The two-dimensional(2D) perovskite(including pure-2D and quasi-2D) is formed by introducing large-group ammonium halides into conventional bulk perovskite. In the past twenty years, 2D perovskite materials were wi...The two-dimensional(2D) perovskite(including pure-2D and quasi-2D) is formed by introducing large-group ammonium halides into conventional bulk perovskite. In the past twenty years, 2D perovskite materials were widely developed with the enriched species and advanced physicalknowledge in material characteristics as well as optoelectronic device applications. To review achievments in 2D perovskite,the fundamental mechanism and properties of 2D perovskite are introduced to offer insight into device performance.Moreover, the preparation methods of 2D perovskite films are summarized and compared. The latest successful applications of the 2D perovskite in the solar cells and light-emitting diodes fields, especially the advanced stability of 2D perovskite solar cells(PeSCs) and the efficient 2D perovskite lightemitting diodes(PeLEDs), are also achieved. Furthermore, the challenges and outlook of 2D perovskite materials are proposed.展开更多
基金supported by the National Key Research and Development Program of China (2016YFA0202401)the 111 Project (B16016)+1 种基金the National Natural Science Foundation of China (51572080, 51702096 and U1705256)the Fundamental Research Funds for the Central Universities (2017XS080)
文摘The two-dimensional(2D) perovskite(including pure-2D and quasi-2D) is formed by introducing large-group ammonium halides into conventional bulk perovskite. In the past twenty years, 2D perovskite materials were widely developed with the enriched species and advanced physicalknowledge in material characteristics as well as optoelectronic device applications. To review achievments in 2D perovskite,the fundamental mechanism and properties of 2D perovskite are introduced to offer insight into device performance.Moreover, the preparation methods of 2D perovskite films are summarized and compared. The latest successful applications of the 2D perovskite in the solar cells and light-emitting diodes fields, especially the advanced stability of 2D perovskite solar cells(PeSCs) and the efficient 2D perovskite lightemitting diodes(PeLEDs), are also achieved. Furthermore, the challenges and outlook of 2D perovskite materials are proposed.