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Response of CH_4 emission of paddy fields to land management practices at a microcosmic cultivation scale in China 被引量:10
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作者 SHAOJiang-an HUANGXue-xia +3 位作者 GAOMing WEIChao-fu XIEDe-ti CAIZu-cong 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2005年第4期691-698,共8页
The terrestrial ecosystem may be either a source or a sink of CH_4 in rice paddies, depending, to a great extent, on the change of ecosystem types and land use patterns. CH_4 emission fluxes from paddy fields under 4 ... The terrestrial ecosystem may be either a source or a sink of CH_4 in rice paddies, depending, to a great extent, on the change of ecosystem types and land use patterns. CH_4 emission fluxes from paddy fields under 4 cultivation patterns (conventional plain culture of rice(T1), no-tillage and ridge culture of rice(T2), no-tillage and ridge culture of rice and wheat (T3), and rice-wheat rotation(T4)) were measured with the closed chamber technique in 1996 and 1998 in Chongqing, China. The results showed that differences existed in CH_4 emission from paddy fields under these land management practices. In 1996 and 1998, CH_4 emission was 71 48% and 78 82%(T2), 65 93% and 57 18%(T3), and 61 53% and 34 22%(T4) of that in T1 during the rice growing season. During the non-rice growing season, CH_4 emission from rice fields was 76 23% in T2 and 38 69% in T1 The accumulated annual CH_4 emission in T2, T3 and T4 in 1996 decreased by 33 53%, 63 30% and 65 73%, respectively, as compared with that in T1 In 1998, the accumulated annual CH_4 emission in T1, T2, T3 and T4 was 116 96 g/m^2, 68 44 g/m^2, 19 70 g/m^2 and 11 80 g/m^2, respectively. Changes in soil physical and chemical properties, in thermal and moisture conditions in the soil and in rice plant growth induced by different land use patterns were the dominant causes for the difference in CH_4 emission observed. The relative contribution of various influencing factors to CH_4 emission from paddy fields differed significantly under different land use patterns. However, the general trend was that chlorophyll content in rice leaves, air temperature and temperature at the 5 cm soil layer play a major role in CH_4 emission from paddy fields and the effects of illumination, relative humidity and water layer depth in the paddy field and CH_4 concentration in the crop canopy were relatively non-significant. Such conservative land use patterns as no-tillage and ridge culture of rice with or without rotation with wheat are thought to be beneficial to reducing CH_4 emission from paddy fields and are, therefore, recommended as a significant solution to the problems of global(climatic) change. 展开更多
关键词 land use pattern microcosmic cultivation scale fluxes of CH_4 emission paddy field
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Seasonal Variations of CH_4 Emissions in the Yangtze River Delta Region of China Are Driven by Agricultural Activities 被引量:2
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作者 Wenjing HUANG Timothy JGRIFFIS +2 位作者 Cheng HU Wei XIAO Xuhui LEE 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2021年第9期1537-1551,共15页
Developed regions of the world represent a major atmospheric methane(CH_4) source,but these regional emissions remain poorly constrained.The Yangtze River Delta(YRD) region of China is densely populated(about 16% of C... Developed regions of the world represent a major atmospheric methane(CH_4) source,but these regional emissions remain poorly constrained.The Yangtze River Delta(YRD) region of China is densely populated(about 16% of China's total population) and consists of large anthropogenic and natural CH_4 sources.Here,atmospheric CH_4 concentrations measured at a 70-m tall tower in the YRD are combined with a scale factor Bayesian inverse(SFBI) modeling approach to constrain seasonal variations in CH_4 emissions.Results indicate that in 2018 agricultural soils(AGS,rice production) were the main driver of seasonal variability in atmospheric CH_4 concentration.There was an underestimation of emissions from AGS in the a priori inventories(EDGAR—Emissions Database for Global Atmospheric Research v432 or v50),especially during the growing seasons.Posteriori CH_4 emissions from AGS accounted for 39%(4.58 Tg,EDGAR v432) to 47%(5.21 Tg,EDGAR v50) of the total CH_4 emissions.The posteriori natural emissions(including wetlands and water bodies) were1.21 Tg and 1.06 Tg,accounting for 10.1%(EDGAR v432) and 9.5%(EDGAR v50) of total emissions in the YRD in2018.Results show that the dominant factor for seasonal variations in atmospheric concentration in the YRD was AGS,followed by natural sources.In summer,AGS contributed 42%(EDGAR v432) to 64%(EDGAR v50) of the CH_4 concentration enhancement while natural sources only contributed about 10%(EDGAR v50) to 15%(EDGAR v432).In addition,the newer version of the EDGAR product(EDGAR v50) provided more reasonable seasonal distribution of CH_4 emissions from rice cultivation than the old version(EDGAR v432). 展开更多
关键词 CH_4 emissions WRF-STILT seasonal variations Yangtze River Delta
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Responses of CH_4 Emissions to Nitrogen Addition and Spartina alterniflora Invasion in Minjiang River Estuary, Southeast of China 被引量:10
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作者 MOU Xiaojie LIU Xingtu +1 位作者 TONG Chuan SUN Zhigao 《Chinese Geographical Science》 SCIE CSCD 2014年第5期562-574,共13页
The nitrogen (N) input and Spartina alterniflora invasion in the tidal marsh of the southeast of China are increasingly serious. To evaluate CH4 emissions in the tidal marsh as affected by the N inputs and S. altern... The nitrogen (N) input and Spartina alterniflora invasion in the tidal marsh of the southeast of China are increasingly serious. To evaluate CH4 emissions in the tidal marsh as affected by the N inputs and S. alterniflora invasion, we measured CH4 emissions from plots with vegetated S. alterniflora and native Cyperus malaccensis, and fertilized with exogenous N at the rate of 0 (NO), 21 (N1) and 42 (N2) g N/(m2.yr), respectively, in the Shanyutan marsh in the Minjiang River estuary, the southeast of China. The average CH4 fluxes during the experiment in the C. malaccensis and S. alterniflora plots without N addition were 3.67 mg CHa/(m2.h) and 7.79 mg CH4/(m2-h), respectively, suggesting that the invasion of S. alterniflora into the Minjiang River estuary stimulated CH4 emission. Exogenous N had positive effects on CH4 fluxes both in native and in invaded tidal marsh. The mean CH4 fluxes of NI and N2 treat- ments increased by 31.05% and 123.50% in the C. malaccensis marsh, and 63.88% and 7.55% in the S. alterniflora marsh, respectively, compared to that of NO treatment. The CH4 fluxes in the two marshes were positively correlated with temperature and pH, and nega- tively correlated with electrical conductivity and redox potential (Eh) at different N addition treatments. While the relationships between CH4 fluxes and environmental variables (especially soil temperature, pH and Eh at different depths) tended to decrease with N additions. Significant temporal variability in CH4 fluxes were observed as the N was gradually added to the native and invaded marshes. In order to better assess the global climatic role of tidal marshes as affected by N addition, much more attention should be paid to the short-term temporal variability in CH4 emission. 展开更多
关键词 nitrogen addition CH4 emission tidal marsh Spartina alterniflora invasion temporal variability
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CH_4 emissions and reduction potential in wastewater treatment in China 被引量:5
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作者 MA Zhan-Yun FENG Peng +3 位作者 GAO Qing-Xian LU Yan-Na LIU Jun-Rong LI Wen-Tao 《Advances in Climate Change Research》 SCIE CSCD 2015年第3期216-224,共9页
The treatment of domestic and industrial wastewater is one of the major sources of CH_4 in the Chinese waste sector. On the basis of statistical data and country-specific emission factors, using IPCC methodology, the ... The treatment of domestic and industrial wastewater is one of the major sources of CH_4 in the Chinese waste sector. On the basis of statistical data and country-specific emission factors, using IPCC methodology, the characteristics of CH_4 emissions from wastewater treatment in China were analyzed. The driving factors of CH_4 emissions were studied, and the emission trend and reduction potential were predicted and analyzed according to the current situation. Results show that in 2010, CH_4 emissions from the treatment of domestic and industrial wastewater were0.6110 Mt and 1.6237 Mt, respectively. Eight major industries account for more than 92% of emissions, and CH_4 emissions gradually increased from 2005 to 2010. From the controlling management scenario, we predict that in 2020, CH_4 emissions from the treatment of domestic and industrial wastewater will be 1.0136 Mt and 2.3393 Mt, respectively, and the reduction potential will be 0.0763 Mt and 0.2599 Mt, respectively.From 2010 to 2020, CH_4 emissions from the treatment of domestic and industrial wastewater will increase by 66% and 44%, respectively. 展开更多
关键词 Domestic and industrial wastewater CH4 emissions Reduction scenario emission reduction potential
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Super Rice Cropping Will Enhance Rice Yield and Reduce CH_4 Emission:A Case Study in Nanjing,China 被引量:12
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作者 JIANG Yu WANG Li-li +3 位作者 YAN Xiao-jun TIAN Yun-lu DENG Ai-xing ZHANG Wei-jian 《Rice science》 SCIE 2013年第6期427-433,共7页
A pot experiment was performed to learn the differences in plant productivity and OH4 emission between two rice cultivars, super rice variety Ningjing 1 and traditional variety Zhendao 11, which were currently commerc... A pot experiment was performed to learn the differences in plant productivity and OH4 emission between two rice cultivars, super rice variety Ningjing 1 and traditional variety Zhendao 11, which were currently commercially appUed in Nanjing, China. Similar seasonal changes of CH4 emission fluxes and soil solution CH4 contents were found between the tested cultivars. Although there was no significant difference in plant biomass production between the cultivars, the grain yield of Ningjing 1 was significantly higher by 35.0% (P 〈 0.05) than that of Zhendao 11, whereas the total CH4 emission from Ningjing 1 was 35.2% lower (P 〈 0.05). The main difference in the amounts of CH4 emission between the cultivars occurred in the period from the tillering stage to the heading stage. The biomass-scaled and yield-scaled CH4 emissions were respectively 3.8 and 5.2 mg/g for Ningjing 1, significantly lower than those for Zhendao 11 (7.4 and 12.8 mg/g, respectively). According to the relationships between the plant growth characteristics and the CH4 emission, a stronger root system contributed mainly to the lower CH4 emission of Ningjing 1, as compared with Zhendao 11. Our results demonstrated that super rice has advantages not only in grain productivity but also in CH4 emission mitigation. Further expansion of super rice cropping will enhance rice yield and reduce greenhouse gas emission in China. 展开更多
关键词 global warming food security rice variety rice production CH4 emission East China super rice
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Comparison of Field Measurements of CH_4 Emission from Rice Cultivation in Nanjing, China and in Texas, USA 被引量:3
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作者 黄耀 蒋静艳 +4 位作者 宗良纲 Ronald L.Sass Frank M.Fisher 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2001年第6期1121-1130,共10页
Field measurements of methane emission from rice paddies were made in Nanjing, China and in Texas, USA, respectively. Soil temperature at approximately 10 cm depth of the flooded soils was automatically recorded. Abov... Field measurements of methane emission from rice paddies were made in Nanjing, China and in Texas, USA, respectively. Soil temperature at approximately 10 cm depth of the flooded soils was automatically recorded. Aboveground biomass of rice crop was measured approximately every 10 days in Nanjing and every other week in Texas. Seasonal variation of soil temperature in Nanjing was quite wide with a magnitude of 15.3°C and that in Texas was narrow with a magnitude of 2.9°C. Analysis of methane emission fluxes against soil temperature and rice biomass production demonstrated that the seasonal course of methane emission in Nanjing was mostly attributed to soil temperature changes, while that in Texas was mainly related to rice biomass production. We concluded that under the permanent flooding condition, the seasonal trend of methane emission would be determined by the soil temperature where there was a wide variation of soil temperature, and the seasonal trend would be mainly determined by rice biomass production if there are no additional organic matter inputs and the variation of soil temperature over the rice growing season is small. Key words CH4 emission - Rice paddies - Rice biomass production - Soil temperature This work was supported by grants from TECO/NASA, the United States, the Hundred Talents Program, Chinese Academy of Sciences and the National Key Basic Research Development Foundation (approved # G1999011805), China. 展开更多
关键词 CH4 emission Rice paddies Rice biomass production Soil temperature
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Effects of soil moisture and temperature on CH_4 oxidation and N_2O emission of forest soil 被引量:2
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作者 张秀君 徐慧 陈冠雄 《Journal of Forestry Research》 CAS CSCD 2000年第3期203-206,共4页
Soil samples were taken from depth of 0-12cm in the virgin broad- leaved/Korean pine mixed forest in Changbai Mountain in April, 2000. 20 μL·L-1 and 200 μL·L-1 CH4 and N2O concentration were supplied for a... Soil samples were taken from depth of 0-12cm in the virgin broad- leaved/Korean pine mixed forest in Changbai Mountain in April, 2000. 20 μL·L-1 and 200 μL·L-1 CH4 and N2O concentration were supplied for analysis. Laboratory study on CH4 oxidation and N2O emission in forest soil showed that fresh soil sample could oxidize atmospheric methane and product N2O. Air-dried soil sample could not oxidize atmospheric methane, but could produCt N2O. However, it could oxidize the supplied methane quickly when its concentration was higher than 20 μL·L-1. The oxidation rate of methane was increased with its initial concentration. An addition of water to dry soil caused large pulse of N2O emissions within 2 hours. There were curvilinear correlations between N2O emission and temperature (r2=0.706, p <0.05), and between N2O emission andtwater content (r2=0.2968. p <0.05). These suggested temperature and water content were important factors controlling N2O emission. The correlation between CH4 oxidization and temperature was also found while CH4 was supplied 200 μL·L-1 (r2 =0.3573, p<0.05). Temperature was an important f8Ctor controlling CH4 oxidation. However, when 20 μL·L-1 CH4 was supplied, there was no correlation among CH4 oxidization, N2O emission, temperature and water content. 展开更多
关键词 Air-dried soil Fresh forest soil CH_4 oxidation N_2O emission
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Effect of elevated CO_2 on CH_4 emission 被引量:3
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作者 WANG DaliState Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences , Beijing 100085, China 《Chinese Science Bulletin》 SCIE EI CAS 1999年第13期1153-1157,共5页
Global CH<sub>4</sub> emission may increase under CO<sub>2</sub> enrichment condition, which is projected for the future. CO<sub>2</sub> enrichment could affect CH<sub>4</s... Global CH<sub>4</sub> emission may increase under CO<sub>2</sub> enrichment condition, which is projected for the future. CO<sub>2</sub> enrichment could affect CH<sub>4</sub> emission in two ways: ( ⅰ ) Photosynthesis of plants that also include plants in rice paddies and natural wetlands will be stimulated under CO<sub>2</sub> enrichment condition. CH<sub>4</sub> emission rate may be increased due to the accumulation of more plant biomass, root exudes and soil organic matters. ( ⅱ ) Combined with other global warming forces, CO<sub>2</sub> enrichment may bring a change of atmospheric temperature and precipitation around the world. CH<sub>4</sub> emission will also be changed with the variation of the area and distribution of rice paddies and natural wetlands. 展开更多
关键词 GLOBAL CHANGE CO2 ENRICHMENT CH4 emission.
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CH_4 EMISSION FROM A CHINESE RICE PADDY FIELD 被引量:21
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作者 王明星 戴爱国 +4 位作者 沈壬兴 HelmutSchitz HeinzRennenberg WolfgangSeiler 吴海宝 《Acta meteorologica Sinica》 SCIE 1990年第3期265-275,共11页
CH_4 emission rates have been measured continuously for the early rice of 1988 and late rices of 1987 and 1988 during entire growing seasons in a rice paddy field in Hangzhou,Zhejiang Province,China,by using an automa... CH_4 emission rates have been measured continuously for the early rice of 1988 and late rices of 1987 and 1988 during entire growing seasons in a rice paddy field in Hangzhou,Zhejiang Province,China,by using an automatic sampling and analyzing system.During most parts of the seasons CH_4 emission rates showed strong diurnal variations.Bi-mode patterns with the highest value in the afternoon and a second peak at mid-night were generally found for the early rice,while the highest values were almost always found in the night for the late rice.Bi-mode patterns with a second peak in the afternoon were also found during the reproductive phase of the late rice plants.These diurnal variations may be explained by the diurnal variations of the soil temperature and the activity of rice plants.Strong seasonal variations with one peak in the tillering stage and two during the reproductive phase of rice plants were observed for all the three growing seasons.The seasonal variations may be explained by the activity of rice plants,availability of organic substrates in the soil,and the activity of soil bacteria related to soil temperatures,Fertilization did not show significant effects on the total seasonal CH_4 emissions but slightly changed the pattern of the seasonal variations of the CH_4 emission rates.Averaged over the measuring periods and 8 spots,CH_4 emission rates of 7.8 mg m^(-2) h^(-1) for the early rice and 28.6 mg m^(-2) h^(-1) for the late rice were obtained. Based on these measured data,the total global emission of CH_4 from rice paddies is estimated to be about 90 Tg/yr ranging from 70 to 110,accounting for 20% of the total source of CH_4. 展开更多
关键词 CH4 emission FROM A CHINESE RICE PADDY FIELD
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CH_4 emission and conversion from A^2O and SBR processes in full-scale wastewater treatment plants 被引量:12
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作者 Yan Liu Xiang Cheng +1 位作者 Xiaoxiu Lun Dezhi Sun 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2014年第1期224-230,共7页
Wastewater treatment systems are important anthropogenic sources of CH4 emission. A full-scale experiment was carried out to monitor the CH4 emission from anoxic/anaerobic/oxic process (A2O) and sequencing batch rea... Wastewater treatment systems are important anthropogenic sources of CH4 emission. A full-scale experiment was carried out to monitor the CH4 emission from anoxic/anaerobic/oxic process (A2O) and sequencing batch reactor (SBR) wastewater treatment plants (WWTPs) for one year from May 2011 to April 2012. The main emission unit of the A2O process was an oxic tank, accounting for 76.2% of CH4 emissions; the main emission unit of the SBR process was the feeding and aeration phase, accounting for 99.5% of CH4 emissions. CH4 can be produced in the anaerobic condition, such as in the primary settling tank and anaerobic tank of the A2O process. While CH4 can be consumed in anoxic denitrification or the aeration condition, such as in the anoxic tank and oxic tank of the A2O process and the feeding and aeration phase of the SBR process. The CH4 emission flux and the dissolved CH4 concentration rapidly decreased in the oxic tank of the A2O process. These metrics increased during the first half of the phase and then decreased during the latter half of the phase in the feeding and aeration phase of the SBR process. The CH4 oxidation rate ranged from 32.47% to 89.52% (mean: 67.96%) in the A2O process and from 12.65% to 88.31% (mean: 47.62%) in the SBR process. The mean CH4 emission factors were 0.182 g/ton of wastewater and 24.75 g CH4/(person.year) for the A2O process, and 0.457 g/ton of wastewater and 36.55 g CH4/(person.year) for the SBR process. 展开更多
关键词 CH4 emission production and consumption wastewater treatment plant A2O SBR
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Choice of precipitant and calcination temperature of precursor for synthesis of NiCo_2O_4 for control of CO–CH_4 emissions from CNG vehicles
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作者 Suverna Trivedi Ram Prasad 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2018年第3期62-71,共10页
Compressed natural gas(CNG)is most appropriate an alternative of conventional fuel for automobiles.However,emissions of carbon-monoxide and methane from such vehicles adversely affect human health and environment.Co... Compressed natural gas(CNG)is most appropriate an alternative of conventional fuel for automobiles.However,emissions of carbon-monoxide and methane from such vehicles adversely affect human health and environment.Consequently,to abate emissions from CNG vehicles,development of highly efficient and inexpensive catalysts is necessary.Thus,the present work attempts to scan the effects of precipitants(Na2CO3,KOH and urea)for nickel cobaltite(Ni Co2O4)catalysts prepared by co-precipitation from nitrate solutions and calcined in a lean CO-air mixture at 400℃.The catalysts were used for oxidation of a mixture of CO and CH4(1:1).The catalysts were characterized by X-ray diffractometer,Brunauer–Emmett–Teller surface-area,X-ray photoelectron spectroscopy;temperature programmedreductionandScanningelectronmicroscopycoupledwith Energy-Dispersive X-Ray Spectroscopy.The Na2CO3was adjudged as the best precipitant for production of catalyst,which completely oxidized CO-CH4mixture at the lowest temperature(T(100)=350℃).Whereas,for catalyst prepared using urea,T(100)=362℃.On the other hand the conversion of CO-CH4mixture over the catalyst synthesized by KOH limited to 97%even beyond 400℃.Further,the effect of higher calcination temperatures of 500 and600℃ was examined for the best catalyst.The total oxidation of the mixture was attained at higher temperatures of 375 and 410℃ over catalysts calcined at 500 and 600℃ respectively.Thus,the best precipitant established was Na2CO3and the optimum calcination temperature of 400℃ was found to synthesize the Ni Co2O4catalyst for the best performance in CO-CH4oxidation. 展开更多
关键词 CNG vehicular emissions CO-CH4 oxidation NiG0204 Precipitants CALCINATIONS
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Can soil remediation agents synergistically mitigate rice Cd content and CH_(4)emission from karst paddies?
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作者 Wangbiao Lu Guangneng Zeng +8 位作者 Weijun Luo Jiangju Song Maofei Ni Shuangqin Guo Qi Zhang Chengling Huang Cheng Yang Haijun Du Shijie Wang 《Acta Geochimica》 EI CAS CSCD 2024年第6期1123-1132,共10页
Rice(Oryza sativa L.)paddies are increasingly threatened by cadmium(Cd)pollution,and potentially serve as CH_(4)emitters to the atmosphere.Remediation agents widely mitigate Cd pollution in paddy soil,however,we know ... Rice(Oryza sativa L.)paddies are increasingly threatened by cadmium(Cd)pollution,and potentially serve as CH_(4)emitters to the atmosphere.Remediation agents widely mitigate Cd pollution in paddy soil,however,we know little about their regulations on CH_(4)emission.Here,via adding biochar(B),sulfhydryl-modified palygorskite(SMP),and selenium foliar fertilizer(SFF),we conducted a pot experiment to investigate soil and rice Cd contents together with in-situ CH_(4)f luxes.Compared to CK,the addition of SMP,SFF,and B-SMP reduced Cd in brown rice by 25%to 50%,25%,and 50%to 75%,respectively.Agents 7%B,7%B-0.01%SMP,and SFF reduced CH_(4)emissions by 8.46%,5.30%,and 4.11%,respectively.CH_(4)emission increased gradually along the growing season,with the cumulative CH_(4)fluxes ranging between 338.82 and 619.13 kg hm^(-2).Our results highlight that mixed 7%B-0.01%SMP and SFF showed collaborative eff ects on Cd remediation and CH_(4)emission.This study reveals the feasibility of reducing Cd pollution and CH_(4)emission in karst rice paddies,which hopes to supplement the knowledge of collaborative controls on soil remediation and carbon emission. 展开更多
关键词 Cd content CH_(4) FLUX Remediation agents Synergistical effect Rice paddy
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Optimized tillage methods increase mechanically transplanted rice yield and reduce the greenhouse gas emissions
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作者 Shuang Cheng Zhipeng Xing +3 位作者 Chao Tian Mengzhu Liu Yuan Feng Hongcheng Zhang 《Journal of Integrative Agriculture》 SCIE CAS CSCD 2024年第4期1150-1163,共14页
Biaxia lrotary tillage in dryland(DBRT)can complete biaxial rotary tillage with straw incorporation,secondary suppression,and ditching,and it has been previously studied in direct-seeded rice and wheat.However,the eff... Biaxia lrotary tillage in dryland(DBRT)can complete biaxial rotary tillage with straw incorporation,secondary suppression,and ditching,and it has been previously studied in direct-seeded rice and wheat.However,the effects of DBRT on the mechanically transplanted rice yield and greenhouse gas emissions remain unclear.To evaluate the effects of DBRT on improving the food security of mechanically transplanted rice and reducing the greenhouse gas emissions,we conducted an experiment for two years with wheat straw incorporation.Three tillage methods were set up:DBRT,uniaxial rotary tillage in dryland and paddy(DPURT),and uniaxial rotary tillage in paddy(PURT).The results showed that compared with DPURT and PURT,DBRT increased the yield of machine-transplanted rice by 7.5-11.0%and 13.3-26.7%,respectively,while the seasonal cumulative CH_(4) emissions were reduced by 13.9-21.2%and 30.2-37.0%,respectively,and the seasonal cumulative N_(2)O emissions were increased by 13.5-28.6%and 50.0-73.1%,respectively.Consequently,DBRT reduced the global warming potential by 10.7-15.5%and 23.7-28.6%,respectively,andtheyield-scaledglobalwarmingpotentialby18.2-21.8%and36.4-39.3%,respectively,compared to DPURT and PURT.These results were mainly related to the fact that DBRT significantly reduced soil bulk density and increased soil redox potential(Eh).Therefore,implementing DBRT in machine-transplanted rice fields is feasible,which cannot only increase the rice yield,but also reduce the greenhouse gas emissions. 展开更多
关键词 integrated tillage rice grain yield CH_(4) N_(2)O
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Co_(3)O_(4)as an efficient passive NO_(x) adsorber for emission control during cold-start of diesel engines
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作者 Jinhuang Cai Shijie Hao +3 位作者 Yun Zhang Xiaomin Wu Zhenguo Li Huawang Zhao 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2024年第2期1-7,共7页
The Co_(3)O_(4)nanoparticles,dominated by a catalytically active(110)lattice plane,were synthesized as a low-temperature NO_(x) adsorbent to control the cold start emissions from vehicles.These nanoparticles boast a s... The Co_(3)O_(4)nanoparticles,dominated by a catalytically active(110)lattice plane,were synthesized as a low-temperature NO_(x) adsorbent to control the cold start emissions from vehicles.These nanoparticles boast a substantial quantity of active chemisorbed oxygen and lattice oxygen,which exhibited a NO_(x) uptake capacity commensurate with Pd/SSZ-13 at 100℃.The primary NO_(x) release temperature falls within a temperature range of 200-350℃,making it perfectly suitable for diesel engines.The characterization results demonstrate that chemisorbed oxygen facilitate nitro/nitrites intermediates formation,contributing to the NO_(x) storage at 100℃,while the nitrites begin to decompose within the 150-200℃range.Fortunately,lattice oxygen likely becomes involved in the activation of nitrites into more stable nitrate within this particular temperature range.The concurrent processes of nitrites decomposition and its conversion to nitrates results in a minimal NO_(x) release between the temperatures of 150-200℃.The nitrate formed via lattice oxygen mainly induces the NO_(x) to be released as NO_(2) within a temperature range of 200-350℃,which is advantageous in enhancing the NO_(x) activity of downstream NH_(3)-SCR catalysts,by boosting the fast SCR reaction pathway.Thanks to its low cost,considerable NO_(x) absorption capacity,and optimal release temperature,Co_(3)O_(4)demonstrates potential as an effective material for passive NO_(x) adsorber applications. 展开更多
关键词 emission control COLD-START Low-temperature adsorption Co_(3)O_(4) Nitrate formation
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不同水分管理及耕作制度对广州地区稻田CH_4排放的影响 被引量:17
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作者 卢维盛 张建国 +1 位作者 廖宗文 蔡祖聪 《华南农业大学学报》 CAS CSCD 北大核心 1997年第3期57-61,共5页
1994年利用密闭箱法观测了广州地区早稻和晚稻CH4的排放,结果CH4平均排放通量早稻为0.22~3.81mg/m2·h,晚稻为0.36~17.63mg/m2·h。其中淹水稻田为3.81~17.63mg/m2&... 1994年利用密闭箱法观测了广州地区早稻和晚稻CH4的排放,结果CH4平均排放通量早稻为0.22~3.81mg/m2·h,晚稻为0.36~17.63mg/m2·h。其中淹水稻田为3.81~17.63mg/m2·h,常规灌溉为0.22~2.84mg/m2·h。表明淹水稻田CH4排放显著高于常规灌溉,晚稻高于早稻,水旱轮作能显著减少稻田CH4排放。常规灌溉CH4排放明显低于国内其他稻区,对其原因进行了初步分析。 展开更多
关键词 广州地区 稻田 水分管理 耕作制度 CH_4排放
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广州地区晚季稻田CH_4、N_2O排放研究初报 被引量:8
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作者 杨军 贺丽萍 +3 位作者 杨崇 陈玉芬 吕雪娟 伍时照 《华南农业大学学报》 CAS CSCD 北大核心 1997年第3期62-66,共5页
采用广州地区农民常用施肥类型(1化肥;2有机肥+化肥)和灌溉方式(间歇灌溉),研究晚季稻田CH4、N2O排放规律及排放量。试验初步表明,在一定的施肥量及气候条件下,灌溉水管理是决定CH4、N2O排放量的较主要因素... 采用广州地区农民常用施肥类型(1化肥;2有机肥+化肥)和灌溉方式(间歇灌溉),研究晚季稻田CH4、N2O排放规律及排放量。试验初步表明,在一定的施肥量及气候条件下,灌溉水管理是决定CH4、N2O排放量的较主要因素,而这一因素对CH4、N2O排放量的影响互为相反,即施肥后稻田处于灌溉淹水状态有利于CH4排放而不利于N2O排放;稻田处于干湿状态有利于N2O排放,但非常不利于CH4排放;研究初步结果:施纯化肥水稻田所排放的CH4、N2O总量对温室效应及地球臭氧层破坏的综合影响强度大于施有机肥加化肥水稻田。广州地区晚季稻田CH4排放通量为7.8mg/m2·h;N2O排放通量为226μg/m2·h。 展开更多
关键词 CH_4 N_2O 排放通量 施肥 水稻田
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华东稻田CH_4和N_2O排放 被引量:107
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作者 郑循华 王明星 +4 位作者 王跃思 沈壬兴 上官行健 金继生 李老土 《大气科学》 CSCD 北大核心 1997年第2期231-237,共7页
稻田CH4和N2O排放的季节变化规律完全不同,两者的排放通量随土壤水分条件变化而互为消长,但它们的日变化形式则比较一致。晴天时的CH4和N2O排放日变化规律明显,主要表现为下午单峰模态,有时CH4排放夜间出现一个次峰... 稻田CH4和N2O排放的季节变化规律完全不同,两者的排放通量随土壤水分条件变化而互为消长,但它们的日变化形式则比较一致。晴天时的CH4和N2O排放日变化规律明显,主要表现为下午单峰模态,有时CH4排放夜间出现一个次峰。CH4和N2O排放总量因肥料类型而不同,堆肥加尿素处理比NH4HCO3处理少排放N2O30%,多排放CH412%。 展开更多
关键词 华东 稻田 CH4 N2O 排放
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Modeling Methane Emission from Rice Paddy Soils:Ⅱ.Model Validation and Application 被引量:4
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作者 HUANGYAO R.L.SASS 《Pedosphere》 SCIE CAS CSCD 1999年第1期11-24,共14页
A simulation model developed by the authors (Huang et al., 1999) was validated against independent field measurements of methane emission from rice paddy soils in Texas of USA, Tuzu Of China and Vercelli of Italy.A si... A simulation model developed by the authors (Huang et al., 1999) was validated against independent field measurements of methane emission from rice paddy soils in Texas of USA, Tuzu Of China and Vercelli of Italy.A simplified version of the simulation model was further validated against methane emission measurements from various regions of the world, including italy, China, Indonesia, Philippines and the United States. Model validation suggested that the seasonal variation of methane emission was mainly regulated by rice growth and development and that methane emission could be predicted from rice net productivity, cultivar character, soil texture and temperature, and organic matter amendments. Model simulations in general agreed with the observations. The comparison between computed and measured methane emission resulted in correlation coefficients r2 values from 0.450 to 0.952, significant at 0.01-0.001 probability level.On the basis of available information on rice cultivated area, growth duration, grain yield, soil texture and temperature, methane emission from rice paddy soils of China's Mainland was estimated for 28 rice cultivated provinces/municipal cities by employing the validated model. The calculated daily methane emission rates, on a provincial scale, ranged from 0.12 to 0.71 g m-2 with an average of 0.26 g m-2. A total amount of 7.92 Tg CH4 per year, ranging from 5.89 to 11.17 Tg year-1, was estimated to be released from Chinese rice paddy soils. Of the total, 45% was emitted from the single-rice growing season, and 19% and 36% were from the early-rice and the late-rice growing seasons, respectively. Approximately 70% of the total was emitted in the region located at latitude between 25°and 32°N. The emissions from rice fields in Sichuan and Hunan provinces were calculated to be 2.34 Tg year-1, accounting for approximately 30% of the total. 展开更多
关键词 CH_4 emission China model estimates model validation rice paddy soils
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芦苇湿地温室气体甲烷(CH_4)排放研究 被引量:67
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作者 黄国宏 肖笃宁 +3 位作者 李玉祥 陈冠雄 杨玉成 赵长伟 《生态学报》 CAS CSCD 北大核心 2001年第9期1494-1497,共4页
用封闭式箱法对辽河三角洲芦苇湿地温室气体 CH4 的观测结果表明 ,其排放有明显的季节变化规律。淹水前 ,土壤为 CH4 汇。淹水期间 ,有大量的 CH4 排放。排水后 ,CH4 排放明显减少。在测定期内 ,CH4 排放通量为 -968~2 73 4 μg CH4 l/... 用封闭式箱法对辽河三角洲芦苇湿地温室气体 CH4 的观测结果表明 ,其排放有明显的季节变化规律。淹水前 ,土壤为 CH4 汇。淹水期间 ,有大量的 CH4 排放。排水后 ,CH4 排放明显减少。在测定期内 ,CH4 排放通量为 -968~2 73 4 μg CH4 l/ (m2· h)。另外 ,土壤中产生的 CH4 主要是通过芦苇植株的传输作用进入到大气中。试验结果还表明 ,有芦苇生长的湿地 CH4 排放是无芦苇生长的 1 5倍。同时 ,建议芦苇田应采用间歇灌溉的水分管理措施 ,这样既能促进植株生长 ,又能减少 CH4 展开更多
关键词 芦苇湿地 CH4排放 植株作用 温室气体
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农垦与放牧对内蒙古草原N_2O、CO_2排放和CH_4吸收的影响 被引量:49
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作者 王跃思 纪宝明 +2 位作者 黄耀 胡玉琼 王艳芬 《环境科学》 EI CAS CSCD 北大核心 2001年第6期7-13,共7页
利用优选静态箱 /气相色谱法 (GC) ,首次对我国内蒙古草原典型地区进行了人类活动对N2 O、CO2 和CH4交换通量影响的实验观测 .结果表明 ,农垦麦田N2 O平均排放通量比原始草原高出 3倍 ,并改变了草甸草原为CO2 汇的性质 ,使其季节排放净... 利用优选静态箱 /气相色谱法 (GC) ,首次对我国内蒙古草原典型地区进行了人类活动对N2 O、CO2 和CH4交换通量影响的实验观测 .结果表明 ,农垦麦田N2 O平均排放通量比原始草原高出 3倍 ,并改变了草甸草原为CO2 汇的性质 ,使其季节排放净通量以C计增加 1 4 .3mg·(m2 ·h) - 1.随放牧强度的增加CO2 排放通量呈线性增长 ,轻牧会引起草原对CH4 吸收的大幅增加 ,而随着放牧压力的增大 ,增加值迅速回落 .农垦麦田与草甸草原相比地 气间CH4 交换无显著变化 ,放牧强度对N2 O排放影响无显著规律 .土壤湿度和温度是影响草原排放N2 O和CO2 、吸收CH4 季节变化形式的关键因子 ,而人类活动仅影响排放强度 .排放和吸收量年际间差异很大 ,但主要受降水的影响 .N2 O和CO2 排放与CH4 展开更多
关键词 内蒙古草原 N2O CO2 CH4 农垦 放牧 草原 温室气体 大气环境 废气排放
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