An innovative complex lidar system deployed on an airborne rotorcraft platform for remote sensing of atmospheric pollution is proposed and demonstrated.The system incorporates integrated-path differential absorption l...An innovative complex lidar system deployed on an airborne rotorcraft platform for remote sensing of atmospheric pollution is proposed and demonstrated.The system incorporates integrated-path differential absorption lidar(DIAL) and coherent-doppler lidar(CDL) techniques using a dual tunable TEA CO_(2)laser in the 9—11 μm band and a 1.55 μm fiber laser.By combining the principles of differential absorption detection and pulsed coherent detection,the system enables agile and remote sensing of atmospheric pollution.Extensive static tests validate the system’s real-time detection capabilities,including the measurement of concentration-path-length product(CL),front distance,and path wind speed of air pollution plumes over long distances exceeding 4 km.Flight experiments is conducted with the helicopter.Scanning of the pollutant concentration and the wind field is carried out in an approximately 1 km slant range over scanning angle ranges from 45°to 65°,with a radial resolution of 30 m and10 s.The test results demonstrate the system’s ability to spatially map atmospheric pollution plumes and predict their motion and dispersion patterns,thereby ensuring the protection of public safety.展开更多
This study focuses on air quality in southern Benin in order to show public authorities what the Beninese populations are exposed to for efficient decision-making. Two sampling campaigns were carried out, one in the w...This study focuses on air quality in southern Benin in order to show public authorities what the Beninese populations are exposed to for efficient decision-making. Two sampling campaigns were carried out, one in the wet period and the other in the dry season. The measurements were taken using a monitor called an “Air Quality Monitor”. For data processing, the multiple comparison methods of Dun (1961) and the Wilcoxon test were used. To maintain legitimacy, all spatial data were included in the official cartographic repository of Benin: WGS 1984, Transverse Mercator Universe Projection (UTM), Zone 31 North. The Moran statistic was used to measure the levels of spatial autocorrelation of the variables studied and to test the significance. In order to locate the spatial subsets, the local spatial association indices of Anselin Local Moran and Getis-Ord, Gi* were used. In terms of results, on the 13 monitoring sites and the 8 parameters chosen to determine air quality, we do not note any significant inter-seasonal difference. Of the eight parameters, only three parameters present spatial autocorrelation leading to predictions of ambient air quality over the entire study area based on the distance separating the points, namely, PM<sub>2.5</sub>, PM<sub>10</sub> and ambient air quality index (AQI). The localities affected by atmospheric pollution in South Benin are located in the south-western part of Benin, headed by Cotonou, which is heavily polluted by CO<sub>2</sub>, TCOV, PM<sub>10</sub> and PM<sub>2.5</sub>.展开更多
Over the past few years, research on the quality of air and microorganisms presen</span><span style="font-family:Verdana;">t in the atmosphere and spore composition of the environment has increas...Over the past few years, research on the quality of air and microorganisms presen</span><span style="font-family:Verdana;">t in the atmosphere and spore composition of the environment has increased significantly, due to concerns over health risks for humans, plants, and animals. This study shows the abundance and diversity of microorganisms </span></span><span style="font-family:Verdana;">and </span><span style="font-family:Verdana;">the</span><span style="font-family:""><span style="font-family:Verdana;"> atmosphere of an urban nucleus, that is, the city of Valladolid (Spain). We considered the conditions of precipitation, humidity </span><span style="font-family:Verdana;">and</span><span style="font-family:Verdana;"> wind, and the presence of some atmospheric pollutants such as nitrogen dioxide and nitrogen monoxide (NO</span><sub><span style="font-family:Verdana;">2</span></sub><span style="font-family:Verdana;">/NO), carbon monoxide (CO), sulfur dioxide, and particulate matter (</span></span><span style="font-family:Verdana;"><i></span><i><span style="font-family:Verdana;">PM</span></i><i><span style="font-family:Verdana;"></i></span></i><span style="font-family:Verdana;">10 and </span><span style="font-family:Verdana;"><i></span><i><span style="font-family:Verdana;">PM</span></i><i><span style="font-family:Verdana;"></i></span></i><span style="font-family:""><span style="font-family:Verdana;">2.5). After their deposition </span><span style="font-family:Verdana;">present</span><span style="font-family:Verdana;"> at five geographic points with different environmental conditions, differences </span><span style="font-family:Verdana;">were</span><span style="font-family:Verdana;"> observed in the proportion of bacteria growth which </span><span style="font-family:Verdana;">w</span></span><span style="font-family:Verdana;">as</span><span style="font-family:Verdana;"> char</span><span style="font-family:Verdana;">acterized by growth in several specific culture media. Most identified the Gram-negative bacteria identified in the air samples collected belong to the genera </span><span style="font-family:Verdana;"><i></span><i><span style="font-family:Verdana;">Staphylococcus</span></i><i><span style="font-family:Verdana;"></i></span></i><span style="font-family:Verdana;"> and </span><span style="font-family:Verdana;"><i></span><i><span style="font-family:Verdana;">Streptococcus</span></i><i><span style="font-family:Verdana;"></i></span></i><span style="font-family:Verdana;">. Gram-positive bacteria were present at a low rate.展开更多
The uncertainty in assessing the numerous atmospheric pollutants transported via wind from arid and semi-arid regions is affecting the glacial ecosystem. In our study area due to the complexity of the system, a promin...The uncertainty in assessing the numerous atmospheric pollutants transported via wind from arid and semi-arid regions is affecting the glacial ecosystem. In our study area due to the complexity of the system, a prominent seasonal difference noticed among major ions(Ca^(2+), Mg^(2+), SO_4^(2-), and NO_3^-). There is a need for understanding the ions cycling as a whole and the directionality of the feedback loops in the system. Therefore, we provide an appraisal of our current hypothesis for seasonal difference in major ion concentration from snow samples for two corresponding years(2013 and 2015) at Dokriani Glacier. A systematic study of chemical compositionsin the shallow snow pit from Dokriani Glacier was undertaken for the pre-monsoon season to understand the cycling of major ions from atmosphere to solute acquisition process. The intimating connections of ions cycling in snow and its temporal behavior was observed and analyzed through various statistical tests. Among major ions, the SO_4^(2-)has the highest concentration among anions on an average considered as 14.21% in 2013 and 29.46% in 2015. On the other side Ca^(2+) is the dominant cation contributing 28.22% in 2013 and 15.3% in 2015 on average. The average ratio of Na+/Cl-was higher in 2013 whereas lower in 2015. The backward trajectory analysis suggests the possible sources of the ions transported from Central Asia through the Western Disturbance(WD) as a prominent source of winter precipitation mainly in the Central Himalaya. Ionicconcentration of Ca^(2+) in cations was highly dominated while in anion SO_4^(2-)played the major role. Factor analysis and correlation matrix suggested that, the precipitation chemistry is mostly influenced by anthropogenic, crustal, and sea salt sources over the studied region. The elemental cycling through ocean, atmosphere and biosphere opens up new ways to understand the geochemical processes operating at the glacierized catchments of the Himalaya. Moreover, increasing the field-based studies in the coming decades would also have the certain advantage in overcoming the conceptual and computational geochemical modelling difficulties.展开更多
To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shan...To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shantou of Guangdong Province on the basis of an overall assessment of regional natural environment, social economic state of development, pollution sources and atmospheric environmental quality. Compared with actual monitoring results in a studied region, simulation values fell within the range of two times of error and were evenly distributed in the two sides of the monitored values. Predicted with the largest emission model method, the largest emission of sulfur dioxide would be 54 279.792 tons per year in 2010. Conclusion The mathematical model established and revised on the basis of GIS is more rational and suitable for the regional characteristics of total amount control of air pollutants.展开更多
[ Objective] The research aimed to analyze characteristics of the atmospheric particulate pollutants ( PMlo and PM2.s) in Wenzhou City. [Method] We analyzed interannual change rule of the dust haze in Wenzhou during...[ Objective] The research aimed to analyze characteristics of the atmospheric particulate pollutants ( PMlo and PM2.s) in Wenzhou City. [Method] We analyzed interannual change rule of the dust haze in Wenzhou during 1978 -2008. Moreover, we respectively set monitoring points in urban district, industrial park and beauty spot of Wenzhou in summer and winter of 2010. Element, ion and polycyclic aromatic hydrocarbon com- positions and morphology of the particulate matter were analyzed. [ Result] Dust haze in Wenzhou City mainly appeared in winter and spring, which was related to local meteorological condition. In summer and winter, both PMlo and PM2.s concentrations presented the characteristic of industrial park 〉 commercial area 〉 beauty spot. Chain-like particle aggregates and ultrafine particles were main composition of the atmospheric particulate matter in Wenzhou. Contribution rate of the spherical particle amount was smaller than metropolis, which was related to local industry and traffic. Fe element had the most content in particulate matter. Mass concentration was mainly composed of 6 elements, such as Na, Si, S, K, Ca and Fe. Total concentration of the six elements occupied 70% -80% of the 16 elements. SO^- and NH4* in particulate matter were higher. They were mainly from human activity. Main compositions of the polycyclic aromatic hydrocarbon were naphthalene, anthracene, benzo (b) fluoranthene, indeno (1,2, 3-cd) pyrene and benzo (g, h, i) perylene, which was related to abrupt increase of the motor vehicle. [ Condusion] The research provided scientific basis and technology support for controlling atmospheric particulate matter pollution in Wenzhou City by government and related department.展开更多
Through the analysis on the migratory diffusion process of atmospheric pollutants,we proposed to seek atmospheric pollutant source with surface soil sample of data.Based on Gaussian plume model and deposition model,at...Through the analysis on the migratory diffusion process of atmospheric pollutants,we proposed to seek atmospheric pollutant source with surface soil sample of data.Based on Gaussian plume model and deposition model,atmospheric pollutants distribution model was deduced,with which a schema matching source seeking model was established.The model was used to seek the pollutant source by using the arsenic data in the surface soil sample of a city.展开更多
This paper takes seven cities in the Tibet Autonomous Region as the study area,and collects data from more than 20 monitoring stations covering the Tibet Autonomous Region in the ambient air quality online monitoring ...This paper takes seven cities in the Tibet Autonomous Region as the study area,and collects data from more than 20 monitoring stations covering the Tibet Autonomous Region in the ambient air quality online monitoring platform to analyze the spatial and temporal variation characteristics of PM_(10),PM_(2.5),SO_(2),NO_(2),CO and O_(3)MAD 8(ozone daily maximum 8-h average).The results show that(1)the multi-year average PM_(2.5)concentration in Tibet Autonomous Region is 12.03μg/m^(3);the multi-year average PM_(10)concentration is 28.27μg/m^(3);the multi-year average CO concentration is 0.59 mg/m^(3);the multi-year average NO_(2)concentration is 12.34μg/m^(3);the multi-year average SO_(2)concentration is 7.00μg/m^(3);the multi-year average value of O_(3)is 89.54μg/m^(3).The concentrations of atmospheric pollutants all meet the primary concentration limits of the Ambient Air Quality Standards(GB 3095-2012).(2)The air environment in the Tibet Autonomous Region in spring is relatively poor,with about 20%of excellent days and 80%of good days.The air environment is relatively good in summer,autumn and winter,with about 65%-87%of excellent days and 35%-13%of good days.The air environment quality of Tibet Autonomous Region is excellent:winter>autumn>summer>spring,and good:spring>summer>autumn>winter.(3)Except for NO_(2)which is more influenced by automobile exhaust and SO_(2)which is more influenced by man-made source in winter,the ambient air quality in Tibet Autonomous Region is less influenced by industry.The variability characteristics of the six atmospheric pollutants studied in this paper are strongly correlated with the unique natural environment of Tibet(air pressure,altitude,wind speed,temperature,precipitation,solar radiation,etc).展开更多
Air pollution as one of the major environmental issues in modern society,has already brought severe impact to human life and production,thus it is an urgent task for studying environmental and ecological science to so...Air pollution as one of the major environmental issues in modern society,has already brought severe impact to human life and production,thus it is an urgent task for studying environmental and ecological science to solve this issue that has bothered human society for the last centuries.Scientists have endeavored to figure out the laws of atmospheric pollutant diffusion using various mathematical models and statistical models,and drawn some precious conclusions.This paper explored the basic model of atmospheric diffusion—modeling and solution of Gaussian Diffusion Model,clarify its principles and operation forms,then applied the model into the PM_(2.5) atmospheric diffusion cases,make the program planning base on the results of model calculation,and get the final conclusion.展开更多
Studies in various regions of the world have revealed that air pollution can have a significant influence on local climate. This study therefore considers the impact of concentration levels of atmospheric pollutants o...Studies in various regions of the world have revealed that air pollution can have a significant influence on local climate. This study therefore considers the impact of concentration levels of atmospheric pollutants on local climate of Delta state, Nigeria. Monthly and annual averaging of the daily pollutant concentrations and meteorological parameters within the period of investigation was carried out. Descriptive Statistics, correlation analysis, coefficient of determination (R<sup>2</sup>) analysis and least squares regression analysis of the selected meteorological parameters with CH<sub>4</sub> and O<sub>3</sub> concentrations for the period of 2003 to 2012 and NO<sub>2</sub> and CO<sub>2</sub> concentrations for the period of 2011 to 2014 were carried out. The regression relationship was then used to obtain predicted values for the meteorological parameters within the period of investigation. The results of the descriptive statistics of annual averages of CH<sub>4</sub>, O<sub>3</sub>, NO<sub>2</sub> and CO<sub>2</sub> concentrations within the period of investigation revealed that the emission levels breached FEPA and EGASPIN limits. The results of the correlation analysis indicated that CO<sub>2</sub> had a strong significant positive correlation with temperature with a correlation coefficient of 0.962, while a moderate negative correlation coefficient of 0.549 was obtained for CH<sub>4</sub>, and very weak correlation coefficients of -0.167 and 0.077 were obtained for O<sub>3</sub> and NO<sub>2</sub> respectively. CH<sub>4</sub>, O<sub>3</sub> and CO<sub>2</sub> had a moderately significant positive correlation with solar radiation with correlation coefficients of 0.661, 0.571 and 0.656 respectively, while a weak negative correlation coefficient of 0.106 was obtained for NO<sub>2</sub>. CH<sub>4</sub> had a strong significant positive correlation with relative humidity with a correlation coefficient of 0.859, while moderate correlation coefficients of -0.516 and 0.646 were obtained for NO<sub>2</sub> and CO<sub>2</sub> respectively, and a weak correlation coefficient of 0.345 was obtained for O<sub>3</sub>. CO<sub>2</sub> and CH<sub>4</sub> had a strong significant correlation with wind speed with correlation coefficients of 0.951 and -0.906 respectively, while a moderate negative correlation coefficient of 0.518 was obtained for O<sub>3</sub>, and a weak negative correlation coefficient of 0.317 was obtained for NO<sub>2</sub>. The predicted values of the meteorological parameters showed a significant level of agreement with their measured values. Therefore, among the atmospheric pollutants postulated as influencing meteorological parameters, CO<sub>2</sub> appears to be the most strongly significant in explaining temperature variations in this region of Niger Delta, with correlation coefficient of 96.2% and coefficient of determination (R<sup>2</sup>) of 0.926, implying that CO<sub>2</sub> influenced 92.6% variation in temperature in this part of Niger Delta within the period of investigation.展开更多
A critical environmental problem facing the Niger Delta region is Air Pollution. This study therefore analyses concentration levels of atmospheric pollutants in the region. Statistical analysis of CH<sub>4</s...A critical environmental problem facing the Niger Delta region is Air Pollution. This study therefore analyses concentration levels of atmospheric pollutants in the region. Statistical analysis of CH<sub>4</sub> and O<sub>3</sub> concentrations for the period of 2003 to 2012 and NO<sub>2</sub> and CO<sub>2</sub> concentrations for the period of 2011 to 2014 were carried out. The results showed that concentration levels of the pollutants were lower during the rainy season than during the dry year time. This is due to higher occurrences of atmospheric instability during the rainy season. On the other hand, ozone (O<sub>3</sub>) concentration reached its peak value during the peak period of the rainy season unlike the other pollutants. In all likelihood, some of the ozone-depleting substances such as aerosols and atmospheric hydrogen chloride become soluble in water and are being washed off by precipitation during rainy season, thereby leading to increased tropospheric ozone concentration during the rainy season. The study also revealed a steady increase in the concentration of CO<sub>2</sub> within the period of investigation. This steady increase in CO<sub>2</sub> can be traced to the alarming increase in anthropogenic activities which appreciably increases the amount of CO<sub>2</sub> in the atmosphere. Methane (CH<sub>4</sub>) had higher standard deviation values than carbon dioxide (CO<sub>2</sub>), meaning that on a per molecule basis, a proportional rise in CH<sub>4</sub> is much more effective as a greenhouse gas than a similar increase in CO<sub>2</sub>. However, CO<sub>2</sub> has a greater effect than CH<sub>4</sub> on climate change owing to its higher atmospheric concentration. The Mann-Kendall rank statistics of the atmospheric pollutants revealed that the standardization variables U(t<sub>i</sub>) and U'(t<sub>i</sub>) have a sequential fluctuating behavior around a zero level.展开更多
This study focuses on monitoring the exposure of populations in South Benin to atmospheric pollution. Thirteen (13) monitoring points were identified where the Air quality measurements were taken using autonomous elec...This study focuses on monitoring the exposure of populations in South Benin to atmospheric pollution. Thirteen (13) monitoring points were identified where the Air quality measurements were taken using autonomous electronic devices called “Air Quality Monitor”. Calibrated and turned on, the measuring device automatically determines the concentrations of carbon dioxide CO<sub>2</sub>, Total Organic Compounds, methanal (HCHO), particulate matter PM<sub>2.5</sub> and PM<sub>10</sub>, temperature in degrees Fahrenheit and relative humidity (RH). Per site, air pollution levels are recorded for 5 minutes every 30 minutes from 7 a.m. to 6 p.m. After the analyses, it appears that the carbon dioxide CO<sub>2</sub> contents vary from 400 to 1444 ppm with an average of 486.80 ± 184.3 ppm, the daily contents of Total Volatile Organic Compounds from 0.01 to 6 .91 mg/m<sup>3</sup> with a daily average of 0.36 ± 0.65 mg/m<sup>3</sup>, aldehydes from 0.005 to 3 mg/m<sup>3</sup> with an average of 0.05 ± 0.17 mg/m<sup>3</sup>, for particulate matter of diameters less than or equal to 2.5 μm (PM<sub>2.5</sub>) pollution levels vary between 5 and 173.8 μg/m<sup>3</sup> with an average of 21.5 ± 17.62 μg/m<sup>3</sup>. On the other hand, for PM<sub>10</sub>, the contents vary from 5 to 449.6 μg/m<sup>3</sup> with an average of 28.17 ± 31.74 μg/m<sup>3</sup>, the Air Quality Index (AQI) varies from 0, 3 to 243 with an average of 39 ± 33.16. From the results observed, it appears that the south-western part of South Benin is heavily polluted by CO<sub>2</sub>, Total Volatile Organic Compounds, PM<sub>10</sub> and especially PM<sub>2.5</sub> with the city of Cotonou at its head, in particular the Red Star crossroads, the Toyota crossroads and the crossroads after the friendship stadium. The impacts of this pollution could be significant on sensitive people such as the elderly, newborns and patients with acute and chronic respiratory illnesses.展开更多
This paper describes the relation and difference of "emission up to standards" and "total quantity control" ofmain atmospheric pollutants, as well as their legal status. It points out that the tota...This paper describes the relation and difference of "emission up to standards" and "total quantity control" ofmain atmospheric pollutants, as well as their legal status. It points out that the total quantity control is a good approachto solve a problem that environmental quality do not yet reach the requirements in an area where emission concentrationhas came up to standards, or to solve a problem that the interregional transportation of pollutants (e. g. acid rain) arises.And further, it put forward five proposals for the total quantity control.[展开更多
The newly revised and enlarged main contents of the Law of Prevention and Control of Atmospheric Pollution are described, The macro impacts of the law on the power industry development are analyzed mainly in respects ...The newly revised and enlarged main contents of the Law of Prevention and Control of Atmospheric Pollution are described, The macro impacts of the law on the power industry development are analyzed mainly in respects to power demand and readjustment of power structure and layout. clean production and pollution control level, scientific management of environmental protection, in accordance with law as well as changes of construction and operation costs. And finally, several questions worthy to be noted in course of implementation of the new law are enumerated.展开更多
Based on emergency monitoring work flow analysis of atmospheric pollution incidents, key technical problems involved in the atmospheric pollution monitoring scheme based on GIS was studied, including the orientation o...Based on emergency monitoring work flow analysis of atmospheric pollution incidents, key technical problems involved in the atmospheric pollution monitoring scheme based on GIS was studied, including the orientation of the accident site, the inquiry of the distribution of the emergency monitoring units and the groups of experts and the determination of the shortest path of emergency monitoring researchers and equipments arriving to the accident site as well as the integrated technology of Gaussian model with GIS which was mainly researched. The automatic prototype system of the emergency monitoring optimized scheme of the atmospheric pollution based on GIS was analyzed with the case of atmospheric pollution accident in Kunshan.展开更多
The Pb-monitoring program was extended for 6 years from 2002 to 2007 at 17 representative urban sites (6 traffic, 5 industrial, and 6 residential sites), and 3 suburban sites to assess the lead pollution in fine par...The Pb-monitoring program was extended for 6 years from 2002 to 2007 at 17 representative urban sites (6 traffic, 5 industrial, and 6 residential sites), and 3 suburban sites to assess the lead pollution in fine particulate matter (PM2.5) after phasing out leaded gasoline in Shanghai. Compared with Pb levels reported in other places, the Pb pollution in Shanghai is still serious after phasing out leaded gasoline, which remains at high concentration range (213-176 ng/m^3) in PM2.5 in winter. Significant spatial variation of Pb concentrations and strong seasonal variation of higher Pb concentration in winter than that in summer were detected. The size distribution of Pb in particulate matter has a unimodat mode that peaks at approximately 0.154-1.59 μm particle diameter, indicating that Pb is mainly concentrated in fine fraction. Lead in the fine fraction is enriched by a factor of 103-104 relative to Pb abundance in crust. Eight categories of Pb pollution sources were identified in the PM2.5 in the winter of 2007 in Shanghai. The important emission sources among them are vehicle exhaust derived from combustion of unleaded gasoline, metaUurgic industry emission, and coal combustion emission.展开更多
Remote sensing technology, as the most advanced method for collecting data, along with the common ways often used in the past on research of environmental science, was integrated to study the relationship between envi...Remote sensing technology, as the most advanced method for collecting data, along with the common ways often used in the past on research of environmental science, was integrated to study the relationship between environmental pollution of coal mine and spectral characteristics of nearby plants. With compositive index and mean reflectivity at near infrared, a regression equation was established, and a conclusion was made that spectral reflectivity can be used to distinguish regions with different pollution degree. Through testing with real status of the research region, it is verified that this kind of integration and conclusion not only are helpful for human being in controlling the movement law of pollutants and the corresponding change of coal mine environmental quality but also bring a new way for the research of environment problems of coal mine.展开更多
The attainment of suitable ambient air quality standards is a matter of great concern for successfully hosting the ⅩⅩⅣ Olympic Winter Games(OWG). Transport patterns and potential sources of pollutants in Zhangjiako...The attainment of suitable ambient air quality standards is a matter of great concern for successfully hosting the ⅩⅩⅣ Olympic Winter Games(OWG). Transport patterns and potential sources of pollutants in Zhangjiakou(ZJK) were investigated using pollutant monitoring datasets and a dispersion model. The PM_(2.5) concentration during February in ZJK has increased slightly(28%) from 2018 to 2021, mostly owing to the shift of main potential source regions of west-central Inner Mongolia and Mongolian areas(2015–18) to the North China Plain and northern Shanxi Province(NCPS) after 2018.Using CO as an indicator, the relative contributions of the different regions to the receptor site(ZJK) were evaluated based on the source-receptor-relationship method(SRR) and an emission inventory. We found that the relative contribution of pollutants from NCPS increased from 33% to 68% during 2019–21. Central Inner Mongolia(CIM) also has an important impact on ZJK under unfavorable weather conditions. This study demonstrated that the effect of pollution control measures in the NCPS and CIM should be strengthened to ensure that the air quality meets the standard during the ⅩⅩⅣ OWG.展开更多
With rapid economic growth in China, anthropogenic reactive nitrogen (Nr) emissions have more than doubled over the last two or three decades. Atmospheric Nr pollution is an environmental concern in China especially...With rapid economic growth in China, anthropogenic reactive nitrogen (Nr) emissions have more than doubled over the last two or three decades. Atmospheric Nr pollution is an environmental concern in China especially in megacities such as Beijing. In order to identify the impact of emission sources on atmospheric Nr pollution, we measured atmospheric Nr concentrations and their isotopic composition (δ15N) dynamics at three typical sites: landfill, pig farm and road traffic sites in Beijing from April 2010 to March 2011. Passive samplers were used for monitoring ammonia (NH3) and nitrogen dioxide (NO2), two major Nr species, while their δ15N values were measured by a diffusion method combined with mass spectrometer approach. The raw water pool of the landfill and fattening house of the pig farm were important NH3 sources with mean NH3 concentrations being 2,829 and 2,369 μg/m3, respectively, while the road traffic site was a minor NH3 source (10.6 μg/m3). NH3 concentrations at sites besides the landfill and roads were high in summer and low in winter due to the annual variation of temperature and the change of emission source intensity. In contrast, the NH3 concentrations inside the pig farm house were high in winter and low in summer, for the barn windows were open in summer and closed in winter. The mean NO2 concentrations were 89.8, 32.9 and 23.0 μg/m3 at the road traffic, the landfill and pig farm sites, respectively. Due to vehicle fuel combustion, NO2 concentration at the road traffic was the highest among the three sources, and the road traffic was a main NO2 emission source. PM10, pNH4* and pNO3- concentrations in particulate matter were higher in summer than in winter (except PM10 for the pig farm). The δ15NH3 values ranged from -19.14‰ to 7.82‰, with an average of-0.05‰ for the landfill site, and the lowest values were observed in June and July. The δ15NH3 values for the pig farm site ranged from -29.78‰ to-14.05‰ with an average of-24.51‰, and the 515NH3 values were more negative in summer than in the other seasons. The (515NO2 values were -9.63%o to 7.04‰ with an average of -3.72%0 for the road traffic site. The δ15NO2 values were more negative in summer than those in the other seasons. The different δ15N values for the various Nr species in different sources may serve as important indicators for identifying atmospheric Nr sources in megacities. The results may also provide the theoretical basis for research on the atmospheric N deposition and its sources.展开更多
文摘An innovative complex lidar system deployed on an airborne rotorcraft platform for remote sensing of atmospheric pollution is proposed and demonstrated.The system incorporates integrated-path differential absorption lidar(DIAL) and coherent-doppler lidar(CDL) techniques using a dual tunable TEA CO_(2)laser in the 9—11 μm band and a 1.55 μm fiber laser.By combining the principles of differential absorption detection and pulsed coherent detection,the system enables agile and remote sensing of atmospheric pollution.Extensive static tests validate the system’s real-time detection capabilities,including the measurement of concentration-path-length product(CL),front distance,and path wind speed of air pollution plumes over long distances exceeding 4 km.Flight experiments is conducted with the helicopter.Scanning of the pollutant concentration and the wind field is carried out in an approximately 1 km slant range over scanning angle ranges from 45°to 65°,with a radial resolution of 30 m and10 s.The test results demonstrate the system’s ability to spatially map atmospheric pollution plumes and predict their motion and dispersion patterns,thereby ensuring the protection of public safety.
文摘This study focuses on air quality in southern Benin in order to show public authorities what the Beninese populations are exposed to for efficient decision-making. Two sampling campaigns were carried out, one in the wet period and the other in the dry season. The measurements were taken using a monitor called an “Air Quality Monitor”. For data processing, the multiple comparison methods of Dun (1961) and the Wilcoxon test were used. To maintain legitimacy, all spatial data were included in the official cartographic repository of Benin: WGS 1984, Transverse Mercator Universe Projection (UTM), Zone 31 North. The Moran statistic was used to measure the levels of spatial autocorrelation of the variables studied and to test the significance. In order to locate the spatial subsets, the local spatial association indices of Anselin Local Moran and Getis-Ord, Gi* were used. In terms of results, on the 13 monitoring sites and the 8 parameters chosen to determine air quality, we do not note any significant inter-seasonal difference. Of the eight parameters, only three parameters present spatial autocorrelation leading to predictions of ambient air quality over the entire study area based on the distance separating the points, namely, PM<sub>2.5</sub>, PM<sub>10</sub> and ambient air quality index (AQI). The localities affected by atmospheric pollution in South Benin are located in the south-western part of Benin, headed by Cotonou, which is heavily polluted by CO<sub>2</sub>, TCOV, PM<sub>10</sub> and PM<sub>2.5</sub>.
文摘Over the past few years, research on the quality of air and microorganisms presen</span><span style="font-family:Verdana;">t in the atmosphere and spore composition of the environment has increased significantly, due to concerns over health risks for humans, plants, and animals. This study shows the abundance and diversity of microorganisms </span></span><span style="font-family:Verdana;">and </span><span style="font-family:Verdana;">the</span><span style="font-family:""><span style="font-family:Verdana;"> atmosphere of an urban nucleus, that is, the city of Valladolid (Spain). We considered the conditions of precipitation, humidity </span><span style="font-family:Verdana;">and</span><span style="font-family:Verdana;"> wind, and the presence of some atmospheric pollutants such as nitrogen dioxide and nitrogen monoxide (NO</span><sub><span style="font-family:Verdana;">2</span></sub><span style="font-family:Verdana;">/NO), carbon monoxide (CO), sulfur dioxide, and particulate matter (</span></span><span style="font-family:Verdana;"><i></span><i><span style="font-family:Verdana;">PM</span></i><i><span style="font-family:Verdana;"></i></span></i><span style="font-family:Verdana;">10 and </span><span style="font-family:Verdana;"><i></span><i><span style="font-family:Verdana;">PM</span></i><i><span style="font-family:Verdana;"></i></span></i><span style="font-family:""><span style="font-family:Verdana;">2.5). After their deposition </span><span style="font-family:Verdana;">present</span><span style="font-family:Verdana;"> at five geographic points with different environmental conditions, differences </span><span style="font-family:Verdana;">were</span><span style="font-family:Verdana;"> observed in the proportion of bacteria growth which </span><span style="font-family:Verdana;">w</span></span><span style="font-family:Verdana;">as</span><span style="font-family:Verdana;"> char</span><span style="font-family:Verdana;">acterized by growth in several specific culture media. Most identified the Gram-negative bacteria identified in the air samples collected belong to the genera </span><span style="font-family:Verdana;"><i></span><i><span style="font-family:Verdana;">Staphylococcus</span></i><i><span style="font-family:Verdana;"></i></span></i><span style="font-family:Verdana;"> and </span><span style="font-family:Verdana;"><i></span><i><span style="font-family:Verdana;">Streptococcus</span></i><i><span style="font-family:Verdana;"></i></span></i><span style="font-family:Verdana;">. Gram-positive bacteria were present at a low rate.
基金funded by the Department of Science and Technology,Government of India,New Delhi
文摘The uncertainty in assessing the numerous atmospheric pollutants transported via wind from arid and semi-arid regions is affecting the glacial ecosystem. In our study area due to the complexity of the system, a prominent seasonal difference noticed among major ions(Ca^(2+), Mg^(2+), SO_4^(2-), and NO_3^-). There is a need for understanding the ions cycling as a whole and the directionality of the feedback loops in the system. Therefore, we provide an appraisal of our current hypothesis for seasonal difference in major ion concentration from snow samples for two corresponding years(2013 and 2015) at Dokriani Glacier. A systematic study of chemical compositionsin the shallow snow pit from Dokriani Glacier was undertaken for the pre-monsoon season to understand the cycling of major ions from atmosphere to solute acquisition process. The intimating connections of ions cycling in snow and its temporal behavior was observed and analyzed through various statistical tests. Among major ions, the SO_4^(2-)has the highest concentration among anions on an average considered as 14.21% in 2013 and 29.46% in 2015. On the other side Ca^(2+) is the dominant cation contributing 28.22% in 2013 and 15.3% in 2015 on average. The average ratio of Na+/Cl-was higher in 2013 whereas lower in 2015. The backward trajectory analysis suggests the possible sources of the ions transported from Central Asia through the Western Disturbance(WD) as a prominent source of winter precipitation mainly in the Central Himalaya. Ionicconcentration of Ca^(2+) in cations was highly dominated while in anion SO_4^(2-)played the major role. Factor analysis and correlation matrix suggested that, the precipitation chemistry is mostly influenced by anthropogenic, crustal, and sea salt sources over the studied region. The elemental cycling through ocean, atmosphere and biosphere opens up new ways to understand the geochemical processes operating at the glacierized catchments of the Himalaya. Moreover, increasing the field-based studies in the coming decades would also have the certain advantage in overcoming the conceptual and computational geochemical modelling difficulties.
文摘To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shantou of Guangdong Province on the basis of an overall assessment of regional natural environment, social economic state of development, pollution sources and atmospheric environmental quality. Compared with actual monitoring results in a studied region, simulation values fell within the range of two times of error and were evenly distributed in the two sides of the monitored values. Predicted with the largest emission model method, the largest emission of sulfur dioxide would be 54 279.792 tons per year in 2010. Conclusion The mathematical model established and revised on the basis of GIS is more rational and suitable for the regional characteristics of total amount control of air pollutants.
基金Supported by Study on Formation Reason and Early Warning of the Dust Haze and Atmospheric Complex Pollution Control in Wenzhou City ( R20090124)
文摘[ Objective] The research aimed to analyze characteristics of the atmospheric particulate pollutants ( PMlo and PM2.s) in Wenzhou City. [Method] We analyzed interannual change rule of the dust haze in Wenzhou during 1978 -2008. Moreover, we respectively set monitoring points in urban district, industrial park and beauty spot of Wenzhou in summer and winter of 2010. Element, ion and polycyclic aromatic hydrocarbon com- positions and morphology of the particulate matter were analyzed. [ Result] Dust haze in Wenzhou City mainly appeared in winter and spring, which was related to local meteorological condition. In summer and winter, both PMlo and PM2.s concentrations presented the characteristic of industrial park 〉 commercial area 〉 beauty spot. Chain-like particle aggregates and ultrafine particles were main composition of the atmospheric particulate matter in Wenzhou. Contribution rate of the spherical particle amount was smaller than metropolis, which was related to local industry and traffic. Fe element had the most content in particulate matter. Mass concentration was mainly composed of 6 elements, such as Na, Si, S, K, Ca and Fe. Total concentration of the six elements occupied 70% -80% of the 16 elements. SO^- and NH4* in particulate matter were higher. They were mainly from human activity. Main compositions of the polycyclic aromatic hydrocarbon were naphthalene, anthracene, benzo (b) fluoranthene, indeno (1,2, 3-cd) pyrene and benzo (g, h, i) perylene, which was related to abrupt increase of the motor vehicle. [ Condusion] The research provided scientific basis and technology support for controlling atmospheric particulate matter pollution in Wenzhou City by government and related department.
文摘Through the analysis on the migratory diffusion process of atmospheric pollutants,we proposed to seek atmospheric pollutant source with surface soil sample of data.Based on Gaussian plume model and deposition model,atmospheric pollutants distribution model was deduced,with which a schema matching source seeking model was established.The model was used to seek the pollutant source by using the arsenic data in the surface soil sample of a city.
基金Supported by National Natural Science Foundation of China(21677116)National Key Research&Development Program of China(2019YFC1904101)。
文摘This paper takes seven cities in the Tibet Autonomous Region as the study area,and collects data from more than 20 monitoring stations covering the Tibet Autonomous Region in the ambient air quality online monitoring platform to analyze the spatial and temporal variation characteristics of PM_(10),PM_(2.5),SO_(2),NO_(2),CO and O_(3)MAD 8(ozone daily maximum 8-h average).The results show that(1)the multi-year average PM_(2.5)concentration in Tibet Autonomous Region is 12.03μg/m^(3);the multi-year average PM_(10)concentration is 28.27μg/m^(3);the multi-year average CO concentration is 0.59 mg/m^(3);the multi-year average NO_(2)concentration is 12.34μg/m^(3);the multi-year average SO_(2)concentration is 7.00μg/m^(3);the multi-year average value of O_(3)is 89.54μg/m^(3).The concentrations of atmospheric pollutants all meet the primary concentration limits of the Ambient Air Quality Standards(GB 3095-2012).(2)The air environment in the Tibet Autonomous Region in spring is relatively poor,with about 20%of excellent days and 80%of good days.The air environment is relatively good in summer,autumn and winter,with about 65%-87%of excellent days and 35%-13%of good days.The air environment quality of Tibet Autonomous Region is excellent:winter>autumn>summer>spring,and good:spring>summer>autumn>winter.(3)Except for NO_(2)which is more influenced by automobile exhaust and SO_(2)which is more influenced by man-made source in winter,the ambient air quality in Tibet Autonomous Region is less influenced by industry.The variability characteristics of the six atmospheric pollutants studied in this paper are strongly correlated with the unique natural environment of Tibet(air pressure,altitude,wind speed,temperature,precipitation,solar radiation,etc).
基金Program of Regional Tourism Development and Rural Revitalization Coordination Center (2020Z04)。
文摘Air pollution as one of the major environmental issues in modern society,has already brought severe impact to human life and production,thus it is an urgent task for studying environmental and ecological science to solve this issue that has bothered human society for the last centuries.Scientists have endeavored to figure out the laws of atmospheric pollutant diffusion using various mathematical models and statistical models,and drawn some precious conclusions.This paper explored the basic model of atmospheric diffusion—modeling and solution of Gaussian Diffusion Model,clarify its principles and operation forms,then applied the model into the PM_(2.5) atmospheric diffusion cases,make the program planning base on the results of model calculation,and get the final conclusion.
文摘Studies in various regions of the world have revealed that air pollution can have a significant influence on local climate. This study therefore considers the impact of concentration levels of atmospheric pollutants on local climate of Delta state, Nigeria. Monthly and annual averaging of the daily pollutant concentrations and meteorological parameters within the period of investigation was carried out. Descriptive Statistics, correlation analysis, coefficient of determination (R<sup>2</sup>) analysis and least squares regression analysis of the selected meteorological parameters with CH<sub>4</sub> and O<sub>3</sub> concentrations for the period of 2003 to 2012 and NO<sub>2</sub> and CO<sub>2</sub> concentrations for the period of 2011 to 2014 were carried out. The regression relationship was then used to obtain predicted values for the meteorological parameters within the period of investigation. The results of the descriptive statistics of annual averages of CH<sub>4</sub>, O<sub>3</sub>, NO<sub>2</sub> and CO<sub>2</sub> concentrations within the period of investigation revealed that the emission levels breached FEPA and EGASPIN limits. The results of the correlation analysis indicated that CO<sub>2</sub> had a strong significant positive correlation with temperature with a correlation coefficient of 0.962, while a moderate negative correlation coefficient of 0.549 was obtained for CH<sub>4</sub>, and very weak correlation coefficients of -0.167 and 0.077 were obtained for O<sub>3</sub> and NO<sub>2</sub> respectively. CH<sub>4</sub>, O<sub>3</sub> and CO<sub>2</sub> had a moderately significant positive correlation with solar radiation with correlation coefficients of 0.661, 0.571 and 0.656 respectively, while a weak negative correlation coefficient of 0.106 was obtained for NO<sub>2</sub>. CH<sub>4</sub> had a strong significant positive correlation with relative humidity with a correlation coefficient of 0.859, while moderate correlation coefficients of -0.516 and 0.646 were obtained for NO<sub>2</sub> and CO<sub>2</sub> respectively, and a weak correlation coefficient of 0.345 was obtained for O<sub>3</sub>. CO<sub>2</sub> and CH<sub>4</sub> had a strong significant correlation with wind speed with correlation coefficients of 0.951 and -0.906 respectively, while a moderate negative correlation coefficient of 0.518 was obtained for O<sub>3</sub>, and a weak negative correlation coefficient of 0.317 was obtained for NO<sub>2</sub>. The predicted values of the meteorological parameters showed a significant level of agreement with their measured values. Therefore, among the atmospheric pollutants postulated as influencing meteorological parameters, CO<sub>2</sub> appears to be the most strongly significant in explaining temperature variations in this region of Niger Delta, with correlation coefficient of 96.2% and coefficient of determination (R<sup>2</sup>) of 0.926, implying that CO<sub>2</sub> influenced 92.6% variation in temperature in this part of Niger Delta within the period of investigation.
文摘A critical environmental problem facing the Niger Delta region is Air Pollution. This study therefore analyses concentration levels of atmospheric pollutants in the region. Statistical analysis of CH<sub>4</sub> and O<sub>3</sub> concentrations for the period of 2003 to 2012 and NO<sub>2</sub> and CO<sub>2</sub> concentrations for the period of 2011 to 2014 were carried out. The results showed that concentration levels of the pollutants were lower during the rainy season than during the dry year time. This is due to higher occurrences of atmospheric instability during the rainy season. On the other hand, ozone (O<sub>3</sub>) concentration reached its peak value during the peak period of the rainy season unlike the other pollutants. In all likelihood, some of the ozone-depleting substances such as aerosols and atmospheric hydrogen chloride become soluble in water and are being washed off by precipitation during rainy season, thereby leading to increased tropospheric ozone concentration during the rainy season. The study also revealed a steady increase in the concentration of CO<sub>2</sub> within the period of investigation. This steady increase in CO<sub>2</sub> can be traced to the alarming increase in anthropogenic activities which appreciably increases the amount of CO<sub>2</sub> in the atmosphere. Methane (CH<sub>4</sub>) had higher standard deviation values than carbon dioxide (CO<sub>2</sub>), meaning that on a per molecule basis, a proportional rise in CH<sub>4</sub> is much more effective as a greenhouse gas than a similar increase in CO<sub>2</sub>. However, CO<sub>2</sub> has a greater effect than CH<sub>4</sub> on climate change owing to its higher atmospheric concentration. The Mann-Kendall rank statistics of the atmospheric pollutants revealed that the standardization variables U(t<sub>i</sub>) and U'(t<sub>i</sub>) have a sequential fluctuating behavior around a zero level.
文摘This study focuses on monitoring the exposure of populations in South Benin to atmospheric pollution. Thirteen (13) monitoring points were identified where the Air quality measurements were taken using autonomous electronic devices called “Air Quality Monitor”. Calibrated and turned on, the measuring device automatically determines the concentrations of carbon dioxide CO<sub>2</sub>, Total Organic Compounds, methanal (HCHO), particulate matter PM<sub>2.5</sub> and PM<sub>10</sub>, temperature in degrees Fahrenheit and relative humidity (RH). Per site, air pollution levels are recorded for 5 minutes every 30 minutes from 7 a.m. to 6 p.m. After the analyses, it appears that the carbon dioxide CO<sub>2</sub> contents vary from 400 to 1444 ppm with an average of 486.80 ± 184.3 ppm, the daily contents of Total Volatile Organic Compounds from 0.01 to 6 .91 mg/m<sup>3</sup> with a daily average of 0.36 ± 0.65 mg/m<sup>3</sup>, aldehydes from 0.005 to 3 mg/m<sup>3</sup> with an average of 0.05 ± 0.17 mg/m<sup>3</sup>, for particulate matter of diameters less than or equal to 2.5 μm (PM<sub>2.5</sub>) pollution levels vary between 5 and 173.8 μg/m<sup>3</sup> with an average of 21.5 ± 17.62 μg/m<sup>3</sup>. On the other hand, for PM<sub>10</sub>, the contents vary from 5 to 449.6 μg/m<sup>3</sup> with an average of 28.17 ± 31.74 μg/m<sup>3</sup>, the Air Quality Index (AQI) varies from 0, 3 to 243 with an average of 39 ± 33.16. From the results observed, it appears that the south-western part of South Benin is heavily polluted by CO<sub>2</sub>, Total Volatile Organic Compounds, PM<sub>10</sub> and especially PM<sub>2.5</sub> with the city of Cotonou at its head, in particular the Red Star crossroads, the Toyota crossroads and the crossroads after the friendship stadium. The impacts of this pollution could be significant on sensitive people such as the elderly, newborns and patients with acute and chronic respiratory illnesses.
文摘This paper describes the relation and difference of "emission up to standards" and "total quantity control" ofmain atmospheric pollutants, as well as their legal status. It points out that the total quantity control is a good approachto solve a problem that environmental quality do not yet reach the requirements in an area where emission concentrationhas came up to standards, or to solve a problem that the interregional transportation of pollutants (e. g. acid rain) arises.And further, it put forward five proposals for the total quantity control.[
文摘The newly revised and enlarged main contents of the Law of Prevention and Control of Atmospheric Pollution are described, The macro impacts of the law on the power industry development are analyzed mainly in respects to power demand and readjustment of power structure and layout. clean production and pollution control level, scientific management of environmental protection, in accordance with law as well as changes of construction and operation costs. And finally, several questions worthy to be noted in course of implementation of the new law are enumerated.
基金Supported by Scientific and Technological Projects of China "863" Plan
文摘Based on emergency monitoring work flow analysis of atmospheric pollution incidents, key technical problems involved in the atmospheric pollution monitoring scheme based on GIS was studied, including the orientation of the accident site, the inquiry of the distribution of the emergency monitoring units and the groups of experts and the determination of the shortest path of emergency monitoring researchers and equipments arriving to the accident site as well as the integrated technology of Gaussian model with GIS which was mainly researched. The automatic prototype system of the emergency monitoring optimized scheme of the atmospheric pollution based on GIS was analyzed with the case of atmospheric pollution accident in Kunshan.
基金supported by the National Natural Sci-ence Foundation of China (No. 10775172, 10675159)the Major Project of Knowledge Innovation Program of Chinese Academy of Sciences (No.KJCX3.SYW.N3)This work has been performed under the approval of the Photon Factory (PF) Program Advisory Committee (No.2007G502)
文摘The Pb-monitoring program was extended for 6 years from 2002 to 2007 at 17 representative urban sites (6 traffic, 5 industrial, and 6 residential sites), and 3 suburban sites to assess the lead pollution in fine particulate matter (PM2.5) after phasing out leaded gasoline in Shanghai. Compared with Pb levels reported in other places, the Pb pollution in Shanghai is still serious after phasing out leaded gasoline, which remains at high concentration range (213-176 ng/m^3) in PM2.5 in winter. Significant spatial variation of Pb concentrations and strong seasonal variation of higher Pb concentration in winter than that in summer were detected. The size distribution of Pb in particulate matter has a unimodat mode that peaks at approximately 0.154-1.59 μm particle diameter, indicating that Pb is mainly concentrated in fine fraction. Lead in the fine fraction is enriched by a factor of 103-104 relative to Pb abundance in crust. Eight categories of Pb pollution sources were identified in the PM2.5 in the winter of 2007 in Shanghai. The important emission sources among them are vehicle exhaust derived from combustion of unleaded gasoline, metaUurgic industry emission, and coal combustion emission.
文摘Remote sensing technology, as the most advanced method for collecting data, along with the common ways often used in the past on research of environmental science, was integrated to study the relationship between environmental pollution of coal mine and spectral characteristics of nearby plants. With compositive index and mean reflectivity at near infrared, a regression equation was established, and a conclusion was made that spectral reflectivity can be used to distinguish regions with different pollution degree. Through testing with real status of the research region, it is verified that this kind of integration and conclusion not only are helpful for human being in controlling the movement law of pollutants and the corresponding change of coal mine environmental quality but also bring a new way for the research of environment problems of coal mine.
基金the National Key Scientific and Technological Infrastructure project “Earth System Science Numerical Simulator Facility” (Earth Lab)
文摘The attainment of suitable ambient air quality standards is a matter of great concern for successfully hosting the ⅩⅩⅣ Olympic Winter Games(OWG). Transport patterns and potential sources of pollutants in Zhangjiakou(ZJK) were investigated using pollutant monitoring datasets and a dispersion model. The PM_(2.5) concentration during February in ZJK has increased slightly(28%) from 2018 to 2021, mostly owing to the shift of main potential source regions of west-central Inner Mongolia and Mongolian areas(2015–18) to the North China Plain and northern Shanxi Province(NCPS) after 2018.Using CO as an indicator, the relative contributions of the different regions to the receptor site(ZJK) were evaluated based on the source-receptor-relationship method(SRR) and an emission inventory. We found that the relative contribution of pollutants from NCPS increased from 33% to 68% during 2019–21. Central Inner Mongolia(CIM) also has an important impact on ZJK under unfavorable weather conditions. This study demonstrated that the effect of pollution control measures in the NCPS and CIM should be strengthened to ensure that the air quality meets the standard during the ⅩⅩⅣ OWG.
基金supported by the National Basic Research Program of China(2014CB954202)the National Natural Science Foundation of China(40425007,41071151,31421092)the Suzhou University Startup Foundation for Doctor(2015jb04)
文摘With rapid economic growth in China, anthropogenic reactive nitrogen (Nr) emissions have more than doubled over the last two or three decades. Atmospheric Nr pollution is an environmental concern in China especially in megacities such as Beijing. In order to identify the impact of emission sources on atmospheric Nr pollution, we measured atmospheric Nr concentrations and their isotopic composition (δ15N) dynamics at three typical sites: landfill, pig farm and road traffic sites in Beijing from April 2010 to March 2011. Passive samplers were used for monitoring ammonia (NH3) and nitrogen dioxide (NO2), two major Nr species, while their δ15N values were measured by a diffusion method combined with mass spectrometer approach. The raw water pool of the landfill and fattening house of the pig farm were important NH3 sources with mean NH3 concentrations being 2,829 and 2,369 μg/m3, respectively, while the road traffic site was a minor NH3 source (10.6 μg/m3). NH3 concentrations at sites besides the landfill and roads were high in summer and low in winter due to the annual variation of temperature and the change of emission source intensity. In contrast, the NH3 concentrations inside the pig farm house were high in winter and low in summer, for the barn windows were open in summer and closed in winter. The mean NO2 concentrations were 89.8, 32.9 and 23.0 μg/m3 at the road traffic, the landfill and pig farm sites, respectively. Due to vehicle fuel combustion, NO2 concentration at the road traffic was the highest among the three sources, and the road traffic was a main NO2 emission source. PM10, pNH4* and pNO3- concentrations in particulate matter were higher in summer than in winter (except PM10 for the pig farm). The δ15NH3 values ranged from -19.14‰ to 7.82‰, with an average of-0.05‰ for the landfill site, and the lowest values were observed in June and July. The δ15NH3 values for the pig farm site ranged from -29.78‰ to-14.05‰ with an average of-24.51‰, and the 515NH3 values were more negative in summer than in the other seasons. The (515NO2 values were -9.63%o to 7.04‰ with an average of -3.72%0 for the road traffic site. The δ15NO2 values were more negative in summer than those in the other seasons. The different δ15N values for the various Nr species in different sources may serve as important indicators for identifying atmospheric Nr sources in megacities. The results may also provide the theoretical basis for research on the atmospheric N deposition and its sources.