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聚甲基苄基二烯丙基氯化铵的制备及脱色性能
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作者 孙运通 张秀娟 +2 位作者 陶贤平 贾旭 张跃军 《高分子材料科学与工程》 EI CAS CSCD 北大核心 2019年第9期1-7,共7页
通过水溶液聚合法,采用引发剂一次性加入三阶段升温工艺,以甲基苄基二烯丙基氯化铵(DAMBAC)为单体,偶氮二异丁脒盐酸盐(V-50)为引发剂,乙二胺四乙酸四钠盐(Na4EDTA)为金属离子络合剂,对聚甲基苄基二烯丙基氯化铵(PDAMBAC)制备工艺条件... 通过水溶液聚合法,采用引发剂一次性加入三阶段升温工艺,以甲基苄基二烯丙基氯化铵(DAMBAC)为单体,偶氮二异丁脒盐酸盐(V-50)为引发剂,乙二胺四乙酸四钠盐(Na4EDTA)为金属离子络合剂,对聚甲基苄基二烯丙基氯化铵(PDAMBAC)制备工艺条件采用响应曲面优化法(RSM),得到聚合物最佳制备条件为:w(DAMBAC)=82.5%,m(V-50)∶m(DAMBAC)=3.03%,m(Na4EDTA)∶m(DAMBAC)=0.0147%,T1=61.8℃,T2=70.6℃和T3=85.0℃,各阶段均反应3 h。在实验范围内,各因素的影响顺序分别为T1>T2>T3、w(DAMBAC)>m(V-50)∶m(DAMBAC)>m(Na4EDTA)∶m(DAMBAC),得到聚合物重均相对分子质量(Mw)最高值为7.86×104,单体转化率(Conv.)为90.85%。模拟活性染料废水脱色性能对比实验表明,以脱色率为考察指标,该聚合物对活性染料模拟废水的脱色效果明显优于传统的二烯丙基季铵盐均聚物--聚二甲基二烯丙基氯化铵,PDAMBAC对3种活性染料的脱色率均达到了96.00%以上,最佳投加量条件下对C.I.活性红3BF、C.I.活性蓝KN-R和C.I.活性黄3RF染料的脱色率分别为96.01%、97.21%和99.70%,分别比PDMDAAC的脱色率高9.14%、56.64%和10.42%。 展开更多
关键词 甲基苄基二烯丙基氯化铵 均聚 响应曲面优化 相对分子质量 絮凝
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Towards a programming framework for activity-oriented context-aware applications
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作者 Xuansong LI xianping tao Jian LU 《Frontiers of Computer Science》 SCIE EI CSCD 2017年第6期987-1006,共20页
Context-aware system is an emerging research area in recent years. Context plays an important role in these systems. In most existing work, context is treated as all rel- ative elements in the environment of an applic... Context-aware system is an emerging research area in recent years. Context plays an important role in these systems. In most existing work, context is treated as all rel- ative elements in the environment of an application, and the scope of context is predefined by the developers during the development. However, it is difficult to analyze, specify, and organize everything in the environment accurately and com- pletely; and even when it is possible, the developed applica- tions are difficult to extend or modify as the requests for en- vironment may change over time. In this paper, we focus on activity-oriented context-aware (AOCA) applications where the requests for environment are highly dependent on user activities, and propose a programming framework for devel- oping AOCA applications. In particular, we first present a concept model for describing the notions of activity-oriented context. Next, based on the concept model, we describe the details of the programming framework as well as a develop- ment tool. Moreover, we provide a platform to support the runtime of AOCA applications, and demonstrate the advan- tages of our programming framework through experimental evaluations. 展开更多
关键词 pervasive computing context-awareness context-aware programming framework activity-orientedcontext
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