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Probing Molecular Dynamics with Ultrafast Electron Diffraction
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作者 zhuo-ran ma Feng-feng Qi Dao Xiang 《Chinese Journal of Chemical Physics》 SCIE CAS CSCD 2021年第1期15-29,I0011,共16页
Recent progress in ultrafast lasers,ultrafast X-rays and ultrafast electron beams has made it possible to watch the motion of atoms in real time through pumpprobe technique.In this review,we focus on how the molecular... Recent progress in ultrafast lasers,ultrafast X-rays and ultrafast electron beams has made it possible to watch the motion of atoms in real time through pumpprobe technique.In this review,we focus on how the molecular dynamics can be studied with ultrafast electron diffraction where the dynamics is initiated by a pumping laser and then probed by pulsed electron beams.This technique allows one to track the molecular dynamics with femtosecond time resolution and Angstr6m spatial resolution.We present the basic physics and latest development of this technique.Representative applications of ultrafast electron diffraction in studies of laser-induced molecular dynamics are also discussed.This table-top technique is complementary to X-ray free-electron laser and we expect it to have a strong impact in studies of chemical dynamics. 展开更多
关键词 Ultrafast electron diffraction Gas phase PHOTOCHEMISTRY Molecular dynamics PUMP-PROBE
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NIPAD: a non-invasive power-based anomaly detection scheme for programmable logic controllers 被引量:4
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作者 Yu-jun XIAO Wen-yuan XU +2 位作者 Zhen-hua JIA zhuo-ran ma Dong-lian QI 《Frontiers of Information Technology & Electronic Engineering》 SCIE EI CSCD 2017年第4期519-534,共16页
Industrial control systems (ICSs) are widely used in critical infrastructures, making them popular targets for attacks to cause catastrophic physical damage. As one of the most critical components in ICSs, the progr... Industrial control systems (ICSs) are widely used in critical infrastructures, making them popular targets for attacks to cause catastrophic physical damage. As one of the most critical components in ICSs, the programmable logic controller (PLC) controls the actuators directly. A PLC executing a malicious program can cause significant property loss or even casualties. The number of attacks targeted at PLCs has increased noticeably over the last few years, exposing the vulnerability of the PLC and the importance of PLC protection. Unfortunately, PLCs cannot be protected by traditional intrusion detection systems or antivirus software. Thus, an effective method for PLC protection is yet to be designed. Motivated by these concerns, we propose a non-invasive power- based anomaly detection scheme for PLCs. The basic idea is to detect malicious software execution in a PLC through analyzing its power consumption, which is measured by inserting a shunt resistor in series with the CPU in a PLC while it is executing instructions. To analyze the power measurements, we extract a discriminative feature set from the power trace, and then train a long short-term memory (LSTM) neural network with the features of normal samples to predict the next time step of a normal sample. Finally, an abnormal sample is identified through comparing the predicted sample and the actual sample. The advantages of our method are that it requires no software modification on the original system and is able to detect unknown attacks effectively. The method is evaluated on a lab testbed, and for a trojan attack whose difference from the normal program is around 0.63%, the detection accuracy reaches 99.83%. 展开更多
关键词 Industrial control system Programmable logic controller Side-channel Anomaly detection Long short-term memory neural networks
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