Layered Ag-graphene films synthesized by Gamma ray irradiation for stable lithium metal ano des in carb on ate-based electrolytes

Lithium metal batteries are considered as high energy density battery systems with very promising prospects and have bee n widely studied.However,The uncon trollable plating/strippi ng behavior,infinite volume change and den drites formation of lithium metal anode restrict the applicati on.The unc on trolled n ucleati on of lithium caused by the non uniform multi-physical field distributions,can lead to the undesirable lithium deposition.Herein,a graphene composite uniformly loaded with Ag nano-particles(Ag NPs)is prepared through a facile Gamma ray irradiation method and assembled into self-supported film with layered structure(Ag-rGO film).Whe n such film is used as a lithium metal an ode host,the uncontrolled deposition is converted into a highly nucleation-induced process.On one hand,the Ag NPs distributed between the in terlayers of graphe ne can preferentially induce lithium nu cleati on and en able uniform deposition morphology of lithium between interlayers.On the other hand,the stable layered graphene structure can accommodate volume change,stabilize the interface between anode and electrolyte and inhibit dendrites formation.Therefore,the layered Ag-rGO film as anode host can reach a high Coulombic efficiency over 93.3% for 200 cycle(786 h)at a current density of 1 mA cm^(-2) for 2 mAh cm^(-2) in carbonate-based electrolyte.This work proposes a facile Gamma ray irradiation method to prepare metal/3D-skeleton structure as lithium anode host and demonstrates the potential to regulate the lithium metal deposition behaviors via manipulating the distribution of lithiophilic metal(e.g.Ag)in 3D frameworks.This may offer a practicable thinking for the subsequent design of the lithium metal anode.

Synthesis of New Structures and Substances in Dense Gases H2, D2 and He under Irradiation by Braking 10 MeV y-rays in Cu0.98Be0.02 Pressure Chamber

High-pressure chambers filled with gaseous hydrogen （HHPC）, deuterium （DHPC） and helium （HeHPC） under different initial pressures from about I kbar up to 3 kbar were irradiated with braking γ-rays of threshold energy 10 MeV during varying periods of exposure at the electron beam currents 22-24μA. Upon opening of these chambers, a lot of new synthesized structures with unusual element compositions very different from the initial ones were found. The described phenomena agree well with a series of studies by authors carried out under the action of γ-rays on dense gases of hydrogen, deuterium and helium in the presence of chosen metals in the reaction chamber.

Irradiation Effect of γ Rays on Diamond-Like Carbon Films

Diamond like carbon films, prepared by RF glow discharge on glass substrates, were irradiated by γ rays. The as deposited and irradiated films were characterized by Raman spectroscopy, electrical resistivity, and infrared transmittance. It is shown that the irradiation of the γ rays can lead to the breaking of SP 3 C H and SP 2 C H bonds, slight increasing of SP 3 C C bonds, and induced hydrogen recombination with H 2 molecules, subsequently diffusing to the surface of the films. When the γ rays irradiation dose reached 10×10 4 Gy, the numbers of SP 3 C H bonds was decreased by about 50%, the resistivity of irradiated DLC films was increased, and the diamond like character of the films became more obvious. The structure of DLC films was modified when irradiated by γ rays. The irradiation mechanisms are briefly discussed.

Differential Expression of Retrotransposon WIS 2-1A Response to Vacuum, Low-Energy N^+ Implantation and ^(60)Coγ-ray Irradiation in Wheat

Mutagenesis and retrotransposons have a close relationship, but little attention has been paid yet to the activity of retrotransposons produced by physical mutagens. The variation of retrotransposon WIS 2-1A activity in wheat （Triticum aestivum L.） embryos at three different growth times （30 h, 45 h and 60 h） was investigated after they had been treated with N^＋ implantation in a vacuum of 5× 10^-2 Pa and irradiation by ^60Coγ-ray respectively. For each of the three growth times the expression of WIS 2-1A showed almost entirely a same trend of downregulation, upregulation, then downregulation, and upregulation again with the increase in dose of N^＋ implantation, but the expression appeared irregular with the increase in irradiation of ^60Coγ-ray. In conclusion, the acutely activating effect of WIS 2-1A stimulated by vacuum and high dose N^＋ implantation within a shorter incubation time may provide a convenient tool to advance the research on mutagenic breeding and function genes.

Effects on Agronomic Traits of M_1 by Pollen of Upland Cotton Irradiated by ^(60)Co-γ Ray

[Objective] The aim was to provide reference for research on radiation and breeding of cotton pollen through irradiating common ripe pollen grain of upland cotton by 60Co-γ Ray of varied doses. [Method] Ripe pollen grains of upland cotton were irradiated by 60Co-γ Ray with doses of 5, 10, 15, and 20 Gy, respectively, to learn radiation effect and select appropriate dose. [Result] Most properties of M1 obviously showed variation when dose was over 10 Gy; vitality, growth, and fertility were greatly inhibited when dose was 15 Gy which was almost semi-lethal concentration, and variation species were richest at the same time, which provided materi- als for practical breeding. [Conclusion] 60Co-γ Ray of 15 Gy is more suitable for mutagenesis research on ripe pollen grains of upland cotton.

Thermal Properties of Crosslinking Modified Ultrahigh Molecular Weight Polyethylene Fibers by Ultra-Violet Irradiation

By means of ultra-violet(UV)irradiation with photoini-tiator and multifunctional crosslinking agent,thecrosslinking modification of ultrahigh molecular weightpolyethylene(UHMWPE)fibers prepared by gel-spin-ning was carried out.Thermal properties of fiber sampleswere examined using differential scanning calorimetry(DSC),thermomechanical analysis(TMA)apparatusand a manual device.The results indicated that the opti-mal irradiation energy is 250-400 mJ/cm^2,heat-andcreep-resistant behaviors of modified fibers have beenimproved.

Impact of the displacement damage in channel and source/drain regions on the DC characteristics degradation in deep-submicron MOSFETs after heavy ion irradiation

This paper mainly reports the permanent impact of displacement damage induced by heavy-ion strikes on the deepsubmicron MOSFETs. Upon the heavy ion track through the device, it can lead to displacement damage, including the vacancies and the interstitials. As the featured size of device scales down, the damage can change the dopant distribution in the channel and source/drain regions through the generation of radiation-induced defects and thus have significant impacts on their electrical characteristics. The measured results show that the radiation-induced damage can cause DC characteristics degradations including the threshold voltage, subthreshold swing, saturation drain current, transconductanee, etc. The radiation-induced displacement damage may become the dominant issue while it was the secondary concern for the traditional devices after the heavy ion irradiation. The samples are also irradiated by Co- 60 gamma ray for comparison with the heavy ion irradiation results. Corresponding explanations and analysis are discussed.

Irradiation-induced EMT is associated with activation of TGF-β and restriction of BMP signaling in esophageal cancer cells

Objective: Irradiation may enhance migration and/or invasiveness of cancer cells in vitro and in vivo, the mechanism of which may be associated with epithelial-mesenchymal transition (EMT). The present study explored the mechanisms of EMT induced by irradiation in esophageal cancer cells. Methods: Human esophageal cancer cell line EC109 was treated with increased doses of irradiation (0 Gy, 20 Gy, 40 Gy and 60 Gy). Cell morphology was observed. Expressions of E-cadherin and vimentin were determined by immunofluorescence assay or western blot. Secretion of transforming growth factor-β1 (TGF-β1) by cells was determined by enzyme-linked immunosorbent assay (ELISA), and the expressions of Smad2/3 and phosphorated Smad2 (p-Smad2) were also examined by Western blot. The mRNA expressions of BMP-4, a bone morphogenetic protein (BMP) ligand, and two secreted BMP antagonists (Chordin and Gremlin), were detected with reverse transcription-polymerase chain reaction (RT-PCR). Cell migratory capacity was evaluated. Results: Irradiation induced EMT in EC109 cells in a dose-dependent manner as evidenced by morphological changes, decreased expression of E-cadherin and increased expression of vimentin, and increased cell motility. The secretion of TGF-β1 and expression of p-Smad2 were gradually increased in an irradiation dose-dependent manner, but the Smad2/3 protein levels remained stable. The mRNA expression of BMP-4 was gradually down-regulated, but the expressions of Chordin and Gremlin were gradually up-regulated in cells treated with increased doses of irradiation. Conclusion: Irradiation can induce EMT in esophageal cancer cells in a dose-dependent manner, and the mechanism may be associated with activation of TGF-β and restriction of BMP signaling.

Depolymerization of <i>α</i>- &<i>β</i>-Chitosan by <i>e</i>-Beam Irradiation

α- and β-chitosan with molecular weight of 190,000 and 800,000 respectively, were depolymerized by e-beam irradiation with various doses. The radiation yield of scission (Gs) and degradation rate of the chitosans were identified. The synergistic chemical degradation in the presence of hydrogen peroxide is more effective at lower doses. Mw of β-chitosan was dramatically decreased from 800,000 to 21,030 at the irradiation dose 5 kGy, on the other hand, that of α-chitosan was decreased much more gradually from 190,000 to 36,000. The values of Gs at 10 kGy in the solution without H2O2 and with H2O2 were respectively 6.09 × 10-5 mol/cal and 30.6 × 10-5 mol/cal for α-Chitosan, and 8.18 × 10-5 mol/cal and 43.8 × 10-5 mol/cal for β-chitosan. It was obviously effective on depolymerization by using the combination of e-beam and H2O2. α-Chitosan molecules are likely to adopt a diffuse conformation in the solution and make the different morphologies depending on the concentration.

方ray可解方程组与rayS^＊-阵的图论特征

给出了系数矩阵为方阵的复线性方程组为ray可解、非负ray可解及全非零ray可解等的图论特征刻画,得到了这些方程组的解的ray模式的图论表述.应用这些结论还给出了ray S*-阵和ray S-阵的图论特征刻画,及其他若干类特殊的复线性方程组的ray可解性条件.

Preparation, characterization, and antibacterial activity of γ-irradiated silver nanoparticles in aqueous gelatin

Colloidal silver nanoparticles （Ag-NPs） were obtained through γ-irradiation of aqueous solutions containing AgNO3 and gelatin as a silver source and stabilizer, respectively. The absorbed dose of γ-irradiation influences the particle diameter of the Ag-NPs, as evidenced from surface plasmon resonance （SPR） and transmission electron microscopy （TEM） images. When the γ-irradiation dose was increased （from 2 to 50 kGy）, the mean particle size was decreased continuously as a result of γ-induced Ag-NPs fragmentation. The antibacterial properties of the Ag-NPs were tested against Methicillinresistant Staphylococcus aureus （MRSA） （Gram-positive） and Pseudomonas aeruginosa （P.a） （Gram-negative） bacteria. This approach reveals that the γ-irradiation-mediated method is a promising simple route for synthesizing highly stable Ag-NPs in aqueous solutions with good antibacterial properties for different applications.

An algorithm to resolve γ-rays from charged cosmic rays with DAMPE

The DArk Matter Particle Explorer（DAMPE）,also known as Wukong in China,which was launched on 2015 December 17,is a new high energy cosmic ray and γ-ray satellite-borne observatory.One of the main scientific goals of DAMPE is to observe Ge V-Te V high energy γ-rays with accurate energy,angular and time resolution,to indirectly search for dark matter particles and for the study of high energy astrophysics. Due to the comparatively higher fluxes of charged cosmic rays with respect to γ-rays,it is challenging to identify γ-rays with sufficiently high efficiency,minimizing the amount of charged cosmic ray contamination. In this work we present a method to identify γ-rays in DAMPE data based on Monte Carlo simulations,using the powerful electromagnetic/hadronic shower discrimination provided by the calorimeter and the veto detection of charged particles provided by the plastic scintillation detector. Monte Carlo simulations show that after this selection the number of electrons and protons that contaminate the selected γ-ray events at～10 Ge V amounts to less than 1% of the selected sample.Finally,we use flight data to verify the effectiveness of the method by highlighting known γ-ray sources in the sky and by reconstructing preliminary light curves of the Geminga pulsar.

On the intrinsic shape of the gamma-ray spectrum for Fermi blazars

The curvature of the γ-ray spectrum in blazars may reflect the intrinsic distribution of emitting electrons, which will further give some information on the possible acceleration and cooling processes in the emitting region. The γ-ray spectra of Fermi blazars are normally fitted either by a single power-law（PL） or a log-normal（call Logarithmic Parabola, LP） form. The possible reason for this difference is not clear. We statistically explore this issue based on the different observational properties of 1419 Fermi blazars in the 3 LAC Clean Sample. We find that the γ-ray flux（100 Me V–100 Ge V） and variability index follow bimodal distributions for PL and LP blazars, where the γ-ray flux and variability index show a positive correlation. However, the distributions of γ-ray luminosity and redshift follow a unimodal distribution. Our results suggest that the bimodal distribution of γ-ray fluxes for LP and PL blazars may not be intrinsic and all blazars may have an intrinsically curved γ-ray spectrum, and the PL spectrum is just caused by the fitting effect due to less photons.

Research on Irradiation Electric Field for Charged Particles Beam with High Energy

Irradiation protection of the nonlinear optical devices used in the spacecraft and next generation active laser system must be solved. The first problem was to find the irradiation damage mechanism of the nonlinear materials. In this paper the irradiation electronic field originating from high speed charged particle beams was discussed. The calculating model of the electronic field, based on the relativistic mechanics and electro-magnetic theory, was founded. The common characters of the irradiation electronic field were predicted and the fields of α ray and β ray were calculated by means of our model. The simulating results showed that the intensity of the electric field increased with the energy or the intensity of the beam. The results also showed that the field change trend of α ray and β ray was similar, but the field value was quite different. When the beam intensity I = 100 μA and the beam energy εm = 500 Mev, the electronic field values were about 3.5 × 107 v/m for α ray and 2.4 × 1011 v/m for β ray.

A statistical classification of the unassociated gamma-ray sources in the second Fermi Large Area Telescope Catalog

With the assistance of the identified/associated sources in the second Fermi Large Area Telescope （LAT） catalog, we analyze and resolve the spatial distribution and the distributions of the gamma-ray spectral and variability indices of the remaining 575 unassociated Fermi LAT sources. Consequently, it is suggested that the unassociated sources could statistically consist of Galactic supernova remnants/pulsar wind nebulae, BL Lacertae objects, fiat spectrum radio quasars and other types of active galaxies with fractions of 25%, 29%, 41% and 5%, respectively.

THE RELATIONSHIP BETWEEN RADIATION DOSE AND CHROMOSOME ABERRATIONS AND MICRONUCLEI IN RABBITS EXPOSED TO FRACTIONATED WHOLE-BODY ^(60)Co GAMMA RAYS

The frequencies of chromosome aberrationsand micronuclei showed an increase withdoses after irradiation of rabbitsexposed to fractionated or single whole-body 60Co gamma rays.At most dose points,

Possible modulated γ-ray emission from the transitional millisecond pulsar binary PSR J1023+0038

We report the results from our analysis of Fermi Large Area Telescope （LAT） data for the transitional millisecond pulsar binary PSR J1023＋0038. The time period of the data is nearly 9 yr, and that after the source＇s transition, in June 2013 from the disk-free state to the active state of having an accretion disk, is approximately 4 yr. We identify a high-energy 〉5.5 GeV component in the source＇s spectrum in the active state, and find this component is only significantly detected in half of the orbital phase centered at the descending node （when the pulsar is moving towards the Earth）. Considering the pulsar scenario proposed for multi-frequency emission from the source, in which the pulsar is still active and a cold-relativistic pulsar wind inverse-Compton scatters the photons from the accretion disk, we discuss the origin of the high-energy component. In order to explain the observed spectrum, a power-law distribution of particles, with an index of ~3, in the pulsar wind is required, while the orbital variations are possibly due to changes in power-law index as a function of orbital phase.

Searching forγ-ray counterparts to very faint X-ray transient neutron star binaries

Very faint X-ray transients （VFXTs） are a group of X-ray binaries with low luminosities, displaying peak X-ray luminosities during their outbursts of only 1034-1036 erg s^-1. Using γ-ray data obtained with the Large Area Telescope （LAT） onboard the Fermi Gamma-Ray Space Telescope （Fermi）, we investigate their possible nature of containing rotation-powered pulsars, or more specifically being transitional millisecond pulsars （MSPs）. Among more than 40 known VFXTs, we select 12 neutron star systems. We analyze the LAT data for the fields of 12 VFXTs in the energy range 0.2-300GeV, but do not find any counterparts likely detected by Fermi. We obtain luminosity upper limits for the 12 sources. While the distances to the sources are largely uncertain, the upper limits are comparable to the luminosities of two transitional systems, PSR J1023-0038 and XSS J12270-4859. From our study, we conclude that no evidence is found at γ-rays for the suggestion that some VFXTs could contain rotation-powered MSPs （or be transitional MSP systems）.

Study of temporal and spectral characteristics of the X-ray emission from solar flares

Temporal and spectral characteristics of X-ray emission from 60 flares of intensity ≥C class observed by the Solar X-ray Spectrometer （SOXS） during 2003-2011 are presented. We analyze the X-ray emission observed in four and three energy bands by the Si and Cadmium-Zinc-Telluride （CZT） detectors, respectively. The number of peaks in the intensity profile of the flares varies between 1 and 3. We find moderate correlation （R ~=0.2） between the rise time and the peak flux of the first peak of the flare irrespective of energy band, which is indicative of its energy-independent nature. Moreover, the magnetic field complexity of the flaring region is found to be highly anti-correlated （R = 0.61） with the rise time of the flares while positively correlated （R = 0.28） with the peak flux of the flare. The time delay between the peak of the X-ray emission in a given energy band and that in 25-30keV decreases with increasing energy, suggesting conduction cooling is dominant in the lower energies. Analysis of 340 spectra from 14 flares reveals that the peak of differential emission measure （DEM） evolution is delayed by 60-360 s relative to that of the temperature, and this time delay is inversely proportional to the peak flux of the flare. We conclude that temporal and intensity characteristics of flares are dependent on energy as well as the magnetic field configuration of the active region.

Possible Contribution of Mature γ-ray Pulsars to Cosmic-ray Positrons

We restudy the possible contribution of mature gamma-ray pulsars to cosmic ray positrons based on the new version of outer gap model. In this model, the inclination angle and average properties of the outer gap are taken into account, and more mature pulsars can have the outer gap and emit high energy photons. Half of the primary particles in the outer gaps will flow back toward the star surface and emit synchrotron photons, which can produce electron/positron pairs by the cascade of pair production. Some of these pairs will escape from the light cylinder and be accelerated to relativistic energies in the pulsar wind driven by low-frequency electromagnetic waves. Using a Monte Carlo method, we obtain a sample of mature gamma-ray pulsars and then calculate the production of the positrons from these pulsars. The observed excess of cosmic positrons can be well explained by this model.