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2002~2022年北京大气气溶胶光学特性的地基遥感连续观测
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作者 陈洪滨 施红蓉 +1 位作者 范学花 夏祥鳌 《大气科学》 CSCD 北大核心 2024年第1期347-358,共12页
长时间序列的气溶胶光学特性观测资料是定量研究气溶胶辐射和气候效应的重要基础,也是空气质量和环境健康研究的重要数据来源。本文系统评述了全球AERONET(Aerosol Robotic Network)观测网,并介绍了我国最长观测时间的AEROENT北京站发... 长时间序列的气溶胶光学特性观测资料是定量研究气溶胶辐射和气候效应的重要基础,也是空气质量和环境健康研究的重要数据来源。本文系统评述了全球AERONET(Aerosol Robotic Network)观测网,并介绍了我国最长观测时间的AEROENT北京站发展状况和一些研究成果;使用北京站长达20余年的观测数据,针对AERONET观测网的光学辐射产品的多时间尺度变化特征进行系统分析,讨论了长期观测的重要性和迫切性。 展开更多
关键词 气溶胶 光学特性 AERONET(Aerosol Robotic Network)北京站 气候效应
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冬春两湖盆地地区大气气溶胶污染的年代际变化特征及其与东亚经向风南北反相位的联系
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作者 姜玉洁 张玲 +2 位作者 朱寿鹏 白永清 智协飞 《大气科学》 CSCD 北大核心 2024年第2期773-788,共16页
基于MERRA-2及ERA5逐月再分析资料,本文采用EOF分析、线性回归和合成分析等方法,分析了1980~2020年长江流域中游两湖盆地地区气溶胶光学厚度(AOD)的年代际变化特征及东亚经向风南北反位相模态对其的影响。结果表明,在年代际尺度上两湖... 基于MERRA-2及ERA5逐月再分析资料,本文采用EOF分析、线性回归和合成分析等方法,分析了1980~2020年长江流域中游两湖盆地地区气溶胶光学厚度(AOD)的年代际变化特征及东亚经向风南北反位相模态对其的影响。结果表明,在年代际尺度上两湖盆地地区AOD呈现非线性的变化趋势,20世纪80、90年代处于低值,21世纪初AOD持续升高,2010年后开始下降。空间场上表现为全区一致的变化特征,高值区主要位于两湖盆地中部,以洞庭湖为中心呈南北纵向分布。进一步对两湖盆地AOD年代际变化与大气环流异常关系的分析表明,在东亚经向风南北反相模的影响下,偏北风输送是影响两湖盆地AOD年代际变化的主要气象原因。在年代际尺度上,当西伯利亚高压的强度、面积增大,东亚大槽西移,西北太平洋副热带高压脊线南移时,东亚经向风南北反相模趋于正相位(即长江以北有异常偏南风、长江以南有异常偏北风)。此时,两湖盆地位于气旋性环流异常的底部,在异常的偏北风的作用下,西北地区的气溶胶向两湖盆地输送加强。且两湖盆地处于两个异常气旋性环流的中间,气压梯度小,风速偏弱,使得两湖盆地气溶胶输入大于输出,促进21世纪初AOD年代际升高。 展开更多
关键词 AOD (aerosol optical depth) 年代际 两湖盆地 冬春 经向风南北反相模
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Simulation of the Ecosystem Productivity Responses to Aerosol Diffuse Radiation Fertilization Effects over the Pan-Arctic during 2001–19 被引量:1
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作者 Zhiding ZHANG Xu YUE +3 位作者 Hao ZHOU Jun ZHU Yadong LEI Chenguang TIAN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第1期84-96,共13页
The pan-Arctic is confronted with air pollution transported from lower latitudes.Observations have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).Whil... The pan-Arctic is confronted with air pollution transported from lower latitudes.Observations have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).While such DRFEs have been explored at low to middle latitudes,the aerosol impacts on pan-Arctic ecosystems and the contributions by anthropogenic and natural emission sources remain less quantified.Here,we perform regional simulations at 0.2o×0.2ousing a well-validated vegetation model(Yale Interactive terrestrial Biosphere,YIBs)in combination with multi-source of observations to quantify the impacts of aerosol DRFEs on the net primary productivity(NPP)in the pan-Arctic during 2001-19.Results show that aerosol DRFEs increase pan-Arctic NPP by 2.19 Pg C(12.8%)yr^(-1)under clear-sky conditions,in which natural and anthropogenic sources contribute to 8.9% and 3.9%,respectively.Under all-sky conditions,such DRFEs are largely dampened by cloud to only 0.26 Pg C(1.24%)yr^(-1),with contributions of 0.65% by natural and 0.59% by anthropogenic species.Natural aerosols cause a positive NPP trend of 0.022% yr^(-1)following the increased fire activities in the pan-Arctic.In contrast,anthropogenic aerosols induce a negative trend of-0.01% yr^(-1)due to reduced emissions from the middle latitudes.Such trends in aerosol DRFEs show a turning point in the year of 2007 with more positive NPP trends by natural aerosols but negative NPP trends by anthropogenic aerosols thereafter.Though affected by modeling uncertainties,this study suggests a likely increasing impact of aerosols on terrestrial ecosystems in the pan-Arctic under global warming. 展开更多
关键词 diffuse radiation fertilization effects anthropogenic aerosols natural aerosols pan-Arctic net primary productivity
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Anthropogenic Influence on Decadal Changes in Concurrent Hot and Dry Events over China around the Mid-1990s 被引量:1
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作者 Qin SU Buwen DONG +1 位作者 Fangxing TIAN Nicholas P.KLINGAMAN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第2期233-246,共14页
The frequency and duration of observed concurrent hot and dry events(HDEs) over China during the growing season(April–September) exhibit significant decadal changes across the mid-1990s. These changes are characteriz... The frequency and duration of observed concurrent hot and dry events(HDEs) over China during the growing season(April–September) exhibit significant decadal changes across the mid-1990s. These changes are characterized by increases in HDE frequency and duration over most of China, with relatively large increases over southeastern China(SEC), northern China(NC), and northeastern China(NEC). The frequency of HDEs averaged over China in the present day(PD,1994–2011) is double that in the early period(EP, 1964–81);the duration of HDEs increases by 60%. Climate experiments with the Met Office Unified Model(MetUM-GOML2) are used to estimate the contributions of anthropogenic forcing to HDE decadal changes over China. Anthropogenic forcing changes can explain 60%–70% of the observed decadal changes,suggesting an important anthropogenic influence on HDE changes over China across the mid-1990s. Single-forcing experiments indicate that the increase in greenhouse gas(GHG) concentrations dominates the simulated decadal changes,increasing the frequency and duration of HDEs throughout China. The change in anthropogenic aerosol(AA) emissions significantly decreases the frequency and duration of HDEs over SEC and NC, but the magnitude of the decrease is much smaller than the increase induced by GHGs. The changes in HDEs in response to anthropogenic forcing are mainly due to the response of climatological mean surface air temperatures. The contributions from changes in variability and changes in climatological mean soil moisture and evapotranspiration are relatively small. The physical processes associated with the response of HDEs to GHG and AA changes are also revealed. 展开更多
关键词 concurrent hot and dry events decadal variation greenhouse gases aerosol emissions
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Composition optimization and performance prediction for ultra-stable water-based aerosol based on thermodynamic entropy theory
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作者 Tingting Kang Canjun Yan +6 位作者 Xinying Zhao Jingru Zhao Zixin Liu Chenggong Ju Xinyue Zhang Yun Zhang Yan Wu 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2024年第3期437-446,共10页
Water-based aerosol is widely used as an effective strategy in electro-optical countermeasure on the battlefield used to the preponderance of high efficiency,low cost and eco-friendly.Unfortunately,the stability of th... Water-based aerosol is widely used as an effective strategy in electro-optical countermeasure on the battlefield used to the preponderance of high efficiency,low cost and eco-friendly.Unfortunately,the stability of the water-based aerosol is always unsatisfactory due to the rapid evaporation and sedimentation of the aerosol droplets.Great efforts have been devoted to improve the stability of water-based aerosol by using additives with different composition and proportion.However,the lack of the criterion and principle for screening the effective additives results in excessive experimental time consumption and cost.And the stabilization time of the aerosol is still only 30 min,which could not meet the requirements of the perdurable interference.Herein,to improve the stability of water-based aerosol and optimize the complex formulation efficiently,a theoretical calculation method based on thermodynamic entropy theory is proposed.All the factors that influence the shielding effect,including polyol,stabilizer,propellant,water and cosolvent,are considered within calculation.An ultra-stable water-based aerosol with long duration over 120 min is obtained with the optimal fogging agent composition,providing enough time for fighting the electro-optic weapon.Theoretical design guideline for choosing the additives with high phase transition temperature and low phase transition enthalpy is also proposed,which greatly improves the total entropy change and reduce the absolute entropy change of the aerosol cooling process,and gives rise to an enhanced stability of the water-based aerosol.The theoretical calculation methodology contributes to an abstemious time and space for sieving the water-based aerosol with desirable performance and stability,and provides the powerful guarantee to the homeland security. 展开更多
关键词 Ultra-stable Water-based aerosol Thermodynamic entropy Composition optimization Performance prediction
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Electric field and force characteristic of dust aerosol particles on the surface of high-voltage transmission line
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作者 刘滢格 李兴财 +2 位作者 王娟 马鑫 孙文海 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第1期368-378,共11页
High-voltage transmission lines play a crucial role in facilitating the utilization of renewable energy in regions prone to desertification. The accumulation of atmospheric particles on the surface of these lines can ... High-voltage transmission lines play a crucial role in facilitating the utilization of renewable energy in regions prone to desertification. The accumulation of atmospheric particles on the surface of these lines can significantly impact corona discharge and wind-induced conductor displacement. Accurately quantifying the force exerted by particles adhering to conductor surfaces is essential for evaluating fouling conditions and making informed decisions. Therefore, this study investigates the changes in electric field intensity along branched conductors caused by various fouling layers and their resulting influence on the adhesion of dust particles. The findings indicate that as individual particle size increases, the field strength at the top of the particle gradually decreases and eventually stabilizes at approximately 49.22 k V/cm, which corresponds to a field strength approximately 1.96 times higher than that of an unpolluted transmission line. Furthermore,when particle spacing exceeds 15 times the particle size, the field strength around the transmission line gradually decreases and approaches the level observed on non-adhering surface. The electric field remains relatively stable. In a triangular arrangement of three particles, the maximum field strength at the tip of the fouling layer is approximately 1.44 times higher than that of double particles and 1.5 times higher compared to single particles. These results suggest that particles adhering to the transmission line have a greater affinity for adsorbing charged particles. Additionally, relevant numerical calculations demonstrate that in dry environments, the primary adhesion forces between particles and transmission lines follow an order of electrostatic force and van der Waals force. Specifically, at the minimum field strength, these forces are approximately74.73 times and 19.43 times stronger than the gravitational force acting on the particles. 展开更多
关键词 high-voltage current electric field aerosol particles force characteristic
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Experimental investigation on effective aerosol scavenging using different spray configurations with pre-injection of water mist for Fukushima Daiichi decommissioning
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作者 Rui-Cong Xu Avadhesh Kumar Sharma +2 位作者 Erdal Ozdemir Shuichiro Miwa Shunichi Suzuki 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第5期154-172,共19页
During the decommissioning of the Fukushima Daiichi nuclear power plant,it is important to consider the retrieval of resolidified debris both in air and underwater configurations.For the subsequent retrieval of debris... During the decommissioning of the Fukushima Daiichi nuclear power plant,it is important to consider the retrieval of resolidified debris both in air and underwater configurations.For the subsequent retrieval of debris from the reactor building,the resolidified debris must be cut into smaller pieces using various cutting methods.During the cutting process,aerosol particles are expected to be generated at the submicron scale.It has been noted that such aerosols sizing within the Greenfield gap(0.1-1μm)are difficult to remove effectively using traditional spraying methods.Therefore,to improve the aerosol removal efficiency of the spray system,a new aerosol agglomeration method was recently proposed,which involves injecting water mist to enlarge the sizes of the aerosol particles before removing them using water sprays.In this study,a series of experiments were performed to clarify the proper spray configurations for effective aerosol scavenging and to improve the performance of the water mist.The experimental results showed that the spray flow rate and droplet characteristics are important factors for the aerosol-scavenging efficiency and performance of the water mist.The results obtained from this study will be helpful for the optimization of the spray system design for effective aerosol scavenging during the decommissioning of the Fukushima Daiichi plant. 展开更多
关键词 Fukushima Daiichi decommissioning Aerosol scavenging Multiphase flow Spray system Aerosol-mist agglomeration
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A Deep-Learning and Transfer-Learning Hybrid Aerosol Retrieval Algorithm for FY4-AGRI:Development and Verification over Asia
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作者 Disong Fu Hongrong Shi +9 位作者 Christian AGueymard Dazhi Yang Yu Zheng Huizheng Che Xuehua Fan Xinlei Han Lin Gao Jianchun Bian Minzheng Duan Xiangao Xia 《Engineering》 SCIE EI CAS CSCD 2024年第7期164-174,共11页
The Advanced Geosynchronous Radiation Imager(AGRI)is a mission-critical instrument for the Fengyun series of satellites.AGRI acquires full-disk images every 15 min and views East Asia every 5 min through 14 spectral b... The Advanced Geosynchronous Radiation Imager(AGRI)is a mission-critical instrument for the Fengyun series of satellites.AGRI acquires full-disk images every 15 min and views East Asia every 5 min through 14 spectral bands,enabling the detection of highly variable aerosol optical depth(AOD).Quantitative retrieval of AOD has hitherto been challenging,especially over land.In this study,an AOD retrieval algorithm is proposed that combines deep learning and transfer learning.The algorithm uses core concepts from both the Dark Target(DT)and Deep Blue(DB)algorithms to select features for the machinelearning(ML)algorithm,allowing for AOD retrieval at 550 nm over both dark and bright surfaces.The algorithm consists of two steps:①A baseline deep neural network(DNN)with skip connections is developed using 10 min Advanced Himawari Imager(AHI)AODs as the target variable,and②sunphotometer AODs from 89 ground-based stations are used to fine-tune the DNN parameters.Out-of-station validation shows that the retrieved AOD attains high accuracy,characterized by a coefficient of determination(R2)of 0.70,a mean bias error(MBE)of 0.03,and a percentage of data within the expected error(EE)of 70.7%.A sensitivity study reveals that the top-of-atmosphere reflectance at 650 and 470 nm,as well as the surface reflectance at 650 nm,are the two largest sources of uncertainty impacting the retrieval.In a case study of monitoring an extreme aerosol event,the AGRI AOD is found to be able to capture the detailed temporal evolution of the event.This work demonstrates the superiority of the transfer-learning technique in satellite AOD retrievals and the applicability of the retrieved AGRI AOD in monitoring extreme pollution events. 展开更多
关键词 Aerosol optical depth Retrieval algorithm Deep learning Transfer learning Advanced Geosynchronous Radiation IMAGER
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Aerosol deposition technology and its applications in batteries
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作者 Xinyu Wang Ramon Alberto Paredes Camacho +6 位作者 Xiaoyu Xu Yumei Wang Yi Qiang Hans Kungl Ruediger-AEichel Yunfeng Zhang Li Lu 《Nano Materials Science》 EI CAS CSCD 2024年第1期24-37,共14页
Aerosol deposition(AD)method is a kind of additive manufacturing technology for fabricating dense films such as metals and ceramics at room temperature.It resolves the challenge of integrating ceramic films onto tempe... Aerosol deposition(AD)method is a kind of additive manufacturing technology for fabricating dense films such as metals and ceramics at room temperature.It resolves the challenge of integrating ceramic films onto temperaturesensitive substrates,including metals,glasses,and polymers.It should be emphasized that the AD is a spray coating technology that uses powder without thermal assistance to generate films with high density.Compared to the traditional sputter-based approach,the AD shows several advantages in efficiency,convenience,better interfacial bonding and so on.Therefore,it opens some possibilities to the field of batteries,especially all-solidstate batteries(ASSBs)and draws much attention not only for research but also for large scale applications.The purpose of this work is to provide a critical review on the science and technology of AD as well as its applications in the field of batteries.The process,mechanism and effective parameters of AD,and recent developments in AD applications in the field of batteries will be systematically reviewed so that a trend for AD will be finally provided. 展开更多
关键词 Aerosol deposition Room temperature impact consolidation Ceramic film All-solid-state battery Spray coating technology
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Contribution of Satellite Observations in the Optical and Microphysical Characterization of Aerosols in Burkina Faso, West Africa
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作者 Nébon Bado Serge Dimitri Bazyomo +4 位作者 Germain Wende Pouiré Ouedraogo Bruno Korgo Mamadou Simina Dramé Florent P. Kieno Sié Kam 《Atmospheric and Climate Sciences》 2024年第1期154-171,共18页
In this work, we proceed to an optical and microphysical analysis of the observations reversed by the MODIS, SeaWiFS, MISR and OMI sensors with the aim of proposing the best-adapted airborne sensor for better monitori... In this work, we proceed to an optical and microphysical analysis of the observations reversed by the MODIS, SeaWiFS, MISR and OMI sensors with the aim of proposing the best-adapted airborne sensor for better monitoring of aerosols in Burkina Faso. To this end, a comparison of AOD between satellite observations and in situ measurements at the Ouagadougou site reveals an underestimation of AERONET AOD except for OMI which overestimates them. Also, an inter-comparison done based on the linear regression line representation shows the correlation between the aerosol models incorporated in the airborne sensor inversion algorithms and the aerosol population probed. This can be seen through the correlation coefficients R which are 0.84, 0.64, 0.55 and 0.054 for MODIS, SeaWiFS, MISR and OMI respectively. Furthermore, an optical analysis of aerosols in Burkina Faso by the MODIS sensor from 2001 to 2016 indicates a large spatial and temporal variability of particles strongly dominated by desert dust. This is corroborated by the annual and seasonal cycles of the AOD at 550 nm and the Angström coefficient measured in the spectral range between 412 nm and 470 nm. A zoom on a few sites chosen according to the three climatic zones confirms the majority presence of mineral aerosols in Burkina Faso, whose maxima are observed in spring and summer. 展开更多
关键词 AERONET Airborne Sensors AEROSOL Optical and Microphysical Properties
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Some Features of Black Carbon Aerosols Connected with Regional Climate Over Pristine Environment
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作者 Saurabh Yadav Panuganti C.S.Devara +4 位作者 S.M.Sonbawne B.S.Murthy S.Tiwari S.Wadhwa A.Kumar 《Journal of Atmospheric Science Research》 2024年第1期1-18,共18页
The authors report the results of aethalometer black carbon(BC)aerosol measurements carried out over a rural(pristine)site,Panchgaon,Haryana State,India during the winter months of 2021-2022 and 2022-2023.They are com... The authors report the results of aethalometer black carbon(BC)aerosol measurements carried out over a rural(pristine)site,Panchgaon,Haryana State,India during the winter months of 2021-2022 and 2022-2023.They are compared with collocated and concurrent observations from the Air Quality Monitoring Station(AQMS),which provides synchronous air pollution and surface meteorological parameters.Secular variations in BC mass concentration are studied and explained with variations in local meteorological parameters.The biomass burning fire count retrievals from NASA-NOAA VIIRS satellite,and backward airmass trajectories from NOAA-ERL HYSPLIT Model analysis have also been utilized to explain the findings.They reveal that the north-west Indian region contributes maximum to the BC mass concentration over the study site during the study period.Moreover,the observed BC mass concentrations corroborate the synchronous fire count,primary and secondary pollutant concentrations.The results were found to aid the development of mitigation methods to achieve a sustainable climate system. 展开更多
关键词 Carbonaceous aerosols Dual-spot technique Temporal variations Primary and secondary pollutants Stubble burning Long-range transport Satellite products
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Mongolia Contributed More than 42%of the Dust Concentrations in Northern China in March and April 2023 被引量:3
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作者 Siyu CHEN Dan ZHAO +8 位作者 Jianping HUANG Jiaqi HE Yu CHEN Junyan CHEN Hongru BI Gaotong LOU Shikang DU Yue ZHANG Fan YANG 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2023年第9期1549-1557,共9页
Dust storms are one of the most frequent meteorological disasters in China,endangering agricultural production,transportation,air quality,and the safety of people’s lives and property.Against the backdrop of climate ... Dust storms are one of the most frequent meteorological disasters in China,endangering agricultural production,transportation,air quality,and the safety of people’s lives and property.Against the backdrop of climate change,Mongolia’s contribution to China’s dust cannot be ignored in recent years.In this study,we used the Weather Research and Forecasting model coupled with Chemistry(WRF-Chem),along with dynamic dust sources and the HYSPLIT model,to analyze the contributions of different dust sources to dust concentrations in northern China in March and April 2023.The results show that the frequency of dust storms in 2023 was the highest observed in the past decade.Mongolia and the Taklimakan Desert were identified as two main dust sources contributing to northern China.Specifically,Mongolia contributed more than 42%of dust,while the Taklimakan Desert accounted for 26%.A cold high-pressure center,a cold front,and a Mongolian cyclone resulted in the transport of dust aerosols from Mongolia and the Taklimakan Desert to northern China,where they affected most parts of the region.Moreover,two machine learning methods[the XGBoost algorithm and the Synthetic Minority Oversampling Technique(SMOTE)]were used to forecast the dust storms in March 2023,based on ground observations and WRF-Chem simulations over East Asia.XGBoost-SMOTE performed well in predicting hourly PM10 concentrations in China in March 2023,with a mean absolute error of 33.8μg m−3 and RMSE of 54.2μg m−3. 展开更多
关键词 dust aerosol Mongolian dust transboundary contribution WRF-Chem HYSPLIT model
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Fluorescence Properties and Chemical Composition of Fine Particles in the Background Atmosphere of North China
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作者 Ping LI Siyao YUE +13 位作者 Xiaoyang YANG Di LIU Qiang ZHANG Wei HU Shengjie HOU Wanyu ZHAO Hong REN Gang LI Yuanguan GAO Junjun DENG Qiaorong XIE Yele SUN Zifa WANG Pingqing FU 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2023年第7期1159-1174,共16页
To understand the aerosol characteristics in a regional background environment,fine-particle(PM_(2.5),n=228)samples were collected over a one-year period at the Shangdianzi(SDZ)station,which is a Global Atmospheric Wa... To understand the aerosol characteristics in a regional background environment,fine-particle(PM_(2.5),n=228)samples were collected over a one-year period at the Shangdianzi(SDZ)station,which is a Global Atmospheric Watch regional background station in North China.The chemical and optical characteristics of PM_(2.5)were analyzed,including organic carbon,elemental carbon,water-soluble organic carbon,water-soluble inorganic ions,and fluorescent components of watersoluble organic matter.The source factors of major aerosol components are apportioned,and the sources of the fluorescent chromophores are further analyzed.The major chemical components of PM_(2.5)at SDZ were NO_(3)^(-),organic matter,SO_(4)^(2-),and NH_(4)^(+).Annually,water-soluble organic carbon contributed 48%±15%to the total organic carbon.Secondary formation(52%)and fossil fuel combustion(63%)are the largest sources of water-soluble organic matter and water-insoluble organic matter,respectively.In addition,three humic-like and one protein-like matter were identified via parallel factor analysis for excitation–emission matrices.The fluorescence intensities of the components were highest in winter and lowest in summer,indicating the main impact of burning sources.This study contributes to understanding the chemical and optical characteristics of ambient aerosols in the background atmosphere. 展开更多
关键词 fine aerosols excitation-emission matrix fluorescence properties primary biological aerosols Shangdianzi
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A Statistical Algorithm for Retrieving Background Value of Absorbing Aerosol Index Based on TROPOMI Measurements
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作者 Fuying TANG Weihe WANG +4 位作者 Fuqi SI Haijin ZHOU Yuhan LUO Dongshang YANG Yuanyuan QIAN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2023年第6期1104-1116,共13页
The ultraviolet aerosol index(UVAI) is essential for monitoring the absorbing aerosols during aerosol events. UVAI depends on the absorbing aerosol concentration, the viewing geometry, and the temporal drift of radiom... The ultraviolet aerosol index(UVAI) is essential for monitoring the absorbing aerosols during aerosol events. UVAI depends on the absorbing aerosol concentration, the viewing geometry, and the temporal drift of radiometric sensitivity. To efficiently detect absorbing aerosols with the highest precision and to improve the accuracy of long-term UVAI estimates,the background UVAI must be examined through the UVAI retrieval. This study presents a statistical method that calculates the background value of UVAI using TROPOspheric Monitoring Instrument(TROPOMI) observation data over the Pacific Ocean under clear-sky scenes. Radiative transfer calculations were performed to simulate the dependence of UVAI on aerosol type and viewing geometry. We firstly applied the background UVAI to reducing the effects of viewing geometry and the degradation of the TROPOMI irradiance measurements on the UVAI. The temporal variability of the background UVAI under the same viewing geometry and aerosol concentration was identified. Radiative transfer calculations were performed to study the changes in background UVAI using Aerosol Optical Depth from the Moderate Resolution Imaging Spectroradiometer(MODIS) and reflectance measurements from TROPOMI as input. The trends of the temporal variations in the background UVAI agreed with the simulations. Alterations in the background UVAI expressed the reflectance variations driven by the changes in satellite state. Decreasing trends in solar irradiance at 340 and 380 nm due to instrument degradation were identified. Our findings are valuable because they can be applied to future retrievals of UVAI from the Environmental Trace Gases Monitoring Instrument(EMI) onboard the Chinese GaoFen-5 satellite. 展开更多
关键词 ultraviolet aerosol index background UVAI TROPOMI reflectance DEGRADATION
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Temporal and Spatial Distribution of SARS-CoV-2 Aerosols in a Large-Scale Fangcang Shelter Hospital in Shanghai,China
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作者 Jiafu Jiang Zhe Yin +23 位作者 Jing Li Leili Jia Rulin He Wenhui Yang Jihu Yang Hang Fan Sen Zhang Yunfei Wang Zengming Zhao Haoran Peng Lizhong Li Yi Yang Shi-Yong Fan Rong Xiang Jianshu Guo Jinjin Wang Juanning Wei Fengling Zhou Ding Liu Ping Zhao Yujun Cui Yunxi Liu Dongsheng Zhou Gang Dong 《Engineering》 SCIE EI CAS CSCD 2023年第9期222-233,共12页
The coronavirus disease 2019(COVID-19)pandemic caused by frequently mutating severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)has had a worldwide impact.However,detailed data on the potential aerosol transmi... The coronavirus disease 2019(COVID-19)pandemic caused by frequently mutating severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)has had a worldwide impact.However,detailed data on the potential aerosol transmission of SARS-CoV-2 in real-world and controlled laboratory settings remain sparse.During the COVID-19 pandemic in Shanghai,China in 2022,samples were collected in a Fangcang shelter hospital,a large-scale temporary hospital rapidly built by converting the existing National Exhibition and Convention Center(Shanghai)into a health care facility.Aerosol samples at different sites and intervals around patients and in public areas,surface samples,and pharyngeal swab samples from corresponding patients were included.Samples were tested for SARS-CoV-2 using real-time quantitative polymerase chain reaction(RT-qPCR)assays,followed by sequencing if the cycle threshold(Ct)value was<30.The positivity rate for SARS-CoV-2 in aerosol samples was high in contaminated zones(37.5%,104/277),especially around the bed(41.2%,68/165)and near ventilation inlets(45.2%,14/31).The prevalence of SARS-CoV-2 around the bed,public areas,and air inlets of exhaust vents fluctuated and was closely related to the positivity rate among patients at corresponding sampling sites.Some surface samples of different personal protective equipment from medical staff had high positivity rates.Sixty sequences of joined ORF1ab and spike genes obtained from sixty samples represented two main clusters of Omicron SARS-CoV-2.There was consistency in virus sequences from the same patient and their environment,and the detected virus sequences matched those of virus strains in circulation during the collection periods,which indicated a high likelihood of cross-contamination in the Fangcang shelter hospital.In summary,the results provide a quantitative and real landscape of the aerosol transmission of SARS-CoV-2 and a patient-centered view of contamination in large and enclosed spaces and offer a useful guide for taking targeted measures to avoid nosocomial infections during the management of SARS-CoV-2 or other respiratory virus diseases in a Fangcang shelter hospital. 展开更多
关键词 Coronavirus disease 2019 Severe acute respiratory syndrome coronavirus 2 AEROSOLS Fangcang shelter hospital China
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Spinal fusion is an aerosol generating procedure
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作者 Joanna Lind Langner Nicole Segovia Pham +3 位作者 Ann Richey Yousi Oquendo Shayna Mehta John Schoeneman Vorhies 《World Journal of Orthopedics》 2023年第5期340-347,共8页
BACKGROUND Transmission of severe acute respiratory syndrome coronavirus 2 can occur during aerosol generating procedures.Several steps in spinal fusion may aerosolize blood but little data exists to quantify the risk... BACKGROUND Transmission of severe acute respiratory syndrome coronavirus 2 can occur during aerosol generating procedures.Several steps in spinal fusion may aerosolize blood but little data exists to quantify the risk this may confer upon surgeons.Aerosolized particles containing infectious coronavirus are typically 0.5-8.0μm.AIM To measure the generation of aerosols during spinal fusion using a handheld optical particle sizer(OPS).METHODS We quantified airborne particle counts during five posterior spinal instrumentation and fusions(9/22/2020-10/15/2020)using an OPS near the surgical field.Data were analyzed by 3 particle size groups:0.3-0.5μm/m^(3),1.0-5.0μm/m^(3),and 10.0μm/m^(3).We used hierarchical logistic regression to model the odds of a spike in aerosolized particle counts based on the step in progress.A spike was defined as a>3 standard deviation increase from average baseline levels.RESULTS Upon univariate analysis,bovie(P<0.0001),high speed pneumatic burring(P=0.009),and ultrasonic bone scalpel(P=0.002)were associated with increased 0.3-0.5μm/m^(3)particle counts relative to baseline.Bovie(P<0.0001)and burring(P<0.0001)were also associated with increased 1-5μm/m^(3)and 10μm/m^(3)particle counts.Pedicle drilling was not associated with increased particle counts in any of the size ranges measured.Our logistic regression model demonstrated that bovie(OR=10.2,P<0.001),burring(OR=10.9,P<0.001),and bone scalpel(OR=5.9,P<0.001)had higher odds of a spike in 0.3-0.5μm/m^(3)particle counts.Bovie(OR=2.6,P<0.001),burring(OR=5.8,P<0.001),and bone scalpel(OR=4.3,P=0.005)had higher odds of a spike in 1-5μm/m^(3)particle counts.Bovie(OR=0.3,P<0.001)and drilling(OR=0.2,P=0.011)had significantly lower odds of a spike in 10μm/m^(3)particle counts relative to baseline.CONCLUSION Several steps in spinal fusion are associated with increased airborne particle counts in the aerosol size range.Further research is warranted to determine if such particles have the potential to contain infectious viruses.Previous research has shown that electrocautery smoke may be an inhalation hazard for surgeons but here we show that usage of the bone scalpel and high-speed burr also have the potential to aerosolize blood. 展开更多
关键词 Optical particle sizers AEROSOL COVID-19 Orthopaedic procedures Spinal fusion SARS-CoV-2
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Effects of Spring Biomass Burning in the Indochina Peninsula on May Precipitation in South China
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作者 Qianqian Mao Shuyu Liu Yu Huang 《Journal of Water Resource and Protection》 CAS 2023年第5期179-193,共15页
Each year, during the dry season that precedes the summer wind and rainfall Indo-China Peninsula (ICP), significant biomass burning occurs and reaches its peak from March to April. This biomass burning generates large... Each year, during the dry season that precedes the summer wind and rainfall Indo-China Peninsula (ICP), significant biomass burning occurs and reaches its peak from March to April. This biomass burning generates large amounts of aerosols that impact East Asia and surrounding areas through the Asian monsoon. This study aims to investigate the potential connection between biomass burning over the ICP and precipitation in South China during May, along with the physical processes involved. The analysis is based on GLDAS soil moisture reanalysis data and CPC (NOAA) precipitation data covering the period from 1980 to 2021. The research findings indicate a negative (positive) correlation between biomass burning in the ICP region during spring and precipitation in the same region (South China) during May. The circulation patterns corresponding to years with biomass-burning emission anomalies are further investigated, and the impact of biomass-burning emissions in spring on soil moisture and temperature is examined. The results suggest that biomass-burning emissions can significantly affect atmospheric circulation and precipitation, ultimately leading to anomalous precipitation in South China. 展开更多
关键词 Indo-China Peninsula Biomass-Burning Aerosols Atmospheric Circulation PRECIPITATION
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Changes in Aerosol Optical Depth over the Arctic Ocean as Seen by CALIOP, MAIAC, and MODIS C6.1
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作者 Nicole Mölders Mariel Friberg 《Journal of Environmental Protection》 2023年第6期419-440,共22页
Due to the recent increase in Arctic shipping, 2006-2020 June to October Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 (C6.1), and Mult... Due to the recent increase in Arctic shipping, 2006-2020 June to October Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 (C6.1), and Multi-Angle Implementation of Atmospheric Correction (MAIAC) retrieved aerosol optical depth (AOD) data were examined for changes in AOD from period 1 (P1, 2006-2012) to period 2 (P2, 2014-2020 (P2). Herein, AOD was statistically analyzed on a 0.25° × 0.25° grid and in the airsheds over the various ocean basins over the Arctic north of 59.75°N. According to heatmaps of the correlation between AOD and ship traffic, and AOD and fire emissions for the airsheds, all three AOD products captured the observed inter-annual variability in wildfire occurrence well, and showed wildfire emissions over Siberia were more severe in P2 than P1. Except for the Atlantic, North, and Baltic Seas, Beaufort Sea, and Barents Sea, all three AOD products indicated that AOD was higher over the various basins in P2 than P1, but disagreed on the magnitude. This fact suggests that the detection of changes in the typical low AOD over the Arctic Ocean might be rather qualitative than quantitative. While all products captured increases in AOD due to ships at berth, only MODIS C6.1 caught the elevated AOD due to shipping on the Siberian rivers. Obviously, sub-daily resolutions are required to capture increased AOD due to short-term events like a traveling ship or short-interval fire. 展开更多
关键词 Arctic Aerosol Optical Depth Changes in Aerosol Optical Depth Arctic Ship-Emissions Impacts on AOD Boreal Wildfire Impacts on AOD
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Weathering the Storm: Mitigating Hurricanes with Ground-Based CCN and Lightning
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作者 Venkata Chaganti Murali Krishna Cheruvu 《Journal of Geoscience and Environment Protection》 2023年第12期13-27,共15页
This research introduces a groundbreaking methodology aimed at mitigating storm and hurricane intensity through the application of a ground-based, manually operated Cloud Condensation Nuclei (CCN) Generator. To meet t... This research introduces a groundbreaking methodology aimed at mitigating storm and hurricane intensity through the application of a ground-based, manually operated Cloud Condensation Nuclei (CCN) Generator. To meet the demand for more comprehensive context and rationale, this study explores the escalating challenges presented by the growing intensity of hurricanes, exemplified by Hurricane IAN (2022). The controlled release of environmentally friendly aerosols into the atmosphere, achieved by combusting selected wood pieces and organic edible materials, is a pivotal response to the escalating threat of extreme weather events. By generating CCN, the novel approach seeks to augment positive lightning in the eyewall, providing a potential solution to the intensification of hurricanes. Results illustrate the successful implementation of the methodology, with released aerosols effectively reaching the clouds for seeding, thus contributing to the modification of convection in the outer wall of Hurricane IAN and consequent intensity reduction. Rigorous experiments, incorporating considerations of various parameters such as wind patterns and the experimental location in Sarasota City, emphasize the scientific rigor applied to weakening Hurricane IAN. This comprehensive approach not only holds promise in mitigating hurricane intensity but also sheds light on the potential impact of cloud seeding in reducing the severity of future hurricanes, addressing a critical need for sustainable solutions to climate-related challenges. 展开更多
关键词 IAN 2022 Hurricane Mitigation LIGHTNING AEROSOL Cloud Condensation Nuclei (CCN)
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Current Status of Rn-220 Chamber Carrier Aerosol Modulation Research
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作者 Yanan Liu Yu Cheng 《Journal of Geoscience and Environment Protection》 2023年第4期30-36,共7页
Radon is the most important source of natural radiation to human beings and the second major causative agent of lung cancer other than smoking. In recent years, the hazards of human exposure to thoron (Rn-220), anothe... Radon is the most important source of natural radiation to human beings and the second major causative agent of lung cancer other than smoking. In recent years, the hazards of human exposure to thoron (Rn-220), another isotope of radon, and its progeny have gained consensus. To accurately evaluate the dose level and hazards of Rn-220 and its progeny, a standard Rn-220 chamber with strong regulation ability for Rn-220 and its progeny needs to be established for the scale or calibration of measurement instruments. This paper describes the hazards, sources, behavioral characteristics of Rn-220 and its progeny, and some representative Rn-220 chambers established in various countries. 展开更多
关键词 THORON Rn-220 Chamber Aerosol Modulation
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