Negative air ions are natural components of the air we breathe Forests are the main continuous natural source of negative air ions (NAI). The spatio-temporal patterns of negative air ions were explored in Shanghai, ...Negative air ions are natural components of the air we breathe Forests are the main continuous natural source of negative air ions (NAI). The spatio-temporal patterns of negative air ions were explored in Shanghai, based on monthly monitoring in 15 parks from March 2009 to February 2010. In each park, sampling sites were selected in forests and open spaces. The annual variation in negative air ion concentrations (NAIC) showed peak values from June to October and minimum values from December to January. NAIC were highest in summer and autumn, intermediate in spring, and lowest in winter. During spring and summer, NAIC in open spaces were significantly higher in rural areas than those in suburban areas. However, there were no significant differences in NAIC at forest sites among seasons. For open spaces, total suspended particles (TSP) were the dominant determining factor of NAIC in sum- mer, and air temperature and air humidity were the dominant determining factors of NAIC in spring, which were tightly correlated with Shanghai's ongoing urbanization and its impacts on the environment. R is suggested that urbanization could induce variation in NAIC along the urban-rural gradient, but that may not change the temporal variation pattern. Fur- thermore, the effects of urbanization on NAIC were limited in non-vegetated or less-vegetated sites, such as open spaces, but not in well-vegetated areas, such as urban forests. Therefore, we suggest that urban greening, especially urban forest, has significant resistance to theeffect of urbanization on NAIC.展开更多
Atmosphere is the basic environmental element on which human beings depend for survival and development,and its environmental quality is directly related to sustainable socio-economic development.China is currently in...Atmosphere is the basic environmental element on which human beings depend for survival and development,and its environmental quality is directly related to sustainable socio-economic development.China is currently in a period of accelerated urbanization,accompanied by industrialization and urbanization bringing environmental pollution problems more and more prominent.Therefore,it is particularly important to strengthen the management of atmospheric quality and improve the level of atmospheric environment.To this end,the spatial and temporal distribution characteristics of AQI and six types of air pollutants in eight prefecture-level cities were analysed and studied using the month-by-month air quality monitoring data of Sichuan Province from 2017 to 2021.The results show that:(1)according to the Ambient Air Quality Standards,Chengdu,Mianyang,Zigong,Luzhou and Deyang do not meet the concentration limits of PM_(2.5),Zigong and Suining do not meet the concentration limits of PM_(10),Chengdu does not meet the concentration limits of NO_(2),and all eight cities meet the concentration limits of NO_(2)and SO_(2).(2)The seasonal concentration changes of PM_(2.5),PM_(10)and NO_(2)have the same characteristics,showing that they are winter>spring>autumn>summer.The seasonal concentration changes of CO are winter>autumn>spring>summer;the seasonal concentration changes of SO_(2)are winter>spring>summer>autumn;the seasonal concentration changes of O_(3)are summer>spring>autumn>winter.展开更多
In 2016 WHO reported that Kolkata is the second most polluted city inIndia behind Delhi. Albeit the number of registered vehicles in Kolkatais much less compare to Delhi. Kolkata has encountered a decade longbattle ag...In 2016 WHO reported that Kolkata is the second most polluted city inIndia behind Delhi. Albeit the number of registered vehicles in Kolkatais much less compare to Delhi. Kolkata has encountered a decade longbattle against change of old vehicles and fuel types. So, this paper madean attempt to explore the dynamics of air pollution in the city speciallypre and post period of vehicle and fuel change in the city. The objectivesof the paper include looking at spatiotemporal change of air pollution inthe city. Besides, the paper additionally illuminates on the role of landuse functions and pollution in the city. The analysis shows that after theimplementation of regulatory measures air pollution in the city reduced tosome extent but effects of the measure gradually diminished. It is foundthat land use function as well as dynamics of metropolitan area plays crucialrole in the air pollution of the city.展开更多
A synergistic pathway is regarded as a critical measure for tackling the intertwined challenges of climate change and air pollution in China. However, there is as yet no indicator that can comprehensively reflect such...A synergistic pathway is regarded as a critical measure for tackling the intertwined challenges of climate change and air pollution in China. However, there is as yet no indicator that can comprehensively reflect such synergistic effects;hence, existing studies lack a consistent framework for comparison. Here, we introduce a new synergistic indicator defined as the pollutant generation per gross domestic product (GDP) and adopt an integrated analysis framework by linking the logarithmic mean Divisia index (LMDI) method, response surface model (RSM), and global exposure mortality model (GEMM) to evaluate the synergistic effects of carbon mitigation on both air pollutant reduction and public health in China. The results show that synergistic effects played an increasingly important role in the emissions mitigation of SO_(2), NOx, and primary particulate matter with an aerodynamic diameter no greater than 2.5 μm (PM2.5), and the synergistic mitigation of pollutants respectively increase from 3.1, 1.4, and 0.3 Mt during the 11th Five-Year Plan (FYP) (2006–2010) to 5.6, 3.7, and 1.9 Mt during the 12th FYP (2011–2015). Against the non-control scenario, synergistic effects alone contributed to a 15% reduction in annual mean PM2.5 concentration, resulting in the prevention of 0.29 million (95% confidential interval: 0.28–0.30) PM2.5-attributable excess deaths in 2015. Synergistic benefits to air quality improvement and public health were remarkable in the developed and population-dense eastern provinces and municipalities. With the processes of urbanization and carbon neutrality in the future, synergistic effects are expected to continue to increase. Realizing climate targets in advance in developed regions would concurrently bring strong synergistic effects to air quality and public health.展开更多
This paper analyses the features and dynamic changes of the spatial layout of air transportation utilization among different provinces in China. It makes use of data for the airport throughput and socio-economic devel...This paper analyses the features and dynamic changes of the spatial layout of air transportation utilization among different provinces in China. It makes use of data for the airport throughput and socio-economic development of every province throughout the country in the years 2006 and 2015, and employs airport passenger and cargo throughput per capita and per unit of GDP as measures of regional air transportation utilization, which is significant for refining indicators of regional air transportation scale and comparing against them. It also analyzes the spatial differences of coupling between the regional air transportation utilization indicators and the key influencing factors on regional air transportation demand and utilization, which include per capita GDP, urbanization rate, and population density. Based on these key influencing factors, it establishes a multiple linear regression model to conduct forecasting of each province's future airport passenger and cargo throughput as well as throughput growth rates. The findings of the study are as follows:(1) Between 2006 and 2015, every province throughout the country showed a trend of year on year growth in their airport passenger and cargo throughput per capita. Throughput per capita grew fastest in Hebei, with a rise of 780%, and slowest in Beijing, with a rise of 38%. Throughput per capita was relatively high in western and southeastern coastal regions, and relatively low in northern and central regions. Airport passenger and cargo throughput per unit of GDP showed growth in provinces with relatively slow economic development, and showed negative growth in provinces with relatively rapid economic development. Throughput per unit of GDP grew fastest in Hebei, rising 265% between 2006 and 2015, and Hunan had the fastest negative growth, with a fall of 44% in the same period. Southwestern regions had relatively high throughput per unit of GDP, while in central, northern, and northeastern regions it was relatively low.(2) Strong correlation exists between airport passenger and cargo throughput per capita and per capita GDP, urbanization rate, and population density. Throughput per capita has positive correlation with per capita GDP and urbanization rate in all regions, and positive correlation with population density in most regions. Meanwhile, there is weak correlation between airport passenger and cargo throughput per unit of GDP and per capita GDP, urbanization rate, and population density, with positive correlation in some regions and negative correlation in others.(3) Between 2015 and 2025, it is estimated that all provinces experience a trend of rapid growth in their airport passenger and cargo throughput. Inner Mongolia and Hebei will see the fastest growth, rising221% and 155%, respectively, while Yunnan, Sichuan, and Hubei will see the slowest growth, with increases of 62%, 63%, and 65%, respectively.展开更多
To investigate the air quality change during the COVID-19 pandemic,we analyzed spatiotemporal variations of six criteria pollutants in nine typical urban agglomerations in China using ground-based data and examined me...To investigate the air quality change during the COVID-19 pandemic,we analyzed spatiotemporal variations of six criteria pollutants in nine typical urban agglomerations in China using ground-based data and examined meteorological influences through correlation analysis and backward trajectory analysis under different responses.Concentrations of PM2.5,PM10,NO2,SO2 and CO in urban agglomerations respectively decreased by 18%–45%(30%–62%),17%–53%(22%–39%),47%-64%(14%–41%),9%–34%(0%–53%)and 16%-52%(23%–56%)during Lockdown(Post-lockdown)period relative to Pre-lockdown period.PM2.5 pollution events occurred during Lockdown in Beijing-Tianjin-Hebe(BTH)and Middle and South Liaoning(MSL),and daily O3 concentration rose to gradeⅡstandard in Post-lockdown period.Distinct from the nationwide slump of NO2 during Lockdown period,a rebound(~40%)in Post-lockdown period was observed in Cheng-Yu(CY),Yangtze River Middle-Reach(YRMR),Yangtze River Delta(YRD)and Pearl River Delta(PRD).With slightly higher wind speed compared with 2019,the reduction of PM2.5(51%–62%)in Post-lockdown period is more than2019(15%–46%)in HC(Harbin-Changchun),MSL,BTH,CP(Central Plain)and SP(ShandongPeninsula),suggesting lockdown measures are effective to PM2.5 alleviation.Although O3 concentrations generally increased during the lockdown,its increment rate declined compared with 2019 under similar sunlight duration and temperature.Additionally,unlike HC,MSL and BTH,which suffered from additional(>30%)air masses from surrounding areas after the lockdown,the polluted air masses reaching YRD and PRD mostly originated from the long-distance transport,highlighting the importance of joint regional governance.展开更多
PM_(2.5) has become an increasing public concern recently because of its visibility reduction and severe health risks. For the whole year of 2013, hourly PM_(2.5) data of 496 monitoring sites scattered in 74 citie...PM_(2.5) has become an increasing public concern recently because of its visibility reduction and severe health risks. For the whole year of 2013, hourly PM_(2.5) data of 496 monitoring sites scattered in 74 cities of China are collected to analyze temporal and spatial variability of PM_(2.5) concentration. Different temporal scales(seasonal variation, monthly variation and daily variation) and spatial scales(urban versus rural, typical areas and national scale) are discussed. Results show that PM_(2.5) concentration changes significantly in both long-term and short-term scales. An apparent bimodal pattern exists in daily variation of PM_(2.5) concentration and the daytime peak appears around 10:00 am while the lowest concentration appears around 16:00 pm. Spatial autocorrelation analysis and Ordinary Kriging are used to characterize spatial variability. Moran's I of PM_(2.5) concentration in three typical regions, the Beijing-Tianjin-Hebei region, the Yangtze River Delta region and the Pearl River Delta region, is 0.906, 0.693, 0.746, respectively, which indicates that PM_(2.5) is strong spatial correlated. Spatial distribution of annual PM_(2.5) concentration simulated by Ordinary Kriging shows that 7.94 million km2(83%) areas fail in meeting the requirement of China's National Ambient Air Quality Standards Level-2(35 mg/m3) and there are at least three concentrated highly polluted areas across the country.展开更多
Based on satellite image data and China's Statistical Yearbooks(2000 to 2014), we estimated the total mass of crop residue burned, and the proportion of residue burned in the field vs.indoors as domestic fuel. The ...Based on satellite image data and China's Statistical Yearbooks(2000 to 2014), we estimated the total mass of crop residue burned, and the proportion of residue burned in the field vs.indoors as domestic fuel. The total emissions of various pollutants from the burning of crop residue were estimated for 2000-2014 using the emission factor method. The results indicate that the total amount of crop residue and average burned mass were 8690.9 Tg and4914.6 Tg, respectively. The total amount of emitted pollutants including CO2, CO, NOx,VOCs, PM(2.5), OC(organic carbon), EC(element carbon) and TC(total carbon) were 4212.4–8440.9 Tg, 192.8–579.4 Tg, 4.8–19.4 Tg, 18.6–61.3 Tg, 18.8–49.7 Tg, 6.7–31.3 Tg, 2.3–4.7 Tg, and8.5–34.1 Tg, respectively. The emissions of pollutants released from crop residue burning were found to be spatially variable, with the burning of crop residue mainly occurring in Northeast, North and South China. In addition, pollutant emissions per unit area(10 km ×10 km) were mostly concentrated in the central and eastern regions of China. Emissions of CO2, NOx, VOCs, OC and TC were mainly from rice straw burning, while burning of corn and wheat residues contributed most to emissions of CO, PM(2.5) and EC. The increased ratio of PM(2.5) emissions from crop residue burning to the total emitted from industry during the study period is attributed to the implementation of strict emissions management policies in Chinese industry. This study also provides baseline data for assessment of the regional atmospheric environment.展开更多
High concentrations of PM_(2.5) are universally considered as a main cause for haze formation. Therefore, it is important to identify the spatial heterogeneity and influencing factors of PM_(2.5) concentrations for re...High concentrations of PM_(2.5) are universally considered as a main cause for haze formation. Therefore, it is important to identify the spatial heterogeneity and influencing factors of PM_(2.5) concentrations for regional air quality control and management. In this study, PM_(2.5) data from 2000 to 2015 was determined from an inversion of NASA atmospheric remote sensing images. Using geo-statistics, geographic detectors, and geo-spatial analysis methods, the spatio-temporal evolution patterns and driving factors of PM_(2.5) concentration in China were evaluated. The main results are as follows.(1) In general, the average concentration of PM_(2.5) in China increased quickly and reached its peak value in 2006; subsequently, concentrations remained between 21.84 and 35.08 μg/m3.(2) PM_(2.5) is strikingly heterogeneous in China, with higher concentrations in the north and east than in the south and west. In particular, areas with relatively high PM_(2.5) concentrations are primarily in four regions, the Huang-Huai-Hai Plain, Lower Yangtze River Delta Plain, Sichuan Basin, and Taklimakan Desert. Among them, Beijing-Tianjin-Hebei Region has the highest concentration of PM_(2.5).(3) The center of gravity of PM_(2.5) has generally moved northeastward, which indicates an increasingly serious haze in eastern China. High-value PM_(2.5) concentrations have moved eastward, while low-value PM_(2.5) has moved westward.(4) Spatial autocorrelation analysis indicates a significantly positive spatial correlation. The "High-High" PM_(2.5) agglomeration areas are distributed in the Huang-Huai-Hai Plain, Fenhe-Weihe River Basin, Sichuan Basin, and Jianghan Plain regions. The "Low-Low" PM_(2.5) agglomeration areas include Inner Mongolia and Heilongjiang, north of the Great Wall, Qinghai-Tibet Plateau, and Taiwan, Hainan, and Fujian and other southeast coastal cities and islands.(5) Geographic detection analysis indicates that both natural and anthropogenic factors account for spatial variations in PM_(2.5) concentration. Geographical location, population density, automobile quantity, industrial discharge, and straw burning are the main driving forces of PM_(2.5) concentration in China.展开更多
基金supported by the National Natural Science Foundation of China(No.40971041)
文摘Negative air ions are natural components of the air we breathe Forests are the main continuous natural source of negative air ions (NAI). The spatio-temporal patterns of negative air ions were explored in Shanghai, based on monthly monitoring in 15 parks from March 2009 to February 2010. In each park, sampling sites were selected in forests and open spaces. The annual variation in negative air ion concentrations (NAIC) showed peak values from June to October and minimum values from December to January. NAIC were highest in summer and autumn, intermediate in spring, and lowest in winter. During spring and summer, NAIC in open spaces were significantly higher in rural areas than those in suburban areas. However, there were no significant differences in NAIC at forest sites among seasons. For open spaces, total suspended particles (TSP) were the dominant determining factor of NAIC in sum- mer, and air temperature and air humidity were the dominant determining factors of NAIC in spring, which were tightly correlated with Shanghai's ongoing urbanization and its impacts on the environment. R is suggested that urbanization could induce variation in NAIC along the urban-rural gradient, but that may not change the temporal variation pattern. Fur- thermore, the effects of urbanization on NAIC were limited in non-vegetated or less-vegetated sites, such as open spaces, but not in well-vegetated areas, such as urban forests. Therefore, we suggest that urban greening, especially urban forest, has significant resistance to theeffect of urbanization on NAIC.
基金Supported by Physical and Chemical Characteristics and Source Analysis of Atmospheric Particulate Matter in Lhasa,Tibet(21677116)National Natural Science Foundation of China,National Key Research&Development Program of China(2019YFC1904101)。
文摘Atmosphere is the basic environmental element on which human beings depend for survival and development,and its environmental quality is directly related to sustainable socio-economic development.China is currently in a period of accelerated urbanization,accompanied by industrialization and urbanization bringing environmental pollution problems more and more prominent.Therefore,it is particularly important to strengthen the management of atmospheric quality and improve the level of atmospheric environment.To this end,the spatial and temporal distribution characteristics of AQI and six types of air pollutants in eight prefecture-level cities were analysed and studied using the month-by-month air quality monitoring data of Sichuan Province from 2017 to 2021.The results show that:(1)according to the Ambient Air Quality Standards,Chengdu,Mianyang,Zigong,Luzhou and Deyang do not meet the concentration limits of PM_(2.5),Zigong and Suining do not meet the concentration limits of PM_(10),Chengdu does not meet the concentration limits of NO_(2),and all eight cities meet the concentration limits of NO_(2)and SO_(2).(2)The seasonal concentration changes of PM_(2.5),PM_(10)and NO_(2)have the same characteristics,showing that they are winter>spring>autumn>summer.The seasonal concentration changes of CO are winter>autumn>spring>summer;the seasonal concentration changes of SO_(2)are winter>spring>summer>autumn;the seasonal concentration changes of O_(3)are summer>spring>autumn>winter.
文摘In 2016 WHO reported that Kolkata is the second most polluted city inIndia behind Delhi. Albeit the number of registered vehicles in Kolkatais much less compare to Delhi. Kolkata has encountered a decade longbattle against change of old vehicles and fuel types. So, this paper madean attempt to explore the dynamics of air pollution in the city speciallypre and post period of vehicle and fuel change in the city. The objectivesof the paper include looking at spatiotemporal change of air pollution inthe city. Besides, the paper additionally illuminates on the role of landuse functions and pollution in the city. The analysis shows that after theimplementation of regulatory measures air pollution in the city reduced tosome extent but effects of the measure gradually diminished. It is foundthat land use function as well as dynamics of metropolitan area plays crucialrole in the air pollution of the city.
基金supported by the National Natural Science Foundation of China(72025401,71974108,and 72140003)the Tsinghua University-INDITEX Sustainable Development Fund.
文摘A synergistic pathway is regarded as a critical measure for tackling the intertwined challenges of climate change and air pollution in China. However, there is as yet no indicator that can comprehensively reflect such synergistic effects;hence, existing studies lack a consistent framework for comparison. Here, we introduce a new synergistic indicator defined as the pollutant generation per gross domestic product (GDP) and adopt an integrated analysis framework by linking the logarithmic mean Divisia index (LMDI) method, response surface model (RSM), and global exposure mortality model (GEMM) to evaluate the synergistic effects of carbon mitigation on both air pollutant reduction and public health in China. The results show that synergistic effects played an increasingly important role in the emissions mitigation of SO_(2), NOx, and primary particulate matter with an aerodynamic diameter no greater than 2.5 μm (PM2.5), and the synergistic mitigation of pollutants respectively increase from 3.1, 1.4, and 0.3 Mt during the 11th Five-Year Plan (FYP) (2006–2010) to 5.6, 3.7, and 1.9 Mt during the 12th FYP (2011–2015). Against the non-control scenario, synergistic effects alone contributed to a 15% reduction in annual mean PM2.5 concentration, resulting in the prevention of 0.29 million (95% confidential interval: 0.28–0.30) PM2.5-attributable excess deaths in 2015. Synergistic benefits to air quality improvement and public health were remarkable in the developed and population-dense eastern provinces and municipalities. With the processes of urbanization and carbon neutrality in the future, synergistic effects are expected to continue to increase. Realizing climate targets in advance in developed regions would concurrently bring strong synergistic effects to air quality and public health.
基金National Natural Science Foundation of China,No.41171433Philosophy and Social Science Foundation of China,No.16BJY039
文摘This paper analyses the features and dynamic changes of the spatial layout of air transportation utilization among different provinces in China. It makes use of data for the airport throughput and socio-economic development of every province throughout the country in the years 2006 and 2015, and employs airport passenger and cargo throughput per capita and per unit of GDP as measures of regional air transportation utilization, which is significant for refining indicators of regional air transportation scale and comparing against them. It also analyzes the spatial differences of coupling between the regional air transportation utilization indicators and the key influencing factors on regional air transportation demand and utilization, which include per capita GDP, urbanization rate, and population density. Based on these key influencing factors, it establishes a multiple linear regression model to conduct forecasting of each province's future airport passenger and cargo throughput as well as throughput growth rates. The findings of the study are as follows:(1) Between 2006 and 2015, every province throughout the country showed a trend of year on year growth in their airport passenger and cargo throughput per capita. Throughput per capita grew fastest in Hebei, with a rise of 780%, and slowest in Beijing, with a rise of 38%. Throughput per capita was relatively high in western and southeastern coastal regions, and relatively low in northern and central regions. Airport passenger and cargo throughput per unit of GDP showed growth in provinces with relatively slow economic development, and showed negative growth in provinces with relatively rapid economic development. Throughput per unit of GDP grew fastest in Hebei, rising 265% between 2006 and 2015, and Hunan had the fastest negative growth, with a fall of 44% in the same period. Southwestern regions had relatively high throughput per unit of GDP, while in central, northern, and northeastern regions it was relatively low.(2) Strong correlation exists between airport passenger and cargo throughput per capita and per capita GDP, urbanization rate, and population density. Throughput per capita has positive correlation with per capita GDP and urbanization rate in all regions, and positive correlation with population density in most regions. Meanwhile, there is weak correlation between airport passenger and cargo throughput per unit of GDP and per capita GDP, urbanization rate, and population density, with positive correlation in some regions and negative correlation in others.(3) Between 2015 and 2025, it is estimated that all provinces experience a trend of rapid growth in their airport passenger and cargo throughput. Inner Mongolia and Hebei will see the fastest growth, rising221% and 155%, respectively, while Yunnan, Sichuan, and Hubei will see the slowest growth, with increases of 62%, 63%, and 65%, respectively.
基金supported by the National Natural Science Foundation of China(No.21777094)the Science and Technology Commission of Shanghai Municipality(CN)(Nos.19DZ1205004,20DZ1204004)。
文摘To investigate the air quality change during the COVID-19 pandemic,we analyzed spatiotemporal variations of six criteria pollutants in nine typical urban agglomerations in China using ground-based data and examined meteorological influences through correlation analysis and backward trajectory analysis under different responses.Concentrations of PM2.5,PM10,NO2,SO2 and CO in urban agglomerations respectively decreased by 18%–45%(30%–62%),17%–53%(22%–39%),47%-64%(14%–41%),9%–34%(0%–53%)and 16%-52%(23%–56%)during Lockdown(Post-lockdown)period relative to Pre-lockdown period.PM2.5 pollution events occurred during Lockdown in Beijing-Tianjin-Hebe(BTH)and Middle and South Liaoning(MSL),and daily O3 concentration rose to gradeⅡstandard in Post-lockdown period.Distinct from the nationwide slump of NO2 during Lockdown period,a rebound(~40%)in Post-lockdown period was observed in Cheng-Yu(CY),Yangtze River Middle-Reach(YRMR),Yangtze River Delta(YRD)and Pearl River Delta(PRD).With slightly higher wind speed compared with 2019,the reduction of PM2.5(51%–62%)in Post-lockdown period is more than2019(15%–46%)in HC(Harbin-Changchun),MSL,BTH,CP(Central Plain)and SP(ShandongPeninsula),suggesting lockdown measures are effective to PM2.5 alleviation.Although O3 concentrations generally increased during the lockdown,its increment rate declined compared with 2019 under similar sunlight duration and temperature.Additionally,unlike HC,MSL and BTH,which suffered from additional(>30%)air masses from surrounding areas after the lockdown,the polluted air masses reaching YRD and PRD mostly originated from the long-distance transport,highlighting the importance of joint regional governance.
基金Supported by the National Natural Science Foundation of China(41571385)
文摘PM_(2.5) has become an increasing public concern recently because of its visibility reduction and severe health risks. For the whole year of 2013, hourly PM_(2.5) data of 496 monitoring sites scattered in 74 cities of China are collected to analyze temporal and spatial variability of PM_(2.5) concentration. Different temporal scales(seasonal variation, monthly variation and daily variation) and spatial scales(urban versus rural, typical areas and national scale) are discussed. Results show that PM_(2.5) concentration changes significantly in both long-term and short-term scales. An apparent bimodal pattern exists in daily variation of PM_(2.5) concentration and the daytime peak appears around 10:00 am while the lowest concentration appears around 16:00 pm. Spatial autocorrelation analysis and Ordinary Kriging are used to characterize spatial variability. Moran's I of PM_(2.5) concentration in three typical regions, the Beijing-Tianjin-Hebei region, the Yangtze River Delta region and the Pearl River Delta region, is 0.906, 0.693, 0.746, respectively, which indicates that PM_(2.5) is strong spatial correlated. Spatial distribution of annual PM_(2.5) concentration simulated by Ordinary Kriging shows that 7.94 million km2(83%) areas fail in meeting the requirement of China's National Ambient Air Quality Standards Level-2(35 mg/m3) and there are at least three concentrated highly polluted areas across the country.
基金supported by the Fujian Agriculture and Forestry University Funds for Distinguished Young Scholar(No.xjq201613)the National Natural Science Foundation of China(No.31400552)+1 种基金the International Science and Technology Cooperation Program of Fujian Agriculture and Forestry University(No.KXB16008A)the Asia-Pacific Network for Sustainable Forest Management and Rehabilitation(APFnet/2010/FPF/001)Phase II
文摘Based on satellite image data and China's Statistical Yearbooks(2000 to 2014), we estimated the total mass of crop residue burned, and the proportion of residue burned in the field vs.indoors as domestic fuel. The total emissions of various pollutants from the burning of crop residue were estimated for 2000-2014 using the emission factor method. The results indicate that the total amount of crop residue and average burned mass were 8690.9 Tg and4914.6 Tg, respectively. The total amount of emitted pollutants including CO2, CO, NOx,VOCs, PM(2.5), OC(organic carbon), EC(element carbon) and TC(total carbon) were 4212.4–8440.9 Tg, 192.8–579.4 Tg, 4.8–19.4 Tg, 18.6–61.3 Tg, 18.8–49.7 Tg, 6.7–31.3 Tg, 2.3–4.7 Tg, and8.5–34.1 Tg, respectively. The emissions of pollutants released from crop residue burning were found to be spatially variable, with the burning of crop residue mainly occurring in Northeast, North and South China. In addition, pollutant emissions per unit area(10 km ×10 km) were mostly concentrated in the central and eastern regions of China. Emissions of CO2, NOx, VOCs, OC and TC were mainly from rice straw burning, while burning of corn and wheat residues contributed most to emissions of CO, PM(2.5) and EC. The increased ratio of PM(2.5) emissions from crop residue burning to the total emitted from industry during the study period is attributed to the implementation of strict emissions management policies in Chinese industry. This study also provides baseline data for assessment of the regional atmospheric environment.
基金The Strategic Priority Research Program of the Chinese Academy of Sciences,No.XDA19040401China Postdoctoral Science Foundation,No.2016M600121+1 种基金National Natural Science Foundation of China,No.41701173,No.41501137The State Key Laboratory of Resources and Environmental Information System
文摘High concentrations of PM_(2.5) are universally considered as a main cause for haze formation. Therefore, it is important to identify the spatial heterogeneity and influencing factors of PM_(2.5) concentrations for regional air quality control and management. In this study, PM_(2.5) data from 2000 to 2015 was determined from an inversion of NASA atmospheric remote sensing images. Using geo-statistics, geographic detectors, and geo-spatial analysis methods, the spatio-temporal evolution patterns and driving factors of PM_(2.5) concentration in China were evaluated. The main results are as follows.(1) In general, the average concentration of PM_(2.5) in China increased quickly and reached its peak value in 2006; subsequently, concentrations remained between 21.84 and 35.08 μg/m3.(2) PM_(2.5) is strikingly heterogeneous in China, with higher concentrations in the north and east than in the south and west. In particular, areas with relatively high PM_(2.5) concentrations are primarily in four regions, the Huang-Huai-Hai Plain, Lower Yangtze River Delta Plain, Sichuan Basin, and Taklimakan Desert. Among them, Beijing-Tianjin-Hebei Region has the highest concentration of PM_(2.5).(3) The center of gravity of PM_(2.5) has generally moved northeastward, which indicates an increasingly serious haze in eastern China. High-value PM_(2.5) concentrations have moved eastward, while low-value PM_(2.5) has moved westward.(4) Spatial autocorrelation analysis indicates a significantly positive spatial correlation. The "High-High" PM_(2.5) agglomeration areas are distributed in the Huang-Huai-Hai Plain, Fenhe-Weihe River Basin, Sichuan Basin, and Jianghan Plain regions. The "Low-Low" PM_(2.5) agglomeration areas include Inner Mongolia and Heilongjiang, north of the Great Wall, Qinghai-Tibet Plateau, and Taiwan, Hainan, and Fujian and other southeast coastal cities and islands.(5) Geographic detection analysis indicates that both natural and anthropogenic factors account for spatial variations in PM_(2.5) concentration. Geographical location, population density, automobile quantity, industrial discharge, and straw burning are the main driving forces of PM_(2.5) concentration in China.