The influence of yttrium on the corrosion behavior of Mg–Y alloys has been investigated by electrochemical measurements,scanning electron microscope(SEM)observation,X-ray diffraction(XRD),and X-ray photoelectron spec...The influence of yttrium on the corrosion behavior of Mg–Y alloys has been investigated by electrochemical measurements,scanning electron microscope(SEM)observation,X-ray diffraction(XRD),and X-ray photoelectron spectroscopy(XPS)analysis in NaCl solution.The corrosion resistance decreased with increasing Y content due to increasing Y-rich zone.The solid-dissolved Y improved the chemical activity of the substrate which promoted the corrosion reaction by forming Y2O3.The corrosion resistance was improved by increasing the Y concentration of matrix and proper net Y-rich structure.The sample has the best corrosion resistance when all the Y element was dissolved into the matrix of Mg–5Y in 0.1 M NaCl.展开更多
Kansu (KS) profile is located in the east of Yili basin, western Xinjiang, where typical loess sediments are distributed. The magnetic parameters (such as IRM, SIRM SOFT, and M) and grain size in the KS profile we...Kansu (KS) profile is located in the east of Yili basin, western Xinjiang, where typical loess sediments are distributed. The magnetic parameters (such as IRM, SIRM SOFT, and M) and grain size in the KS profile were analyzed in the study. The results showed that the magnetic property of KS loess is dominated by ferrimagnetic minerals, such as magnetite and maghemite. Antiferromagnetic and superparamagnetic minerals also exist in the profile, but had less impact on magnetic susceptibility. Compared with the typical loess sediments of the central Loess Plateau in China, the strata of Kansu profile contained more magnetic minerals and hard magnetic minerals. The analysis of grain size for magnetic minerals indicated that the properties of loess and paleosol were respectively dominated by PSD/MD and coarse SSD magnetite. The research found that the contents of magnetic minerals in loess and paleosol sequences in Kansu profile were similar, but the proportion of fine grained magnetite and soft magnetic minerals were varying, which implies a positive relationship between the value of magnetic susceptibility and intensity of pedogenesis.展开更多
We present a new method for calculation of quasi-potential,which is a key concept in the large deviation theory.This method adopts the"ordered"idea in the ordered upwind algorithm and different from the fini...We present a new method for calculation of quasi-potential,which is a key concept in the large deviation theory.This method adopts the"ordered"idea in the ordered upwind algorithm and different from the finite difference upwind scheme,the first-order line integral is used as its update rule.With sufficient accuracy,the new simplified method can greatly speed up the computational time.Once the quasi-potential has been computed,the minimum action path(MAP)can also be obtained.Since the MAP is of concern in most stochastic situations,the effectiveness of this new method is checked by analyzing the accuracy of the MAP.Two cases of isotropic diffusion and anisotropic diffusion are considered.It is found that this new method can both effectively compute the MAPs for systems with isotropic diffusion and reduce the computational time.Meanwhile anisotropy will affect the accuracy of the computed MAP.展开更多
This article investigates the variations of contamination levels of heavy metals such as copper, lead, chromium, cadmium, zinc, arsenic, and mercury over time in surface sediments of the Changjiang River Estuary (CRE...This article investigates the variations of contamination levels of heavy metals such as copper, lead, chromium, cadmium, zinc, arsenic, and mercury over time in surface sediments of the Changjiang River Estuary (CRE), Yellow River Estuary (YRE), Pearl River Estuary (PRE), and their adjacent coastal areas in China. The contamination factor (CF), pollution load index (PLI), and geoaccumulation index (Igeo) are used to evaluate the quality of the surface sediments in the study areas. The results showed that the CRE, YRE, and their adjacent coastal areas were at a low risk of contamination in terms of heavy metals, while the PRE and its adjacent coastal area were at a moderate level. By comparison, the concentrations of heavy metals in the surface sediments of the YRE and its adjacent coastal area were relatively lower than those in the CRE, PRE, and their adjacent coastal areas.展开更多
Lithium-sulfur(Li-S)batteries are anticipated as one of the most promising candidates for the highenergy-density storage systems.However,the insulating nature and shuttling effect of sulfur severely limits their perfo...Lithium-sulfur(Li-S)batteries are anticipated as one of the most promising candidates for the highenergy-density storage systems.However,the insulating nature and shuttling effect of sulfur severely limits their performance.The incorporation of sulfur with carbon materials has been deemed as one of the most powerful strategies to improve electrical conductivity and suppress soluble polysulfide shuttling.Herein,a novel three-dimensional carbon framework(3DCF)is prepared and employed as a sulfur host(3DCF@S)for Li-S batteries.The 3DCF not only supplies abundant paths for lithium ion diffusion and electron transport,but also strengthens polysulfide immobilization during the lithium/sulfur conversion reactions.As a result,the 3DCF@S with high sulfur content of 90%exhibits a high capacity of 1366 mA h/g at 0.1 C and excellent cycling stability with a satisfactory capacity of 601 mA h/g after 600 cycles at 2.0 C.The resultant Li-S button battery based 3DCF@S electrode could power a light-emitting diode for 2 h.The acquired 3DCF@S is expected to be widely used in Li-S batteries and this study will promote developments of carbon/sulfur composites for Li-S batteries.展开更多
This article examines a viscoelastic plate that is driven parametrically by a non-Guassian colored noise,which is simplified to an Ornstein-Uhlenbeck process based on the approximation method.To examine the moment sta...This article examines a viscoelastic plate that is driven parametrically by a non-Guassian colored noise,which is simplified to an Ornstein-Uhlenbeck process based on the approximation method.To examine the moment stability property of the viscoelastic system,we use the stochastic averaging method,Girsanov theorem and Feynmann-Kac formula to derive the approximate analytic expansion of the moment Lyapunov exponent.Furthermore,the Monte Carlo simulation results for the original system are given to check the accuracy of the approximate analytic results.At the end of this paper,results are presented to show some quantitative pictures of the effects of the system parameters,noise parameters and viscoelastic parameters on the stability of the viscoelastic plate.展开更多
The noise-induced transition of the augmented Lotka-Volterra system is investigated under vanishingly small noise.Populations will ultimately go extinct because of intrinsic noise,and different extinction routes may o...The noise-induced transition of the augmented Lotka-Volterra system is investigated under vanishingly small noise.Populations will ultimately go extinct because of intrinsic noise,and different extinction routes may occur due to the Freidlin-Wentzell large deviation theory.The relation between the most probable extinction route(MPER)and heteroclinic bifurcation is studied in this paper.The MPERs and the quasi-potentials in different regimes of parameters are analyzed in detail.Before the bifurcation,the predator goes extinct,and the prey will survive for a long time.Then,the heteroclinic bifurcation changes the MPER wherein both species go extinct.The heteroclinic cycle plays a role in transferring the most probable extinction state.Moreover,the analyses of the weak noise limit can contribute to predicting the stochastic behavior under finite small noise.Both the heteroclinic bifurcation and the rotational deterministic vector field can reduce the action necessary for the MPER.展开更多
基金the National Basic Research Program of China(grant number:2013CB632205)National Natural Science Foundation of China(grant number:51501199).
文摘The influence of yttrium on the corrosion behavior of Mg–Y alloys has been investigated by electrochemical measurements,scanning electron microscope(SEM)observation,X-ray diffraction(XRD),and X-ray photoelectron spectroscopy(XPS)analysis in NaCl solution.The corrosion resistance decreased with increasing Y content due to increasing Y-rich zone.The solid-dissolved Y improved the chemical activity of the substrate which promoted the corrosion reaction by forming Y2O3.The corrosion resistance was improved by increasing the Y concentration of matrix and proper net Y-rich structure.The sample has the best corrosion resistance when all the Y element was dissolved into the matrix of Mg–5Y in 0.1 M NaCl.
基金funded by the National 973 Project (2009CB421308)the Natural Science Foundation of China (40871080 and 90502008)
文摘Kansu (KS) profile is located in the east of Yili basin, western Xinjiang, where typical loess sediments are distributed. The magnetic parameters (such as IRM, SIRM SOFT, and M) and grain size in the KS profile were analyzed in the study. The results showed that the magnetic property of KS loess is dominated by ferrimagnetic minerals, such as magnetite and maghemite. Antiferromagnetic and superparamagnetic minerals also exist in the profile, but had less impact on magnetic susceptibility. Compared with the typical loess sediments of the central Loess Plateau in China, the strata of Kansu profile contained more magnetic minerals and hard magnetic minerals. The analysis of grain size for magnetic minerals indicated that the properties of loess and paleosol were respectively dominated by PSD/MD and coarse SSD magnetite. The research found that the contents of magnetic minerals in loess and paleosol sequences in Kansu profile were similar, but the proportion of fine grained magnetite and soft magnetic minerals were varying, which implies a positive relationship between the value of magnetic susceptibility and intensity of pedogenesis.
基金the National Natural Science Foundation of China(Grant Nos.11772149 and 12172167)the Project Funded by the Priority Academic Program Development of Jiangsu Higher Education Institutions(PAPD)the Research Fund of State Key Laboratory of Mechanics and Control of Mechanical Structures(Grant No.MCMS-I19G01).
文摘We present a new method for calculation of quasi-potential,which is a key concept in the large deviation theory.This method adopts the"ordered"idea in the ordered upwind algorithm and different from the finite difference upwind scheme,the first-order line integral is used as its update rule.With sufficient accuracy,the new simplified method can greatly speed up the computational time.Once the quasi-potential has been computed,the minimum action path(MAP)can also be obtained.Since the MAP is of concern in most stochastic situations,the effectiveness of this new method is checked by analyzing the accuracy of the MAP.Two cases of isotropic diffusion and anisotropic diffusion are considered.It is found that this new method can both effectively compute the MAPs for systems with isotropic diffusion and reduce the computational time.Meanwhile anisotropy will affect the accuracy of the computed MAP.
文摘This article investigates the variations of contamination levels of heavy metals such as copper, lead, chromium, cadmium, zinc, arsenic, and mercury over time in surface sediments of the Changjiang River Estuary (CRE), Yellow River Estuary (YRE), Pearl River Estuary (PRE), and their adjacent coastal areas in China. The contamination factor (CF), pollution load index (PLI), and geoaccumulation index (Igeo) are used to evaluate the quality of the surface sediments in the study areas. The results showed that the CRE, YRE, and their adjacent coastal areas were at a low risk of contamination in terms of heavy metals, while the PRE and its adjacent coastal area were at a moderate level. By comparison, the concentrations of heavy metals in the surface sediments of the YRE and its adjacent coastal area were relatively lower than those in the CRE, PRE, and their adjacent coastal areas.
基金financially supported by the National Postdoctoral Science Foundation(2016YFA0200100)the Project of Education Department of Jiangxi Province(Grant No.GJJ160649)Doctoral startup fund of Jiangxi University of Science and Technology(Grant No.3401223242)。
文摘Lithium-sulfur(Li-S)batteries are anticipated as one of the most promising candidates for the highenergy-density storage systems.However,the insulating nature and shuttling effect of sulfur severely limits their performance.The incorporation of sulfur with carbon materials has been deemed as one of the most powerful strategies to improve electrical conductivity and suppress soluble polysulfide shuttling.Herein,a novel three-dimensional carbon framework(3DCF)is prepared and employed as a sulfur host(3DCF@S)for Li-S batteries.The 3DCF not only supplies abundant paths for lithium ion diffusion and electron transport,but also strengthens polysulfide immobilization during the lithium/sulfur conversion reactions.As a result,the 3DCF@S with high sulfur content of 90%exhibits a high capacity of 1366 mA h/g at 0.1 C and excellent cycling stability with a satisfactory capacity of 601 mA h/g after 600 cycles at 2.0 C.The resultant Li-S button battery based 3DCF@S electrode could power a light-emitting diode for 2 h.The acquired 3DCF@S is expected to be widely used in Li-S batteries and this study will promote developments of carbon/sulfur composites for Li-S batteries.
基金supported by the National Natural Science Foundation of China (Grant Nos. 11072107 and 91016022)the Specialized Research Fund for the Doctoral Program of Higher Education of China (GrantNo.20093218110003)
文摘This article examines a viscoelastic plate that is driven parametrically by a non-Guassian colored noise,which is simplified to an Ornstein-Uhlenbeck process based on the approximation method.To examine the moment stability property of the viscoelastic system,we use the stochastic averaging method,Girsanov theorem and Feynmann-Kac formula to derive the approximate analytic expansion of the moment Lyapunov exponent.Furthermore,the Monte Carlo simulation results for the original system are given to check the accuracy of the approximate analytic results.At the end of this paper,results are presented to show some quantitative pictures of the effects of the system parameters,noise parameters and viscoelastic parameters on the stability of the viscoelastic plate.
基金the National Natural Science Foundation of China(Grant Nos.11772149,and 12172167)A Project Funded by the Priority Academic Program Development of Jiangsu Higher Education In-stitutions(PAPD)and The Research Fund of State Key Laboratory of Me-chanics and Control of Mechanical Structures(Grant No.MCMS-I-19G0l).
文摘The noise-induced transition of the augmented Lotka-Volterra system is investigated under vanishingly small noise.Populations will ultimately go extinct because of intrinsic noise,and different extinction routes may occur due to the Freidlin-Wentzell large deviation theory.The relation between the most probable extinction route(MPER)and heteroclinic bifurcation is studied in this paper.The MPERs and the quasi-potentials in different regimes of parameters are analyzed in detail.Before the bifurcation,the predator goes extinct,and the prey will survive for a long time.Then,the heteroclinic bifurcation changes the MPER wherein both species go extinct.The heteroclinic cycle plays a role in transferring the most probable extinction state.Moreover,the analyses of the weak noise limit can contribute to predicting the stochastic behavior under finite small noise.Both the heteroclinic bifurcation and the rotational deterministic vector field can reduce the action necessary for the MPER.