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Preparation of PrFe_(x)Co_(1-x)O_(3)/Mt catalyst and study on degradation of 2-hydroxybenzoic acid wastewater by catalytic wet peroxide oxidation
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作者 Binxia Zhao yijia gao +3 位作者 Tiancheng Hun Xiaoxiao Fan Nan Shao Xiaoqian Chen 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2024年第1期286-297,共12页
In this study,the perovskite nanocomposite PrFe_(x)Co_(1-x)O_(3)(Pr(S))was successfully synthesized by the sol-gel method;PrFe_(x)Co_(1-x)O_(3)/Al-pillared montmorillonite(Pr(S)/Mt)catalysts were prepared by impregnat... In this study,the perovskite nanocomposite PrFe_(x)Co_(1-x)O_(3)(Pr(S))was successfully synthesized by the sol-gel method;PrFe_(x)Co_(1-x)O_(3)/Al-pillared montmorillonite(Pr(S)/Mt)catalysts were prepared by impregnation(D)method and solid-melting(G)method,respectively,with Pr(S)as the active component and Al-pillared montmorillonite as the carrier.The catalysts were applied to treat the 2-hydroxybenzoic acid(2-HA)-simulated wastewater by catalytic wet peroxide oxidation(CWPO)technique,and the chemical oxygen demand(COD)removal rate and the 2-HA degradation rate were used as indicators to evaluate the catalytic performance.The results of the experiment indicated that the solid-melting method was more conducive to preparing the catalyst when the Co/Fe molar ratio of 7:3 and the optimal structural properties of the catalysts were achieved.The influence of operating parameters,including reaction temperature,catalyst dosage,H_(2)O_(2)dosage,pH,and initial 2-HA concentration,were optimized for the degradation of 2-HA by CWPO.The results showed that 97.64%of 2-HA degradation and 75.23%of COD removal rate were achieved under more suitable experimental conditions.In addition,after the catalyst was used five times,the degradation rate of 2-HA could still reach 76.93%,which implied the high stability and reusability of the catalyst.The high catalytic activity of the catalyst was due to the doping of Co into PrFeO_(3),which could promote the generation of HO·,and the high stability could be attributed to the loading of Pr(S)onto Al-Mt,which reduced the leaching of reactive metals.The study of reaction mechanism and kinetics showed that the whole degradation process conformed to the pseudo-firstorder kinetic equation,and the Langmuir-Hinshelwood method was applied to demonstrate that catalysis was dominant in the degradation process. 展开更多
关键词 MONTMORILLONITE PEROVSKITE Catalytic wet peroxide oxidation(CWPO) 2-Hydroxybenzoic acid
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Comparison of Spring Radish Varieties with Entire Leaves
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作者 Xiaomin YU Chenchen XIAO +2 位作者 Weizhen LI yijia gao Shisheng LI 《Agricultural Biotechnology》 CAS 2021年第6期16-18,共3页
[Objectives]This study was conducted to select spring radish varieties with better growth,higher yield and better nutrition.[Methods]A new spring radish combination(2019MUA×Lixiang)was obtained through traditiona... [Objectives]This study was conducted to select spring radish varieties with better growth,higher yield and better nutrition.[Methods]A new spring radish combination(2019MUA×Lixiang)was obtained through traditional hybridization methods,and various characters of this line were compared with its parents and commercial spring radish.The radish varieties such as Lixiang radish,2019MUA×Lixiang,2019MUA,commercial variety Zhongluo No.1 and Huangzhou radish were respectively compared and studied in detail in terms of botanical characters,entire leaf bolting ratios,nutritional physiological indexes and so on.[Results]The new radish combination 2019MUA×Lixiang has better indexes,and is more suitable for spring planting.[Conclusions]The study provides a reference basis for the selection on radish planted in Spring. 展开更多
关键词 Spring radish Botanical characters Rate of bolting Physiological index
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