One hallmark of Weyl semimetals is the emergence of Fermi arcs(FAs) in surface Brillouin zones, where FAs connect the projected Weyl nodes of opposite chiralities. Unclosed FAs can give rise to various exotic effects ...One hallmark of Weyl semimetals is the emergence of Fermi arcs(FAs) in surface Brillouin zones, where FAs connect the projected Weyl nodes of opposite chiralities. Unclosed FAs can give rise to various exotic effects that have attracted tremendous research interest. Configurations of FAs are usually thought to be determined fully by the band topology of the bulk states, which seems impossible to manipulate. Here, we show that FAs can be simply modified by a surface gate voltage. Because the penetration length of the surface states depends on the in-plane momentum, a surface gate voltage induces an effective energy dispersion. As a result, a continuous deformation of the surface band can be implemented by tuning the surface gate voltage. In particular, as the saddle point of the surface band meets the Fermi energy, the topological Lifshitz transition takes place for the FAs,during which the Weyl nodes switch their partners connected by the FAs. Accordingly, the magnetic Weyl orbits composed of the FAs on opposite surfaces and chiral Landau bands inside the bulk change their configurations.We show that such an effect can be probed by the transport measurements in a magnetic field, in which the switch-on and switch-off conductances by the surface gate voltage signal the Lifshitz transition. Our work opens a new route for manipulating the FAs by surface gates and exploring novel transport phenomena associated with the topological Lifshitz transition.展开更多
The Weyl semimetal has emerged as a new topologically nontrivial phase of matter,hosting low-energy excitations of massless Weyl fermions.Here,we present a comprehensive study of a type-ⅡWeyl semimetal WP2.Transport ...The Weyl semimetal has emerged as a new topologically nontrivial phase of matter,hosting low-energy excitations of massless Weyl fermions.Here,we present a comprehensive study of a type-ⅡWeyl semimetal WP2.Transport studies show a butterfly-like magnetoresistance at low temperature,reflecting the anisotropy of the electron Fermi surfaces.This four-lobed feature gradually evolves into a two-lobed variant with an increase in temperature,mainly due to the reduced relative contribution of electron Fermi surfaces compared to hole Fermi surfaces for magnetoresistance.Moreover,an angle-dependent Berry phase is also discovered,based on quantum oscillations,which is ascribed to the effective manipulation of extremal Fermi orbits by the magnetic field to feel nearby topological singularities in the momentum space.The revealed topological character and anisotropic Fermi surfaces of the WP2 substantially enrich the physical properties of Weyl semimetals,and show great promises in terms of potential topological electronic and Fermitronic device applications.展开更多
We investigate the topological phase transition driven by non-local electronic correlations in a realistic quantum anomalous Hall model consisting of d_(xy)–d_(x^(2)-y^(2)) orbitals. Three topologically distinct phas...We investigate the topological phase transition driven by non-local electronic correlations in a realistic quantum anomalous Hall model consisting of d_(xy)–d_(x^(2)-y^(2)) orbitals. Three topologically distinct phases defined in the noninteracting limit evolve to different charge density wave phases under correlations. Two conspicuous conclusions were obtained: The topological phase transition does not involve gap-closing and the dynamical fluctuations significantly suppress the charge order favored by the next nearest neighbor interaction. Our study sheds light on the stability of topological phase under electronic correlations, and we demonstrate a positive role played by dynamical fluctuations that is distinct to all previous studies on correlated topological states.展开更多
Topological materials (TMs) have gained intensive attention due to their novel behaviors compared with topologically trivial materials. Among various TMs, Dirac semimetal (DSM) has been studied extensively. Although s...Topological materials (TMs) have gained intensive attention due to their novel behaviors compared with topologically trivial materials. Among various TMs, Dirac semimetal (DSM) has been studied extensively. Although several DSMs have been proposed and verified experimentally, the suitable DSM for realistic applications is still lacking. Thus finding ideal DSMs and providing detailed analyses to them are of both fundamental and technological importance. Here, we sort out 8 (nearly) ideal DSMs from thousands of topological semimetals in Nature 566(7745), 486 (2019). We show the concrete positions of the Dirac points in the Brillouin zone for these materials and clarify the symmetryprotection mechanism for these Dirac points as well as their low-energy effective models. Our results provide a useful starting point for future study such as topological phase transition under strain and transport study based on these effective models. These DSMs with high mobilities are expected to be applied in fabrication of functional electronic devices.展开更多
Recently,competing electronic instabilities,including superconductivity and density-wave-like order,have been discovered in vanadium-based kagome metals AV_(3)Sb_(5)(A=K,Rb,Cs)with a nontrivial band topology.This find...Recently,competing electronic instabilities,including superconductivity and density-wave-like order,have been discovered in vanadium-based kagome metals AV_(3)Sb_(5)(A=K,Rb,Cs)with a nontrivial band topology.This finding stimulates considerable interest to study the interplay of these competing electronic orders and possible exotic excitations in the superconducting state.Here,we performed51V and133Cs nuclear magnetic resonance(NMR)measurements on a CsV_(3)Sb_(5)single crystal to clarify the nature of density-wave-like transition in these kagome superconductors.A first-order structural transition is unambiguously revealed below T_(s)~94 K by observing the sudden splitting of Knight shift in^(51)V NMR spectrum.Moreover,combined with^(133)Cs NMR spectrum,the present result confirms a three-dimensional structural modulation.By further analyzing the anisotropy of Knight shift and 1/T_(1)T at^(51)V nuclei,we proposed that the orbital order is the primary electronic order induced by the firstorder structural transition,which is supported by further analysis on electric field gradient at^(51)V nuclei.In addition,the evidence for possible orbital fluctuations is also revealed above T_(s).The present work sheds light on a rich orbital physics in kagome superconductors AV_(3)Sb_(5).展开更多
Valley,the energy extrema in the electronic band structure at momentum space,is regarded as a new degree of freedom of electrons,in addition to charge and spin.The studies focused on valley degree of freedom now form ...Valley,the energy extrema in the electronic band structure at momentum space,is regarded as a new degree of freedom of electrons,in addition to charge and spin.The studies focused on valley degree of freedom now form an emerging field of condensed-matter physics,i.e.,valleytronics,whose development is exactly following that of spintronics,which focuses on the spin degree of freedom.展开更多
Performing angle-resolved photoemission spectroscopy(ARPES) and theoretical calculations for ZrSnTe, we find a nodal line in the kx-ky plane with a tiny gap and two nodal lines without gaps along the kzdirection. The ...Performing angle-resolved photoemission spectroscopy(ARPES) and theoretical calculations for ZrSnTe, we find a nodal line in the kx-ky plane with a tiny gap and two nodal lines without gaps along the kzdirection. The constant energy contours are plotted in the kx-ky plane at a photon energy of 30 e V to examine the gapping feature of the nodal line. In addition, we depict the band dispersions along the Γ-M and Γ-X directions from the ARPES images at photon energies ranging from 24 to 40 e V. The kz mapping confirms the presence of stable Dirac points with obvious kzdependences along the M-A and X-R directions. In this paper, we report the two types of nodal lines associated with the theoretical local-density approximation calculations, broadening the horizons of nodal-line semimetal research.展开更多
Coexistence of non-trivial band topology and intrinsic magnetic order not only leads to emergent phenomena but also allows for the tunability of the exotic properties from different degrees of freedom. By performing t...Coexistence of non-trivial band topology and intrinsic magnetic order not only leads to emergent phenomena but also allows for the tunability of the exotic properties from different degrees of freedom. By performing transport measurements at synergetic extreme conditions, here we report on pressure engineering of intertwined structural, magnetic, and topological phase transitions in an antiferromagnetic Dirac semimetal NdSb. We show that the original antiferromagnetic state is strengthened in the lowpressure region while destabilized upon further compression close to the critical pressure where a structural transition from Fm-3m phase to P4/mmm phase takes place at P~18 GPa, forming a yurt-shaped evolution in response to magnetic field,pressure and temperature. Concomitant with the structural transition, NdSb simultaneously carries on a magnetic transition to the ferromagnetic state. Moreover, theoretical calculations unravel that the ferromagnetic tetragonal phase presents nontrivial features of Weyl fermions. These findings offer new important insight into the microscopic interplay among lattice, spin, and relativistic fermions in lanthanide monopnictides.展开更多
Unsaturated magnetoresistance (MR) has been reported in type-II Weyl semimetal WTe2, manifested as a perfect compensation of opposite carriers. We report linear MR (LMR) in WTe2 crystals, the onset of which was id...Unsaturated magnetoresistance (MR) has been reported in type-II Weyl semimetal WTe2, manifested as a perfect compensation of opposite carriers. We report linear MR (LMR) in WTe2 crystals, the onset of which was identified by constructing the MR mobility spectra for weak fields. The LMR further increased and became dominant for fields stronger than 20 T, while the parabolic MR gradually decayed. The LMR was also observed in high-pressure conditions.展开更多
基金supported by the National Natural Science Foundation of China (Grant Nos. 12074172, 12222406, and 12174182)the State Key Program for Basic Researches of China (Grant No. 2021YFA1400403)+1 种基金the Fundamental Research Funds for the Central Universities, the startup grant at Nanjing Universitythe Excellent Programme at Nanjing University。
文摘One hallmark of Weyl semimetals is the emergence of Fermi arcs(FAs) in surface Brillouin zones, where FAs connect the projected Weyl nodes of opposite chiralities. Unclosed FAs can give rise to various exotic effects that have attracted tremendous research interest. Configurations of FAs are usually thought to be determined fully by the band topology of the bulk states, which seems impossible to manipulate. Here, we show that FAs can be simply modified by a surface gate voltage. Because the penetration length of the surface states depends on the in-plane momentum, a surface gate voltage induces an effective energy dispersion. As a result, a continuous deformation of the surface band can be implemented by tuning the surface gate voltage. In particular, as the saddle point of the surface band meets the Fermi energy, the topological Lifshitz transition takes place for the FAs,during which the Weyl nodes switch their partners connected by the FAs. Accordingly, the magnetic Weyl orbits composed of the FAs on opposite surfaces and chiral Landau bands inside the bulk change their configurations.We show that such an effect can be probed by the transport measurements in a magnetic field, in which the switch-on and switch-off conductances by the surface gate voltage signal the Lifshitz transition. Our work opens a new route for manipulating the FAs by surface gates and exploring novel transport phenomena associated with the topological Lifshitz transition.
基金Supported by the National Natural Science Foundation of China(Grant Nos.11974324,11804326,U1832151,and 11674296),the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDC07010000)the National Key Research and Development Program of China(Grant No.2017YFA0403600)+4 种基金the Anhui Initiative in Quantum Information Technologies(Grant No.AHY170000)the Hefei Science Center CAS(Grant No.2018HSC-UE014)the Jiangsu Provincial Science Foundation for Youth(Grant No.BK20170821)the National Natural Science Foundation of China for Youth(Grant No.11804160)the Anhui Provincial Natural Science Foundation(Grant No.1708085MF136)。
文摘The Weyl semimetal has emerged as a new topologically nontrivial phase of matter,hosting low-energy excitations of massless Weyl fermions.Here,we present a comprehensive study of a type-ⅡWeyl semimetal WP2.Transport studies show a butterfly-like magnetoresistance at low temperature,reflecting the anisotropy of the electron Fermi surfaces.This four-lobed feature gradually evolves into a two-lobed variant with an increase in temperature,mainly due to the reduced relative contribution of electron Fermi surfaces compared to hole Fermi surfaces for magnetoresistance.Moreover,an angle-dependent Berry phase is also discovered,based on quantum oscillations,which is ascribed to the effective manipulation of extremal Fermi orbits by the magnetic field to feel nearby topological singularities in the momentum space.The revealed topological character and anisotropic Fermi surfaces of the WP2 substantially enrich the physical properties of Weyl semimetals,and show great promises in terms of potential topological electronic and Fermitronic device applications.
基金supported by the National Natural Science Foundation of China (Grant No. 11874263)the National Key R&D Program of China (Grant No. 2017YFE0131300)Shanghai Technology Innovation Action Plan (2020-Integrated Circuit Technology Support Program 20DZ1100605,2021-Fundamental Research Area 21JC1404700)。
文摘We investigate the topological phase transition driven by non-local electronic correlations in a realistic quantum anomalous Hall model consisting of d_(xy)–d_(x^(2)-y^(2)) orbitals. Three topologically distinct phases defined in the noninteracting limit evolve to different charge density wave phases under correlations. Two conspicuous conclusions were obtained: The topological phase transition does not involve gap-closing and the dynamical fluctuations significantly suppress the charge order favored by the next nearest neighbor interaction. Our study sheds light on the stability of topological phase under electronic correlations, and we demonstrate a positive role played by dynamical fluctuations that is distinct to all previous studies on correlated topological states.
基金supported by the National Natural Science Foundation of China (Nos.11525417,11834006,51721001,and 11790311)the National Key R&D Program of China (Nos.2018YFA0305704 and 2017YFA0303203).
文摘Topological materials (TMs) have gained intensive attention due to their novel behaviors compared with topologically trivial materials. Among various TMs, Dirac semimetal (DSM) has been studied extensively. Although several DSMs have been proposed and verified experimentally, the suitable DSM for realistic applications is still lacking. Thus finding ideal DSMs and providing detailed analyses to them are of both fundamental and technological importance. Here, we sort out 8 (nearly) ideal DSMs from thousands of topological semimetals in Nature 566(7745), 486 (2019). We show the concrete positions of the Dirac points in the Brillouin zone for these materials and clarify the symmetryprotection mechanism for these Dirac points as well as their low-energy effective models. Our results provide a useful starting point for future study such as topological phase transition under strain and transport study based on these effective models. These DSMs with high mobilities are expected to be applied in fabrication of functional electronic devices.
基金supported by the National Key R&D Program of China(Grant Nos.2017YFA0303000,and 2016YFA0300201)the National Natural Science Foundation of China(Grant Nos.11888101,and 12034004)+2 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB25000000)the Anhui Initiative in Quantum Information Technologies(Grant No.AHY160000)the Collaborative Innovation Program of Hefei Science Center,CAS(Grant No.2019HSCCIP007)。
文摘Recently,competing electronic instabilities,including superconductivity and density-wave-like order,have been discovered in vanadium-based kagome metals AV_(3)Sb_(5)(A=K,Rb,Cs)with a nontrivial band topology.This finding stimulates considerable interest to study the interplay of these competing electronic orders and possible exotic excitations in the superconducting state.Here,we performed51V and133Cs nuclear magnetic resonance(NMR)measurements on a CsV_(3)Sb_(5)single crystal to clarify the nature of density-wave-like transition in these kagome superconductors.A first-order structural transition is unambiguously revealed below T_(s)~94 K by observing the sudden splitting of Knight shift in^(51)V NMR spectrum.Moreover,combined with^(133)Cs NMR spectrum,the present result confirms a three-dimensional structural modulation.By further analyzing the anisotropy of Knight shift and 1/T_(1)T at^(51)V nuclei,we proposed that the orbital order is the primary electronic order induced by the firstorder structural transition,which is supported by further analysis on electric field gradient at^(51)V nuclei.In addition,the evidence for possible orbital fluctuations is also revealed above T_(s).The present work sheds light on a rich orbital physics in kagome superconductors AV_(3)Sb_(5).
基金This work was supported by the National Key Research and Development Program of China(2017YFA0303403)Shanghai Science and Technology Innovation Action Plan(No.19JC1416700)+1 种基金the NSF of China(No.51572085,11774092)ECNU Multifunctional Platform for Innovation.
文摘Valley,the energy extrema in the electronic band structure at momentum space,is regarded as a new degree of freedom of electrons,in addition to charge and spin.The studies focused on valley degree of freedom now form an emerging field of condensed-matter physics,i.e.,valleytronics,whose development is exactly following that of spintronics,which focuses on the spin degree of freedom.
基金supported by the National Key R&D Program of China(Grant No.2018YFA0306800)the National Natural Science Foundation of China(Grant Nos.11714154,11790311,and 11774151)+1 种基金the Fundamental Research Funds for the Central Universities(Grant No.020414380110)the Program for High-Level Entrepreneurial and Innovative Talents Introduction,Jiangsu Province
文摘Performing angle-resolved photoemission spectroscopy(ARPES) and theoretical calculations for ZrSnTe, we find a nodal line in the kx-ky plane with a tiny gap and two nodal lines without gaps along the kzdirection. The constant energy contours are plotted in the kx-ky plane at a photon energy of 30 e V to examine the gapping feature of the nodal line. In addition, we depict the band dispersions along the Γ-M and Γ-X directions from the ARPES images at photon energies ranging from 24 to 40 e V. The kz mapping confirms the presence of stable Dirac points with obvious kzdependences along the M-A and X-R directions. In this paper, we report the two types of nodal lines associated with the theoretical local-density approximation calculations, broadening the horizons of nodal-line semimetal research.
基金supported by the National Key Research and Development Program of China(Grant Nos.2018YFA0305700,and 2021YFA1600204)the National Natural Science Foundation of China(Grant Nos.12174395,12174397,U1932152,U1832209,U19A2093,12004004,and 11874362)+6 种基金the Natural Science Foundation of Anhui Province(Grant Nos.2008085QA40,and 1908085QA18)the Key Project of Natural Scientific Research of Universities in Anhui Province(Grant No.KJ2021A0068)the Users with Excellence Project of Hefei Center CAS(Grant Nos.2021HSCUE008,and 2020HSC-UE015)the Collaborative Innovation Program of Hefei Science Center,CAS(2020HSC-CIP014)supported by the High Magnetic Field Laboratory of Anhui Province(Grant Nos.AHHM-FX-2020-02,and AHHM-FX-2021-03)supported by the Youth Innovation Promotion Association CAS(Grant No.2020443)supported by DOE-NNSA’s Office of Experimental Sciencesa U.S.Department of Energy(DOE)Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory(Grant No.DE-AC02-06CH11357)。
文摘Coexistence of non-trivial band topology and intrinsic magnetic order not only leads to emergent phenomena but also allows for the tunability of the exotic properties from different degrees of freedom. By performing transport measurements at synergetic extreme conditions, here we report on pressure engineering of intertwined structural, magnetic, and topological phase transitions in an antiferromagnetic Dirac semimetal NdSb. We show that the original antiferromagnetic state is strengthened in the lowpressure region while destabilized upon further compression close to the critical pressure where a structural transition from Fm-3m phase to P4/mmm phase takes place at P~18 GPa, forming a yurt-shaped evolution in response to magnetic field,pressure and temperature. Concomitant with the structural transition, NdSb simultaneously carries on a magnetic transition to the ferromagnetic state. Moreover, theoretical calculations unravel that the ferromagnetic tetragonal phase presents nontrivial features of Weyl fermions. These findings offer new important insight into the microscopic interplay among lattice, spin, and relativistic fermions in lanthanide monopnictides.
文摘Unsaturated magnetoresistance (MR) has been reported in type-II Weyl semimetal WTe2, manifested as a perfect compensation of opposite carriers. We report linear MR (LMR) in WTe2 crystals, the onset of which was identified by constructing the MR mobility spectra for weak fields. The LMR further increased and became dominant for fields stronger than 20 T, while the parabolic MR gradually decayed. The LMR was also observed in high-pressure conditions.