Tandem catalytic reactions have attracted extensive interest because of their ability to reduce reaction steps,energy consumption,and waste.However,the construction of highly efficient tandem catalytic systems is stil...Tandem catalytic reactions have attracted extensive interest because of their ability to reduce reaction steps,energy consumption,and waste.However,the construction of highly efficient tandem catalytic systems is still a significant challenge due to the problematic integration of multiple active sites in one reaction system and the incompatibility of different reaction conditions.Although metal nanoparticles(MNPs)supported on porous framework materials have shown excellent catalytic performances in various reactions,their cooperative catalysis for tandem reactions is rarely reported.展开更多
基金support from the National Key Research and Development Program of China(nos.2018YFA0208600 and 2018YFA0704502)NSFC(nos.22071245,21671188,21871263,and 21520102001)+2 种基金Key Research Program of Frontier Science,CAS(no.QYZDJ-SSW-SLH045)Strategic Priority Research Program of the Chinese Academy of Sciences(no.XDB20000000)and Youth Innovation Promotion Association,CAS(no.Y201850).
文摘Tandem catalytic reactions have attracted extensive interest because of their ability to reduce reaction steps,energy consumption,and waste.However,the construction of highly efficient tandem catalytic systems is still a significant challenge due to the problematic integration of multiple active sites in one reaction system and the incompatibility of different reaction conditions.Although metal nanoparticles(MNPs)supported on porous framework materials have shown excellent catalytic performances in various reactions,their cooperative catalysis for tandem reactions is rarely reported.