The difficulty of obtaining high-intensity localized light spots for optical probes leads to their lack of good applications in nanoimaging.Here we demonstrate a Fabry–Pérot resonance flat-based plasmonic fiber prob...The difficulty of obtaining high-intensity localized light spots for optical probes leads to their lack of good applications in nanoimaging.Here we demonstrate a Fabry–Pérot resonance flat-based plasmonic fiber probe(FPFP).The simulation results show that the probe can obtain a nanofocusing spot at the tip with the radially polarized mode.The Fabry–Pérot interference structure is used to control the plasmon propagation on the surface of the probe,it effectively improves the local spot intensity at the tip.Furthermore,the experimental results verify that the FPFP(tip curvature radius is 20 nm)prepared by chemical etching method can obtain a nanofocusing spot at the tip.The nanoimaging of the gold slit structure demonstrates the nanoimaging capability of the FPFP,the 36.9 nm slit width is clearly identified by the FPFP.展开更多
Delivering light to the nanoscale using a flexible and easily integrated fiber platform holds potential in various fields of quantum science and bioscience.However,rigorous optical alignment,sophisticated fabrication ...Delivering light to the nanoscale using a flexible and easily integrated fiber platform holds potential in various fields of quantum science and bioscience.However,rigorous optical alignment,sophisticated fabrication process,and low spatial resolution of the fiber-based nanoconcentrators limit the practical applications.Here,a broadband azimuthal plasmon interference nanofocusing technique on a fiber-coupled spiral tip is demonstrated for fiber-based near-field optical nanoimaging.The spiral plasmonic fiber tip fabricated through a robust and reproducible process can reverse the polarization and modulate the mode field of the surface plasmon polaritons in three-dimensionally azimuthal direction,resulting in polarization-insensitive,broad-bandwidth,and azimuthal interference nanofocusing.By integrating this with a basic scanning near-field optical microscopy,a high optical resolution of 31 nm and beyond is realized.The high performance and the easy incorporation with various existing measurement platforms offered by this fiber-based nanofocusing technique have great potential in near-field optics,tip-enhanced Raman spectroscopy,nonlinear spectroscopy,and quantum sensing.展开更多
Flexible photodetectors are fundamental components for developing wearable systems,which can be widely used for medical detection,environmental monitoring and flexible imaging.However,compared with 3D materials,lowdim...Flexible photodetectors are fundamental components for developing wearable systems,which can be widely used for medical detection,environmental monitoring and flexible imaging.However,compared with 3D materials,lowdimensional materials have degraded performance,a key challenge for current flexible photodetectors.Here,a highperformance broadband photodetector has been proposed and fabricated.By combining the high mobility of graphene(Gr)with the strong light–matter interactions of single-walled carbon nanotubes(SWCNTs)and molybdenum disulfide(MoS2),the flexible photodetector exhibits a greatly improved photoresponse covering the visible to near-infrared range.Additionally,a thin layer of gadolinium iron garnet(Gd_(3)Fe_(5)O_(12),GdlG)film is introduced to improve the interface of the double van der Waals heterojunctions to reduce the dark current.The SWCNT/GdIG/Gr/GdIG/MoS2 flexible photodetector exhibits a high photoresponsivity of 47.375 A/W and a high detectivity of 1.952×1012 Jones at 450 nm,a high photoresponsivity of 109.311 A/W and a high detectivity of 4.504×10^(12) Jones at 1080 nm,and good mechanical stability at room temperature.This work demonstrates the good capacity of GdIGassisted double van der Waals heterojunctions on flexible substrates and provides a new solution for constructing high-performance flexible photodetectors.展开更多
The properties of near-field optics have always been the focus of nano-measurement technology.The 11th order effective nearfield optical signal with an incident laser wavelength of 1,550 nm is obtained using a platinu...The properties of near-field optics have always been the focus of nano-measurement technology.The 11th order effective nearfield optical signal with an incident laser wavelength of 1,550 nm is obtained using a platinum-coated optical probe(Pt–Si probe).The experimental results show that the local electric field intensity of the Pt–Si probe is nearly 30 times higher than that of silicon probe(Si probe).Therefore,the highest 7th order near-field optical imaging results are obtained with the Pt–Si probe.Further,near-field optical imaging is performed on samples such as gold grids and carbon nanotubes using the Pt–Si probe.The measurement results show that the high-order signal has the characteristics of less background,higher signal-to-noise ratio,and resolution up to 5.7 nm.展开更多
基金the National Science Fund for Distinguished Young Scholars(No.52225507).
文摘The difficulty of obtaining high-intensity localized light spots for optical probes leads to their lack of good applications in nanoimaging.Here we demonstrate a Fabry–Pérot resonance flat-based plasmonic fiber probe(FPFP).The simulation results show that the probe can obtain a nanofocusing spot at the tip with the radially polarized mode.The Fabry–Pérot interference structure is used to control the plasmon propagation on the surface of the probe,it effectively improves the local spot intensity at the tip.Furthermore,the experimental results verify that the FPFP(tip curvature radius is 20 nm)prepared by chemical etching method can obtain a nanofocusing spot at the tip.The nanoimaging of the gold slit structure demonstrates the nanoimaging capability of the FPFP,the 36.9 nm slit width is clearly identified by the FPFP.
基金The authors would like to acknowledge the support by the National Science Fund for Distinguished Young Scholars(No.52225507)the National Key Research and Development Program of China(No.2021YFF0700402)the Key Research and Development Program of Shaanxi Province(No.2021GXLH-Z-029).
文摘Delivering light to the nanoscale using a flexible and easily integrated fiber platform holds potential in various fields of quantum science and bioscience.However,rigorous optical alignment,sophisticated fabrication process,and low spatial resolution of the fiber-based nanoconcentrators limit the practical applications.Here,a broadband azimuthal plasmon interference nanofocusing technique on a fiber-coupled spiral tip is demonstrated for fiber-based near-field optical nanoimaging.The spiral plasmonic fiber tip fabricated through a robust and reproducible process can reverse the polarization and modulate the mode field of the surface plasmon polaritons in three-dimensionally azimuthal direction,resulting in polarization-insensitive,broad-bandwidth,and azimuthal interference nanofocusing.By integrating this with a basic scanning near-field optical microscopy,a high optical resolution of 31 nm and beyond is realized.The high performance and the easy incorporation with various existing measurement platforms offered by this fiber-based nanofocusing technique have great potential in near-field optics,tip-enhanced Raman spectroscopy,nonlinear spectroscopy,and quantum sensing.
基金This work was supported by the China National Funds for Distinguished Young Scientists(No.52225507)the National Key Research and Development Program of China(No.2021YFF0700402)the Fundamental Research Funds for the Central Universities.
文摘Flexible photodetectors are fundamental components for developing wearable systems,which can be widely used for medical detection,environmental monitoring and flexible imaging.However,compared with 3D materials,lowdimensional materials have degraded performance,a key challenge for current flexible photodetectors.Here,a highperformance broadband photodetector has been proposed and fabricated.By combining the high mobility of graphene(Gr)with the strong light–matter interactions of single-walled carbon nanotubes(SWCNTs)and molybdenum disulfide(MoS2),the flexible photodetector exhibits a greatly improved photoresponse covering the visible to near-infrared range.Additionally,a thin layer of gadolinium iron garnet(Gd_(3)Fe_(5)O_(12),GdlG)film is introduced to improve the interface of the double van der Waals heterojunctions to reduce the dark current.The SWCNT/GdIG/Gr/GdIG/MoS2 flexible photodetector exhibits a high photoresponsivity of 47.375 A/W and a high detectivity of 1.952×1012 Jones at 450 nm,a high photoresponsivity of 109.311 A/W and a high detectivity of 4.504×10^(12) Jones at 1080 nm,and good mechanical stability at room temperature.This work demonstrates the good capacity of GdIGassisted double van der Waals heterojunctions on flexible substrates and provides a new solution for constructing high-performance flexible photodetectors.
基金the National Key Research and Development Program of China(No.2021YFF0700402)the Program for Science and Technology Innovation Group of Shaanxi Province(No.2019TD-011)+1 种基金the Key Research and Development Program of Shaanxi Province(No.2020DLGY04-02)the Fundamental Research Funds for the Central Universities for their support.
文摘The properties of near-field optics have always been the focus of nano-measurement technology.The 11th order effective nearfield optical signal with an incident laser wavelength of 1,550 nm is obtained using a platinum-coated optical probe(Pt–Si probe).The experimental results show that the local electric field intensity of the Pt–Si probe is nearly 30 times higher than that of silicon probe(Si probe).Therefore,the highest 7th order near-field optical imaging results are obtained with the Pt–Si probe.Further,near-field optical imaging is performed on samples such as gold grids and carbon nanotubes using the Pt–Si probe.The measurement results show that the high-order signal has the characteristics of less background,higher signal-to-noise ratio,and resolution up to 5.7 nm.