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Accelerated anaerobic dechlorination of DDT in slurry with Hydragric Acrisols using citric acid and anthraquinone-2,6-disulfonate(AQDS) 被引量:5
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作者 Cuiying Liu Xianghua Xu Jianling Fan 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2015年第12期87-94,共8页
The application of electron donor and electron shuttle substances has a vital influence on electron transfer,thus may affect the reductive dechlorination of 1,1,1-trichoro-2,2-bis(p-chlorophenyl)ethane(DDT) in ana... The application of electron donor and electron shuttle substances has a vital influence on electron transfer,thus may affect the reductive dechlorination of 1,1,1-trichoro-2,2-bis(p-chlorophenyl)ethane(DDT) in anaerobic reaction systems.To evaluate the roles of citric acid and anthraquinone-2,6-disulfonate(AQDS) in accelerating the reductive dechlorination of DDT in Hydragric Acrisols that contain abundant iron oxide,a batch anaerobic incubation experiment was conducted in a slurry system with four treatments of(1) control,(2) citric acid,(3) AQDS,and(4) citric acid + AQDS.Results showed that DDT residues decreased by 78.93%-92.11% of the initial quantities after 20 days of incubation,and 1,1-dichloro-2,2-bis(4-chlorophenyl)-ethane(DDD) was the dominant metabolite.The application of citric acid accelerated DDT dechlorination slightly in the first 8 days,while the methanogenesis rate increased quickly,and then the acceleration effect improved after the 8th day while the methanogenesis rate decreased.The amendment by AQDS decreased the Eh value of the reaction system and accelerated microbial reduction of Fe(III) oxides to generate Fe(II),which was an efficient electron donor,thus enhancing the reductive dechlorination rate of DDT.The addition of citric acid + AQDS was most efficient in stimulating DDT dechlorination,but no significant interaction between citric acid and AQDS on DDT dechlorination was observed.The results will be of great significance for developing an efficient in situ remediation strategy for DDT-contaminated sites. 展开更多
关键词 1 1 1-Trichoro-2 2-bis(p-chlorophenyl)ethane (DDT) Anthraquinone-2 6-disulfonate (aqds Electron donor Reductive dechlorination Soil
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蒽醌-2,6-二磺酸钠掺杂聚吡咯修饰阴极对沉积型微生物燃料电池产电性能的影响 被引量:3
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作者 任月萍 付飞 +1 位作者 李秀芬 朱荣 《环境化学》 CAS CSCD 北大核心 2013年第10期1851-1855,共5页
采用化学原位聚合法制备了蒽醌-2,6-二磺酸钠(anthraquinone-2,6-disulfonic acid disodium salt,AQDS)掺杂的聚吡咯(polypyrrole,PPy)修饰阴极.电化学交流阻抗谱(EIS)和塔菲尔(Tafel)测试发现,与空白阴极和PPy修饰阴极相比,PPy-AQDS修... 采用化学原位聚合法制备了蒽醌-2,6-二磺酸钠(anthraquinone-2,6-disulfonic acid disodium salt,AQDS)掺杂的聚吡咯(polypyrrole,PPy)修饰阴极.电化学交流阻抗谱(EIS)和塔菲尔(Tafel)测试发现,与空白阴极和PPy修饰阴极相比,PPy-AQDS修饰阴极的内阻更低,电极反应速率更高.在校园浅水湖中以空白阴极,PPy修饰阴极和PPy-AQDS修饰阴极运行沉积型微生物燃料电池(sediment microbial fuel cell,SMFC)30 d.实验结果表明,PPy-AQDS修饰阴极可以提高SMFC体系的产电能力并提高沉积物中有机质的去除效率.与空白阴极SMFC体系相比,PPy-AQDS修饰阴极SMFC体系的最大功率密度增大了3.7倍,阳极表面沉积物中烧失量(loss on ignition,LOI)和易氧化有机质(readily oxidizable organic matter,ROOM)去除率分别由5.5%和5.5%增大到14.4%和31.9%. 展开更多
关键词 沉积型微生物燃料电池(SMFC) 阴极修饰 聚吡咯(PPy) 蒽醌-2 6-二磺酸钠(aqds)
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Enhanced U(Ⅵ) bioreduction by alginate-immobilized uranium-reducing bacteria in the presence of carbon nanotubes and anthraquinone-2,6-disulfonate 被引量:3
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作者 Weida Wang Yali Feng +4 位作者 Xinhua Tang Haoran Li Zhuwei Du Aifei Yi Xu Zhang 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2015年第5期68-73,共6页
Uranium-reducing bacteria were immobilized with sodium alginate, anthraquinone-2,6-disulfonate(AQDS), and carbon nanotubes(CNTs). The effects of different AQDS-CNTs contents, U(Ⅳ) concentrations, and metal ions... Uranium-reducing bacteria were immobilized with sodium alginate, anthraquinone-2,6-disulfonate(AQDS), and carbon nanotubes(CNTs). The effects of different AQDS-CNTs contents, U(Ⅳ) concentrations, and metal ions on U(Ⅳ) reduction by immobilized beads were examined. Over 97.5% U(Ⅵ)(20 mg/L) was removed in 8 hr when the beads were added to 0.7% AQDS-CNTs, which was higher than that without AQDS-CNTs. This result may be attributed to the enhanced electron transfer by AQDS and CNTs. The reduction of U(Ⅵ) occurred at initial U(Ⅵ) concentrations of 10 to 100 mg/L and increased with increasing AQDS-CNT content from 0.1% to 1%. The presence of Fe(Ⅲ), Cu(Ⅱ) and Mn(Ⅱ)slightly increased U(Ⅵ) reduction, whereas Cr(Ⅵ), Ni(Ⅱ), Pb(Ⅱ), and Zn(Ⅱ) significantly inhibited U(Ⅵ) reduction. After eight successive incubation-washing cycles or 8 hr of retention time(HRT) for 48 hr of continuous operation, the removal efficiency of uranium was above 90% and 92%, respectively. The results indicate that the AQDS-CNT/AL/cell beads are suitable for the treatment of uranium-containing wastewaters. 展开更多
关键词 Uranium Carbon nanotubes(CNTs) Redox mediator Anthraquinone-2 6-disulfonate(aqds Immobilization
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南海北部海域底泥微生物的腐殖质还原性能研究 被引量:3
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作者 吴鹏 赵怡 +1 位作者 洪义国 段舜山 《生态环境学报》 CSCD 北大核心 2011年第1期132-136,共5页
微生物的腐殖质还原过程自1996年发现以来,日益成为环境领域的一个研究热点。以南海北部海域的8个底泥为实验材料,利用蒽醌-2,6,-双磺酸(AQDS)为腐殖质模式物,初步探讨了南海北部8个底泥培养物对腐殖质的还原能力,并探讨了驯化后的8... 微生物的腐殖质还原过程自1996年发现以来,日益成为环境领域的一个研究热点。以南海北部海域的8个底泥为实验材料,利用蒽醌-2,6,-双磺酸(AQDS)为腐殖质模式物,初步探讨了南海北部8个底泥培养物对腐殖质的还原能力,并探讨了驯化后的8个底泥微生物对腐殖质的还原过程。结果发现:从南海北部深海海域到海陆交接的香港米浦红树林的8个底泥样品培养液均能很好的还原AQDS;驯化后的8个站点底泥微生物对腐殖质还原的能力有所不同,在48 h,E425站点培养液中的OD450只有0.74,其余7个站点培养液中的OD450都在2.0~3.0之间,推测其原因是8个站点中腐殖质还原微生物的数量具有明显差异,使得各站点的OD450差异很大。研究结果为认知腐殖质还原微生物的分布和探究腐殖质还原微生物在环境中的生态学意义提供重要的理论依据。 展开更多
关键词 腐殖质还原菌 南海北部海域 底泥 腐殖质还原 蒽醌-2 6-双磺酸
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驯化的西湖底泥还原腐殖质影响因素研究 被引量:4
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作者 徐志伟 陈红 《浙江大学学报(工学版)》 EI CAS CSCD 北大核心 2010年第2期349-352,共4页
利用驯化的西湖底泥,以蒽醌-2,6-双磺酸盐(AQDS)作为腐殖质模式物,初步研究了温度、pH、不同类型氮源、不同种类金属离子等对底泥微生物还原腐殖质的影响.结果发现,在15~45℃下驯化底泥能还原腐殖质,最适反应温度为30~37℃;在反应初... 利用驯化的西湖底泥,以蒽醌-2,6-双磺酸盐(AQDS)作为腐殖质模式物,初步研究了温度、pH、不同类型氮源、不同种类金属离子等对底泥微生物还原腐殖质的影响.结果发现,在15~45℃下驯化底泥能还原腐殖质,最适反应温度为30~37℃;在反应初始pH为4~9的条件下可进行腐殖质还原,最适pH为7;不同类型氮源对微生物还原腐殖质的效果依次为NH4Cl>CO(NH2)2>NaNO3>NaNO2;Mg2+、Mn2+促进了微生物还原腐殖质,而Zn2+、Ni2+、Cu2+部分地抑制了腐殖质还原,Hg2+则完全抑制腐殖质还原. 展开更多
关键词 腐殖质还原菌 蒽醌-2 6-双磺酸盐 腐殖质还原 PH 氮源 金属离子
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Effect of microbial mediated iron plaque reduction on arsenic mobility in paddy soil 被引量:11
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作者 WANG Xinjun CHEN Xueping +2 位作者 YANG Jing WANG Zhaosu SUN Guoxin 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2009年第11期1562-1568,共7页
The potential of microbial mediated iron plaque reduction, and associated arsenic (As) mobility were examined by iron reducing bacteria enriched from As contaminated paddy soil. To our knowledge, this is the first t... The potential of microbial mediated iron plaque reduction, and associated arsenic (As) mobility were examined by iron reducing bacteria enriched from As contaminated paddy soil. To our knowledge, this is the first time to report the impact of microbial iron plaque reduction on As mobility. Iron reduction occurred during the inoculation of iron reducing enrichment culture in the treatments with iron plaque and ferrihydrite as the electron acceptors, respectively. The Fe(II) concentration with the treatment of anthraquinone-2, 6-disulfonic acid (AQDS) and iron reducing bacteria increased much faster than the control. Arsenic released from iron plaque with the iron reduction, and a significant correlation between Fe(II) and total As in culture was observed. However, compared with control, the increasing rate of As was inhibited by iron reducing bacteria especially in the presence of AQDS. In addition, the concentrations of As(III) and As(V) in abiotic treatments were higher than those in the biotic treatments at day 30. These results indicated that both microbial and chemical reductions of iron plaque caused As release from iron plaque to aqueous phase, however, microbial iron reduction induced the formation of more crystalline iron minerals, leading to As sequestration. In addition, the presence of AQDS in solution can accelerate the iron reduction, the As release from iron plaque and subsequently the As retention in the crystalline iron mineral. Thus, our results suggested that it is possible to remediate As contaminated soils by utilizing iron reducing bacteria and AQDS. 展开更多
关键词 iron reducing bacteria iron plaque ARSENIC anthraquinone-2 6-disulfonic acid (aqds paddy soil FERRIHYDRITE
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