The in-situ instrumentation technique for measuring mercury and itsspeciation downstream a utility 100 MW pulverized coal (PC) fired boiler system was developed andconducted by the use of the Ontario hydro method (OHM...The in-situ instrumentation technique for measuring mercury and itsspeciation downstream a utility 100 MW pulverized coal (PC) fired boiler system was developed andconducted by the use of the Ontario hydro method (OHM) consistent with American standard test methodtogether with the semi-continuous emissions monitoring (SCEM) system as well as a mobile laboratoryfor mercury monitoring. The mercury and its speciation concentrations including participate mercuryat three locations of before air preheater, before electrostatic precipitator (ESP) and after ESPwere measured using the OHM and SCEM methods under normal operation conditions of the boiler systemas a result of firing a bituminous coal. The vapor-phase total mercury Hg(VT) concentration declinedwith the decrease of flue gas temperature because of mercury species transformation from oxidizedmercury to particulate mercury as the flue gas moved downstream from the air preheater to the ESPand after the ESP. A good agreement for Hg°, Hg^(2+) and Hg( VT) was obtained between the twomethods in the ash-free area. But in the dense particle-laden flue gas area, there appeared to be abig bias for mercury speciation owing to dust cake formed in the filter of OHM sampling probe. Theparticulateaffinity to the flue gas mercury and the impacts of sampling condition to accuracy ofmeasure were discussed.展开更多
为了改进水文建模过程中的不确定性处理,采用一种融合全局优化和数据同化(Simultaneous Optimization and Data Assimilation,SODA)的混合框架,对Hy MOD模型进行了不确定性分析,并与经典SCEM-UA方法进行了比较。SODA方法具有如下特点:(1...为了改进水文建模过程中的不确定性处理,采用一种融合全局优化和数据同化(Simultaneous Optimization and Data Assimilation,SODA)的混合框架,对Hy MOD模型进行了不确定性分析,并与经典SCEM-UA方法进行了比较。SODA方法具有如下特点:(1)具备较高的参数搜索效率和寻优能力;(2)明确考虑包括输入、输出、参数以及模型结构在内的重要不确定性来源。SODA方法在渭河流域的实例应用结果表明:与SCEM-UA方法相比,SODA方法不仅显著提高了预报精度,而且推求出了性质更为优良的预报区间。SODA方法的成功应用,有助于模型概念的改进及对水文系统功能的理解。展开更多
文摘The in-situ instrumentation technique for measuring mercury and itsspeciation downstream a utility 100 MW pulverized coal (PC) fired boiler system was developed andconducted by the use of the Ontario hydro method (OHM) consistent with American standard test methodtogether with the semi-continuous emissions monitoring (SCEM) system as well as a mobile laboratoryfor mercury monitoring. The mercury and its speciation concentrations including participate mercuryat three locations of before air preheater, before electrostatic precipitator (ESP) and after ESPwere measured using the OHM and SCEM methods under normal operation conditions of the boiler systemas a result of firing a bituminous coal. The vapor-phase total mercury Hg(VT) concentration declinedwith the decrease of flue gas temperature because of mercury species transformation from oxidizedmercury to particulate mercury as the flue gas moved downstream from the air preheater to the ESPand after the ESP. A good agreement for Hg°, Hg^(2+) and Hg( VT) was obtained between the twomethods in the ash-free area. But in the dense particle-laden flue gas area, there appeared to be abig bias for mercury speciation owing to dust cake formed in the filter of OHM sampling probe. Theparticulateaffinity to the flue gas mercury and the impacts of sampling condition to accuracy ofmeasure were discussed.
文摘为了改进水文建模过程中的不确定性处理,采用一种融合全局优化和数据同化(Simultaneous Optimization and Data Assimilation,SODA)的混合框架,对Hy MOD模型进行了不确定性分析,并与经典SCEM-UA方法进行了比较。SODA方法具有如下特点:(1)具备较高的参数搜索效率和寻优能力;(2)明确考虑包括输入、输出、参数以及模型结构在内的重要不确定性来源。SODA方法在渭河流域的实例应用结果表明:与SCEM-UA方法相比,SODA方法不仅显著提高了预报精度,而且推求出了性质更为优良的预报区间。SODA方法的成功应用,有助于模型概念的改进及对水文系统功能的理解。
