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Petrogenesis of early Paleozoic granitoids in the North Qinling Orogen,Central China:Implications for crustal evolution in an accretionary orogen
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作者 Leran Hao Debin yang +3 位作者 Anqi Wang Yikang Quan xiangyu yan Shuo Wang 《Geoscience Frontiers》 SCIE CAS CSCD 2024年第2期183-201,共19页
Accretionary orogens are sites of extensive continental crustal growth and modification.The mechanism by which mafic crust is transformed into silicic melts(i.e.,maturation of continental crust)is important for unders... Accretionary orogens are sites of extensive continental crustal growth and modification.The mechanism by which mafic crust is transformed into silicic melts(i.e.,maturation of continental crust)is important for understanding the formation of the continental crust.The North Qinling Orogen(NQO)is a composite orogenic belt and contains an early Paleozoic accretion-dominated orogenic system,which is ideal for investigating continental crustal maturation.We obtained zircon and monazite U–Pb age and O isotope data,zircon Lu–Hf isotope data,and whole-rock major-and trace-element and Sr–Nd isotope data for early Paleozoic granitoids of the NQO.The granitoids are divided into three groups.Group 1 includes the Taiping tonalite(445±3 Ma),the Manziying syenogranite(445±2 Ma),and the Huoshenmiao granodiorite(436±2 Ma).The Taiping and Huoshenmiao plutons have relatively high SiO_(2)contents(68.64–71.67 wt.%)and Na_(2)O/K_(2)O ratios(1.15–4.19),with enrichments in Rb,Ba,Th,and U and depletions in Nb,Ta,P,and Ti,and they are geochemically similar to sodic arc magmas.The Manziying syenogranite is a peraluminous potassic granite with high K_(2)O contents(4.59–5.27 wt.%).Grantioids from Group 1 have similarly depleted Sr–Nd–Hf–O isotopic features(eHf[t]=+5.9 to+8.8;δ^(18)O=3.98‰–5.41‰),indicative of derivation via partial melting of oceanic arc crust,which suggests that partial melting of oceanic arc crust in a subduction system contributes to the generation of continental crust and causes its maturation.Group 2 consists of the Wuduoshan monzogranite(418±2 Ma)and the Sikeshu granodiorite(423±3 Ma).These plutons have relatively high SiO_(2)(65.59–72.06 wt.%),K_(2)O(3.26–4.79 wt.%),and Al2O3(14.65–16.12 wt.%)contents and Sr/Y(33–87)and(La/Yb)N(23–48)ratios.The Wuduoshan monzogranite has positive zircon eHf(t)(+0.4 to+3.1)and uniformδ^(18)O(6.38‰–8.07‰)values,but the Sikeshu granodiorite has more variable isotopic compositions(eHf[t]=-1.9 to+5.0;δ^(18)O=6.37‰–10.60‰).The Wuduoshan monzogranite and Sikeshu granodiorite have similar whole-rock Sr–Nd isotopic compositions to basement rocks of the NQO.These features indicate that the two plutons formed by partial melting of basement rocks(i.e.,subducted into the lower crust)of the North Qinling unit,along with juvenile crustal material.Group 3 is represented by the Xiaguan monzogranite,which formed at 434–430 Ma,and can be subdivided into heavy rare earth element(REE)-depleted and-enriched units.The former has high Sr/Y(56–98)and(La/Yb)_(N)(34–73)ratios and low MgO(0.13–0.24 wt.%),Cr(0.37–1.69 ppm),and Ni(0.32–1.09 ppm)contents,similar to adakites derived from metabasaltic sources.The heavy REE-enriched nature of the Xiaguan monzogranite may reflect modification of its source by melt or fluid.Our results show that partial melting of enriched oceanic arc crust contributed to crustal maturation in an accretionary orogen.The addition of evolved crustal material also facilitated this process;therefore,the basement rocks and crustal thickness should be considered when assessing crustal dynamics in an accretionary orogen. 展开更多
关键词 Zircon Hf-O isotopes GRANITE Continental crust Accretionary orogen
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装配式村镇住宅轻钢框架结构设计与研究
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作者 陈志华 孙克肇 +3 位作者 周婷 闫翔宇 肖潇 张莫凡 《钢结构(中英文)》 2023年第9期28-36,共9页
在乡村振兴、双碳目标、建筑产业升级、装配式的大背景下,我国村镇经济实现了突飞猛进的发展。在住宅建设热潮的推动下,村镇住宅的发展从量的增加转变为质的提高,居住条件和建设质量的改善越来越成为村镇住宅下一阶段发展的必然要求。... 在乡村振兴、双碳目标、建筑产业升级、装配式的大背景下,我国村镇经济实现了突飞猛进的发展。在住宅建设热潮的推动下,村镇住宅的发展从量的增加转变为质的提高,居住条件和建设质量的改善越来越成为村镇住宅下一阶段发展的必然要求。轻钢框架结构体系具有构件轻便、易于运输、抗震性能优良的特点,适用于村镇地区低层住宅。但已有的焊接、栓接的连接方式不满足低成本、简易施工的预期目的。为此,从村镇地区落后的运输条件和施工条件的立足点出发,提出了一种新型村镇轻钢框架结构体系,包括自攻螺钉连接节点、方钢管组合异形柱等。结合德胜村装配式村镇住宅钢结构房屋,研究了新型体系的结构设计和节点设计方法,详细介绍了其设计与施工过程中所采用的关键技术,包括装配式村镇住宅BIM正向设计技术、简易施工异形柱装配技术、装配化螺旋钢桩承台节点技术、节点简易化连接与安装技术。结果表明:这种新型体系结构设计指标满足相关规范要求,安全可靠;采用范围修正后的英国规范计算的螺钉抗剪承载力和欧洲规范计算的螺钉抗拔承载力,均比实际试验值略小,工程应用偏于安全;所提出的关键技术满足村镇住宅绿色环保、简易施工、经济效益优的内在要求,适于在村镇地区推广应用。 展开更多
关键词 自攻螺钉连接 装配式 村镇住宅 轻钢框架结构
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钢框架-网格墙结构分析与设计
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作者 闫翔宇 张莫凡 +3 位作者 王丹妮 陈志华 李晓斐 王彬 《钢结构(中英文)》 2023年第9期19-27,共9页
网格墙结构是将钢板墙网格化得到的一种新型抗侧力体系,具有抗震性能好、焊接工作量小、构件加工和运输方便、施工安装便捷等优势,符合当前大力发展装配式钢结构的政策要求。目前对网格墙结构的研究主要集中在力学性能方面,但其在实际... 网格墙结构是将钢板墙网格化得到的一种新型抗侧力体系,具有抗震性能好、焊接工作量小、构件加工和运输方便、施工安装便捷等优势,符合当前大力发展装配式钢结构的政策要求。目前对网格墙结构的研究主要集中在力学性能方面,但其在实际工程设计中尚未得到应用。为探索其在实际工程中应用的可行性,以兰州新区保障性住房建设项目(二期)9号楼的钢框架-钢板剪力墙结构为背景,采用钢框架-网格墙结构进行了结构布置与设计,在YJK和MIDAS/Gen软件中建立了结构计算模型,并在相同技术参数和荷载条件下进行了整体结构分析、构件承载力验算以及关键节点设计与分析。在YJK和MIDAS/Gen中对钢框架-网格墙结构进行弹性分析,得到结构的整体指标,并与原钢框架-钢板剪力墙结构的整体指标进行对比,结果表明:钢框架-网格墙结构抗侧力构件沿平面、立面布置规则,两种软件所得各项指标比较接近且均满足JGJ 99-2015《高层民用建筑钢结构技术规程》和GB 50011-2010《建筑抗震设计规范》的要求,虽然其抗侧刚度略低于钢框架-钢板剪力墙结构,但钢网格墙的用钢量和焊接工程量均低于相应的钢板剪力墙。对构件承载力进行验算时,由于钢网格墙T型钢构件计算长度算法尚不明确,无法采用一阶弹性分析法进行构件稳定性计算,因而采用直接分析法对构件进行了验算,考虑整体初始缺陷和构件初始缺陷,进行各荷载组合下的非线性分析,结果表明:所有钢构件的强度应力比均小于1.0,构件承载力满足GB 50017-2017《钢结构设计标准》要求。鱼尾板作为T型钢与边缘构件间的连接构件,对钢网格墙耗能性能的发挥至关重要,为确保连接的可靠性,对鱼尾板的力学性能进行深入分析,在有限元软件ABAQUS中建立该钢网格墙的3层局部子结构精细化有限元模型,施加荷载包络组合作用下的柱顶内力、梁上荷载以及各层柱顶侧向位移后进行分析,结果表明,在设计荷载下鱼尾板、T型钢构件、边缘构件均不出现屈服,继续侧向加载至鱼尾板出现屈服时,此时大部分T型钢构件、梁端以及底层柱脚受压侧早已经出现截面屈服,满足“强节点、弱构件”的设计要求。 展开更多
关键词 钢网格墙 装配式建筑 抗侧性能 直接分析设计法 节点分析
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轻钢框架-网格墙结构施工关键技术及抗侧性能研究
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作者 刘子杰 闫翔宇 +4 位作者 张莫凡 杨艳 陈志华 贾莉 芦燕 《钢结构(中英文)》 2023年第9期45-52,共8页
随着新型城镇化的推进,装配式钢结构建筑比例逐年提高,但是现有钢结构体系用于村镇建筑时存在着住宅品质不优、构件标准化程度低、运输安装不便、建造质量低下、污染及浪费严重等问题,亟需研发低成本、易安装、生态化的村镇装配式住宅... 随着新型城镇化的推进,装配式钢结构建筑比例逐年提高,但是现有钢结构体系用于村镇建筑时存在着住宅品质不优、构件标准化程度低、运输安装不便、建造质量低下、污染及浪费严重等问题,亟需研发低成本、易安装、生态化的村镇装配式住宅轻钢结构体系以及相应的建造技术。轻钢框架-网格墙结构不仅具有抗震性能优良、构件轻便、易于运输的优点,而且节点可采用完全装配式的螺栓连接或自攻螺钉连接,施工安装简便。为了研究这种结构形式的简易施工关键技术以及抗侧性能,建造了一栋采用全螺钉连接的轻钢框架-钢、木、竹网格墙混合结构体系的单层房屋,并对其进行了原位试验。以该工程中的一榀轻钢框架-网格墙为例,从柱脚、基础、框架安装、钢网格墙安装、墙板安装等方面阐述轻钢框架-网格墙的简易施工建造技术,并通过原位静力试验得到了其抗侧性能。研究表明,这种轻钢框架-网格墙易于安装,能够节省人力物力,适于在村镇地区推广应用,且采用该建造技术完成的轻钢框架-网格墙结构的抗侧性能能够满足设计要求。 展开更多
关键词 网格墙结构 施工关键技术 原位试验 自攻螺钉节点
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气力输送关键装置及管内流动特性研究现状及展望 被引量:1
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作者 周甲伟 闫翔宇 +2 位作者 郑泽冰 王庆辉 上官林建 《过程工程学报》 CAS CSCD 北大核心 2023年第5期649-661,共13页
气力输送具有清洁安全、空间集约、配置灵活且易于自动化等特点,是颗粒类散体物料常用的绿色输送技术,在化工、食品、制药、能源等多个领域得到广泛应用。同时,该技术也存在输送工艺复杂、颗粒输送状态瞬变且难以准确预测等难题,采用不... 气力输送具有清洁安全、空间集约、配置灵活且易于自动化等特点,是颗粒类散体物料常用的绿色输送技术,在化工、食品、制药、能源等多个领域得到广泛应用。同时,该技术也存在输送工艺复杂、颗粒输送状态瞬变且难以准确预测等难题,采用不同输送工艺时物料输送特性的多手段表征和预测一直是该技术的研究热点。本文在综述气力输送系统构成、常用供料装置结构特点的基础上,对计算流体力学与离散元耦合(CFD-DEM)数值模拟方法、常用测量装置和分析方法在气力输送特性研究的应用进行归纳,总结了当前气力输送流型演变、输送系统压力损失等输送特性的相关研究成果,并对气力输送研究进行展望,讨论了未来研究需关注的几个思考点。 展开更多
关键词 气力输送 实验测量 计算流体力学和离散单元耦合 输送流型 压力损失
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外加酶强化剩余污泥与厨余垃圾渗滤液混合厌氧消化
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作者 薛同站 孙鑫 +4 位作者 李卫华 刘晓吉 王坤 闫祥宇 杨厚云 《过程工程学报》 CAS CSCD 北大核心 2023年第8期1208-1219,共12页
为了研究水解酶对剩余污泥和厨余垃圾渗滤液混合厌氧消化产气性能的影响,以城市污水处理厂剩余污泥和厨余垃圾渗滤液为底物,在混合比为1:1和2:1混合液中分别加入比例为1:1,1:2和2:1 (总酶加入量60 mg/g TS)的蛋白酶和纤维素酶,在38±... 为了研究水解酶对剩余污泥和厨余垃圾渗滤液混合厌氧消化产气性能的影响,以城市污水处理厂剩余污泥和厨余垃圾渗滤液为底物,在混合比为1:1和2:1混合液中分别加入比例为1:1,1:2和2:1 (总酶加入量60 mg/g TS)的蛋白酶和纤维素酶,在38±0.5℃的温度下进行混合厌氧消化。结果表明,在剩余污泥与厨余垃圾渗滤液2:1混合厌氧消化体系中1:1投加蛋白酶和纤维素酶时产气性能和处置效果最佳。其日产甲烷峰值为60.15 mL/g VS,比单独消化污泥提高了1.84倍,比同底物不加酶时提高了70.49%;甲烷总产量为296.17 mL/g VS,比单独消化污泥提高了75.99%,比同底物不加酶时提高了62.87%;总固体(TS)和挥发性固体(VS)去除率分别为41.43%和67.32%,比单独消化污泥分别提高了14.74和27.89个百分点,比同组不加酶的混合液分别提高了8.34和21.99个百分点,且消化过程中没有出现氨抑制和挥发性脂肪酸(VFAs)积累的状况。利用三维激发矩阵荧光光谱结合平行因子法分析,发现混合厌氧消化过程中存在的荧光物质主要有类蛋白质、类富里酸和类胡敏酸,在消化的不同时间段蛋白质荧光强度存在明显差异,加酶的实验组中这一变化更加显著。此结果可为剩余污泥和厨余垃圾的减量化和资源化提供借鉴。 展开更多
关键词 水解酶 剩余污泥 厨余垃圾渗滤液 厌氧消化 三维激发矩阵荧光光谱
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Cost-effectiveness analysis on COVID-19 surveillance strategy of large-scale sports competition 被引量:2
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作者 Xuechun Wang Yiru Cai +6 位作者 Bo Zhang xiangyu Zhang Lianhao Wang xiangyu yan Mingchen Zhao Yuan Zhang Zhongwei Jia 《Infectious Diseases of Poverty》 SCIE 2022年第2期53-62,共10页
Background:Nucleic acid test(NAT)could effectively control the spread of COVID-19 caused by large-scale sports competitions.However,quantitative analysis on the appropriate frequency of NAT is scarce,and the cost-effe... Background:Nucleic acid test(NAT)could effectively control the spread of COVID-19 caused by large-scale sports competitions.However,quantitative analysis on the appropriate frequency of NAT is scarce,and the cost-effectiveness and necessity of high-frequency NAT remain to be fully explored and validated.This study aims to optimize the COVID-19 surveillance strategies through cost-effectiveness analysis for the Tokyo 2020 Olympic Games and the upcoming Beijing 2022 Olympic Winter Games.Methods:A total of 18 scenarios were designed regarding the NAT frequency,symptom monitoring,and strengthening close-contact control.An agent-based stochastic dynamic model was used to compare the cost-effectiveness of different NAT scenarios and optimize the surveillance strategies.The dynamics of the proposed model included the arrival and departure of agents,transmission of the disease according to Poisson processes,and quarantine of agents based on regular NATs and symptom onset.Accumulative infections,cost,and incremental cost-effectiveness ratio(ICER)were simulated in the frame of the model.ICER was used to compare the cost-effectiveness of different scenarios.Univariate sensitivity analysis was performed to test the robustness of the results.Results:In Scenario 16,where the competition-related personnel(CRP)received NAT daily and national sports delegation(NSD)with quarantined infections accepted an additional NAT daily,accumulative infection was 320.90(90 initial infections),the total cost was(United States Dollar)USD 8920000,and the cost of detecting out each infection was USD 27800.Scenario 16 would reduce the total cost by USD 22570000(avoid 569.61 infections),USD 1420000(avoid 47.2 infections)compared with Scenario 10(weekly NAT,strengthened close contact control)and Scenario 7(daily NAT,no strengthened close contact control),respectively.Sensitivity analysis showed that the result was most sensitive to the change in basic reproductive number.Conclusions:High-frequency NATs such as bidaily,daily,and twice a day were cost-effective.NAT daily for CRP with strengthening close-contact control could be prioritized in defense against COVID-19 at large-scale sports competitions.This study could assist policymakers by assessing the cost-effectiveness of NAT scenarios and provide the host country with an optimal COVID-19 surveillance strategy. 展开更多
关键词 COST-EFFECTIVENESS Sports competition SURVEILLANCE COVID-19 Nucleic acid test Stochastic dynamic model
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Exploring the Bridge Cases’Role in the Transmission of the SARSCoV-2 Delta Variant—Ruili City,Yunnan Province,China,July–September 2021 被引量:4
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作者 xiangyu yan Litao Chang +4 位作者 Zekun Wang Linhui Hao Zhongwei Jia Bo Zhang Tiejun Shui 《China CDC weekly》 2021年第50期1065-1070,共6页
Summary What is already known about this topic?The severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)Delta variant has proved to have increased transmissibility,and mutations that can cause partial immune esc... Summary What is already known about this topic?The severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)Delta variant has proved to have increased transmissibility,and mutations that can cause partial immune escape,which makes its transmission more insidious.What is added by this report?This study showed that probable cases who had negative results in nucleic acid testing but had positive IgM test result and/or IgG test value of over 20 S/CO in antibodies testing. 展开更多
关键词 DELTA testing value
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Operando optical fiber monitoring of nanoscale and fast temperature changes during photo-electrocatalytic reactions 被引量:1
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作者 ZHI LI YONGGUANG XIAO +8 位作者 FU LIU xiangyu yan DAOTONG YOU KAIWEI LI LIXI ZENG MINGSHAN ZHU GAOZHI XIAO JACQUES ALBERT TUAN GUO 《Light(Science & Applications)》 SCIE EI CAS CSCD 2022年第9期2086-2097,共12页
In situ and continuous monitoring of thermal effects is essential for understanding photo-induced catalytic processes at catalyst's surfaces.However,existing techniques are largely unable to capture the rapidly ch... In situ and continuous monitoring of thermal effects is essential for understanding photo-induced catalytic processes at catalyst's surfaces.However,existing techniques are largely unable to capture the rapidly changing temperatures occurring in sub-μm layers at liquid-solid interfaces exposed to light.To address this,a sensing system based on a gold-coated conventional single-mode optical fiber with a tilted fiber Bragg grating inscribed in the fiber core is proposed and demonstrated.The spectral transmission from these devices is made up of a dense comb of narrowband resonances that can differentiate between localized temperatures rapid changes at the catalyst's surface and those of the environment.By using the gold coating of the fiber as an electrode in an electrochemical reactor and exposing it to light,thermal effects in photo-induced catalysis at the interface can be decoded with a temperature resolution of 0.1℃and a temporal resolution of 0.1 sec,without perturbing the catalytic operation that is measured simultaneously.As a demonstration,stable and reproducible correlations between the light-to-heat conversion and catalytic activities over time were measured for two different catalysis processes(linear and nonlinear).These kinds of sensing applications are ideally suited to the fundamental qualities of optical fiber sensors,such as their compact size,flexible shape,and remote measurement capability,thereby opening the way for various thermal monitoring in hard-to-reach spaces and rapid catalytic reaction processes. 展开更多
关键词 CATALYSIS CATALYST thereby
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一种适用于非圆形建筑平面的新型球面弦支穹顶结构静力性能研究
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作者 闫翔宇 巩昊 +4 位作者 张起舞 于敬海 陈志华 王少华 王政凯 《钢结构(中英文)》 2021年第4期1-10,共10页
现有球面弦支穹顶结构主要适用于平面投影为标准圆形的建筑,其结构周圈的支座位于同一标高。当建筑要求的平面为多边形或者由多段不同直径圆弧构成的不规则曲线形状时,现有常规的球面弦支穹顶布置形式无法满足该类建筑的需求。为研究球... 现有球面弦支穹顶结构主要适用于平面投影为标准圆形的建筑,其结构周圈的支座位于同一标高。当建筑要求的平面为多边形或者由多段不同直径圆弧构成的不规则曲线形状时,现有常规的球面弦支穹顶布置形式无法满足该类建筑的需求。为研究球面弦支穹顶在平面投影为多边形或多段圆弧构成的非标准圆形建筑中的适用性,介绍了一种新型球面弦支穹顶结构体系,该体系适用于非圆建筑平面,通过采用位于不同标高内的支座将受力性能较好的球面弦支穹顶结构应用到平面投影不规则的建筑中。其平面投影轮廓轴线由八段圆弧组成,长轴尺寸89.89 m,短轴尺寸82.674 m,短轴方向矢高4.104 m,长轴方向矢高4.876 m。上层单层网壳采用K8+联方型网格布置,共设置了五道环索和撑杆。研究了矢跨比、撑杆长度、环索初拉力、环索截面积和支座水平刚度等参数变化对该新型弦支穹顶结构的结构位移、杆件内力和支座反力等静力性能的影响规律。研究结果表明:1)随着短轴矢跨比、撑杆长度、环索初拉力、环索截面积和支座水平刚度的增大,新型球面弦支穹顶结构最大竖向位移减小。2)网壳最大轴力随着撑杆长度、环索初拉力、环索截面积和支座水平刚度的增大而减小,不随短轴矢跨比变化。撑杆内力和环索内力随着短轴矢跨比和支座水平刚度的增大而减小,随着环索初拉力的增大而增大,随着撑杆长度和环索截面积变化复杂。环索节点不平衡力随着短轴矢跨比、撑杆长度和支座水平刚度的增大而减小,随着环索初拉力和环索截面积的增大而增大。3)随着短轴矢跨比增大,支座水平反力基本不变,而支座竖向反力减小;随着撑杆长度和环索截面积的增加,支座水平反力减小,而支座竖向反力增加;随着环索初拉力的增大,支座水平反力、支座竖向反力值减小;随着支座水平刚度的增大,支座水平反力增大,而支座竖向反力减小。 展开更多
关键词 结构工程 新型球面弦支穹顶 静力性能 参数化分析 非圆形建筑平面
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Association between Drug Co-use Networks and HIV Infection:A Latent Profile Analysis in Chinese Mainland 被引量:1
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作者 Bo Zhang xiangyu yan +3 位作者 Yongjie Li He Zhu Zuhong Lu Zhongwei Jia 《Fundamental Research》 CAS 2021年第5期552-558,共7页
Persons who use drugs are a high-risk subpopulation for HIV infection because more than one drug user often take drugs together,which increases the risk of HIV transmission.For the PWUDs who had tested for HIV,we extr... Persons who use drugs are a high-risk subpopulation for HIV infection because more than one drug user often take drugs together,which increases the risk of HIV transmission.For the PWUDs who had tested for HIV,we extracted data on demographic characteristics,drug types,injection drug use behavior,encrypted IDs of co-users,and drug use location from the National Dynamic Management and Control Database for Persons Who Use Drugs between January 2008 and July 2016.We mapped and classified Co-UDs’networks and estimated the risk of HIV infection.Drug co-use networks were formulated on the basis of connections between PWUDs at the same time and location.Latent profile analysis(LPA)and logistic regression models were used to cluster the classes and to estimate the HIV infection risk among them,respectively.A total of 470967 PWUDs were included,among whom 69529 Co-UDs formed 7001 networks,which were categorized into three classes:Class A(n=211,3.0%)had large networks,with more members(median 10.0(IQR:8.0-14.5)),and comprised depressant and stimulant users located in central and eastern China;Class B(n=3770,53.8%)was dominated by depressant users(median 3.0(IQR:3.0-4.0))across the country;Class C(n=3020,43.1%)was dominated by stimulant users(median 3.0(IQR:3.0-4.0))located in central and eastern China.The HIV infection rates were 9.71%,3.33%,and 0.33%in Classes A,B,and C,respectively.Compared with Class A,Classes B and C were associated with decreased odds of HIV infection.Our findings suggest that more attention should be paid to larger networks,with a relatively high HIV infection risk,to enhance prevention and intervention strategies. 展开更多
关键词 Network Persons who use drugs HIV Depressant STIMULANT China
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Microwave hydrothermal synthesis of lanthanum oxyfluoride nanorods for photocatalytic nitrogen fixation:Effect of Pr doping
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作者 xiangyu yan Da Dai +4 位作者 Kun Ma Shixiang Zuo Wenjie Liu Xiazhang Li Chao Yao 《Frontiers of Materials Science》 SCIE CSCD 2020年第1期43-51,共9页
Photocatalytic fixation of nitrogen has been recognized as a green and promising strategy for ammonia synthesis under ambient conditions.However,the efficient reduction of nitrogen remains a challenge due to high acti... Photocatalytic fixation of nitrogen has been recognized as a green and promising strategy for ammonia synthesis under ambient conditions.However,the efficient reduction of nitrogen remains a challenge due to high activation energy of nitrogen and low utilization of solar energy.Herein,lanthanum oxyfluoride with different doping content of Pr3+(LaOF:xPr3+)upconversion nanorods were synthesized by microwave hydrothermal method.Results indicated that the doping of Pr3+generated considerable defects on the surface of LaOF which acted as the adsorption and activation center for nitrogen.Meanwhile,the Pr3+ion narrowed the band gap and broadened the light response range of LaOF because LaOF:Pr3+can upconvert visible light into ultraviolet light,which excite LaOF nanorods and improve the utilization of solar light.The doping amount of Pr3+had critical effect on the photocatalytic nitrogen fixation performance which reached as high as 180μmol·L?1·ho1 when the molar ratio of Pr3+to LaOF was optimized to be 2%. 展开更多
关键词 LaOF defect UPCONVERSION photocatalysis nitrogen FIXATION
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Construction of upconversion fluoride/attapulgite nanocomposite for visible-light-driven photocatalytic nitrogen fixation
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作者 Xuhua YE xiangyu yan +4 位作者 Xini CHU Shixiang ZUO Wenjie LIU Xiazhang LI Chao YAO 《Frontiers of Materials Science》 SCIE CSCD 2020年第4期469-480,共12页
Developing photocatalysts with wide spectrum absorption and strong nitrogen activation is critical for nitrogen fixation under mild conditions.Herein,one-dimensional natural clay attapulgite(ATP)supported YFg:Sm^3+wer... Developing photocatalysts with wide spectrum absorption and strong nitrogen activation is critical for nitrogen fixation under mild conditions.Herein,one-dimensional natural clay attapulgite(ATP)supported YFg:Sm^3+were successfully synthesized via microwave hydrothermal method,and the composites were employed as the catalyst for photocatalytic nitrogen fixation under visible-light irradiation.Results indicated that the production of ammonia reached as high as 41.2 mg·L^-1 within 3 h when the molar ratio of Sm^3+and the mass fraction of YF3:Sm^3+were optimized.The enhanced fixation performance is mainly due to that the modified ATP fibber with abundant active sites and the doped fluoride with defective vacancy facilitate the adsorption and activation of N2.Furthermore,the upconversion property of YF3:Sm^3+increases the harvesting of visible-light energy,meanwhile the Z-scheme heterostructure built between YF:Sm^3+and modified ATP inhibits the recombination of charge carriers and retains high redox potentials for N2 reduction. 展开更多
关键词 photocatalysis nitrogen fixation ATTAPULGITE UPCONVERSION Z-scheme
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COVID-19 Vaccination Rates of People Who Use Drugs—Chengdu City,Sichuan Province,China,November 2021–February 2022
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作者 Erri Du Pengyu Jiang +4 位作者 Chaowei Zhang Shan Zhang xiangyu yan Yongjie Li Zhongwei Jia 《China CDC weekly》 2022年第37期817-822,I0002,共7页
What is already known about this topic?Few studies have reported that people who use drugs(PWUDs)have much lower coronavirus disease 2019(COVID-19)vaccination rates than the general population,especially with no relat... What is already known about this topic?Few studies have reported that people who use drugs(PWUDs)have much lower coronavirus disease 2019(COVID-19)vaccination rates than the general population,especially with no relative information reported in China specifically.What is added by this report?This study seminally uncovers that the vaccination rate among PWUDs was about 79.34%in one district of Chengdu City,Sichuan Province,China.Assuming that unvaccinated PWUDs with disease records were really not eligible for vaccination,the vaccination rate goes up to 87.25%among the studied PWUDs.The study implies that PWUDs were not left behind in the vaccination drive against COVID-19 in China.What are the implications for public health practice?In pandemics like COVID-19,government leadership and the overall planning and distribution of public health products are critical in achieving national health equity.However,in order to do this as well as avoid discrimination or exclusion among specific portions of the general population,it’s necessary to understand the vaccination rates and behaviors of at-risk groups such as PWUD’s. 展开更多
关键词 VACCINATION Chengdu DISTRICT
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Internet Data for Improving Prevention and Control of Global Infectious Diseases
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作者 Zhongwei Jia xiangyu yan +1 位作者 Yongjie Li Jiaqi Ma 《China CDC weekly》 2020年第52期1009-1012,共4页
By the end of 2018,there were about 5.1 billion internet users worldwide who accounted for 67%of the total population(1).Health problems have emerged following widespread use of the internet as a new model of social a... By the end of 2018,there were about 5.1 billion internet users worldwide who accounted for 67%of the total population(1).Health problems have emerged following widespread use of the internet as a new model of social activity,such as anonymous personal attacks or abuse and information leakages.A more potent threat is the unverified information being provided by the internet or electronic media that can lead to unsubstantiated judgments and improper responses to information regarding an individual’s health status. 展开更多
关键词 INTERNET INTERNET INDIVIDUAL
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