In the phase diagram of the nickel-based superconductor Ba_(1-x)Sr_(x)Ni_(2)As_(2),T_(C) has been found to be enhanced sixfold near the quantum critical point(QCP) x=0.71 compared with the parent compound.However,the ...In the phase diagram of the nickel-based superconductor Ba_(1-x)Sr_(x)Ni_(2)As_(2),T_(C) has been found to be enhanced sixfold near the quantum critical point(QCP) x=0.71 compared with the parent compound.However,the mechanism is still under debate.Here,we report a detailed investigation of the superconducting properties near the QCP(x≈0.7) by utilizing scanning tunneling microscopy and spectroscopy.The temperature-dependent superconducting gap and magnetic vortex state were obtained and analyzed in the framework of the Bardeen-Cooper-Schrieffer model.The ideal isotropic s-wave superconducting gap excludes the long-speculated nematic fluctuations while preferring strong electron-phonon coupling as the mechanism for T_(C) enhancement near the QCP.The lower than expected gap ratio of Δ/(k_(B) T_(C)) is rooted in the fact that Ba_(1-x)Sr_(x)Ni_(2)As_(2) falls into the dirty limit with a serious pair breaking effect similar to the parent compound.展开更多
We revisited the vortex states of 2H-Nb Se2towards zero fields by a low-temperature scanning tunneling microscope.Fine structures of the anisotropic vortex states were distinguished, one is a spatially non-splitting z...We revisited the vortex states of 2H-Nb Se2towards zero fields by a low-temperature scanning tunneling microscope.Fine structures of the anisotropic vortex states were distinguished, one is a spatially non-splitting zero bias peak, and the other is an in-gap conductance anomaly resembling evolved crossing features around the center of the three nearest vortices.Both of them distribute solely along the next nearest neighboring direction of the vortex lattice and become unresolved in much higher magnetic fields, implying an important role played by the vortex–vortex interactions. To clarify these issues,we have studied the intrinsic vortex states of the isolated trapped vortex in zero fields at 0.45 K. It is concluded that the anisotropic zero bias peak is attributed to the superconducting gap anisotropy, and the spatially evolved crossing features are related to the vortex–vortex interaction. The vortex core size under the zero-field limit is determined. These results provide a paradigm for studying the inherent vortex states of type-II superconductors especially based on an isolated vortex.展开更多
To reveal the intrinsic properties of the basic superconducting units,i.e.,the single layered FeSe/FeAs in iron-based superconductors or CuO_(2) planes in cuprate superconductors,is a necessary prerequisite for unders...To reveal the intrinsic properties of the basic superconducting units,i.e.,the single layered FeSe/FeAs in iron-based superconductors or CuO_(2) planes in cuprate superconductors,is a necessary prerequisite for understanding the mechanism of high-Tc superconductivity.Up to now,an isolated FeAs layer has rarely been studied due to the difficulty in materials synthesis.Here,we report a scanning tunneling microscopy/spectroscopy(STM/STS)study on the iron-based superconductor KCa_(2)Fe_(4)As_(4)F_(2).In situ cleavage produced a single FeAs layer covered by a reconstructed K surface,which is isolated from the bulk by the underlying CaF layer and shows multi-band superconductivity with a much lower T_(c) than its bulk counterpart.In the exposed As-terminated regions with coverage of scattered K atoms,a pseudogap was observed,leading to an inhomogeneous superconductivity without long-range phase coherence in real space,which is remarkably similar to the high-T_(c) cuprate superconductors.These results provide a new perspective to understanding the origin of superconductivity in iron-based superconductors.展开更多
The recent discovery of superconductivity(SC)and charge density wave(CDW)in kagome metals AV3Sb5(A=K,Rb,Cs)provides an ideal playground for the study of emergent electronic orders.Application of moderate pressure lead...The recent discovery of superconductivity(SC)and charge density wave(CDW)in kagome metals AV3Sb5(A=K,Rb,Cs)provides an ideal playground for the study of emergent electronic orders.Application of moderate pressure leads to a two-dome-shaped SC phase regime in CsV_(3)Sb_(5) accompanied by the destabilizing of CDW phase.Nonetheless,the nature of this pressure-tuned SC state and its interplay with the CDW are yet to be explored.Here,we perform soft point-contact spectroscopy(SPCS)measurements in CsV_(3)Sb_(5) to investigate the evolution of superconducting order parameter with pressure.Surprisingly,we find that the superconducting gap is significantly enhanced between the two SC domes,at which the zero-resistance temperature is suppressed and the transition is remarkably broadened.Moreover,the temperature-dependence of the SC gap in this pressure range severely deviates from the conventional Bardeen-Cooper-Schrieffer(BCS)behavior,evidencing for strong Cooper pair phase fluctuations.These findings reveal the complex intertwining of the CDW with SC in the compressed CsV_(3)Sb_(5),suggesting striking parallel to the cuprate superconductor La2xBaxCuO4.Our results point to the essential role of charge degree of freedom in the development of intertwining electronic orders,and thus provide new constraints for theories.展开更多
基金Project supported by the National Key R&D Program of China (Grant Nos. 2022YFA1403203, 2022YFA1403400, and 2021YFA1400400)the Innovation Program for Quantum Science and Technology (Grant No. 2021ZD0302802)+2 种基金the National Natural Science Foundation of China (Grant Nos. 12074002, 12104004, 12204008, and 12374133)the Chinese Academy of Sciences (Grant Nos. XDB33000000 and GJTD-2020-01)the Major Basic Program of Natural Science Foundation of Shandong Province (Grant No. ZR2021ZD01)。
文摘In the phase diagram of the nickel-based superconductor Ba_(1-x)Sr_(x)Ni_(2)As_(2),T_(C) has been found to be enhanced sixfold near the quantum critical point(QCP) x=0.71 compared with the parent compound.However,the mechanism is still under debate.Here,we report a detailed investigation of the superconducting properties near the QCP(x≈0.7) by utilizing scanning tunneling microscopy and spectroscopy.The temperature-dependent superconducting gap and magnetic vortex state were obtained and analyzed in the framework of the Bardeen-Cooper-Schrieffer model.The ideal isotropic s-wave superconducting gap excludes the long-speculated nematic fluctuations while preferring strong electron-phonon coupling as the mechanism for T_(C) enhancement near the QCP.The lower than expected gap ratio of Δ/(k_(B) T_(C)) is rooted in the fact that Ba_(1-x)Sr_(x)Ni_(2)As_(2) falls into the dirty limit with a serious pair breaking effect similar to the parent compound.
基金Project supported by the National Key R&D Program of China (Grant No. 2022YFA1403203)the Innovation Program for Quantum Science and Technology (Grant No. 2021ZD0302802)+3 种基金the National Natural Science Foundation of China (Grant Nos. 12074002, 12374133, and 11804379)the Major Basic Program of Natural Science Foundation of Shandong Province (Grant No. ZR2021ZD01)the supports of the National Natural Science Foundation of China (Grant No. 12274001)the Natural Science Foundation of Anhui Province (Grant No. 2208085MA09)。
文摘We revisited the vortex states of 2H-Nb Se2towards zero fields by a low-temperature scanning tunneling microscope.Fine structures of the anisotropic vortex states were distinguished, one is a spatially non-splitting zero bias peak, and the other is an in-gap conductance anomaly resembling evolved crossing features around the center of the three nearest vortices.Both of them distribute solely along the next nearest neighboring direction of the vortex lattice and become unresolved in much higher magnetic fields, implying an important role played by the vortex–vortex interactions. To clarify these issues,we have studied the intrinsic vortex states of the isolated trapped vortex in zero fields at 0.45 K. It is concluded that the anisotropic zero bias peak is attributed to the superconducting gap anisotropy, and the spatially evolved crossing features are related to the vortex–vortex interaction. The vortex core size under the zero-field limit is determined. These results provide a paradigm for studying the inherent vortex states of type-II superconductors especially based on an isolated vortex.
基金supported by the National Key Research and Development Program of China(Grant Nos.2018YFA0305602,2022YFA1403203,and 2017YFA0303201)the National Natural Science Foundation of China(Grant Nos.12074002,92265104,12022413,11674331,and 12104004)+2 种基金the“Strategic Priority Research Program(B)”of the Chinese Academy of Sciences(Grant No.XDB33030100)the Major Basic Program of Natural Science Foundation of Shandong Province(Grant No.ZR2021ZD01)supported by the High Magnetic Field Laboratory of Anhui Province,China。
文摘To reveal the intrinsic properties of the basic superconducting units,i.e.,the single layered FeSe/FeAs in iron-based superconductors or CuO_(2) planes in cuprate superconductors,is a necessary prerequisite for understanding the mechanism of high-Tc superconductivity.Up to now,an isolated FeAs layer has rarely been studied due to the difficulty in materials synthesis.Here,we report a scanning tunneling microscopy/spectroscopy(STM/STS)study on the iron-based superconductor KCa_(2)Fe_(4)As_(4)F_(2).In situ cleavage produced a single FeAs layer covered by a reconstructed K surface,which is isolated from the bulk by the underlying CaF layer and shows multi-band superconductivity with a much lower T_(c) than its bulk counterpart.In the exposed As-terminated regions with coverage of scattered K atoms,a pseudogap was observed,leading to an inhomogeneous superconductivity without long-range phase coherence in real space,which is remarkably similar to the high-T_(c) cuprate superconductors.These results provide a new perspective to understanding the origin of superconductivity in iron-based superconductors.
基金supported by the National Natural Science Foundation of China(11888101 and 11534010)the National Key Research and Development Program of the Ministry of Science and Technology of China(2017YFA0303001 and 2019YFA0704900)+5 种基金the Anhui Initiative in Quantum Information Technologies(AHY160000)the Science Challenge Project of China(TZ2016004)the Key Research Program of Frontier Sciences,CAS,China(QYZDYSSWSLH021)the Strategic Priority Research Program of the Chinese Academy of Sciences(XDB25000000)the Collaborative Innovation Program of Hefei Science Center,CAS(2020HSC-CIP014)the Fundamental Research Funds for the Central Universities(WK3510000011).
文摘The recent discovery of superconductivity(SC)and charge density wave(CDW)in kagome metals AV3Sb5(A=K,Rb,Cs)provides an ideal playground for the study of emergent electronic orders.Application of moderate pressure leads to a two-dome-shaped SC phase regime in CsV_(3)Sb_(5) accompanied by the destabilizing of CDW phase.Nonetheless,the nature of this pressure-tuned SC state and its interplay with the CDW are yet to be explored.Here,we perform soft point-contact spectroscopy(SPCS)measurements in CsV_(3)Sb_(5) to investigate the evolution of superconducting order parameter with pressure.Surprisingly,we find that the superconducting gap is significantly enhanced between the two SC domes,at which the zero-resistance temperature is suppressed and the transition is remarkably broadened.Moreover,the temperature-dependence of the SC gap in this pressure range severely deviates from the conventional Bardeen-Cooper-Schrieffer(BCS)behavior,evidencing for strong Cooper pair phase fluctuations.These findings reveal the complex intertwining of the CDW with SC in the compressed CsV_(3)Sb_(5),suggesting striking parallel to the cuprate superconductor La2xBaxCuO4.Our results point to the essential role of charge degree of freedom in the development of intertwining electronic orders,and thus provide new constraints for theories.
基金supported by the National Key Research and Development Program of China(2018YFA0704200,2017YFA0302904,2019YFA0308500,and 2018YFA0305602)the National Natural Science Foundation of China(12074414,12074002,52072401,11804379,and 11774402)+1 种基金the Recruitment Program for Leading Talent Team of Anhui Province(2019-16)the Strategic Priority Research Program of Chinese Academy of Sciences(XDB25000000)。