为解决氙(Xe)的九种稳定同位素质量差异大(约9.6%),质谱探测器接收难的问题,利用Helix MC Plus静态气体质谱仪,建立一种测量Xe全部稳定同位素丰度比的高精度质谱分析方法,快速、准确获得Xe的全部稳定同位素丰度。首先对混合气体样品中...为解决氙(Xe)的九种稳定同位素质量差异大(约9.6%),质谱探测器接收难的问题,利用Helix MC Plus静态气体质谱仪,建立一种测量Xe全部稳定同位素丰度比的高精度质谱分析方法,快速、准确获得Xe的全部稳定同位素丰度。首先对混合气体样品中的Xe进行提取分离与纯化等条件实验,减小其他惰性气体及活性组分对Xe同位素分析测量的影响,再使用跳峰和多接收两种方式相结合的测量方法,实现在进样量极小时,基于Helix MC Plus型静态气体质谱仪的Xe全部稳定同位素的高精度测量,并利用天然丰度Xe标准气体对配制的混合气体样品测量结果进行线性校正。结果表明,在进样量约1.12×10^(-12)mol条件下,法拉第杯测量129 Xe/^(132)Xe、^(130)Xe/^(132)Xe、^(131)Xe/^(132)Xe、^(134)Xe/^(132)Xe、^(136)Xe/^(132)Xe丰度比的相对标准偏差≤0.24%,对于使用计数法测量124 Xe/^(132)Xe、126 Xe/^(132)Xe丰度比的相对标准偏差分别为0.22%和0.39%。本方法稳定性好、精度高,可以实现痕量Xe稳定同位素的丰度比质谱分析测试。展开更多
Compact flame-holders for afterburners are an increasing requirement for modern aero engines.However,flame-holder design is non-trivial since high inlet temperatures,velocities,and elaborate structures induce complex ...Compact flame-holders for afterburners are an increasing requirement for modern aero engines.However,flame-holder design is non-trivial since high inlet temperatures,velocities,and elaborate structures induce complex turbulence,combustion,and spray coupling in modern afterburners.In this work,the LES-pdf and stochastic fields-Lagrangian particle spray methods are used to investigate methane and aviation kerosene combustion structures formed by new-type concave flame-holders.The flow pattern,combustion mode,and flame structure of gaseous and liquid fuel around a concave flame-holder are analyzed,discussed,and compared with experimental results.Results reveal that the flame stability of a concave flame-holder is better than that of the non-concave one.Furthermore,when using liquid fuel,the concave flame-holder forms a stable and compact flame.These results suggest concave flame-holders are a promising design for compact afterburners.展开更多
Aerosol radionuclides (131I, 134Cs, 137Cs) and gaseous radioactive xenon (133Xe) were monitored at Xi'an, China following the accident at the Fukushima nuclear power plant in March 2011. The additional annual effe...Aerosol radionuclides (131I, 134Cs, 137Cs) and gaseous radioactive xenon (133Xe) were monitored at Xi'an, China following the accident at the Fukushima nuclear power plant in March 2011. The additional annual effective dose attributable to the Fukushima emissions was much lower than the public annual effective dose from natural radiation, according to Chinese national standards. The monitoring results were compared with data from other countries as well as with the radionuclide concentrations observed in Xi'an after the Chernobyl nuclear accident in 1986. Possible transport pathways of the released radionuclides from Fukushima to Xi'an were investigated. The occurrence of an anticyclone in the Pacific Ocean region and the extended period over which the radionuclides were released made the determination transport pathways complex, but divergence in the plume and easterly flow evidently brought the initial suite of radionuclides to Xi'an.展开更多
文摘为解决氙(Xe)的九种稳定同位素质量差异大(约9.6%),质谱探测器接收难的问题,利用Helix MC Plus静态气体质谱仪,建立一种测量Xe全部稳定同位素丰度比的高精度质谱分析方法,快速、准确获得Xe的全部稳定同位素丰度。首先对混合气体样品中的Xe进行提取分离与纯化等条件实验,减小其他惰性气体及活性组分对Xe同位素分析测量的影响,再使用跳峰和多接收两种方式相结合的测量方法,实现在进样量极小时,基于Helix MC Plus型静态气体质谱仪的Xe全部稳定同位素的高精度测量,并利用天然丰度Xe标准气体对配制的混合气体样品测量结果进行线性校正。结果表明,在进样量约1.12×10^(-12)mol条件下,法拉第杯测量129 Xe/^(132)Xe、^(130)Xe/^(132)Xe、^(131)Xe/^(132)Xe、^(134)Xe/^(132)Xe、^(136)Xe/^(132)Xe丰度比的相对标准偏差≤0.24%,对于使用计数法测量124 Xe/^(132)Xe、126 Xe/^(132)Xe丰度比的相对标准偏差分别为0.22%和0.39%。本方法稳定性好、精度高,可以实现痕量Xe稳定同位素的丰度比质谱分析测试。
基金National Science and Technology Major Project (2017-Ⅰ-0004-0005)National Natural Science Foundation of China (91741125)。
文摘Compact flame-holders for afterburners are an increasing requirement for modern aero engines.However,flame-holder design is non-trivial since high inlet temperatures,velocities,and elaborate structures induce complex turbulence,combustion,and spray coupling in modern afterburners.In this work,the LES-pdf and stochastic fields-Lagrangian particle spray methods are used to investigate methane and aviation kerosene combustion structures formed by new-type concave flame-holders.The flow pattern,combustion mode,and flame structure of gaseous and liquid fuel around a concave flame-holder are analyzed,discussed,and compared with experimental results.Results reveal that the flame stability of a concave flame-holder is better than that of the non-concave one.Furthermore,when using liquid fuel,the concave flame-holder forms a stable and compact flame.These results suggest concave flame-holders are a promising design for compact afterburners.
文摘Aerosol radionuclides (131I, 134Cs, 137Cs) and gaseous radioactive xenon (133Xe) were monitored at Xi'an, China following the accident at the Fukushima nuclear power plant in March 2011. The additional annual effective dose attributable to the Fukushima emissions was much lower than the public annual effective dose from natural radiation, according to Chinese national standards. The monitoring results were compared with data from other countries as well as with the radionuclide concentrations observed in Xi'an after the Chernobyl nuclear accident in 1986. Possible transport pathways of the released radionuclides from Fukushima to Xi'an were investigated. The occurrence of an anticyclone in the Pacific Ocean region and the extended period over which the radionuclides were released made the determination transport pathways complex, but divergence in the plume and easterly flow evidently brought the initial suite of radionuclides to Xi'an.
