The single event effect(SEE) sensitivity of silicon–germanium heterojunction bipolar transistor(Si Ge HBT) irradiated by 100-Me V proton is investigated. The simulation results indicate that the most sensitive positi...The single event effect(SEE) sensitivity of silicon–germanium heterojunction bipolar transistor(Si Ge HBT) irradiated by 100-Me V proton is investigated. The simulation results indicate that the most sensitive position of the Si Ge HBT device is the emitter center, where the protons pass through the larger collector-substrate(CS) junction. Furthermore, in this work the experimental studies are also carried out by using 100-Me V proton. In order to consider the influence of temperature on SEE, both simulation and experiment are conducted at a temperature of 93 K. At a cryogenic temperature, the carrier mobility increases, which leads to higher transient current peaks, but the duration of the current decreases significantly.Notably, at the same proton flux, there is only one single event transient(SET) that occurs at 93 K. Thus, the radiation hard ability of the device increases at cryogenic temperatures. The simulation results are found to be qualitatively consistent with the experimental results of 100-Me V protons. To further evaluate the tolerance of the device, the influence of proton on Si Ge HBT after gamma-ray(^(60)Coγ) irradiation is investigated. As a result, as the cumulative dose increases, the introduction of traps results in a significant reduction in both the peak value and duration of the transient currents.展开更多
Neutron computed tomography(NCT)is widely used as a noninvasive measurement technique in nuclear engineering,thermal hydraulics,and cultural heritage.The neutron source intensity of NCT is usually low and the scan tim...Neutron computed tomography(NCT)is widely used as a noninvasive measurement technique in nuclear engineering,thermal hydraulics,and cultural heritage.The neutron source intensity of NCT is usually low and the scan time is long,resulting in a projection image containing severe noise.To reduce the scanning time and increase the image reconstruction quality,an effective reconstruction algorithm must be selected.In CT image reconstruction,the reconstruction algorithms can be divided into three categories:analytical algorithms,iterative algorithms,and deep learning.Because the analytical algorithm requires complete projection data,it is not suitable for reconstruction in harsh environments,such as strong radia-tion,high temperature,and high pressure.Deep learning requires large amounts of data and complex models,which cannot be easily deployed,as well as has a high computational complexity and poor interpretability.Therefore,this paper proposes the OS-SART-PDTV iterative algorithm,which uses the ordered subset simultaneous algebraic reconstruction technique(OS-SART)algorithm to reconstruct the image and the first-order primal–dual algorithm to solve the total variation(PDTV),for sparse-view NCT three-dimensional reconstruction.The novel algorithm was compared with other algorithms(FBP,OS-SART-TV,OS-SART-AwTV,and OS-SART-FGPTV)by simulating the experimental data and actual neutron projection experiments.The reconstruction results demonstrate that the proposed algorithm outperforms the FBP,OS-SART-TV,OS-SART-AwTV,and OS-SART-FGPTV algorithms in terms of preserving edge structure,denoising,and suppressing artifacts.展开更多
In radiation measurement and digital nuclear spectrum systems,traditional nuclear signal processing circuits in nuclear electronics have been gradually replaced by digital algorithm modules with the application of hig...In radiation measurement and digital nuclear spectrum systems,traditional nuclear signal processing circuits in nuclear electronics have been gradually replaced by digital algorithm modules with the application of highperformance programmable hardware logic devices(such as FPGA or DSP).Referring to the digital realization method of inverse RC integral circuit systems,the function of the pole-zero cancellation(PZC)circuit was analyzed,a new modified cascade equivalent model of PZC was established,and the time-domain digital PZC(DPZC)recursive algorithm was derived in detail in this study.Two parameters kIand k_(D)are included in the new algorithm,where kIshould match the exponential decay time constant of the input signal to realize the pole-zero compensation,while the decay time constant of the output signal can be changed with the adjustable parameter k_(D)(which is larger than the decay time constant of the input signal).Based on the new DPZC algorithm module,two trapezoidal(triangular)shaping filters were designed and implemented.The amplitude–frequency characteristics of the output signal of the proposed trapezoidal shaping algorithm and the convolution trapezoidal shaping algorithm were compared,with fixed peaking time.The results show that the trapezoidal shaping algorithm based on DPZC can better suppress high-frequency noise.Finally,based on the Na I(Tl)scintillator(u75 mm×75 mm)detector and^(137)Cs source,the effect of the k_(D)value on the energy resolution of the DPZC trapezoidal(triangular)shaping algorithm was studied.The experimental results show that,with an increase in k_(D),the energy resolution of the system improved and reached the maximum when k_(D)was greater than 10,and the optimal energy resolution of the system was 7.72%.展开更多
In order to investigate the effect of Ag doping(ZnS(Ag)) and Zn vacancy(V_(Zn)) on the alpha particle detection performance of wurtzite(WZ) ZnS as a scintillation cell component, the electronic structure and optical p...In order to investigate the effect of Ag doping(ZnS(Ag)) and Zn vacancy(V_(Zn)) on the alpha particle detection performance of wurtzite(WZ) ZnS as a scintillation cell component, the electronic structure and optical properties of ZnS, ZnS(Ag), and V_(Zn)were studied by firstprinciple calculation based on the density functional theory. The results show that the band gaps of ZnS, ZnS(Ag),and V_(Zn)are 2.17, 1.79, and 2.37 eV, respectively. Both ZnS(Ag) and V_(Zn)enhance the absorption and reflection of the low energy photons. A specific energy, about 2.9 eV,leading to decrease of detection efficiency is observed. The results indicate that Ag doping has a complex effect on the detection performance. It is beneficial to produce more visible light photons than pure WZ ZnS when exposed to the same amount of radiation, while the increase of the absorption to visible light photons weakens the detection performance. Zn vacancy has negative effect on the detection performance. If we want to improve the detection performance of WZ ZnS, Ag doping will be a good way,but we should reduce the absorption to visible light photons and control the number of Zn vacancy rigorously.展开更多
To investigate the damage profiles of high-fluence low-energy proton irradiation on superconducting materials and related devices, Raman characterization and electrical transport measurement of 40-keV-proton irradiate...To investigate the damage profiles of high-fluence low-energy proton irradiation on superconducting materials and related devices, Raman characterization and electrical transport measurement of 40-keV-proton irradiated YBa_2Cu_3O_(7-x)(YBCO) thin films are carried out. From micro-Raman spectroscopy and x-ray diffraction studies, the main component of proton-radiation-induced defects is found to be the partial transition of superconducting orthorhombic phase to the semiconducting tetragonal phase and non-superconducting secondary phase. The results indicate that the defects induced in the conducting CuO_2 planes, such as increased oxygen vacancies and interstitials, can result in an increase in the resistivity but a decrease in the transition temperature TCwith the increase in the fluence of proton irradiation, which is confirmed in the electrical transport measurements. Especially, zero-resistance temperature TC_0 is not observed at a fluence of 10^(15)p/cm^2.Furthermore, the variation of activation energy U_0 can be explained by the plastic-flux creep theory, which indicates that the plastic deformation and entanglement of vortices in a weakly pinned vortex liquid are caused by disorders of point-like defects. Point-like disorders are demonstrated to be the main contribution to the low-energy proton radiation damage in YBCO thin films. These disorders are likely to cause flux creep by thermally assisted flux flow, which may increase noise and reduce the precision of superconducting devices.展开更多
The most critical part of a neutron computed tomography(NCT) system is the image processing algorithm,which directly affects the quality and speed of the reconstructed images.Various types of noise in the system can d...The most critical part of a neutron computed tomography(NCT) system is the image processing algorithm,which directly affects the quality and speed of the reconstructed images.Various types of noise in the system can degrade the quality of the reconstructed images.Therefore,to improve the quality of the reconstructed images of NCT systems,efficient image processing algorithms must be used.The anisotropic diffusion filtering(ADF) algorithm can not only effectively suppress the noise in the projection data,but also preserve the image edge structure information by reducing the diffusion at the image edges.Therefore,we propose the application of the ADF algorithm for NCT image reconstruction.To compare the performance of different algorithms in NCT systems,we reconstructed images using the ordered subset simultaneous algebraic reconstruction technique(OS-SART) algorithm with different regular terms as image processing algorithms.In the iterative reconstruction,we selected two image processing algorithms,the Total Variation and split Bregman solved total variation algorithms,for comparison with the performance of the ADF algorithm.Additionally,the filtered back-projection algorithm was used for comparison with an iterative algorithm.By reconstructing the projection data of the numerical and clock models,we compared and analyzed the effects of each algorithm applied in the NCT system.Based on the reconstruction results,OS-SART-ADF outperformed the other algorithms in terms of denoising,preserving the edge structure,and suppressing artifacts.For example,when the 3D Shepp–Logan was reconstructed at 25 views,the root mean square error of OS-SART-ADF was the smallest among the four iterative algorithms,at only 0.0292.The universal quality index,mean structural similarity,and correlation coefficient of the reconstructed image were the largest among all algorithms,with values of 0.9877,0.9878,and 0.9887,respectively.展开更多
Lithium metal batteries(LMBs) are ideal candidates for next-generation high energy density energy storage systems.However,uncontrollable growth of Li dendrites due to uneven Li plating has restricted the practical app...Lithium metal batteries(LMBs) are ideal candidates for next-generation high energy density energy storage systems.However,uncontrollable growth of Li dendrites due to uneven Li plating has restricted the practical application of the Li metal anode.Here,we develop a highly lithiophilic Zn coating on commercial Cu foil as a substrate for Li metal anode to settle above issues.We find that the lithiophilic nature of Zn can facilitate homogeneous nucleation and deposition of Li on Cu current collector surface.In addition,the uniform Zn coating can not only decrease the nucleation overpotential but also regulate the electric field distribution.Benefiting from the coated Zn layer,the designed anode for half-cell and full-cell tests shows better electrochemical performances compared with the untreated Cu foil.This work provides a simple and effective way to enable a promising dendrite-free lithium metal anode for large-scale industrial applications.展开更多
Layer-by-layer polyelectrolyte self-assembly, a common method for preparing high-quality ultra-thin films, was employed to direct the self-assembly behavior of polystyrene-block-poly(methyl methacrylate)(PS-b-PMMA) bl...Layer-by-layer polyelectrolyte self-assembly, a common method for preparing high-quality ultra-thin films, was employed to direct the self-assembly behavior of polystyrene-block-poly(methyl methacrylate)(PS-b-PMMA) block copolymer for the first time. Differing from the previous neutral polymer brushes anchored to silicon substrates via chemical modification, polyelectrolyte multilayers(PEMs) were anchored by electrostatic interaction and provided a stable, smooth, and neutral interface. In the present study, PS-b-PMMA was deposited on poly(acrylamide hydrochloride)/poly(acrylic acid)(PAH/PAA) PEMs prepared by layer-by-layer self-assembly to successfully yield vertical nanodomains after thermal annealing. Seven layered PEMs revealed an excellent, smooth surface, with a low roughness of 0.6 nm. The periodic structure with interlamellar spacing of 47 nm was determined by grazing-incidence small-angle X-ray scattering(GISAXS). The morphology of the PS-b-PMMA nanodomains depended on the polyanion-to-polycation concentration ratio, which is related to the interaction between the block copolymer and the substrate. Our results demonstrate that layer-by-layer self-assembly is a helpful method for the phase separation of block polymers and the fabrication of vertical, ordered nanodomains.展开更多
Objective Neutron energy spectrum unfolding is a key technique for neutron detection.It is essentially an inversion problem.The GRAVEL algorithm has been widely used in this field,and the PRIP algorithm transforms neu...Objective Neutron energy spectrum unfolding is a key technique for neutron detection.It is essentially an inversion problem.The GRAVEL algorithm has been widely used in this field,and the PRIP algorithm transforms neutron energy spectrum unfolding into a typical nonnegative linear complementarity problem and solves it by interior point algorithm for potential reduction.Methods These two algorithms are applied to unfold several different neutron energy test spectra and actual D-T fusion neutron energy spectrum.Results and Conclusion By comparison,it can be concluded that the PRIP algorithm is highly computationally efficient and fast converging,and the GRAVEL algorithm solution results match up more with the expected results.展开更多
The current-mode-counting method is a new approach to observing transient processes,especially in transient nuclear fusion,based on the non-homogeneous Poisson process(NHPP)model.In this paper,a new measurement proces...The current-mode-counting method is a new approach to observing transient processes,especially in transient nuclear fusion,based on the non-homogeneous Poisson process(NHPP)model.In this paper,a new measurement process model of the pulsed radiation field produced by transient nuclear fusion is built based on the NHPP.A simulated measurement is performed using the model,and the current signal from the detector is obtained by simulation based on Poisson process thinning.The neutron time spectrum is reconstructed and is in good agreement with the theoretical value,with its maximum error of a characteristic parameter less than 2.3%.Verification experiments were carried out on a CPNG-6 device at the China Institute of Atomic Energy,with a detection system with a nanosecond response time.The experimental charge amplitude spectra are in good agreement with those obtained by the traditional counting mode,and the characteristic parameters of the time spectrum are in good agreement with the theoretical values.This shows that the current-mode-counting method is effective for the observation of transient nuclear fusion processes.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant Nos.61574171,61704127,11875229,51872251,and 12027813)。
文摘The single event effect(SEE) sensitivity of silicon–germanium heterojunction bipolar transistor(Si Ge HBT) irradiated by 100-Me V proton is investigated. The simulation results indicate that the most sensitive position of the Si Ge HBT device is the emitter center, where the protons pass through the larger collector-substrate(CS) junction. Furthermore, in this work the experimental studies are also carried out by using 100-Me V proton. In order to consider the influence of temperature on SEE, both simulation and experiment are conducted at a temperature of 93 K. At a cryogenic temperature, the carrier mobility increases, which leads to higher transient current peaks, but the duration of the current decreases significantly.Notably, at the same proton flux, there is only one single event transient(SET) that occurs at 93 K. Thus, the radiation hard ability of the device increases at cryogenic temperatures. The simulation results are found to be qualitatively consistent with the experimental results of 100-Me V protons. To further evaluate the tolerance of the device, the influence of proton on Si Ge HBT after gamma-ray(^(60)Coγ) irradiation is investigated. As a result, as the cumulative dose increases, the introduction of traps results in a significant reduction in both the peak value and duration of the transient currents.
基金supported by the National Key Research and Development Program of China(No.2022YFB1902700)the Joint Fund of Ministry of Education for Equipment Pre-research(No.8091B042203)+5 种基金the National Natural Science Foundation of China(No.11875129)the Fund of the State Key Laboratory of Intense Pulsed Radiation Simulation and Effect(No.SKLIPR1810)the Fund of Innovation Center of Radiation Application(No.KFZC2020020402)the Fund of the State Key Laboratory of Nuclear Physics and Technology,Peking University(No.NPT2023KFY06)the Joint Innovation Fund of China National Uranium Co.,Ltd.,State Key Laboratory of Nuclear Resources and Environment,East China University of Technology(No.2022NRE-LH-02)the Fundamental Research Funds for the Central Universities(No.2023JG001).
文摘Neutron computed tomography(NCT)is widely used as a noninvasive measurement technique in nuclear engineering,thermal hydraulics,and cultural heritage.The neutron source intensity of NCT is usually low and the scan time is long,resulting in a projection image containing severe noise.To reduce the scanning time and increase the image reconstruction quality,an effective reconstruction algorithm must be selected.In CT image reconstruction,the reconstruction algorithms can be divided into three categories:analytical algorithms,iterative algorithms,and deep learning.Because the analytical algorithm requires complete projection data,it is not suitable for reconstruction in harsh environments,such as strong radia-tion,high temperature,and high pressure.Deep learning requires large amounts of data and complex models,which cannot be easily deployed,as well as has a high computational complexity and poor interpretability.Therefore,this paper proposes the OS-SART-PDTV iterative algorithm,which uses the ordered subset simultaneous algebraic reconstruction technique(OS-SART)algorithm to reconstruct the image and the first-order primal–dual algorithm to solve the total variation(PDTV),for sparse-view NCT three-dimensional reconstruction.The novel algorithm was compared with other algorithms(FBP,OS-SART-TV,OS-SART-AwTV,and OS-SART-FGPTV)by simulating the experimental data and actual neutron projection experiments.The reconstruction results demonstrate that the proposed algorithm outperforms the FBP,OS-SART-TV,OS-SART-AwTV,and OS-SART-FGPTV algorithms in terms of preserving edge structure,denoising,and suppressing artifacts.
基金the financial supports from the National Natural Science Foundation of China(No.51701172)Educational Commission of Hunan Province,China(No.20B579)+2 种基金Major Program of Hunan Province,China(No.2018RS3091)China Postdoctoral Science Foundation(No.2018M632977)the Natural Science Foundation of Hunan Province,China(No.2018JJ3504).
基金supported by the National Natural Science Foundation of China(Nos.11975060,12005026,and 12075038)the Fund of Robot Technology Used for Special Environment Key Laboratory of Sichuan Province(No.19kftk02)。
文摘In radiation measurement and digital nuclear spectrum systems,traditional nuclear signal processing circuits in nuclear electronics have been gradually replaced by digital algorithm modules with the application of highperformance programmable hardware logic devices(such as FPGA or DSP).Referring to the digital realization method of inverse RC integral circuit systems,the function of the pole-zero cancellation(PZC)circuit was analyzed,a new modified cascade equivalent model of PZC was established,and the time-domain digital PZC(DPZC)recursive algorithm was derived in detail in this study.Two parameters kIand k_(D)are included in the new algorithm,where kIshould match the exponential decay time constant of the input signal to realize the pole-zero compensation,while the decay time constant of the output signal can be changed with the adjustable parameter k_(D)(which is larger than the decay time constant of the input signal).Based on the new DPZC algorithm module,two trapezoidal(triangular)shaping filters were designed and implemented.The amplitude–frequency characteristics of the output signal of the proposed trapezoidal shaping algorithm and the convolution trapezoidal shaping algorithm were compared,with fixed peaking time.The results show that the trapezoidal shaping algorithm based on DPZC can better suppress high-frequency noise.Finally,based on the Na I(Tl)scintillator(u75 mm×75 mm)detector and^(137)Cs source,the effect of the k_(D)value on the energy resolution of the DPZC trapezoidal(triangular)shaping algorithm was studied.The experimental results show that,with an increase in k_(D),the energy resolution of the system improved and reached the maximum when k_(D)was greater than 10,and the optimal energy resolution of the system was 7.72%.
基金supported by the National Natural Science Foundation of China(Nos.11275071 and 11305061)the Fundamental Research Funds for the Central Universities(Nos.2014MS53 and 2014ZZD09)the Student’s Platform for Innovation and Entrepreneurship Training Program of North China Electric Power University(No.15129)
文摘In order to investigate the effect of Ag doping(ZnS(Ag)) and Zn vacancy(V_(Zn)) on the alpha particle detection performance of wurtzite(WZ) ZnS as a scintillation cell component, the electronic structure and optical properties of ZnS, ZnS(Ag), and V_(Zn)were studied by firstprinciple calculation based on the density functional theory. The results show that the band gaps of ZnS, ZnS(Ag),and V_(Zn)are 2.17, 1.79, and 2.37 eV, respectively. Both ZnS(Ag) and V_(Zn)enhance the absorption and reflection of the low energy photons. A specific energy, about 2.9 eV,leading to decrease of detection efficiency is observed. The results indicate that Ag doping has a complex effect on the detection performance. It is beneficial to produce more visible light photons than pure WZ ZnS when exposed to the same amount of radiation, while the increase of the absorption to visible light photons weakens the detection performance. Zn vacancy has negative effect on the detection performance. If we want to improve the detection performance of WZ ZnS, Ag doping will be a good way,but we should reduce the absorption to visible light photons and control the number of Zn vacancy rigorously.
基金Project supported by the National Natural Science Foundation of China(Grant No.61473023)the Aerospace Science and Technology Innovation Fund,CASCInternational S&T Cooperation Program of China(ISTCP)(Grant No.2015DFR80190)
文摘To investigate the damage profiles of high-fluence low-energy proton irradiation on superconducting materials and related devices, Raman characterization and electrical transport measurement of 40-keV-proton irradiated YBa_2Cu_3O_(7-x)(YBCO) thin films are carried out. From micro-Raman spectroscopy and x-ray diffraction studies, the main component of proton-radiation-induced defects is found to be the partial transition of superconducting orthorhombic phase to the semiconducting tetragonal phase and non-superconducting secondary phase. The results indicate that the defects induced in the conducting CuO_2 planes, such as increased oxygen vacancies and interstitials, can result in an increase in the resistivity but a decrease in the transition temperature TCwith the increase in the fluence of proton irradiation, which is confirmed in the electrical transport measurements. Especially, zero-resistance temperature TC_0 is not observed at a fluence of 10^(15)p/cm^2.Furthermore, the variation of activation energy U_0 can be explained by the plastic-flux creep theory, which indicates that the plastic deformation and entanglement of vortices in a weakly pinned vortex liquid are caused by disorders of point-like defects. Point-like disorders are demonstrated to be the main contribution to the low-energy proton radiation damage in YBCO thin films. These disorders are likely to cause flux creep by thermally assisted flux flow, which may increase noise and reduce the precision of superconducting devices.
基金supported by the National Key Research and Development Program of China (No. 2022YFB1902700)the National Natural Science Foundation of China (No. 11875129)+3 种基金the Fund of the State Key Laboratory of Intense Pulsed Radiation Simulation and Effect (No. SKLIPR1810)Fund of Innovation Center of Radiation Application (No. KFZC2020020402)Fund of the State Key Laboratory of Nuclear Physics and Technology,Peking University (No. NPT2020KFY08)the Joint Innovation Fund of China National Uranium Co.,Ltd.,State Key Laboratory of Nuclear Resources and Environment,East China University of Technology (No. 2022NRE-LH-02)。
文摘The most critical part of a neutron computed tomography(NCT) system is the image processing algorithm,which directly affects the quality and speed of the reconstructed images.Various types of noise in the system can degrade the quality of the reconstructed images.Therefore,to improve the quality of the reconstructed images of NCT systems,efficient image processing algorithms must be used.The anisotropic diffusion filtering(ADF) algorithm can not only effectively suppress the noise in the projection data,but also preserve the image edge structure information by reducing the diffusion at the image edges.Therefore,we propose the application of the ADF algorithm for NCT image reconstruction.To compare the performance of different algorithms in NCT systems,we reconstructed images using the ordered subset simultaneous algebraic reconstruction technique(OS-SART) algorithm with different regular terms as image processing algorithms.In the iterative reconstruction,we selected two image processing algorithms,the Total Variation and split Bregman solved total variation algorithms,for comparison with the performance of the ADF algorithm.Additionally,the filtered back-projection algorithm was used for comparison with an iterative algorithm.By reconstructing the projection data of the numerical and clock models,we compared and analyzed the effects of each algorithm applied in the NCT system.Based on the reconstruction results,OS-SART-ADF outperformed the other algorithms in terms of denoising,preserving the edge structure,and suppressing artifacts.For example,when the 3D Shepp–Logan was reconstructed at 25 views,the root mean square error of OS-SART-ADF was the smallest among the four iterative algorithms,at only 0.0292.The universal quality index,mean structural similarity,and correlation coefficient of the reconstructed image were the largest among all algorithms,with values of 0.9877,0.9878,and 0.9887,respectively.
基金Project supported by the National Natural Science Foundation of China(No.51275450)the National Basic Research Program of China(973 Program)(No.2014CB046403)the Science Fund for Creative Research Groups of National Natural Science Foundation of China(No.51521064)
基金the National Natural Science Foundation of China(Nos.U1904216,51771236 and 51901249)the Innovation-Driven Project of Central South University(No.2020CX007)the Natural Science Foundation of Hunan Province(No.2020JJ5719)。
文摘Lithium metal batteries(LMBs) are ideal candidates for next-generation high energy density energy storage systems.However,uncontrollable growth of Li dendrites due to uneven Li plating has restricted the practical application of the Li metal anode.Here,we develop a highly lithiophilic Zn coating on commercial Cu foil as a substrate for Li metal anode to settle above issues.We find that the lithiophilic nature of Zn can facilitate homogeneous nucleation and deposition of Li on Cu current collector surface.In addition,the uniform Zn coating can not only decrease the nucleation overpotential but also regulate the electric field distribution.Benefiting from the coated Zn layer,the designed anode for half-cell and full-cell tests shows better electrochemical performances compared with the untreated Cu foil.This work provides a simple and effective way to enable a promising dendrite-free lithium metal anode for large-scale industrial applications.
基金financially supported by the National Natural Science Foundation of China (Nos. 11605149, 11405259, U1932118, and U1732123)the Natural Science Foundation of Hunan Province (No. 2017JJ3309)+3 种基金the China Postdoctoral Science Foundation (No. 2017 M622595)the Zhejiang Public Service Technology Research Program/Analytical Test (No. LGC19F040001)the National Key R&D Program of China (No. 2017YFA0403000)the Science and Technology Commission of Shanghai Municipality (No. 17JC1400802)
文摘Layer-by-layer polyelectrolyte self-assembly, a common method for preparing high-quality ultra-thin films, was employed to direct the self-assembly behavior of polystyrene-block-poly(methyl methacrylate)(PS-b-PMMA) block copolymer for the first time. Differing from the previous neutral polymer brushes anchored to silicon substrates via chemical modification, polyelectrolyte multilayers(PEMs) were anchored by electrostatic interaction and provided a stable, smooth, and neutral interface. In the present study, PS-b-PMMA was deposited on poly(acrylamide hydrochloride)/poly(acrylic acid)(PAH/PAA) PEMs prepared by layer-by-layer self-assembly to successfully yield vertical nanodomains after thermal annealing. Seven layered PEMs revealed an excellent, smooth surface, with a low roughness of 0.6 nm. The periodic structure with interlamellar spacing of 47 nm was determined by grazing-incidence small-angle X-ray scattering(GISAXS). The morphology of the PS-b-PMMA nanodomains depended on the polyanion-to-polycation concentration ratio, which is related to the interaction between the block copolymer and the substrate. Our results demonstrate that layer-by-layer self-assembly is a helpful method for the phase separation of block polymers and the fabrication of vertical, ordered nanodomains.
基金Financial supports from the Fundamental Research Funds for the Central Universities(No.2016XS61)National Natural Science Foundation of China(No.1150050900)the Opening Foundation of State Key Laboratory of Intense Pulsed Radiation Simulation and Effect are gratefully acknowledged.
文摘Objective Neutron energy spectrum unfolding is a key technique for neutron detection.It is essentially an inversion problem.The GRAVEL algorithm has been widely used in this field,and the PRIP algorithm transforms neutron energy spectrum unfolding into a typical nonnegative linear complementarity problem and solves it by interior point algorithm for potential reduction.Methods These two algorithms are applied to unfold several different neutron energy test spectra and actual D-T fusion neutron energy spectrum.Results and Conclusion By comparison,it can be concluded that the PRIP algorithm is highly computationally efficient and fast converging,and the GRAVEL algorithm solution results match up more with the expected results.
基金supported by the National Natural Science Foundation of China(No.51275450)the Fundamental Research Funds for the Central Universities(No.2013FZA4004)the Science Fund for Creative Research Groups of National Natural Science Foundation of China(No.51521064)
基金National Natural Science Foundation of China(1435010,11575145,11922507)。
文摘The current-mode-counting method is a new approach to observing transient processes,especially in transient nuclear fusion,based on the non-homogeneous Poisson process(NHPP)model.In this paper,a new measurement process model of the pulsed radiation field produced by transient nuclear fusion is built based on the NHPP.A simulated measurement is performed using the model,and the current signal from the detector is obtained by simulation based on Poisson process thinning.The neutron time spectrum is reconstructed and is in good agreement with the theoretical value,with its maximum error of a characteristic parameter less than 2.3%.Verification experiments were carried out on a CPNG-6 device at the China Institute of Atomic Energy,with a detection system with a nanosecond response time.The experimental charge amplitude spectra are in good agreement with those obtained by the traditional counting mode,and the characteristic parameters of the time spectrum are in good agreement with the theoretical values.This shows that the current-mode-counting method is effective for the observation of transient nuclear fusion processes.