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Highly efficient tandem Z-scheme heterojunctions for visible light-based photocatalytic oxygen evolution reaction
被引量:
3
1
作者
Yi Lu
xing-kai cui
+1 位作者
Cheng-xiao Zhao
Xiao-fei Yang
《Water Science and Engineering》
EI
CAS
CSCD
2020年第4期299-306,共8页
Oxygen is important in maintaining a clean and reliable water environment.Designing heterojunction photocatalysts that can evolve oxygen from water splitting through an artificial Z-scheme pathway is a promising strat...
Oxygen is important in maintaining a clean and reliable water environment.Designing heterojunction photocatalysts that can evolve oxygen from water splitting through an artificial Z-scheme pathway is a promising strategy for solving environmental problems.In this study,flower-like MoS2 nanostructures were fabricated via a simple hydrothermal process,and the electrostatic-based assembly ion-exchange method was used to construct a tandem Ag3PO4/MoS2/g-C3N4(AMC)heterojunction.The as-synthesized photocatalyst exhibited significant improvements in harvesting visible light and transporting charge carriers.Moreover,the catalyst that was similar to the Z-scheme with intimate interface contact exhibited a strong oxygen evolution performance.The oxygen evolution activity of the optimal AMC-10 catalyst was approximately 11 times that of the pristine Ag3PO4.The results indicated that addition of a small amount of the flower-like MoS2 could significantly enhance the efficiency of oxygen evolution by the heterojunction.The findings in this study provide an alternative pathway for rationally designing efficient oxygen-evolving photocatalysts in order to improve the quality of water and rehabilitate the water environment.©2020 Hohai University.Production and hosting by Elsevier B.V.This is an open access article under the CC BY-NC-ND license(http://creativecommons.org/licenses/by-nc-nd/4.0/).
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关键词
Z-scheme
Graphitic
carbon
nitride
MoS2
Ag3PO4
Oxygen
evolution
reaction
Water
splitting
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题名
Highly efficient tandem Z-scheme heterojunctions for visible light-based photocatalytic oxygen evolution reaction
被引量:
3
1
作者
Yi Lu
xing-kai cui
Cheng-xiao Zhao
Xiao-fei Yang
机构
College of Science
School of Materials Science and Engineering
出处
《Water Science and Engineering》
EI
CAS
CSCD
2020年第4期299-306,共8页
基金
This work was supported by the National Natural Science Foundation of China(Grant No.21975129)
the Start-up Fund from Nanjing Forestry University.
文摘
Oxygen is important in maintaining a clean and reliable water environment.Designing heterojunction photocatalysts that can evolve oxygen from water splitting through an artificial Z-scheme pathway is a promising strategy for solving environmental problems.In this study,flower-like MoS2 nanostructures were fabricated via a simple hydrothermal process,and the electrostatic-based assembly ion-exchange method was used to construct a tandem Ag3PO4/MoS2/g-C3N4(AMC)heterojunction.The as-synthesized photocatalyst exhibited significant improvements in harvesting visible light and transporting charge carriers.Moreover,the catalyst that was similar to the Z-scheme with intimate interface contact exhibited a strong oxygen evolution performance.The oxygen evolution activity of the optimal AMC-10 catalyst was approximately 11 times that of the pristine Ag3PO4.The results indicated that addition of a small amount of the flower-like MoS2 could significantly enhance the efficiency of oxygen evolution by the heterojunction.The findings in this study provide an alternative pathway for rationally designing efficient oxygen-evolving photocatalysts in order to improve the quality of water and rehabilitate the water environment.©2020 Hohai University.Production and hosting by Elsevier B.V.This is an open access article under the CC BY-NC-ND license(http://creativecommons.org/licenses/by-nc-nd/4.0/).
关键词
Z-scheme
Graphitic
carbon
nitride
MoS2
Ag3PO4
Oxygen
evolution
reaction
Water
splitting
分类号
X703 [环境科学与工程—环境工程]
O643.36 [理学—物理化学]
O644.1 [理学—物理化学]
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Highly efficient tandem Z-scheme heterojunctions for visible light-based photocatalytic oxygen evolution reaction
Yi Lu
xing-kai cui
Cheng-xiao Zhao
Xiao-fei Yang
《Water Science and Engineering》
EI
CAS
CSCD
2020
3
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