The optical nonlinearity in polycrystalline zinc selenide(ZnSe),excited with 775 nm,1 kHz femtosecond laser pulses was investigated via the nonlinear transmission with material thickness and the Z scan technique.The m...The optical nonlinearity in polycrystalline zinc selenide(ZnSe),excited with 775 nm,1 kHz femtosecond laser pulses was investigated via the nonlinear transmission with material thickness and the Z scan technique.The measured two photon absorption coefficientβwas intensity dependent,inferring that reverse saturated absorption(RSA)is also relevant dur-ing high intensity excitation in ZnSe.At low peak intensity I<5 GW cm^(-2),we findβ=3.5 cm GW^(-1) at 775 nm.The spec-tral properties of the broad blueish two-photon induced fluorescence(460 nm-500 nm)was studied,displaying self-ab-sorption near the band edge while the upper state lifetime was measured to be τ_(e)~3.3 ns.Stimulated emission was ob-served when pumping a 0.5 mm thick polycrystalline ZnSe sample within an optical cavity,confirmed by significant line narrowing fromΔλ=11 nm(cavity blocked)toΔλ=2.8 nm at peak wavelength λ_(p)=475 nm while the upper state life-time also decreased.These results suggest that with more optimum pumping conditions and crystal cooling,polycrystal-line ZnSe might reach lasing threshold via two-photon pumping atλ=775 nm.展开更多
文摘The optical nonlinearity in polycrystalline zinc selenide(ZnSe),excited with 775 nm,1 kHz femtosecond laser pulses was investigated via the nonlinear transmission with material thickness and the Z scan technique.The measured two photon absorption coefficientβwas intensity dependent,inferring that reverse saturated absorption(RSA)is also relevant dur-ing high intensity excitation in ZnSe.At low peak intensity I<5 GW cm^(-2),we findβ=3.5 cm GW^(-1) at 775 nm.The spec-tral properties of the broad blueish two-photon induced fluorescence(460 nm-500 nm)was studied,displaying self-ab-sorption near the band edge while the upper state lifetime was measured to be τ_(e)~3.3 ns.Stimulated emission was ob-served when pumping a 0.5 mm thick polycrystalline ZnSe sample within an optical cavity,confirmed by significant line narrowing fromΔλ=11 nm(cavity blocked)toΔλ=2.8 nm at peak wavelength λ_(p)=475 nm while the upper state life-time also decreased.These results suggest that with more optimum pumping conditions and crystal cooling,polycrystal-line ZnSe might reach lasing threshold via two-photon pumping atλ=775 nm.
