The impacts of low and high-frequency variability from teleconnections between large scale atmospheric processes and local weather as well as emissions changes on concentrations of particulate matter of 2.5 μm or les...The impacts of low and high-frequency variability from teleconnections between large scale atmospheric processes and local weather as well as emissions changes on concentrations of particulate matter of 2.5 μm or less in diameter ([PM2.5]) were examined for the Fairbanks Metropolitan Area (FMA). October to March and May to August mean [PM2.5] were 1.8 and 3.1 μg·m-3 higher for positive than negative annual mean Pacific Decadal Oscillation. Annual mean [PM2.5] were 3.8 μg·m-3 lower for positive than negative Southern Oscillation Index. On 1999-2018 average, [PM2.5] decreased 2.9 μg·m-3·decade-1. On average over October to March, decadal and inter-annual variability caused higher or similar differences in mean observed [PM2.5] and its species than emission-control measures. The 2006 implementation of Tier 2 for new vehicles decreased observed sulfate concentrations the strongest (~4.95 μg·m-3·decade-1) of all occurred emissions changes. On average, observed [PM2.5] showed elevated values at all sites when wind blew from directions of hot springs. The same was found for the sulfate, ammonium and non-metal components of PM2.5. Observations showed that these geothermal waters contain sulfate, ammonia, boric acid and non-metals. Hot springs of such composition are known to emit hydrogen sulfide and ammonia that can serve as precursors for ammonium and sulfate aerosols.展开更多
文摘The impacts of low and high-frequency variability from teleconnections between large scale atmospheric processes and local weather as well as emissions changes on concentrations of particulate matter of 2.5 μm or less in diameter ([PM2.5]) were examined for the Fairbanks Metropolitan Area (FMA). October to March and May to August mean [PM2.5] were 1.8 and 3.1 μg·m-3 higher for positive than negative annual mean Pacific Decadal Oscillation. Annual mean [PM2.5] were 3.8 μg·m-3 lower for positive than negative Southern Oscillation Index. On 1999-2018 average, [PM2.5] decreased 2.9 μg·m-3·decade-1. On average over October to March, decadal and inter-annual variability caused higher or similar differences in mean observed [PM2.5] and its species than emission-control measures. The 2006 implementation of Tier 2 for new vehicles decreased observed sulfate concentrations the strongest (~4.95 μg·m-3·decade-1) of all occurred emissions changes. On average, observed [PM2.5] showed elevated values at all sites when wind blew from directions of hot springs. The same was found for the sulfate, ammonium and non-metal components of PM2.5. Observations showed that these geothermal waters contain sulfate, ammonia, boric acid and non-metals. Hot springs of such composition are known to emit hydrogen sulfide and ammonia that can serve as precursors for ammonium and sulfate aerosols.
