Zero-dimensional environmentally friendly carbon quantum dots(CQDs)combined with two-di-mensional materials have a wide range of applications in optoelec-tronic devices.We combined steady-state and transient absorp-ti...Zero-dimensional environmentally friendly carbon quantum dots(CQDs)combined with two-di-mensional materials have a wide range of applications in optoelec-tronic devices.We combined steady-state and transient absorp-tion spectroscopies to study the energy transfer dynamics between CQDs and molybdenum disulfide(MoS_(2)).Transient absorption plots showed photoinduced absorption and stimulated emission features,which involved the intrinsic and defect states of CQDs.Adding MoS_(2)to CQDs solution,the lowest unoccupied molecular orbital of CQDs transferred energy to MoS_(2),which quenched the intrinsic emission at 390 nm.With addition of MoS_(2),CQD-MoS_(2)composites quenched defect emission at 490 nm and upward absorption,which originated from another energy transfer from the defect state.Two energy transfer paths between CQDs and MoS_(2)were efficiently manipulated by changing the concentration of MoS_(2),which laid a foundation for improving device performance.展开更多
The effect of final-state dynamic correlation is investigated for ionization of atomic hydrogen by 75-keV proton impact by analyzing double differential cross sections.The final state is represented by a continuum cor...The effect of final-state dynamic correlation is investigated for ionization of atomic hydrogen by 75-keV proton impact by analyzing double differential cross sections.The final state is represented by a continuum correlated wave(CCW-PT)function which accounts for the interaction between the projectile and the target nucleus(PT interaction).The correlated final state is nonseparable solutions of the wave equation combining the dynamics of the electron motion relative to the target and projectile,satisfying the Redmond’s asymptotic conditions corresponding to long range interactions.The transition matrix is evaluated using the CCW-PT function and the undistorted initial state.Both the correlation effects and the PT interaction are analyzed by the present calculations.The convergence of the continuous correlated final state is examined carefully.Our results are compared with the absolute experimental data measured by Laforge et al.[Phys.Rev.Lett.103,053201(2009)]and Schulz et al.[Phys.Rev.A 81,052705(2010)],as well as other theoretical models(especially the results of the latest non perturbation theory).We have shown that the dynamic correlation plays an important role in the ionization of atomic hydrogen by proton impact.While overall agreement between theory and the experimental data is encouraging,detailed agreement is still lacking.However,such an analysis is meaningful because it provides valuable information about the dynamical correlation and PT interaction in the CCW-PT theoretical model.展开更多
基金supported by the National Natural Science Foundation of China(No.61805134 and No.11974229)Applied Basic Research Program in Shanxi Province,China(No.201801D221016 and No.202103021223254)+2 种基金Scientific and Technological Innovation Pro-grams of Higher Education Institutions in Shanxi(No.2020L0235 and No.2021L257)Linfen Key Re-search and Development Program(No.2028)Graduate Innovation Project in Shanxi Province(No.2022Y498).
文摘Zero-dimensional environmentally friendly carbon quantum dots(CQDs)combined with two-di-mensional materials have a wide range of applications in optoelec-tronic devices.We combined steady-state and transient absorp-tion spectroscopies to study the energy transfer dynamics between CQDs and molybdenum disulfide(MoS_(2)).Transient absorption plots showed photoinduced absorption and stimulated emission features,which involved the intrinsic and defect states of CQDs.Adding MoS_(2)to CQDs solution,the lowest unoccupied molecular orbital of CQDs transferred energy to MoS_(2),which quenched the intrinsic emission at 390 nm.With addition of MoS_(2),CQD-MoS_(2)composites quenched defect emission at 490 nm and upward absorption,which originated from another energy transfer from the defect state.Two energy transfer paths between CQDs and MoS_(2)were efficiently manipulated by changing the concentration of MoS_(2),which laid a foundation for improving device performance.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11974229 and 11274215)。
文摘The effect of final-state dynamic correlation is investigated for ionization of atomic hydrogen by 75-keV proton impact by analyzing double differential cross sections.The final state is represented by a continuum correlated wave(CCW-PT)function which accounts for the interaction between the projectile and the target nucleus(PT interaction).The correlated final state is nonseparable solutions of the wave equation combining the dynamics of the electron motion relative to the target and projectile,satisfying the Redmond’s asymptotic conditions corresponding to long range interactions.The transition matrix is evaluated using the CCW-PT function and the undistorted initial state.Both the correlation effects and the PT interaction are analyzed by the present calculations.The convergence of the continuous correlated final state is examined carefully.Our results are compared with the absolute experimental data measured by Laforge et al.[Phys.Rev.Lett.103,053201(2009)]and Schulz et al.[Phys.Rev.A 81,052705(2010)],as well as other theoretical models(especially the results of the latest non perturbation theory).We have shown that the dynamic correlation plays an important role in the ionization of atomic hydrogen by proton impact.While overall agreement between theory and the experimental data is encouraging,detailed agreement is still lacking.However,such an analysis is meaningful because it provides valuable information about the dynamical correlation and PT interaction in the CCW-PT theoretical model.
