Space radiation with inherently broadband spectral flux poses a huge danger to astronauts and electronics on aircraft,but it is hard to simulate such feature with conventional radiation sources. Using a tabletop laser...Space radiation with inherently broadband spectral flux poses a huge danger to astronauts and electronics on aircraft,but it is hard to simulate such feature with conventional radiation sources. Using a tabletop laser-plasma accelerator, we can reproduce exponential energy particle beams as similar as possible to these in space radiation. We used such an electron beam to study the electron radiation effects on the surface structure and performance of two-dimensional material(Fe PS3).Energetic electron beam led to bulk sample cleavage and damage between areas of uneven thickness. For the Fe PS3sheet sample, electron radiation transformed it from crystalline state to amorphous state, causing the sample surface to rough.The full widths at the half maximum of characteristic Raman peaks became larger, and the intensities of characteristic Raman peaks became weak or even disappeared dramatically under electron radiation. This trend became more obvious for thinner samples, and this phenomenon was attributed to the cleavage of P–P and P–S bonds, destabilizing the bipyramid structure of [P2S6]4-unit. The results are of great significance for testing the maximum allowable radiation dose for the two-dimensional material, implying that Fe PS3cannot withstand such energetic electron radiation without an essential shield.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.11975308)the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDA25050200)Science Challenge Project(Grant No.TZ2018001)。
文摘Space radiation with inherently broadband spectral flux poses a huge danger to astronauts and electronics on aircraft,but it is hard to simulate such feature with conventional radiation sources. Using a tabletop laser-plasma accelerator, we can reproduce exponential energy particle beams as similar as possible to these in space radiation. We used such an electron beam to study the electron radiation effects on the surface structure and performance of two-dimensional material(Fe PS3).Energetic electron beam led to bulk sample cleavage and damage between areas of uneven thickness. For the Fe PS3sheet sample, electron radiation transformed it from crystalline state to amorphous state, causing the sample surface to rough.The full widths at the half maximum of characteristic Raman peaks became larger, and the intensities of characteristic Raman peaks became weak or even disappeared dramatically under electron radiation. This trend became more obvious for thinner samples, and this phenomenon was attributed to the cleavage of P–P and P–S bonds, destabilizing the bipyramid structure of [P2S6]4-unit. The results are of great significance for testing the maximum allowable radiation dose for the two-dimensional material, implying that Fe PS3cannot withstand such energetic electron radiation without an essential shield.
