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【导读】中国现代天文学摇篮
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作者 吴雪峰 《大学科普》 2024年第1期43-43,共1页
中国科学院紫金山天文台前身是成立于1928年的国立中央研究院天文研究所,1950年更为现名,是我国自主建立的第一个现代天文学研究机构。紫金山天文台的建成标志着中国现代天文学研究的开始,被誉为“中国现代天文学摇篮”。从1913年高鲁... 中国科学院紫金山天文台前身是成立于1928年的国立中央研究院天文研究所,1950年更为现名,是我国自主建立的第一个现代天文学研究机构。紫金山天文台的建成标志着中国现代天文学研究的开始,被誉为“中国现代天文学摇篮”。从1913年高鲁先生下决心建造一座中国人自己的现代化天文台,到1934年余青松先生在紫金山上的天堡峰实现高鲁先生的宏愿,再到新中国成立后张钰哲先生站在中国天文事业全局发展的高度制定规划并推动形成了当前中国科学院和部分高校天文研究机构以及部分天文科普教育基地的分布格局,一代又一代紫金山天文台科技工作者严谨求实,勤奋开拓,不辱使命,为我国天文学事业的发展,为国家经济建设和航天事业的腾飞做出了重要的积极贡献。 展开更多
关键词 紫金山天文台 中国科学院 国立中央研究院 科技工作者 天文研究 张钰哲 全局发展 积极贡献
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An Intermediate-field Fast Radio Burst Model and the Quasi-periodic Oscillation
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作者 Jie-Shuang Wang Xinyu Li +1 位作者 Zigao Dai xuefeng wu 《Research in Astronomy and Astrophysics》 SCIE CAS CSCD 2023年第3期93-99,共7页
Quasi-periodic oscillation(QPO)signals are discovered in some fast radio bursts(FRBs)such as FRB 20191221A,as well as in the X-ray burst associated with the galactic FRB from SGR 1935+2154.We revisit the intermediatef... Quasi-periodic oscillation(QPO)signals are discovered in some fast radio bursts(FRBs)such as FRB 20191221A,as well as in the X-ray burst associated with the galactic FRB from SGR 1935+2154.We revisit the intermediatefield FRB model where the radio waves are generated as fast-magnetosonic waves through magnetic reconnection near the light cylinder.The current sheet in the magnetar wind is compressed by a low frequency pulse emitted from the inner magnetosphere to trigger magnetic reconnection.By incorporating the wave dynamics of the magnetosphere,we demonstrate how the FRB frequency,the single pulse width,and luminosity are determined by the period,magnetic field,QPO frequency and quake energetics of the magnetar.We find that this model can naturally and self-consistently interpret the X-ray/radio event from SGR 1935+2154 and the QPO in FRB20191221A.It can also explain the observed wide energy range of repeating FRBs in a narrow bandwidth. 展开更多
关键词 PERIODIC FIELD NARROW
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Surface Cu^(+) modified ZnIn_(2)S_(4) for promoted visible-light photocatalytic hydrogen evolution 被引量:1
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作者 Wen Li Jia Wen Jing Li +6 位作者 Hai Yang Yuan xuefeng wu Yuanwei Liu Sheng Dai Qilin Cheng Peng Fei Liu Hua Gui Yang 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2022年第11期341-348,I0009,共9页
Surface modification by metal ion has been considered a promising strategy to enhance the photocatalytic activity by extending optical response and improving charge separation and transportation.Here,univalent copper ... Surface modification by metal ion has been considered a promising strategy to enhance the photocatalytic activity by extending optical response and improving charge separation and transportation.Here,univalent copper species were modified on ZnIn_(2)S_(4)photocatalyst via an in-situ photodeposition method,exhibiting a much higher H2evolution rate of 41.10±3.43 mmol g^(-1)h^(-1)and an impressive apparent quantum efficiency(AQE)of 20.81%at 420±15 nm.Our characterizations indicate that the surface modification by copper species can broaden light utilization as well as promote charge separation and transportation.Besides,the density functional theory(DFT)results further exhibit that the energy levels(LUMO and HOMO)for copper-surface modified ZnIn_(2)S_(4)present spatial separation,locating on the Zn-S and In-S layers,respectively,which can suppress the recombination of electron and hole and thus achieves higher photocatalytic H2evolution efficiency. 展开更多
关键词 Surface modification Univalent copper species Charge separation and transportation HOMO-LUMO spatial separation Photocatalytic hydrogen evolution
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Science with the 2.5-meter Wide Field Survey Telescope(WFST) 被引量:4
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作者 Tinggui Wang Guilin Liu +59 位作者 Zhenyi Cai Jinjun Geng Min Fang Haoning He Ji-an Jiang Ning Jiang Xu Kong Bin Li Ye Li Wentao Luo Zhizheng Pan xuefeng wu Ji Yang Jiming Yu Xianzhong Zheng Qingfeng Zhu Yi-Fu Cai Yuanyuan Chen Zhiwei Chen Zigao Dai Lulu Fan Yizhong Fan Wenjuan Fang Zhicheng He Lei Hu Maokai Hu Zhiping Jin Zhibo Jiang Guoliang Li Fan Li Xuzhi Li Runduo Liang Zheyu Lin Qingzhong Liu Wenhao Liu Zhengyan Liu Wei Liu Yao Liu Zheng Lou Han Qu Zhenfeng Sheng Jianchun Shi Yiping Shu Zhenbo Su Tianrui Sun Hongchi Wang Huiyuan Wang Jian Wang Junxian Wang Daming Wei Junjie Wei Yongquan Xue Jingzhi Yan Chao Yang Ye Yuan Yefei Yuan Hongxin Zhang Miaomiao Zhang Haibin Zhao Wen Zhao 《Science China(Physics,Mechanics & Astronomy)》 SCIE EI CAS CSCD 2023年第10期155-202,共48页
The Wide Field Survey Telescope(WFST) is a dedicated photometric surveying facility being built jointly by University of Science and Technology of China(USTC) and the Purple Mountain Observatory(PMO). It is equipped w... The Wide Field Survey Telescope(WFST) is a dedicated photometric surveying facility being built jointly by University of Science and Technology of China(USTC) and the Purple Mountain Observatory(PMO). It is equipped with a 2.5-meter diameter primary mirror, an active optics system, and a mosaic CCD camera with 0.73 gigapixels on the primary focal plane for highquality image capture over a 6.5-square-degree field of view. The installation of WFST near the summit of Saishiteng mountain in the Lenghu region is scheduled in summer of 2023, and the operation is planned to start three months later. WFST will scan the northern sky in four optical bands(u, g, r and i) at cadences from hourly/daily in the deep high-cadence survey(DHS) program, to semi-weekly in the wide field survey(WFS) program. During a photometric night, a nominal 30 s exposure in the WFS program will reach a depth of 22.27, 23.32, 22.84, and 22.31(AB magnitudes) in these four bands, respectively, allowing for the detection of a tremendous amount of transients in the low-z universe and a systematic investigation of the variability of Galactic and extragalactic objects. In the DHS program, intranight 90 s exposures as deep as 23(u) and 24 mag(g), in combination with target of opportunity follow-ups, will provide a unique opportunity to explore energetic transients in demand for high sensitivities, including the electromagnetic counterparts of gravitational wave events, supernovae within a few hours of their explosions,tidal disruption events and fast, luminous optical transients even beyond redshift of unity. In addition, the final 6-year co-added images, anticipated to reach g■25.8 mag in WFS or 1.5 mags deeper in DHS, will be of fundamental importance to general Galactic and extragalactic science. The highly uniform legacy surveys of WFST will serve as an indispensable complement to those of the Vera C. Rubin Observatory's Legacy Survey of Space and Time(LSST) that monitors the southern sky. 展开更多
关键词 optical telescope time domain astronomy photometric survey SUPERNOVAE multi-messenger events tidal disruption event
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Simultaneously Enhanced Thermal and Mechanical Properties of ZK60 Alloy Reinforced by Oriented Graphene Nanoplatelets
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作者 Baohong Zhu Xian Du +5 位作者 Fanjing Meng xuefeng wu Ke Liu Shubo Li Zhaohui Wang Wenbo Du 《Acta Metallurgica Sinica(English Letters)》 SCIE EI CAS CSCD 2023年第12期1999-2012,共14页
The lamellar and orientational characteristics of graphene nanoplatelets(GNPs)are crucial for reinforcing metal matrix composites,particularly in terms of their thermal properties.Two kinds of GNPs with plane sizes of... The lamellar and orientational characteristics of graphene nanoplatelets(GNPs)are crucial for reinforcing metal matrix composites,particularly in terms of their thermal properties.Two kinds of GNPs with plane sizes of 6µm and 80µm were respectively used as reinforcements in ZK60 alloy by powder metallurgy.The oriented distribution of GNPs in the matrix was obtained using a double-pass hot extrusion process,i.e.,a stepped extrusion with two consecutive extrusion ratios(10:1 and 16:1).Reinforced with 0.05 wt%oriented GNPs(80µm),the composite exhibited a tensile yield strength of 257 MPa,ultimate tensile strength of 342 MPa,elongation of 24.7%,and notably enhanced thermal conductivity of 128.3 W(mK)−1 even with refined grain size compared to the ZK60 alloy.The oriented GNPs in the matrix create a favorable path for efficient load and heat transfer,leading to the simultaneously enhancement of mechanical and thermal properties of the GNPs/ZK60 composites.This work is expected to broaden the application potential of GNPs as highly efficient reinforcements and provide a practical method for fabricating metal matrix composites. 展开更多
关键词 Graphene MAGNESIUM ORIENTATION Thermal properties Mechanical properties
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Optical observations of LIGO source GW 170817 by the Antarctic Survey Telescopes at Dome A,Antarctica 被引量:7
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作者 lei hu xuefeng wu +30 位作者 igor andreoni michael c.b.ashley jeff cooke xiangqun cui fujia du zigao dai bozhong gu yi hu haiping lu xiaoyan li zhengyang li ensi liang liangduan liu bin ma zhaohui shang tianrui sun n.b.suntzeff charling tao syed a.uddin lifan wang xiaofeng wang haikun wen di xiao jin xu ji yang shihai yang xiangyan yuan hongyan zhou hui zhang jilin zhou zonghong zhu 《Science Bulletin》 SCIE EI CAS CSCD 2017年第21期1433-1438,共6页
The LIGO detection of gravitational waves(GW) from merging black holes in 2015 marked the beginning of a new era in observational astronomy. The detection of an electromagnetic signal from a GW source is the critical ... The LIGO detection of gravitational waves(GW) from merging black holes in 2015 marked the beginning of a new era in observational astronomy. The detection of an electromagnetic signal from a GW source is the critical next step to explore in detail the physics involved. The Antarctic Survey Telescopes(AST3),located at Dome A, Antarctica, is uniquely situated for rapid response time-domain astronomy with its continuous night-time coverage during the austral winter. We report optical observations of the GW source(GW 170817) in the nearby galaxy NGC 4993 using AST3. The data show a rapidly fading transient at around 1 day after the GW trigger, with the i-band magnitude declining from 17:23 ± 0:13 magnitude to 17:72 ± 0:09 magnitude in ~1:8 h. The brightness and time evolution of the optical transient associated with GW 170817 are broadly consistent with the predictions of models involving merging binary neutron stars. We infer from our data that the merging process ejected about ~10^(-2) solar mass of radioactive material at a speed of up to 30% the speed of light. 展开更多
关键词 Gravitational waves Binary neutron stars Gamma-ray bursts
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Loss of hnRNP A1 in murine skeletal muscle exacerbates high-fat diet-induced onset of insulin resistance and hepatic steatosis 被引量:2
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作者 Mingxia Zhao Lihong Shen +11 位作者 Zijun Ouyang Manru Li Guoliang Deng Chenxi Yang Wei Zheng Lingdong Kong xuefeng wu Xudong wu Wenjie Guo Ye Yin Qiang Xu Yang Sun 《Journal of Molecular Cell Biology》 SCIE CAS CSCD 2020年第4期277-290,共14页
Impairment of glucose(Glu)uptake and storage by skeletal muscle is a prime risk factor for the development of metabolic diseases.Heterogeneous nuclear ribonucleoprotein A1(hnRNP Al)is a highly abundant RNA-binding pro... Impairment of glucose(Glu)uptake and storage by skeletal muscle is a prime risk factor for the development of metabolic diseases.Heterogeneous nuclear ribonucleoprotein A1(hnRNP Al)is a highly abundant RNA-binding protein that has been implicated in diverse cellular functions.The aim of this study was to investigate the function of hnRNP A1 on muscle tissue insulin sensitivity and systemic Glu homeostasis.Our results showed that conditional deletion of hnRNP Al in the muscle gave rise to a severe insulin resistance phenotype in mice fed a high-fat diet(HFD).Conditional knockout mice fed a HFD showed exacerbated obesity,insulin resistance,and hepatic steatosis.In vitro interference of hnRNP Al in C2C12 myotubes impaired insulin signal transduction and inhibited Glu uptake,whereas hnRNP Al overexpression in C2C12 myotubes protected against insulin resistance induced by supraphysiological concentrations of insulin.The expression and stability of glycogen synthase(gysl)mRNA were also decreased in the absence of hnRNP A l.Mechanistically,hnRNP Al interacted with gys l and stabilized its mRNA,thereby promoting glycogen synthesis and maintaining the insulin sensitivity in muscle tissue.Taken together,our findings are the first to show that reduced expression of hnRNP Al in skeletal muscle affects the metabolic properties and systemic insulin sensitivity by inhibiting glycogen synthesis. 展开更多
关键词 hnRNP A1 insulin resistance hepatic steatosis glycogen synthesis
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Observatory science with eXTP
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作者 Jean J.M.in 't Zand Enrico Bozzo +181 位作者 JinLu Qu Xiang-Dong Li Lorenzo Amati Yang Chen Immacolata Donnarumma Victor Doroshenko Stephen A.Drake Margarita Hernanz Peter A.Jenke Thomas J.Maccarone Simin Mahmoodifar Domitilla de Martino Alessandra De Rosa Elena M.Rossi Antonia Rowlinson Gloria Sala Giulia Stratta Thomas M.Tauris Joern Wilms xuefeng wu Ping Zhou Iván Agudo Diego Altamirano Jean-Luc Atteia Nils A.andersson M.Cristina Baglio David R.Ballantyne Altan Baykal Ehud Behar Tomaso Belloni Sudip Bhattacharyya Stefano Bianchi Anna Bilous Pere Blay Joao Braga Sφren Brandt Edward F.Brown Niccolo Bucciantini Luciano Burderi Edward M.Cackett Riccardo Campana Sergio Campana Piergiorgio Casella Yuri Cavecchi Frank Chambers Liang Chen Yu-Peng Chen Jér?me Chenevez Maria Chernyakova ChiChuan Jin Riccardo Ciolfi Elisa Costantini Andrew Cumming Antonino D'Aì Zi-Gao Dai Filippo D'Ammando Massimiliano De Pasquale Nathalie Degenaar Melania Del Santo Valerio D'Elia Tiziana Di Salvo Gerry Doyle Maurizio Falanga XiLong Fan Robert D.Ferdman Marco Feroci Federico Fraschetti Duncan K.Galloway Angelo F.Gambino Poshak Gandhi MingYu Ge Bruce Gendre Ramandeep Gill Diego G?tz Christian Gouiffès Paola Grandi Jonathan Granot Manuel Güdel Alexander Heger Craig O.Heinke Jeroen Homan Rosario Iaria Kazushi Iwasawa Luca Izzo Long Ji Peter G.Jonker Jordi José Jelle S.Kaastra Emrah Kalemci Oleg Kargaltsev Nobuyuki Kawai Laurens Keek Stefanie Komossa Ingo Kreykenbohm Lucien Kuiper Devaky Kunneriath Gang Li En-Wei Liang Manuel Linares Francesco Longo FangJun Lu Alexander A.Lutovinov Denys Malyshev Julien Malzac Antonios Manousakis Ian McHardy Missagh Mehdipour YunPeng Men Mariano Méndez Roberto P.Mignani Romana Mikusincova M.Coleman Miller Giovanni Miniutti Christian Motch Joonas Nättilä Emanuele Nardini Torsten Neubert Paul T.O'Brien Mauro Orlandini Julian P.Osborne Luigi Pacciani Stéphane Paltani Maurizio Paolillo Iossif E.Papadakis Biswajit Paul Alberto Pellizzoni Uria Peretz Miguel A.Pérez Torres Emanuele Perinati Chanda Prescod-Weinstein Pablo Reig Alessandro Riggio Jerome Rodriguez Pablo Rodríguez-Gil Patrizia Romano Agata Rózańska Takanori Sakamoto Tuomo Salmi Ruben Salvaterra andrea Sanna andrea Santangelo Tuomas Savolainen Stéphane Schanne Hendrik Schatz LiJing Shao andy Shearer Steven N.Shore Ben W.Stappers Tod E.Strohmayer Valery F.Suleimanov Jirí Svoboda F.-K.Thielemann Francesco Tombesi Diego F.Torres Eleonora Torresi Sara Turriziani andrea Vacchi Stefano Vercellone Jacco Vink Jian-Min Wang JunFeng Wang Anna L.Watts ShanShan Weng Nevin N.Weinberg Peter J.Wheatley Rudy Wijnands Tyrone E.Woods Stan E.Woosley ShaoLin Xiong YuPeng Xu Zhen Yan George Younes WenFei Yu Feng Yuan Luca Zampieri Silvia Zane andrzej A.Zdziarski Shuang-Nan Zhang Shu Zhang Shuo Zhang Xiao Zhang Michael Zingale 《Science China(Physics,Mechanics & Astronomy)》 SCIE EI CAS CSCD 2019年第2期97-138,共42页
In this White Paper we present the potential of the enhanced X-ray Timing and Polarimetry(eXTP) mission for studies related to Observatory Science targets. These include flaring stars, supernova remnants, accreting wh... In this White Paper we present the potential of the enhanced X-ray Timing and Polarimetry(eXTP) mission for studies related to Observatory Science targets. These include flaring stars, supernova remnants, accreting white dwarfs, low and high mass X-ray binaries, radio quiet and radio loud active galactic nuclei, tidal disruption events, and gamma-ray bursts. eXTP will be excellently suited to study one common aspect of these objects: their often transient nature. Developed by an international Consortium led by the Institute of High Energy Physics of the Chinese Academy of Science, the eXTP mission is expected to be launched in the mid 2020s. 展开更多
关键词 space research in struments nuclear astrophysics flare stars accretion and accretion disks mass loss and stellar winds cataclysmic binaries X-ray binaries supernova remnants active galactic nuclei X-ray bursts gamma-ray bursts gravitational waves
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Hydrophobic 1-octadecanethiol functionalized copper catalyst promotes robust high-current CO_(2) gas-diffusion electrolysis
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作者 Liangyao Xue xuefeng wu +5 位作者 Yuanwei Liu Beibei Xu Xuelu Wang Sheng Dai Pengfei Liu Huagui Yang 《Nano Research》 SCIE EI CSCD 2022年第2期1393-1398,共6页
The electrocatalytic reduction of CO_(2) presents a promising strategy in addressing environmental and energy crisis.Significant progress has been achieved via CO_(2) gas diffusion electrolysis,to react at high select... The electrocatalytic reduction of CO_(2) presents a promising strategy in addressing environmental and energy crisis.Significant progress has been achieved via CO_(2) gas diffusion electrolysis,to react at high selectivity and high rate.However,the gas diffusion layer(GDL)of the gas diffusion electrode(GDE)still suffers from low tolerance and limited active sites.Here,the hydrophobic 1-octadecanethiol molecular was functionalized over the Cu catalyst layer of the GDE,which simultaneously stabilizes the GDL and exposes abundant active solid-liquid-gas three-phase interfaces.The resultant GDE exhibits multi-carbon(C_(2+))product selectivity over faradaic efficiency(FE)of 70.0%in the range of 100 to 800 mA·cm^(-2),with the peak FE^(c2+)of 85.2%at 800 mA·cm^(-2).Notably,the strengthened GDE could continuously drive high-current electrolysis for more than 100 h without flooding.This work opens a new way to improve CO_(2) gas diffusion electrolysis via surface molecular engineering. 展开更多
关键词 CO_(2)reduction reaction gas diffusion electrolysis multi-carbon products molecular engineering HYDROPHOBICITY
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Regulation of antiviral innate immunity by deubiquitinase CYLD
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作者 Minying Zhang Andrew J Lee +1 位作者 xuefeng wu Shao-Cong Sun 《Cellular & Molecular Immunology》 SCIE CAS CSCD 2011年第6期502-504,共3页
An antiviral innate immune response involves induction of type I interferons(IFNs)and their subsequent autocrine and paracrine actions,but the underlying regulatory mechanisms are incompletely understood.Here we repor... An antiviral innate immune response involves induction of type I interferons(IFNs)and their subsequent autocrine and paracrine actions,but the underlying regulatory mechanisms are incompletely understood.Here we report that CYLD,a deubiquitinase that specifically digests lysine 63-linked ubiquitin chains,is required for antiviral host defense.Loss of CYLD renders mice considerably more susceptible to infection by vesicular stomatitis virus(VSV).Consistently,CYLD-deficient dendritic cells are more sensitive to VSV infection.This functional defect was not due to lack of type I IFN production but rather because of attenuated IFN receptor signaling.In the absence of CYLD,IFN-b is ineffective in the induction of antiviral genes and protection of cells from viral infection.These findings establish CYLD as a novel regulator of antiviral innate immunity and suggest a role for CYLD in regulating IFN receptor signaling. 展开更多
关键词 antiviral innate immunity CYLD deubiquitinase INTERFERON VSV
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MIL-125(Ti)中引入高价态钨元素以促进光催化产氢性能
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作者 张诣钧 毛芳欣 +5 位作者 刘袁微 吴雪枫 温春芳 戴升 刘鹏飞 杨化桂 《Science China Materials》 SCIE EI CAS CSCD 2022年第5期1237-1244,共8页
金属有机框架(Metal-organic frameworks, MOFs)材料具有高度可调控的多孔结构以及电子结构,在光催化领域非常有前景.本文利用MOFs的上述特性,将高价态的钨元素连接在MIL-125(Ti)中的Ti-oxo团簇上,得到了W-MIL-125.形成的W–O–Ti结构... 金属有机框架(Metal-organic frameworks, MOFs)材料具有高度可调控的多孔结构以及电子结构,在光催化领域非常有前景.本文利用MOFs的上述特性,将高价态的钨元素连接在MIL-125(Ti)中的Ti-oxo团簇上,得到了W-MIL-125.形成的W–O–Ti结构引发了从金属到团簇的电荷传输(Metal-to-cluster charge transfer, MCCT),且W-MIL-125具有更好的吸光性能.结构和谱学表征证明, MCCT过程能优化电荷的传输路径,有效地实现了载流子空间分离. W-MIL-125在光照条件下展现出更高的产氢性能,高达1110.7±63.7μmol g^(-1)h^(-1),是本体样品产氢速率的4.0倍.本工作为MOFs基材料的局域结构改性以提升光催化性能提供了新的思路. 展开更多
关键词 high-valence state metal-organic frameworks metal-to-cluster charge transfer photocatalytic hydrogen production
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Bandgap opening in MoTe2 thin flakes induced by surface oxidation
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作者 Yuan Gan Jiyuan Liang +11 位作者 Chang-woo Cho Si Li Yanping Guo Xiaoming Ma xuefeng wu Jinsheng Wen Xu Du Mingquan He Chang Liu Shengyuan A.Yang Kedong Wang Liyuan Zhang 《Frontiers of physics》 SCIE CSCD 2020年第3期105-111,共7页
Recently,the layered transition metal dichalcogenide 1T′-MoTe2 has generated considerable interest due to their superconducting and non-trivial topological properties.Here,we present a systematic study on 1T′-MoTe2 ... Recently,the layered transition metal dichalcogenide 1T′-MoTe2 has generated considerable interest due to their superconducting and non-trivial topological properties.Here,we present a systematic study on 1T′-MoTe2 single-crystal and exfoliated thin-flakes by means of electrical transport,scanning tunnelling microscope(STM)measurements and band structure calculations.For a bulk sample,it exhibits large magneto-resistance(MR)and Shubnikov–de Hass oscillations inρxx and a series of Hall plateaus inρxy at low temperatures.Meanwhile,the MoTe2 thin films were intensively investigated with thickness dependence.For samples,without encapsulation,an apparent transition from the intrinsic metallic to insulating state is observed by reducing thickness.In such thin films,we also observed a suppression of the MR and weak anti-localization(WAL)effects.We attributed these effects to disorders originated from the extrinsic surface chemical reaction,which is consistent with the density functional theory(DFT)calculations and in-situ STM results.In contrast to samples without encapsulated protection,we discovered an interesting superconducting transition for those samples with hexagonal Boron Nitride(h-BN)film protection.Our results indicate that the metallic or superconducting behavior is its intrinsic state,and the insulating behavior is likely caused by surface oxidation in few layer 1T’-MoTe2 flakes. 展开更多
关键词 two-dimensional materials metal-insulator transition layered transition metal dichalcogenides(TMDs) surface oxidation
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Ultrathin Hematite Photoanode with Gradient Ti Doping
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作者 Pengfei Liu Chongwu Wang +3 位作者 Lijie Wang xuefeng wu Lirong Zheng Hua Gui Yang 《Research》 EI CAS 2020年第1期883-890,共8页
The poor photoelectrochemical(PEC)performance derived from insufficient charge separation in hematite photoanode crucially limits its application.Gradient doping with band bending in a large region is then considered ... The poor photoelectrochemical(PEC)performance derived from insufficient charge separation in hematite photoanode crucially limits its application.Gradient doping with band bending in a large region is then considered as a promising strategy,facilitating the charge transfer ability due to the built-in electric field.Herein,we developed a synthetic strategy to prepare gradient Ti-doped ultrathin hematite photoelectrode and systematically investigated its PEC performance.The as-synthesized electrode(1.5-6.0%doping level from the surface to the substrate)delivered a photocurrent of about 1.30mAcm^(-2) at 1.23V versus the reversible hydrogen electrode(RHE),which is nearly 100%higher than that of homogeneously doped hematite electrode.The enhanced charge transfer property,induced by the energy band bending due to the built-in electric field,has been further confirmed by electrochemical measurements.This strategy of gradient doping should be adaptable and can be applied for other functional materials in various fields. 展开更多
关键词 electrode DOPING BENDING
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