Supercontinuum(SC)light source has advanced ultrafast laser spectroscopy in condensed matter science,biology,physics,and chemistry.Compared to the frequently used photonic crystal fibers and bulk materials,femtosecond...Supercontinuum(SC)light source has advanced ultrafast laser spectroscopy in condensed matter science,biology,physics,and chemistry.Compared to the frequently used photonic crystal fibers and bulk materials,femtosecond laser filamentation in gases is damage-immune for supercontinuum generation.A bottleneck problem is the strong jitters from filament induced self-heating at kHz repetition rate level.We demonstrated stable kHz supercontinuum generation directly in air with multiple mJ level pulse energy.This was achieved by applying an external DC electric field to the air plasma filament.Beam pointing jitters of the 1 kHz air filament induced SC light were reduced by more than 2 fold.The stabilized high repetition rate laser filament offers the opportunity for stable intense SC generation and its applications in air.展开更多
In this paper,we report the recent progress on the 1 PW/0.1 Hz laser beamline of Shanghai Superintense Ultrafast Laser Facility(SULF).The SULF-1 PW laser beamline is based on the double chirped pulse amplification(CPA...In this paper,we report the recent progress on the 1 PW/0.1 Hz laser beamline of Shanghai Superintense Ultrafast Laser Facility(SULF).The SULF-1 PW laser beamline is based on the double chirped pulse amplification(CPA)scheme,which can generate laser pulses of 50.8 J at 0.1 Hz after the final amplifier;the shot-to-shot energy fluctuation of the amplified pulse is as low as 1.2%(std).After compression,the pulse duration of 29.6 fs is achieved,which can support a maximal peak power of 1 PW.The contrast ratio at-80 ps before main pulse is measured to be 2.5×10^-11.The focused peak intensity is improved by optimizing the angular dispersion in the grating compressor.The maximal focused peak intensity can reach 2.7×10^19W/cm2 even with an f/26.5 off-axis parabolic mirror.The horizontal and vertical angular pointing fluctuations in 1 h are measured to be 1.89 and 2.45μrad,respectively.The moderate repetition rate and the good stability are desirable characteristics for lasermatter interactions.The SULF-1 PW laser beamline is now in the phase of commissioning,and preliminary experiments of particle acceleration and secondary radiation under 300–400 TW/0.1 Hz laser condition have been implemented.The progress on the experiments and the daily stable operation of the laser demonstrate the availability of the SULF-1 PW beamline.展开更多
Remote or standoff detection of greenhouse gases,air pollutants,and biological agents with innovative ultrafast laser technology attracts growing interests in recent years.Hybrid femtosecond/picosecond coherent Raman ...Remote or standoff detection of greenhouse gases,air pollutants,and biological agents with innovative ultrafast laser technology attracts growing interests in recent years.Hybrid femtosecond/picosecond coherent Raman spectroscopy is considered as one of the most versatile techniques due to its great advantages in terms of detection sensitivity and chemical specificity.However,the simultaneous requirement for the femtosecond pump and the picosecond probe increases the complexity of optical system.Herein,we demonstrate that air lasing naturally created inside a filament can serve as an ideal light source to probe Raman coherence excited by the femtosecond pump,producing coherent Raman signal with molecular vibrational signatures.The combination of pulse self-compression effect and air lasing action during filamentation improves Raman excitation efficiency and greatly simplifies the experimental setup.The air-lasing-assisted Raman spectroscopy was applied to quantitatively detect greenhouse gases mixed in air,and it was found that the minimum detectable concentrations of CO_(2) and SF_(6) can reach 0.1%and 0.03%,respectively.The ingenious designs,especially the optimization of pump-seed delay and the choice of perpendicular polarization,ensure a high detection sensitivity and signal stability.Moreover,it is demonstrated that this method can be used for simultaneously measuring CO_(2) and SF_(6) gases and distinguishing ^(12)CO_(2) and ^(13)CO_(2).The developed scheme provides a new route for high-sensitivity standoff detection and combustion diagnosis.展开更多
We theoretically investigate the delay-dependent attosecond transient absorption spectra in the helium atom dressed by an infrared laser pulse in the wavelength range of 800–2400 nm. By numerically solving the three-...We theoretically investigate the delay-dependent attosecond transient absorption spectra in the helium atom dressed by an infrared laser pulse in the wavelength range of 800–2400 nm. By numerically solving the three-dimensional time-dependent Schrdinger equation, we find that the absorption spectrogram exhibits a multiple-fringe structure for using the mid-infrared dressing pulse. The quantitative calculation of the transition matrix between different Floquet states provides direct evidence on the origin of the multiple-fringe structure.Our result shows that the wavelength of the dressing pulse is an important parameter and the unique feature of attosecond transient absorption spectroscopy can be induced in the mid-infrared regime.展开更多
It is accidental, but interesting to celebrate the i0th anniversary of Chinese Optics Letters (COL) after revival from the "most important" day in 2012, December 21, which is closely related to Mayan calendar. The...It is accidental, but interesting to celebrate the i0th anniversary of Chinese Optics Letters (COL) after revival from the "most important" day in 2012, December 21, which is closely related to Mayan calendar. The last decade sees the development of optics in China and around the world, and Nobel Prize awarded to scientists for their excellent work in fiber optics, quantum optics, etc. Up to now, most research results are still published in journals, and COL has been trying to publish the most excellent papers for authors and readers.展开更多
Multidimensional instabilities always develop with time during the process of radiation pressure acceleration,and are detrimental to the generation of monoenergetic proton beams.In this paper,a sharp-front laser is pr...Multidimensional instabilities always develop with time during the process of radiation pressure acceleration,and are detrimental to the generation of monoenergetic proton beams.In this paper,a sharp-front laser is proposed to irradiate a triple-layer target(the proton layer is set between two carbon ion layers)and studied in theory and simulations.It is found that the thin proton layer can be accelerated once to hundreds of MeV with monoenergetic spectra only during the hole-boring(HB)stage.The carbon ions move behind the proton layer in the light-sail(LS)stage,which can shield any further interaction between the rear part of the laser and the proton layer.In this way,proton beam instabilities can be reduced to a certain extent during the entire acceleration process.It is hoped such a mechanism can provide a feasible way to improve the beam quality for proton therapy and other applications.展开更多
A method for inertial confinement fusion driven by powerful long wavelength electromagnetic pulses(EMPs), such as CO2 laser pulses or high power microwave pulses, is proposed. Due to the high efficiency of generating ...A method for inertial confinement fusion driven by powerful long wavelength electromagnetic pulses(EMPs), such as CO2 laser pulses or high power microwave pulses, is proposed. Due to the high efficiency of generating such long wavelength electromagnetic pulses, this method is especially important for the future fusion electricity power. Special fuel targets are designed to overcome the shortcomings of the long wavelength electromagnetic pulses.展开更多
基金This work was supported in part by NSAF(Grant No.U2130123)the International Partnership Program of Chinese Academy of Sciences(Grant Nos.181231KYSB20200033 and 181231KYSB20200040)Shanghai Science and Technology Program(Grant No.21511105000).S.L.C.acknowledges the support of COPL,Laval University,Quebec City,Canada.We thank Dr.Hao Guo,Ms.Na Chen,Mr.Xuan Zhang,Dr.Haiyi Sun from SIOM for help in the experiments and Prof.Howard M.Milchberg from the University of Maryland for the fruitful discussions and his reading of the manuscript.
文摘Supercontinuum(SC)light source has advanced ultrafast laser spectroscopy in condensed matter science,biology,physics,and chemistry.Compared to the frequently used photonic crystal fibers and bulk materials,femtosecond laser filamentation in gases is damage-immune for supercontinuum generation.A bottleneck problem is the strong jitters from filament induced self-heating at kHz repetition rate level.We demonstrated stable kHz supercontinuum generation directly in air with multiple mJ level pulse energy.This was achieved by applying an external DC electric field to the air plasma filament.Beam pointing jitters of the 1 kHz air filament induced SC light were reduced by more than 2 fold.The stabilized high repetition rate laser filament offers the opportunity for stable intense SC generation and its applications in air.
基金the support from the electronacceleration team led by Wentao Wang,Rong Qithe proton-acceleration team led by Hui Zhang+4 种基金supported by the National Natural Science Foundation of China(Nos.11127901,61521093 and 61505234)International S&T Cooperation Program of China(No.2016YFE 0119300)Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDB160301)Technology Commission of Shanghai Municipality(No.2017SHZDZX02)Youth Innovation Promotion Association of the Chinese Academy of Sciences。
文摘In this paper,we report the recent progress on the 1 PW/0.1 Hz laser beamline of Shanghai Superintense Ultrafast Laser Facility(SULF).The SULF-1 PW laser beamline is based on the double chirped pulse amplification(CPA)scheme,which can generate laser pulses of 50.8 J at 0.1 Hz after the final amplifier;the shot-to-shot energy fluctuation of the amplified pulse is as low as 1.2%(std).After compression,the pulse duration of 29.6 fs is achieved,which can support a maximal peak power of 1 PW.The contrast ratio at-80 ps before main pulse is measured to be 2.5×10^-11.The focused peak intensity is improved by optimizing the angular dispersion in the grating compressor.The maximal focused peak intensity can reach 2.7×10^19W/cm2 even with an f/26.5 off-axis parabolic mirror.The horizontal and vertical angular pointing fluctuations in 1 h are measured to be 1.89 and 2.45μrad,respectively.The moderate repetition rate and the good stability are desirable characteristics for lasermatter interactions.The SULF-1 PW laser beamline is now in the phase of commissioning,and preliminary experiments of particle acceleration and secondary radiation under 300–400 TW/0.1 Hz laser condition have been implemented.The progress on the experiments and the daily stable operation of the laser demonstrate the availability of the SULF-1 PW beamline.
基金supported by the National Natural Science Foundation of China(11822410,12034013,12074063)Key Research Program of Frontier Sciences of Chinese Academy of Sciences(QYZDJ-SSW-SLH010)+2 种基金Program of Shanghai Academic Research Leader(20XD1424200)Shanghai Municipal Science and Technology Major Project(2019SHZDZX01)Youth Innovation Promotion Association of CAS(2018284).
文摘Remote or standoff detection of greenhouse gases,air pollutants,and biological agents with innovative ultrafast laser technology attracts growing interests in recent years.Hybrid femtosecond/picosecond coherent Raman spectroscopy is considered as one of the most versatile techniques due to its great advantages in terms of detection sensitivity and chemical specificity.However,the simultaneous requirement for the femtosecond pump and the picosecond probe increases the complexity of optical system.Herein,we demonstrate that air lasing naturally created inside a filament can serve as an ideal light source to probe Raman coherence excited by the femtosecond pump,producing coherent Raman signal with molecular vibrational signatures.The combination of pulse self-compression effect and air lasing action during filamentation improves Raman excitation efficiency and greatly simplifies the experimental setup.The air-lasing-assisted Raman spectroscopy was applied to quantitatively detect greenhouse gases mixed in air,and it was found that the minimum detectable concentrations of CO_(2) and SF_(6) can reach 0.1%and 0.03%,respectively.The ingenious designs,especially the optimization of pump-seed delay and the choice of perpendicular polarization,ensure a high detection sensitivity and signal stability.Moreover,it is demonstrated that this method can be used for simultaneously measuring CO_(2) and SF_(6) gases and distinguishing ^(12)CO_(2) and ^(13)CO_(2).The developed scheme provides a new route for high-sensitivity standoff detection and combustion diagnosis.
基金supported by the National Natural Science Foundation of China(Nos.61690223,11774363,11561121002,61521093,11127901,11227902,and 11574332)the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDB16)the Youth Innovation Promotion Association CAS
文摘We theoretically investigate the delay-dependent attosecond transient absorption spectra in the helium atom dressed by an infrared laser pulse in the wavelength range of 800–2400 nm. By numerically solving the three-dimensional time-dependent Schrdinger equation, we find that the absorption spectrogram exhibits a multiple-fringe structure for using the mid-infrared dressing pulse. The quantitative calculation of the transition matrix between different Floquet states provides direct evidence on the origin of the multiple-fringe structure.Our result shows that the wavelength of the dressing pulse is an important parameter and the unique feature of attosecond transient absorption spectroscopy can be induced in the mid-infrared regime.
文摘It is accidental, but interesting to celebrate the i0th anniversary of Chinese Optics Letters (COL) after revival from the "most important" day in 2012, December 21, which is closely related to Mayan calendar. The last decade sees the development of optics in China and around the world, and Nobel Prize awarded to scientists for their excellent work in fiber optics, quantum optics, etc. Up to now, most research results are still published in journals, and COL has been trying to publish the most excellent papers for authors and readers.
基金supported by the National Natural Science Foundation of China (No. 11575274)Strategic Priority Research Program of the Chinese Academy of Sciences (No. XDB16010600)Ministry of Science and Technology of the People’s Republic of China (Nos. 2016YFA0401102 and 2018YFA0404803)
文摘Multidimensional instabilities always develop with time during the process of radiation pressure acceleration,and are detrimental to the generation of monoenergetic proton beams.In this paper,a sharp-front laser is proposed to irradiate a triple-layer target(the proton layer is set between two carbon ion layers)and studied in theory and simulations.It is found that the thin proton layer can be accelerated once to hundreds of MeV with monoenergetic spectra only during the hole-boring(HB)stage.The carbon ions move behind the proton layer in the light-sail(LS)stage,which can shield any further interaction between the rear part of the laser and the proton layer.In this way,proton beam instabilities can be reduced to a certain extent during the entire acceleration process.It is hoped such a mechanism can provide a feasible way to improve the beam quality for proton therapy and other applications.
文摘A method for inertial confinement fusion driven by powerful long wavelength electromagnetic pulses(EMPs), such as CO2 laser pulses or high power microwave pulses, is proposed. Due to the high efficiency of generating such long wavelength electromagnetic pulses, this method is especially important for the future fusion electricity power. Special fuel targets are designed to overcome the shortcomings of the long wavelength electromagnetic pulses.