Carbonaceous aerosols(CA) are crucial components in the atmospheric PM_(2.5) and derived from diverse sources. One of the major sources for CA is from the incomplete combustion of bituminous coal that has been prevail...Carbonaceous aerosols(CA) are crucial components in the atmospheric PM_(2.5) and derived from diverse sources. One of the major sources for CA is from the incomplete combustion of bituminous coal that has been prevailingly used by household stoves in rural areas for heating during winter. To efficiently eliminate the CA emission, a new household stove(NHS) was developed based on a novel combustion technology and CA emissions from the NHS and a traditional household stove(THS) were comparably investigated under the actual stove operation conditions in a farmer’s house. Compared with the THS, the emission factors of organic carbon(OC), elemental carbon(EC), and water-soluble organic carbon(WSOC) from the NHS were reduced by 96%±1%, 98%±1%, and 91%±1% under the flaming process and 95%±1%, 96%±2%, and 83%±4% under the smoldering process, respectively. Additionally,the mass absorption efficiency of WSOC from the NHS reduced by 3 folds and the radiative forcing by WSOC relative to EC shrank remarkably by a factor of 3-8. Based on the reduction of emissions and light absorption of WSOC, the promotion of the NHS offers a possible solution to achieve the clean combustion of residential solid fuel.展开更多
基金supported by the National Natural Science Foundation of China (Nos. 21876186, 41727805, 41975164)the National Research Program of Key Issues in Air Pollution Control (Nos. DQGG0206, DQGG0103, DQGG0209)。
文摘Carbonaceous aerosols(CA) are crucial components in the atmospheric PM_(2.5) and derived from diverse sources. One of the major sources for CA is from the incomplete combustion of bituminous coal that has been prevailingly used by household stoves in rural areas for heating during winter. To efficiently eliminate the CA emission, a new household stove(NHS) was developed based on a novel combustion technology and CA emissions from the NHS and a traditional household stove(THS) were comparably investigated under the actual stove operation conditions in a farmer’s house. Compared with the THS, the emission factors of organic carbon(OC), elemental carbon(EC), and water-soluble organic carbon(WSOC) from the NHS were reduced by 96%±1%, 98%±1%, and 91%±1% under the flaming process and 95%±1%, 96%±2%, and 83%±4% under the smoldering process, respectively. Additionally,the mass absorption efficiency of WSOC from the NHS reduced by 3 folds and the radiative forcing by WSOC relative to EC shrank remarkably by a factor of 3-8. Based on the reduction of emissions and light absorption of WSOC, the promotion of the NHS offers a possible solution to achieve the clean combustion of residential solid fuel.
