In iron-based superconductor Fe(Se,Te), a flat band-like feature near the Fermi level was observed around the Brillouin zone center in the superconducting state. It is under debate whether this is the evidence on the ...In iron-based superconductor Fe(Se,Te), a flat band-like feature near the Fermi level was observed around the Brillouin zone center in the superconducting state. It is under debate whether this is the evidence on the presence of the BCS–BEC[Bardeen–Cooper–Schrieffer(BCS), Bose–Einstein condensation(BEC)] crossover in the superconductor. High-resolution laser-based angle-resolved photoemission measurements are carried out on high quality single crystals of FeSe_(0.45)Te_(0.55) superconductor to address the issue. By employing different polarization geometries, we have resolved and isolated the dyz band and the topological surface band, making it possible to study their superconducting behaviors separately. The dyz band alone does not form a flat band-like feature in the superconducting state and the measured dispersion can be well described by the BCS picture. We find that the flat band-like feature is formed from the combination of the dyz band and the topological surface state band in the superconducting state. These results reveal the origin of the flat band-like feature and rule out the presence of BCS-BEC crossover in Fe(Se,Te) superconductor.展开更多
The spatially-resolved laser-based high-resolution angle resolved photoemission spectroscopy(ARPES) measurements have been performed on the optimally-doped YBa_(2)Cu_(3)O_(7)-σ(Y123) superconductor. For the first tim...The spatially-resolved laser-based high-resolution angle resolved photoemission spectroscopy(ARPES) measurements have been performed on the optimally-doped YBa_(2)Cu_(3)O_(7)-σ(Y123) superconductor. For the first time, we found the region from the cleaved surface that reveals clear bulk electronic properties. The intrinsic Fermi surface and band structures of Y123 were observed. The Fermi surface-dependent and momentum-dependent superconducting gap was determined which is nodeless and consistent with the d+is gap form.展开更多
High resolution angle-resolved photoemission spectroscopy(ARPES)measurements are carried out on CaKFe_4 As_4,KCa_2 Fe_4 As_4 F_2 and(Ba_(0.6)K_(0.4))Fe_2 As_2 superconductors.Clear evidence of band folding between the...High resolution angle-resolved photoemission spectroscopy(ARPES)measurements are carried out on CaKFe_4 As_4,KCa_2 Fe_4 As_4 F_2 and(Ba_(0.6)K_(0.4))Fe_2 As_2 superconductors.Clear evidence of band folding between the Brillouin zone center and corners with a(π,π)wave vector has been found from the measured Fermi surface and band structures in all the three kinds of superconductors.A dominant √2×√2 surface reconstruction is observed on the cleaved surface of CaKFe_4As_4 by scanning tunneling microscopy(STM)measurements.We propose that the commonly observed √2×√2 reconstruction in the FeAs-based superconductors provides a general scenario to understand the origin of the(π,π)band folding.Our observations provide new insights in understanding the electronic structure and superconductivity mechanism in iron-based superconductors.展开更多
The electronic structure and superconducting gap structure are prerequisites to establish microscopic theories in understanding the superconductivity mechanism of iron-based superconductors.However,even for the most e...The electronic structure and superconducting gap structure are prerequisites to establish microscopic theories in understanding the superconductivity mechanism of iron-based superconductors.However,even for the most extensively studied optimally-doped Ba_(0.6)K_(0.4)Fe_(2)As_(2),there remain outstanding controversies on its electronic structure and superconducting gap structure.Here we resolve these issues by carrying out high-resolution angle-resolved photoemission spectroscopy(ARPES)measurements on the optimally-doped Ba_(0.6)K_(0.4)Fe_(2)As_(2)superconductor using both Helium lamp and laser light sources.Our results indicate the‘‘flat band"feature observed around the Brillouin zone center in the superconducting state originates from the combined effect of the superconductivity-induced band back-bending and the folding of a band from the zone corner to the center.We found direct evidence of the band folding between the zone corner and the center in both the normal and superconducting state.Our resolution of the origin of the flat band makes it possible to assign the three hole-like bands around the zone center and determine their superconducting gap correctly.Around the zone corner,we observe a tiny electronlike band and an M-shaped band simultaneously in both the normal and superconducting states.The obtained gap size for the bands around the zone corner(~5.5 meV)is significantly smaller than all the previous ARPES measurements.Our results establish a new superconducting gap structure around the zone corner and resolve a number of prominent controversies concerning the electronic structure and superconducting gap structure in the optimally-doped Ba_(0.6)K_(0.4)Fe_(2)As_(2).They provide new insights in examining and establishing theories in understanding superconductivity mechanism in iron-based superconductors.展开更多
基金Projects supported by the National Key Research and Development Program of China(GrantNos.2021YFA1401800,2022YFA1604200,2022YFA1403900,and2023YFA1406000)the National Natural Science Foundation of China(Grant Nos.12488201,12374066,12074411,and 12374154)+3 种基金the Strategic Priority Research Program(B)of the Chinese Academy of Sciences(Grant Nos.XDB25000000 and XDB33000000)the Innovation Program for Quantum Science and Technology(Grant No.2021ZD0301800)the Youth Innovation Promotion Association of the Chinese Academy of Sciences(Grant No.Y2021006)the Synergetic Extreme Condition User Facility(SECUF)。
文摘In iron-based superconductor Fe(Se,Te), a flat band-like feature near the Fermi level was observed around the Brillouin zone center in the superconducting state. It is under debate whether this is the evidence on the presence of the BCS–BEC[Bardeen–Cooper–Schrieffer(BCS), Bose–Einstein condensation(BEC)] crossover in the superconductor. High-resolution laser-based angle-resolved photoemission measurements are carried out on high quality single crystals of FeSe_(0.45)Te_(0.55) superconductor to address the issue. By employing different polarization geometries, we have resolved and isolated the dyz band and the topological surface band, making it possible to study their superconducting behaviors separately. The dyz band alone does not form a flat band-like feature in the superconducting state and the measured dispersion can be well described by the BCS picture. We find that the flat band-like feature is formed from the combination of the dyz band and the topological surface state band in the superconducting state. These results reveal the origin of the flat band-like feature and rule out the presence of BCS-BEC crossover in Fe(Se,Te) superconductor.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 11888101 and 11974404)the National Key Research and Development Program of China (Grant Nos. 2021YFA1401800 and 2018YFA0704200)+3 种基金the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grant Nos. XDB25000000 and XDB33000000)the Youth Innovation Promotion Association of CAS (Grant No. Y2021006)Innovation Program for Quantum Science and Technology (Grant No. 2021ZD0301800)the Synergetic Extreme Condition User Facility (SECUF)。
文摘The spatially-resolved laser-based high-resolution angle resolved photoemission spectroscopy(ARPES) measurements have been performed on the optimally-doped YBa_(2)Cu_(3)O_(7)-σ(Y123) superconductor. For the first time, we found the region from the cleaved surface that reveals clear bulk electronic properties. The intrinsic Fermi surface and band structures of Y123 were observed. The Fermi surface-dependent and momentum-dependent superconducting gap was determined which is nodeless and consistent with the d+is gap form.
基金Supported by the National Key Research and Development Program of China (Grant Nos.2016YFA0300300,2017YFA0302900,2018YFA0704200 and 2019YFA0308000)the National Natural Science Foundation of China (Grant Nos.11888101,11922414 and11874405)+2 种基金the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grant No.XDB25000000)the Youth Innovation Promotion Association of CAS (Grant No.2017013)the Research Program of Beijing Academy of Quantum Information Sciences (Grant No.Y18G06)。
文摘High resolution angle-resolved photoemission spectroscopy(ARPES)measurements are carried out on CaKFe_4 As_4,KCa_2 Fe_4 As_4 F_2 and(Ba_(0.6)K_(0.4))Fe_2 As_2 superconductors.Clear evidence of band folding between the Brillouin zone center and corners with a(π,π)wave vector has been found from the measured Fermi surface and band structures in all the three kinds of superconductors.A dominant √2×√2 surface reconstruction is observed on the cleaved surface of CaKFe_4As_4 by scanning tunneling microscopy(STM)measurements.We propose that the commonly observed √2×√2 reconstruction in the FeAs-based superconductors provides a general scenario to understand the origin of the(π,π)band folding.Our observations provide new insights in understanding the electronic structure and superconductivity mechanism in iron-based superconductors.
基金financial support from the National Key Research and Development Program of China(2016YFA0300300,2017YFA0302900,2018YFA0704200 and 2019YFA0308000)the National Natural Science Foundation of China(11888101,11922414,11874405,and 62022089)+2 种基金the Strategic Priority Research Program(B)of the Chinese Academy of Sciences(XDB25000000 and XDB33000000)the Youth Innovation Promotion Association of CAS(2017013 and 2019007)the Research Program of Beijing Academy of Quantum Information Sciences(Y18G06)。
文摘The electronic structure and superconducting gap structure are prerequisites to establish microscopic theories in understanding the superconductivity mechanism of iron-based superconductors.However,even for the most extensively studied optimally-doped Ba_(0.6)K_(0.4)Fe_(2)As_(2),there remain outstanding controversies on its electronic structure and superconducting gap structure.Here we resolve these issues by carrying out high-resolution angle-resolved photoemission spectroscopy(ARPES)measurements on the optimally-doped Ba_(0.6)K_(0.4)Fe_(2)As_(2)superconductor using both Helium lamp and laser light sources.Our results indicate the‘‘flat band"feature observed around the Brillouin zone center in the superconducting state originates from the combined effect of the superconductivity-induced band back-bending and the folding of a band from the zone corner to the center.We found direct evidence of the band folding between the zone corner and the center in both the normal and superconducting state.Our resolution of the origin of the flat band makes it possible to assign the three hole-like bands around the zone center and determine their superconducting gap correctly.Around the zone corner,we observe a tiny electronlike band and an M-shaped band simultaneously in both the normal and superconducting states.The obtained gap size for the bands around the zone corner(~5.5 meV)is significantly smaller than all the previous ARPES measurements.Our results establish a new superconducting gap structure around the zone corner and resolve a number of prominent controversies concerning the electronic structure and superconducting gap structure in the optimally-doped Ba_(0.6)K_(0.4)Fe_(2)As_(2).They provide new insights in examining and establishing theories in understanding superconductivity mechanism in iron-based superconductors.