In this paper,we define a new class of control functions through aggregate special functions.These class of control functions help us to stabilize and approximate a tri-additiveψ-functional inequality to get a better...In this paper,we define a new class of control functions through aggregate special functions.These class of control functions help us to stabilize and approximate a tri-additiveψ-functional inequality to get a better estimation for permuting tri-homomorphisms and permuting tri-derivations in unital C*-algebras and Banach algebras by the vector-valued alternative fixed point theorem.展开更多
To better understand the role of the-NH_(2)group in adsorption process of phenolic wastewaters,NH_(2)-functionalized MIL-53(Al)composites with activated carbon(NH_(2)-M(Al)@(B)AC)were prepared.The results showed that ...To better understand the role of the-NH_(2)group in adsorption process of phenolic wastewaters,NH_(2)-functionalized MIL-53(Al)composites with activated carbon(NH_(2)-M(Al)@(B)AC)were prepared.The results showed that the-NH_(2)group could increase the mesopore volume for composites,which promotes mass transfer and full utilization of active sites,because hierarchical mesopore structure makes the adsorbent easier to enter the internal adsorption sites.Furthermore,the introduction of the-NH_(2)group can improve the adsorption capacity,decrease the activation energy,and enhance the interaction between the adsorbent and p-nitrophenol,demonstrating that the-NH_(2)group plays a crucial role in the adsorption of p-nitrophenol.The density functional theory calculation results show that the H-bond interaction between the-NH_(2)group in the adsorbent and the-NO_(2)in the p-nitrophenol(adsorption energy of -35.5 kJ·mol^(-1)),and base-acid interaction between the primary-NH_(2)group in the adsorbent and the acidic-OH group in the p-nitrophenol(adsorption energy of -27.3 kJ·mol^(-1))are predominant mechanisms for adsorption in terms of the NH_(2)-functionalized adsorbent.Both NH_(2)-functionalized M(Al)@AC and M(Al)@BAC composites exhibited higher p-nitrophenol adsorption capacity than corresponding nonfunctionalized composites.Among the composites,the NH_(2)-M(Al)@BAC had the highest p-nitrophenol adsorption capacity of 474 mg·g^(-1).展开更多
Cubic equations of state(EOSs) are simple and easy at calculation. One way of improving the accuracy of a cubic EOS is through the modification of temperature-dependent energy parameter by using alpha-function.The ind...Cubic equations of state(EOSs) are simple and easy at calculation. One way of improving the accuracy of a cubic EOS is through the modification of temperature-dependent energy parameter by using alpha-function.The industrial applications of natural gas are very wide and as a result, prediction of thermodynamic properties and phase behavior of natural gas is an important part of design for such processes. In this work we develop a newα-function for the Peng-Robinson(PR) EOS with the parameters optimized especially for natural gas components.The parameters are generalized as a linear function of acentric factor. The results are compared to the predictions from original PR EOS and other α-functions in literature. It is shown that the new α-function presents a good accuracy with the average deviation of 1.42% for natural gas components.展开更多
In this paper, we reported a first-principles investigation on the structural and electronic properties of O adsorption on the γ-TiAI(111) surface, to illustrate the oxidation process. It has been found that: (1...In this paper, we reported a first-principles investigation on the structural and electronic properties of O adsorption on the γ-TiAI(111) surface, to illustrate the oxidation process. It has been found that: (1) rather than stopping with one full monolayer of coverage, oxygen adsorption continues till two monolayer coverage, rendering an oxide-like structure; (2) full structural relaxation makes the surface oxide layer denser and more stable, which hinders the subsequent O adsorption (oxidation) process. In addition, the transformation from metal to oxide surface was identified by analyzing the local density of states through the oxidation steps, which was in good agreement with experimental results.展开更多
Humic acid(HA)was carbonized at 300,400 and 500℃ and then functionalized with 1 wt%–12 wt%Fe(Ⅲ)respectively[CHA300/400/500-Fe(Ⅲ)].Adsorption of such Fe(III)-functionalized carbonized HA as adsorbents to aqueous te...Humic acid(HA)was carbonized at 300,400 and 500℃ and then functionalized with 1 wt%–12 wt%Fe(Ⅲ)respectively[CHA300/400/500-Fe(Ⅲ)].Adsorption of such Fe(III)-functionalized carbonized HA as adsorbents to aqueous tetracycline(TC:25 mg·L^-1)was studied.The adsorption equilibrium time for CHA400-Fe(Ⅲ)to TC was 6 h faster and the adsorption removal efficiency(Re)was two times higher than that of HA/CHA.The adsorption Reof CHA400-Fe(Ⅲ)loaded 10%iron[CHA400-(10%)Fe(Ⅲ)]to TC could reach 99.8%at 8 h and still kept80.6%after 8 cycles.The adsorption kinetics were well fitted to the pseudo-second-order equation and the adsorption isotherms could be well delineated via Langmuir equations(R^2N 0.99),indicating that the homogeneous chemical adsorption of TC occurred on the adsorbents.The main adsorption mechanisms of TC were complexation Fe(III)and hydrophobic distribution.Electropositive and electronegative repulsion between TC and CHA400-(10%)Fe(Ⅲ)at lowly p H(2)and highly p H(8–10)respectively,leaded to the relatively low adsorption capacity and more notable influence of ion concentration.When the p H was between 4 and 8,TC mainly existed in neutral molecules(TCH2),so the influence of ion concentration was not obvious.The dynamic adsorption results showed that the CHA400-(10%)Fe(Ⅲ)could continuously treat about 2.4 L TC(27 mg·L^-1)wastewater with the effluent concentration as low as 0.068 mg·L^-1.Our study suggested a broad application prospect of a new,effective,lowcost and environment-friendly adsorbent CHA400-(10%)Fe(Ⅲ)for treatment of low-concentration TC polluted wastewater.展开更多
The object of this article is to study and develop the generalized fractional calcu- lus operators given by Saigo and Maeda in 1996. We establish generalized fractional calculus formulas involving the product of R-fun...The object of this article is to study and develop the generalized fractional calcu- lus operators given by Saigo and Maeda in 1996. We establish generalized fractional calculus formulas involving the product of R-function, Appell function F3 and a general class of poly- nomials. The results obtained provide unification and extension of the results given by Saxena et al. [13], Srivastava and Grag [17], Srivastava et al. [20], and etc. The results are obtained in compact form and are useful in preparing some tables of operators of fractional calculus. On account of the general nature of the Saigo-Maeda operators, R-function, and a general class of polynomials a large number of new and known results involving Saigo fractional calculus operators and several special functions notably H-function, /-function, Mittag-Leffier function, generalized Wright hypergeometric function, generalized Bessel-Maitland function follow as special cases of our main findings.展开更多
目的:探究2型糖尿病肾病(DN)患者外周血白细胞介素-4(IL-4)、γ-干扰素(INF-γ)、纤溶抑制物(TAFI)表达及其与肾小球滤过功能的相关性。方法:比较分析糖尿病肾病组(n=102)与健康组(n=54)的IL-4、INF-γ及TAFI表达水平;将糖尿病肾病组分...目的:探究2型糖尿病肾病(DN)患者外周血白细胞介素-4(IL-4)、γ-干扰素(INF-γ)、纤溶抑制物(TAFI)表达及其与肾小球滤过功能的相关性。方法:比较分析糖尿病肾病组(n=102)与健康组(n=54)的IL-4、INF-γ及TAFI表达水平;将糖尿病肾病组分为3组,比较分析3组患者的IL-4、INF-γ及TAFI表达水平;采用Spearman分析IL-4、INF-γ及TAFI表达水平与2型DN患者肾小球滤过功能的相关性。结果:糖尿病肾病组IL-4、INF-γ及TAFI水平高于健康组(P<0.05);不同肾功能损伤程度患者IL-4、INF-γ及TAFI比较,差异有统计学意义(P<0.05);Spearman相关性分析结果显示,IL-4与24 h UmAlb负相关(P<0.05),与eGFR、Scr无相关性(P>0.05);INF-γ与eGFR负相关,与Scr、24 h UmAlb正相关(P<0.05);TAFI与eGFR负相关,与Scr、24 h UmAlb正相关(P<0.05)。结论:2型DN患者外周血IL-4、INF-γ及TAFI表达水平与患者的肾小球滤过功能存在相关性,可通过检测外周血IL-4、INF-γ及TAFI的表达水平为2型DN患者肾小球滤过功能的评估和临床治疗提供参考。展开更多
基金partially supported by the Natural Sciences and Engineering Research Council of Canada(2019-03907)。
文摘In this paper,we define a new class of control functions through aggregate special functions.These class of control functions help us to stabilize and approximate a tri-additiveψ-functional inequality to get a better estimation for permuting tri-homomorphisms and permuting tri-derivations in unital C*-algebras and Banach algebras by the vector-valued alternative fixed point theorem.
基金supported by the National Natural Science Foundation of China(22008134)。
文摘To better understand the role of the-NH_(2)group in adsorption process of phenolic wastewaters,NH_(2)-functionalized MIL-53(Al)composites with activated carbon(NH_(2)-M(Al)@(B)AC)were prepared.The results showed that the-NH_(2)group could increase the mesopore volume for composites,which promotes mass transfer and full utilization of active sites,because hierarchical mesopore structure makes the adsorbent easier to enter the internal adsorption sites.Furthermore,the introduction of the-NH_(2)group can improve the adsorption capacity,decrease the activation energy,and enhance the interaction between the adsorbent and p-nitrophenol,demonstrating that the-NH_(2)group plays a crucial role in the adsorption of p-nitrophenol.The density functional theory calculation results show that the H-bond interaction between the-NH_(2)group in the adsorbent and the-NO_(2)in the p-nitrophenol(adsorption energy of -35.5 kJ·mol^(-1)),and base-acid interaction between the primary-NH_(2)group in the adsorbent and the acidic-OH group in the p-nitrophenol(adsorption energy of -27.3 kJ·mol^(-1))are predominant mechanisms for adsorption in terms of the NH_(2)-functionalized adsorbent.Both NH_(2)-functionalized M(Al)@AC and M(Al)@BAC composites exhibited higher p-nitrophenol adsorption capacity than corresponding nonfunctionalized composites.Among the composites,the NH_(2)-M(Al)@BAC had the highest p-nitrophenol adsorption capacity of 474 mg·g^(-1).
文摘Cubic equations of state(EOSs) are simple and easy at calculation. One way of improving the accuracy of a cubic EOS is through the modification of temperature-dependent energy parameter by using alpha-function.The industrial applications of natural gas are very wide and as a result, prediction of thermodynamic properties and phase behavior of natural gas is an important part of design for such processes. In this work we develop a newα-function for the Peng-Robinson(PR) EOS with the parameters optimized especially for natural gas components.The parameters are generalized as a linear function of acentric factor. The results are compared to the predictions from original PR EOS and other α-functions in literature. It is shown that the new α-function presents a good accuracy with the average deviation of 1.42% for natural gas components.
基金supported by the National Basic Research Program of China under grant No.2006CB605103
文摘In this paper, we reported a first-principles investigation on the structural and electronic properties of O adsorption on the γ-TiAI(111) surface, to illustrate the oxidation process. It has been found that: (1) rather than stopping with one full monolayer of coverage, oxygen adsorption continues till two monolayer coverage, rendering an oxide-like structure; (2) full structural relaxation makes the surface oxide layer denser and more stable, which hinders the subsequent O adsorption (oxidation) process. In addition, the transformation from metal to oxide surface was identified by analyzing the local density of states through the oxidation steps, which was in good agreement with experimental results.
基金financially supported by the National Natural Science Foundation of China(No.51641209)。
文摘Humic acid(HA)was carbonized at 300,400 and 500℃ and then functionalized with 1 wt%–12 wt%Fe(Ⅲ)respectively[CHA300/400/500-Fe(Ⅲ)].Adsorption of such Fe(III)-functionalized carbonized HA as adsorbents to aqueous tetracycline(TC:25 mg·L^-1)was studied.The adsorption equilibrium time for CHA400-Fe(Ⅲ)to TC was 6 h faster and the adsorption removal efficiency(Re)was two times higher than that of HA/CHA.The adsorption Reof CHA400-Fe(Ⅲ)loaded 10%iron[CHA400-(10%)Fe(Ⅲ)]to TC could reach 99.8%at 8 h and still kept80.6%after 8 cycles.The adsorption kinetics were well fitted to the pseudo-second-order equation and the adsorption isotherms could be well delineated via Langmuir equations(R^2N 0.99),indicating that the homogeneous chemical adsorption of TC occurred on the adsorbents.The main adsorption mechanisms of TC were complexation Fe(III)and hydrophobic distribution.Electropositive and electronegative repulsion between TC and CHA400-(10%)Fe(Ⅲ)at lowly p H(2)and highly p H(8–10)respectively,leaded to the relatively low adsorption capacity and more notable influence of ion concentration.When the p H was between 4 and 8,TC mainly existed in neutral molecules(TCH2),so the influence of ion concentration was not obvious.The dynamic adsorption results showed that the CHA400-(10%)Fe(Ⅲ)could continuously treat about 2.4 L TC(27 mg·L^-1)wastewater with the effluent concentration as low as 0.068 mg·L^-1.Our study suggested a broad application prospect of a new,effective,lowcost and environment-friendly adsorbent CHA400-(10%)Fe(Ⅲ)for treatment of low-concentration TC polluted wastewater.
基金NBHM Department of Atomic Energy,Government of India,Mumbai for the finanicai assistance under PDF sanction no.2/40(37)/2014/R&D-II/14131
文摘The object of this article is to study and develop the generalized fractional calcu- lus operators given by Saigo and Maeda in 1996. We establish generalized fractional calculus formulas involving the product of R-function, Appell function F3 and a general class of poly- nomials. The results obtained provide unification and extension of the results given by Saxena et al. [13], Srivastava and Grag [17], Srivastava et al. [20], and etc. The results are obtained in compact form and are useful in preparing some tables of operators of fractional calculus. On account of the general nature of the Saigo-Maeda operators, R-function, and a general class of polynomials a large number of new and known results involving Saigo fractional calculus operators and several special functions notably H-function, /-function, Mittag-Leffier function, generalized Wright hypergeometric function, generalized Bessel-Maitland function follow as special cases of our main findings.
文摘目的:探究2型糖尿病肾病(DN)患者外周血白细胞介素-4(IL-4)、γ-干扰素(INF-γ)、纤溶抑制物(TAFI)表达及其与肾小球滤过功能的相关性。方法:比较分析糖尿病肾病组(n=102)与健康组(n=54)的IL-4、INF-γ及TAFI表达水平;将糖尿病肾病组分为3组,比较分析3组患者的IL-4、INF-γ及TAFI表达水平;采用Spearman分析IL-4、INF-γ及TAFI表达水平与2型DN患者肾小球滤过功能的相关性。结果:糖尿病肾病组IL-4、INF-γ及TAFI水平高于健康组(P<0.05);不同肾功能损伤程度患者IL-4、INF-γ及TAFI比较,差异有统计学意义(P<0.05);Spearman相关性分析结果显示,IL-4与24 h UmAlb负相关(P<0.05),与eGFR、Scr无相关性(P>0.05);INF-γ与eGFR负相关,与Scr、24 h UmAlb正相关(P<0.05);TAFI与eGFR负相关,与Scr、24 h UmAlb正相关(P<0.05)。结论:2型DN患者外周血IL-4、INF-γ及TAFI表达水平与患者的肾小球滤过功能存在相关性,可通过检测外周血IL-4、INF-γ及TAFI的表达水平为2型DN患者肾小球滤过功能的评估和临床治疗提供参考。