This paper proposes a new approach for multi-objective robust control. The approach extends the standard generalized l2 (Gl2) and generalized H2 (GH2) conditions to a set of new linear matrix inequality (LMI) constra...This paper proposes a new approach for multi-objective robust control. The approach extends the standard generalized l2 (Gl2) and generalized H2 (GH2) conditions to a set of new linear matrix inequality (LMI) constraints based on a new stability condition. A technique for variable parameterization is introduced to the multi-objective control problem to preserve the linearity of the synthesis variables. Consequently, the multi-channel multi-objective mixed Gl2/GH2 control problem can be solved less conservatively using computationally tractable algorithms developed in the paper.展开更多
A novel temperature fluctuation synthesis/simultaneous densification process was developed for the preparation of Ti3SiC2 bulk ceramics. In this process. Si is used as an in-situ liquid forming phase and it is favorab...A novel temperature fluctuation synthesis/simultaneous densification process was developed for the preparation of Ti3SiC2 bulk ceramics. In this process. Si is used as an in-situ liquid forming phase and it is favorable for both the solid-liquid synthesis and the densification of Ti3SiC2 rainies. The present work demonstrated that the temperature fluctuation synthesis/simultaneous densification process is one of the most effective and simple methods for the preparation of Ti3SiC2 bulk materials providing relatively low synthesis temperature. short reaction time; and simultaneous synthesis and densification. This work also showed the capability to control the microstructure, e.g., the preferred orientation, of the bulk Ti3SiC2 materials simply by applying the hot pressing pressure at different Stages of the temperature fluctuation process. And textured Ti3SiC2 bulk materials with {002} faces of laminated Ti3SiC2 grains normal to the hot pressing axis were prepared.展开更多
This paper is concerned with the robust control synthesis of autonomous underwater vehicle （AUV） for general path following maneuvers. First, we present maneuvering kinematics and vehicle dynamics in a unified frame...This paper is concerned with the robust control synthesis of autonomous underwater vehicle （AUV） for general path following maneuvers. First, we present maneuvering kinematics and vehicle dynamics in a unified framework. Based on H∞ loop-shaping procedure, the 2-DOF autopilot controller has been presented to enhance stability and path tracking. By use of model reduction, the high-order control system is reduced to one with reasonable order, and further the scaled low-order controller has been analyzed in both the frequency and the time domains. Finally, it is shown that the autopilot control system provides robust performance and stability against prescribed levels of uncertainty.展开更多
A new type of 2-DOF(degree of freedom) magnetic levitation system for multi-DOF levitation is proposed. In this system, the force of permanent magnets are used for levitation and controlled by adjusting the reluctance...A new type of 2-DOF(degree of freedom) magnetic levitation system for multi-DOF levitation is proposed. In this system, the force of permanent magnets are used for levitation and controlled by adjusting the reluctance of the magnetic circuit. Using permanent magnets, the feature of this system is effective for saving energy and avoiding heat generation. First, the principle of the levitation system and typical reluctance control methods are described. Second, an experimental device based on the principle is introduced. Finally, the feasibility of this system is considered from linear control theory.展开更多
Multi-objective robust state-feedback controller synthesis problems for linear discrete-time uncertain systems are addressed. Based on parameter-dependent Lyapunov functions, the Gl2 and GH2 norm expressed in terms of...Multi-objective robust state-feedback controller synthesis problems for linear discrete-time uncertain systems are addressed. Based on parameter-dependent Lyapunov functions, the Gl2 and GH2 norm expressed in terms of LMI (Linear Matrix Inequality) characterizations are further generalized to cope with the robust analysis for convex polytopic uncertain system. Robust state-feedback controller synthesis conditions are also derived for this class of uncertain systems. Using the above results, multi-objective state-feedback controller synthesis procedures which involve the LMI optimization technique are developed and less conservative than the existing one. An illustrative example verified the validity of the approach.展开更多
The effects of SO_(2) on an one-pot synthesized Cu-SSZ-13 catalyst for selective reduction of NO_(x) by NH_(3) were examined.The addition of SO_(2) inhibited NO_(x) conversion significantly below 300℃,while no effect...The effects of SO_(2) on an one-pot synthesized Cu-SSZ-13 catalyst for selective reduction of NO_(x) by NH_(3) were examined.The addition of SO_(2) inhibited NO_(x) conversion significantly below 300℃,while no effect on NO_(x) conversion was observed above 300℃.TGA,TPD,and XPS results showed that the deactivation was caused by the formation of(NH4)2SO_(4),SO_(2) chemisorption on the isolated Cu^(2+)ion sites,as well as the formation of CuSO_(4)-like species.Among them,the site-blocking effect of(NH_(4))_(2)SO_(4) on Cu^(2+)was the primary reason for deactivation.Fortunately,89%of deNO_(x) activity of the poisoned catalyst was recovered after thermal treatment at 500℃ in air,where(NH_(4))_(2)SO_(4) was completely decomposed.The activity was further recovered with regeneration temperature increasing to 600℃,removing the adsorbed SO_(2) on the Cu^(2+)sites.The regeneration at 600℃ could not recover the activity completely,because of the high stability of CuSO_(4)-like species.展开更多
Cybernetic decision variants were analyzed in order to use for physical task of active noise cancelation. 10 dB mean active noise cancellation is demonstrated in two decades frequency band by usage of cybernetic decis...Cybernetic decision variants were analyzed in order to use for physical task of active noise cancelation. 10 dB mean active noise cancellation is demonstrated in two decades frequency band by usage of cybernetic decision for acoustical duct physical scale model. The used decision was found on minimization of acoustical field power transfer function from the beginning of waveguide to their end.展开更多
Two-dimensional layered materials have attracted significant interest for their potential applications in electronic and optoelectronics devices. Among them, transition metal dichalcogenides(TMDs), especially molybden...Two-dimensional layered materials have attracted significant interest for their potential applications in electronic and optoelectronics devices. Among them, transition metal dichalcogenides(TMDs), especially molybdenum disulfide(MoS_2), is extensively studied because of its unique properties. Monolayer MoS_2 so far can be obtained by mechanical exfoliation or chemical vapor deposition(CVD). However, controllable synthesis of large area monolayer MoS_2 with high quality needs to be improved and their growth mechanism requires more studies. Here we report a systematical study on controlled synthesis of high-quality monolayer MoS_2 single crystals using low pressure CVD. Large-size monolayer MoS_2 triangles with an edge length up to 405 μm were successfully synthesized. The Raman and photoluminescence spectroscopy studies indicate high homogenous optical characteristic of the synthesized monolayer MoS_2 triangles. The transmission electron microscopy results demonstrate that monolayer MoS_2 triangles are single crystals. The back-gated field effect transistors(FETs) fabricated using the as-grown monolayer MoS_2 show typical n-type semiconductor behaviors with carrier mobility up to 21.8 cm^2 V^(-1) s^(-1), indicating excellent electronic property comparing with previously reported CVD grown MoS_2 monolayer. The MoS_2 FETs also show a high photoresponsivity of 7 A W^(-1), as well as a fast photo-response time of 20 ms. The improved synthesis method recommended here, which makes material preparation much easier, may strongly promote further research and potential applications.展开更多
Two-dimensional molybdenum disulfide(2D MoS_(2))is considered as a promising candidate for many applications due to its unique structure and properties.However,the controllable synthesis of large-scale and high-qualit...Two-dimensional molybdenum disulfide(2D MoS_(2))is considered as a promising candidate for many applications due to its unique structure and properties.However,the controllable synthesis of large-scale and high-quality 2D 1T-phase MoS_(2)is still a challenge.Herein,we present the scalable and controllable synthesis of 2D MoS2 from 2H to 1T@2H phase by using K_(2)SO_(4)salt as a simultaneous high-temperature sulfur source and template.The as-synthesized 1T@2H-2D MoS_(2)exhibits a high yield and can be easily assembled into freestanding electrode with high specific capacitance of 434 F/g at a scan rate of 1 mV/s in LiClO_(4)ethylene carbonate/dimethyl carbonate(EC/DMC).Moreover,various single-crystal 2D transition metal sulfides(WS_(2),PbS,MnS and Ni_(9)S_(8))and 2D S-doped carbon can be synthesized using this method.We believe that this study may provide a new sight for scalable and controllable synthesis of other 2D materials beyond 2D MoS_(2).展开更多
In this paper,CuO_(x)@Ag/CeO_(2) catalysts were synthesized by simple wet-chemical method and equal volume impregnation method.The obtained catalysts were subjected to soot temperature programmed oxidation(soot-TPO)ac...In this paper,CuO_(x)@Ag/CeO_(2) catalysts were synthesized by simple wet-chemical method and equal volume impregnation method.The obtained catalysts were subjected to soot temperature programmed oxidation(soot-TPO)activity tests and were further characterized by various techniques such as X-ray diffraction(XRD),transmission electron microscopy/high-resolution transmission electron microscopy(TEM/HR-TEM),N_(2) physisorption,X-ray photoelectron spectroscopy(XPS)and H_(2)-temperature programmed reduction(H_(2)-TPR).The results show that CuO_(x)@Ag/CeO_(2) synthesized presents well controlled core-shell structures,with nano-cube like Cu_(2)O as the core and Ag decorated polycrystalline CeO_(2) grafting layers as the shell.Such core-shell structured CuO_(x)@Ag/CeO_(2) can successfully construct a secondary oxygen delivery channel(CuO_(x)→CeO_(2)→Ag)to effectively transfer bulk oxygen of the catalyst to the soot,resulting in its excellent soot oxidation activity compared to CuO_(x)@CeO_(2).The potential benefiting effect by Ag introduction over Cu@Ag/Ce can be concluded as:(ⅰ)pumping lattice oxygen and accelerating gaseous O_(2) dissociation to generate significantly increased active surface oxygen content;(ⅱ)modulating a moderate surface oxygen vacancies concentration to maintain more highly active O_(2) species.展开更多
Preparing SnO2 with hierarchical micro/nano structures by hydrothermal, coordination, templating and electrochemical deposition methods and their mechanisms are investigated. The result shows that the echinus-like SnO...Preparing SnO2 with hierarchical micro/nano structures by hydrothermal, coordination, templating and electrochemical deposition methods and their mechanisms are investigated. The result shows that the echinus-like SnO2 prepared by Method 1 is a typical Ostwald mechanism that develops from internally to externally. The cabbage-like SnO2 by Method 2 is produced with oxalic acid as complexing agent to set-up precursor of SnO2, and then precursors are bocked around the body that is around the body being bocked. The nest-like SnO2 by Method 3 is controlled by citric acid as coordinator for the nucleation as well as the grow rate and setup process. Spongy-like SnO2 by Method 4 is produced using PST as template, PST is be infiltered into SnO2 precursor by gravity and capillary and treated thermally to form a multiporous structure. The petal-like SnO2 by Method 5 is formed with crystal deposition emergence due to oxidation-reduction reactions of two electrodes in an electric field. XRD analyses shows that the five results are all pure phase SnO2. It provides basic data for SnOE industrial application.展开更多
The sense of touch as a man-machine communication channel can be as acute as the sense of sight and sound. In some scenarios such as those seen in aerobatics, stunt flying, and combat flights, tactile sensors can even...The sense of touch as a man-machine communication channel can be as acute as the sense of sight and sound. In some scenarios such as those seen in aerobatics, stunt flying, and combat flights, tactile sensors can even outperform the conventional non-contact sensors in terms of situation awareness. Fusion of tactile sensory information with those obtained via sight and sound can avoid diverting the user’s attention away from the operational task at hand as well. In this study, the performance of an operator, to servo control the motion of a 2-dof model helicopter with pitch/yaw maneuverability, subjected to an intuitive body-referenced arrangement of a cluster of vibro-tactile sensors is investigated. A blindfolded operator will then control the helicopter to a safe attraction zone via a joystick based on this tactile sensory information. A fine-tuned local controller would take over for the end-of-motion precise homing. This study can pave the way towards a systematic integration and characterization of tactile sensors in high performance weapon platforms with improved situation awareness in visually awkward maneuvers such as those seen in aerial combat scenarios.展开更多
基金Project supported by the National Natural Science Foundation ofChina (No. 60374028) and the Scientific Research Foundation forReturned Overseas Chinese Scholars Ministry of Education (No.[2004]176)
文摘This paper proposes a new approach for multi-objective robust control. The approach extends the standard generalized l2 (Gl2) and generalized H2 (GH2) conditions to a set of new linear matrix inequality (LMI) constraints based on a new stability condition. A technique for variable parameterization is introduced to the multi-objective control problem to preserve the linearity of the synthesis variables. Consequently, the multi-channel multi-objective mixed Gl2/GH2 control problem can be solved less conservatively using computationally tractable algorithms developed in the paper.
基金the National Outstanding YOung Scientist Foundation Under Grant !No.59925208 the National Natural Science Foundation of China
文摘A novel temperature fluctuation synthesis/simultaneous densification process was developed for the preparation of Ti3SiC2 bulk ceramics. In this process. Si is used as an in-situ liquid forming phase and it is favorable for both the solid-liquid synthesis and the densification of Ti3SiC2 rainies. The present work demonstrated that the temperature fluctuation synthesis/simultaneous densification process is one of the most effective and simple methods for the preparation of Ti3SiC2 bulk materials providing relatively low synthesis temperature. short reaction time; and simultaneous synthesis and densification. This work also showed the capability to control the microstructure, e.g., the preferred orientation, of the bulk Ti3SiC2 materials simply by applying the hot pressing pressure at different Stages of the temperature fluctuation process. And textured Ti3SiC2 bulk materials with {002} faces of laminated Ti3SiC2 grains normal to the hot pressing axis were prepared.
基金a part of the project titled "Development of Key Marine Equipments for Enhancement of Ocean Industry-Development of Underwater Manipulator and Thrusting System Driven by Electric Motor" funded by the Ministry of Land, Transport and Maritime Affairs, Korea
文摘This paper is concerned with the robust control synthesis of autonomous underwater vehicle （AUV） for general path following maneuvers. First, we present maneuvering kinematics and vehicle dynamics in a unified framework. Based on H∞ loop-shaping procedure, the 2-DOF autopilot controller has been presented to enhance stability and path tracking. By use of model reduction, the high-order control system is reduced to one with reasonable order, and further the scaled low-order controller has been analyzed in both the frequency and the time domains. Finally, it is shown that the autopilot control system provides robust performance and stability against prescribed levels of uncertainty.
文摘A new type of 2-DOF(degree of freedom) magnetic levitation system for multi-DOF levitation is proposed. In this system, the force of permanent magnets are used for levitation and controlled by adjusting the reluctance of the magnetic circuit. Using permanent magnets, the feature of this system is effective for saving energy and avoiding heat generation. First, the principle of the levitation system and typical reluctance control methods are described. Second, an experimental device based on the principle is introduced. Finally, the feasibility of this system is considered from linear control theory.
基金Project (No. 60374028) supported by the National Natural ScienceFoundation of China
文摘Multi-objective robust state-feedback controller synthesis problems for linear discrete-time uncertain systems are addressed. Based on parameter-dependent Lyapunov functions, the Gl2 and GH2 norm expressed in terms of LMI (Linear Matrix Inequality) characterizations are further generalized to cope with the robust analysis for convex polytopic uncertain system. Robust state-feedback controller synthesis conditions are also derived for this class of uncertain systems. Using the above results, multi-objective state-feedback controller synthesis procedures which involve the LMI optimization technique are developed and less conservative than the existing one. An illustrative example verified the validity of the approach.
基金Financial supports from the Natural Science Foundation of Tianjin 19JCTPJC42300.
文摘The effects of SO_(2) on an one-pot synthesized Cu-SSZ-13 catalyst for selective reduction of NO_(x) by NH_(3) were examined.The addition of SO_(2) inhibited NO_(x) conversion significantly below 300℃,while no effect on NO_(x) conversion was observed above 300℃.TGA,TPD,and XPS results showed that the deactivation was caused by the formation of(NH4)2SO_(4),SO_(2) chemisorption on the isolated Cu^(2+)ion sites,as well as the formation of CuSO_(4)-like species.Among them,the site-blocking effect of(NH_(4))_(2)SO_(4) on Cu^(2+)was the primary reason for deactivation.Fortunately,89%of deNO_(x) activity of the poisoned catalyst was recovered after thermal treatment at 500℃ in air,where(NH_(4))_(2)SO_(4) was completely decomposed.The activity was further recovered with regeneration temperature increasing to 600℃,removing the adsorbed SO_(2) on the Cu^(2+)sites.The regeneration at 600℃ could not recover the activity completely,because of the high stability of CuSO_(4)-like species.
文摘Cybernetic decision variants were analyzed in order to use for physical task of active noise cancelation. 10 dB mean active noise cancellation is demonstrated in two decades frequency band by usage of cybernetic decision for acoustical duct physical scale model. The used decision was found on minimization of acoustical field power transfer function from the beginning of waveguide to their end.
基金supported by the“Thousands Talents”program for pioneer researcher and his innovation team,ChinaPresident Funding of the Chinese Academy of Sciences,National Natural Science Foundation of China(51272238,21321062,51432005,and 61405040)+1 种基金Beijing Municipal Science&Technology Commission(Z131100006013004 and Z131100006013005)Beijing City Committee of Science and Technology(Z151100003315010)
文摘Two-dimensional layered materials have attracted significant interest for their potential applications in electronic and optoelectronics devices. Among them, transition metal dichalcogenides(TMDs), especially molybdenum disulfide(MoS_2), is extensively studied because of its unique properties. Monolayer MoS_2 so far can be obtained by mechanical exfoliation or chemical vapor deposition(CVD). However, controllable synthesis of large area monolayer MoS_2 with high quality needs to be improved and their growth mechanism requires more studies. Here we report a systematical study on controlled synthesis of high-quality monolayer MoS_2 single crystals using low pressure CVD. Large-size monolayer MoS_2 triangles with an edge length up to 405 μm were successfully synthesized. The Raman and photoluminescence spectroscopy studies indicate high homogenous optical characteristic of the synthesized monolayer MoS_2 triangles. The transmission electron microscopy results demonstrate that monolayer MoS_2 triangles are single crystals. The back-gated field effect transistors(FETs) fabricated using the as-grown monolayer MoS_2 show typical n-type semiconductor behaviors with carrier mobility up to 21.8 cm^2 V^(-1) s^(-1), indicating excellent electronic property comparing with previously reported CVD grown MoS_2 monolayer. The MoS_2 FETs also show a high photoresponsivity of 7 A W^(-1), as well as a fast photo-response time of 20 ms. The improved synthesis method recommended here, which makes material preparation much easier, may strongly promote further research and potential applications.
基金supported by the National Natural Science Foundation of China(Nos.51972124,51872101,51672097,51902115,and 61434001)the National Program for Support of Top-notch Young Professionals,and the program for the HUST Academic Frontier Youth Team.
文摘Two-dimensional molybdenum disulfide(2D MoS_(2))is considered as a promising candidate for many applications due to its unique structure and properties.However,the controllable synthesis of large-scale and high-quality 2D 1T-phase MoS_(2)is still a challenge.Herein,we present the scalable and controllable synthesis of 2D MoS2 from 2H to 1T@2H phase by using K_(2)SO_(4)salt as a simultaneous high-temperature sulfur source and template.The as-synthesized 1T@2H-2D MoS_(2)exhibits a high yield and can be easily assembled into freestanding electrode with high specific capacitance of 434 F/g at a scan rate of 1 mV/s in LiClO_(4)ethylene carbonate/dimethyl carbonate(EC/DMC).Moreover,various single-crystal 2D transition metal sulfides(WS_(2),PbS,MnS and Ni_(9)S_(8))and 2D S-doped carbon can be synthesized using this method.We believe that this study may provide a new sight for scalable and controllable synthesis of other 2D materials beyond 2D MoS_(2).
基金Project supported by National Key R&D Program of China(2017YFC0211102)Natural Science Foundation of the Jiangsu Higher Education Institutions of China(20KJB610005)+2 种基金the Natural Science Foundation of Jiangsu Province(BK20201037)Key Research and Development Program of Anhui Province(202104g01020006)the Scientific Research Fund of Nanjing Institute of Technology(YKJ2019111,YKJ2019110)。
文摘In this paper,CuO_(x)@Ag/CeO_(2) catalysts were synthesized by simple wet-chemical method and equal volume impregnation method.The obtained catalysts were subjected to soot temperature programmed oxidation(soot-TPO)activity tests and were further characterized by various techniques such as X-ray diffraction(XRD),transmission electron microscopy/high-resolution transmission electron microscopy(TEM/HR-TEM),N_(2) physisorption,X-ray photoelectron spectroscopy(XPS)and H_(2)-temperature programmed reduction(H_(2)-TPR).The results show that CuO_(x)@Ag/CeO_(2) synthesized presents well controlled core-shell structures,with nano-cube like Cu_(2)O as the core and Ag decorated polycrystalline CeO_(2) grafting layers as the shell.Such core-shell structured CuO_(x)@Ag/CeO_(2) can successfully construct a secondary oxygen delivery channel(CuO_(x)→CeO_(2)→Ag)to effectively transfer bulk oxygen of the catalyst to the soot,resulting in its excellent soot oxidation activity compared to CuO_(x)@CeO_(2).The potential benefiting effect by Ag introduction over Cu@Ag/Ce can be concluded as:(ⅰ)pumping lattice oxygen and accelerating gaseous O_(2) dissociation to generate significantly increased active surface oxygen content;(ⅱ)modulating a moderate surface oxygen vacancies concentration to maintain more highly active O_(2) species.
基金Supported by fund of the Excellent Science&Technology Innovate Team Program for Young and Middle-aged Talents in University of Hubei Province(T201225)Hubei Provincial Key Laboratory of Plant Anti-Cancer Active Substance Purification and Application,The Second Excellent Teacher Team of Hubei University of Education(2012K203)
文摘Preparing SnO2 with hierarchical micro/nano structures by hydrothermal, coordination, templating and electrochemical deposition methods and their mechanisms are investigated. The result shows that the echinus-like SnO2 prepared by Method 1 is a typical Ostwald mechanism that develops from internally to externally. The cabbage-like SnO2 by Method 2 is produced with oxalic acid as complexing agent to set-up precursor of SnO2, and then precursors are bocked around the body that is around the body being bocked. The nest-like SnO2 by Method 3 is controlled by citric acid as coordinator for the nucleation as well as the grow rate and setup process. Spongy-like SnO2 by Method 4 is produced using PST as template, PST is be infiltered into SnO2 precursor by gravity and capillary and treated thermally to form a multiporous structure. The petal-like SnO2 by Method 5 is formed with crystal deposition emergence due to oxidation-reduction reactions of two electrodes in an electric field. XRD analyses shows that the five results are all pure phase SnO2. It provides basic data for SnOE industrial application.
文摘The sense of touch as a man-machine communication channel can be as acute as the sense of sight and sound. In some scenarios such as those seen in aerobatics, stunt flying, and combat flights, tactile sensors can even outperform the conventional non-contact sensors in terms of situation awareness. Fusion of tactile sensory information with those obtained via sight and sound can avoid diverting the user’s attention away from the operational task at hand as well. In this study, the performance of an operator, to servo control the motion of a 2-dof model helicopter with pitch/yaw maneuverability, subjected to an intuitive body-referenced arrangement of a cluster of vibro-tactile sensors is investigated. A blindfolded operator will then control the helicopter to a safe attraction zone via a joystick based on this tactile sensory information. A fine-tuned local controller would take over for the end-of-motion precise homing. This study can pave the way towards a systematic integration and characterization of tactile sensors in high performance weapon platforms with improved situation awareness in visually awkward maneuvers such as those seen in aerial combat scenarios.
