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CFD simulation of ammonia-based CO_2 absorption in a spray column 被引量:1
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作者 赵杰 金保昇 徐寅 《Journal of Southeast University(English Edition)》 EI CAS 2015年第4期479-488,共10页
A comprehensive computational fluid dynamics(CFD) model is developed based on the gas-liquid two-phase hydrodynamics,gas-liquid mass-transfer theory and chemical reaction kinetics,and the ammonia-based CO2 absorptio... A comprehensive computational fluid dynamics(CFD) model is developed based on the gas-liquid two-phase hydrodynamics,gas-liquid mass-transfer theory and chemical reaction kinetics,and the ammonia-based CO2 absorption in a spray column is numerically studied.The Euler-Lagrange model is applied to describe the behavior of gas-liquid twophase flowand heat transfer.The dual-film theory and related correlations are adopted to model the gas-liquid mass transfer and chemical absorption process.The volatilization model of multi-component droplet is utilized to account for ammonia slippage.The effect of operation parameters on CO2 removal efficiency is numerically studied.The results showa good agreement with the previous experimental data,proving the validity of the proposed model.The profile studies of gasphase velocity and CO2 concentration suggest that the flowfield has a significant impact on the CO2 concentration field.Also,the local CO2 absorption rate is influenced by both local turbulence and the local liquid-gas ratio.Furthermore,the velocity field of gas phase is optimized by the method of adjusting the orifice plate,and the results showthat the CO2 removal efficiency is improved by approximately 4%. 展开更多
关键词 CO_2 absorption spray column computational fluid dynamics(CFD) aqueous ammonia
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Estimation of Pore Size Distribution by CO_2 Adsorption and Its Application in Physical Activation of Precursors 被引量:8
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作者 周理 姚金花 +1 位作者 王瑜 周亚平 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2000年第3期279-282,共4页
The CO2 adsorption data may show more than one section in the Dubinin-Radushkevich-Kaganer(DRK) plot if samples had been over-activated. Each section in the plot represents a range of pore size. The whole DRK plot pro... The CO2 adsorption data may show more than one section in the Dubinin-Radushkevich-Kaganer(DRK) plot if samples had been over-activated. Each section in the plot represents a range of pore size. The whole DRK plot provided information on the pore size distribution(PSD) of a sample, which may be used to monitor the effect of activation conditions in activation processes. 展开更多
关键词 pore size distribution activated carbon CO_2 adsorption ACTIVATION
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IN SITU SEPARATION OF ETHANOL DURING BATCH FERMENTATION WITH CO_2 STRIPPING AND ACTIVATED CARBON ADSORPTION
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作者 岑沛霖 张民权 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 1992年第1期19-27,共9页
In situ separation of ethanol during batch fermentation with CO_2 stripping and activated carbon adsorption was studied. The higher initial glucose concentration and fermentation rate were reached due to the eliminati... In situ separation of ethanol during batch fermentation with CO_2 stripping and activated carbon adsorption was studied. The higher initial glucose concentration and fermentation rate were reached due to the elimination of ethanol inhibition on the cell growth by means of CO_2 stripping. The stripped ethanol vapor was selectively adsorbed by an activated carbon column. The conde(?)sate desorbed from the adsorption column can be higher than 50% by weight. Ar unstructured model was used to simulate the experimental data satisfactorily. 展开更多
关键词 ethanol fermentation CO_2 stripping ADsorption MODEL
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An integrated technology for the absorption and utilization of CO_(2)in alkanolamine solution for the preparation of BaCO_(3)in a high-gravity environment
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作者 Kangrui Nie Ruize Shang +3 位作者 Fuming Miao Liuxiang Wang Youzhi Liu Weizhou Jiao 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2024年第8期117-125,共9页
In this study,an integrated technology is proposed for the absorption and utilization of CO_(2)in alkanolamine solution for the preparation of BaCO_(3)in a high-gravity environment.The effects of absorbent type,high-g... In this study,an integrated technology is proposed for the absorption and utilization of CO_(2)in alkanolamine solution for the preparation of BaCO_(3)in a high-gravity environment.The effects of absorbent type,high-gravity factor,gas/liquid ratio,and initial BaCl2concentration on the absorption rate and amount of CO_(2)and the preparation of BaCO_(3)are investigated.The results reveal that the absorption rate and amount of CO_(2)follow the order of ethyl alkanolamine(MEA)>diethanol amine(DEA)>N-methyldiethanolamine(MDEA),and thus MEA is the most effective absorbent for CO_(2)absorption.The absorption rate and amount of CO_(2)under high gravity are higher than that under normal gravity.Notably,the absorption rate at 75 min under high gravity is approximately 2 times that under normal gravity.This is because the centrifugal force resulting from the high-speed rotation of the packing can greatly increase gas-liquid mass transfer and micromixing.The particle size of BaCO_(3)prepared in the rotating packed bed is in the range of 57.2—89 nm,which is much smaller than that prepared in the bubbling reactor(>100.3 nm),and it also has higher purity(99.6%)and larger specific surface area(14.119 m^(2)·g^(-1)).It is concluded that the high-gravity technology has the potential to increase the absorption and utilization of CO_(2)in alkanolamine solution for the preparation of BaCO_(3).This study provides new insights into carbon emissions reduction and carbon utilization. 展开更多
关键词 High-gravity technology Wet absorption CO_(2)capture Enhanced mass transfer CO_(2)utilization Barium carbonate
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Adsorption behavior of CO_(2)/H_(2)S mixtures in calcite slit nanopores for CO_(2) storage:An insight from molecular perspective
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作者 Cheng Qian Zhen-Hua Rui +4 位作者 Yue-Liang Liu Kai Du Chen Liu Yang Zhao Xiao-Min Ma 《Petroleum Science》 SCIE EI CAS CSCD 2024年第4期2444-2456,共13页
It is acknowledged that injecting CO_(2) into oil reservoirs and saline aquifers for storage is a practical and affordable method for CO_(2) sequestration.Most CO_(2) produced from industrial exhaust contains impurity... It is acknowledged that injecting CO_(2) into oil reservoirs and saline aquifers for storage is a practical and affordable method for CO_(2) sequestration.Most CO_(2) produced from industrial exhaust contains impurity gases such as H_(2)S that might impact CO_(2) sequestration due to competitive adsorption.This study makes a commendable effort to explore the adsorption behavior of CO_(2)/H_(2)S mixtures in calcite slit nanopores.Grand Canonical Monte Carlo(GCMC)simulation is employed to reveal the adsorption of CO_(2),H_(2)S as well as their binary mixtures in calcite nanopores.Results show that the increase in pressure and temperature can promote and inhibit the adsorption capacity of CO_(2) and H_(2)S in calcite nanopores,respectively.CO_(2)exhibits stronger adsorption on calcite surface than H_(2)S.Electrostatic energy plays the dominating role in the adsorption behavior.Electrostatic energy accounts for 97.11%of the CO_(2)-calcite interaction energy and 56.33%of the H_(2)S-calcite interaction energy at 10 MPa and 323.15 K.The presence of H_(2)S inhibits the CO_(2) adsorption in calcite nanopores due to competitive adsorption,and a higher mole fraction of H_(2)S leads to less CO_(2) adsorption.The quantity of CO_(2) adsorbed is lessened by approximately 33%when the mole fraction of H_(2)S reaches 0.25.CO_(2) molecules preferentially occupy the regions near the po re wall and H_(2)S molecules tend to reside at the center of nanopore even when the molar ratio of CO_(2) is low,indicating that CO_(2) has an adsorption priority on the calcite surface over H_(2)S.In addition,moisture can weaken the adsorption of both CO_(2) and H_(2)S,while CO_(2) is more affected.More interestingly,we find that pure CO_(2) is more suitable to be sequestrated in the shallower formations,i.e.,500-1500 m,whereas CO_(2)with H_(2)S impurity should be settled in the deeper reservoirs. 展开更多
关键词 Adsorption behavior CO_(2)/H_(2)S binary mixtures Molecular perspective Calcite slit nanopores CO_(2)sequestration
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Visual experimental study of nanofluids application to promote CO_(2) absorption in a bubble column
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作者 Shangyuan Cheng Guisheng Qi +1 位作者 Yuliang Li Yixuan Yang 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2024年第3期228-237,共10页
The addition of dispersed-phase nanoparticles in the liquid phase can enhance the gas-liquid transfer process as the suspended nanoparticles affect the transfer process inside the fluid through microdisturbance or mic... The addition of dispersed-phase nanoparticles in the liquid phase can enhance the gas-liquid transfer process as the suspended nanoparticles affect the transfer process inside the fluid through microdisturbance or micro-convection effects.In this article,a high-speed digital camera was used to visualize the bubble behavior of CO_(2) in pure water and nanofluids to examine the effects of CO_(2) gas flow rate,nanoparticle solid content and type on the bubble behavior in the fluids.The CO_(2) absorption performance in three water-based nanofluids were compared in a bubbler.And the mass transfer characteristics during CO_(2) bubble absorption and the reasons for the enhanced gas-liquid mass transfer effect of nanoparticles were analyzed.The results showed that the presence of nanoparticles affected the formation process of bubbles in the fluid,shortened the bubble detachment time,reduced the detachment diameter,effectively increased the gas-liquid contact area,and improved the bubbles detachment frequency.The system with MCM-41 corresponded to a higher overall mass transfer coefficient.Uncalined MCM-41 contained surfactant that enhanced foaming behavior in water.This prevented the transfer of CO_(2) to some extent,and the CO_(2) absorption by uncalined MCM-41/H_(2)O was 5.34%higher than that by pure water.Compared with SiO_(2) nanoparticles with the same particle size and the same composition,MCM-41 had a higher adsorption capacity and better hydrophilicity due to its larger specific surface area and rich porous structure,which was more favorable to accelerate the collision between nanoparticles and CO_(2) bubbles to cause micro-convection.Under the condition of 0.1%(mass)solid content,the enhancement of CO_(2) absorption process by MCM-41 nanoparticles was more significant and improved by 16.9%compared with pure water. 展开更多
关键词 Nanofluids CO_(2) absorption Mass transfer MCM-41 Bubble column
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Insights into carbon dioxide sequestration into coal seams through coupled gas flow-adsorption-deformation modelling
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作者 Hywel Thomas Min Chen 《Journal of Rock Mechanics and Geotechnical Engineering》 SCIE CSCD 2024年第1期26-40,共15页
Injecting carbon dioxide(CO_(2))into coal seams may unlock substantial carbon sequestration potential.Since the coal acts like a carbon filter,it can preferentially absorb significant amounts of CO_(2).To explore this... Injecting carbon dioxide(CO_(2))into coal seams may unlock substantial carbon sequestration potential.Since the coal acts like a carbon filter,it can preferentially absorb significant amounts of CO_(2).To explore this further,desorption of the adsorbed gas due to pressure drop is investigated in this paper,to achieve an improved understanding of the long-term fate of injected CO_(2) during post-injection period.This paper presents a dual porosity model coupling gas flow,adsorption and geomechanics for studying coupled processes and effectiveness of CO_(2) sequestration in coals.A new adsorption?desorption model derived based on thermodynamics is incorporated,particularly,the desorption hysteresis is considered.The reliability of the proposed adsorption-desorption isotherm is examined via validation tests.It is indicated that occurrence of desorption hysteresis is attributed to the adsorption-induced pore deformation.After injection ceases,the injected gas continues to propagate further from the injection well,while the pressure in the vicinity of the injection well experiences a significant drop.Although the adsorbed gas near the well also decreases,this decrease is less compared to that in pressure because of desorption hysteresis.The unceasing spread of CO_(2) and drops of pressure and adsorbed gas depend on the degree of desorption hysteresis and heterogeneity of coals,which should be considered when designing CO_(2) sequestration into coal seams. 展开更多
关键词 CO_(2)geological storage Coal seam ADsorption Desorption hysteresis
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The Al_(2)O_(3)and Mn/Al_(2)O_(3)sorbents highly utilized in destructive sorption of NF_(3)
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作者 Yanfei Pan Hejian Li +1 位作者 Li Zheng Xiufeng Xu 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2024年第1期54-62,共9页
NF_(3)is commonly used as an etching and cleaning gas in semiconductor industry,however it is a strongly greenhouse gas.Therefore,the destruction of disposal NF_(3)is an urgent task to migrate the greenhouse effect.Am... NF_(3)is commonly used as an etching and cleaning gas in semiconductor industry,however it is a strongly greenhouse gas.Therefore,the destruction of disposal NF_(3)is an urgent task to migrate the greenhouse effect.Among the technologies for NF_(3)abatement,the destructive sorption of NF_(3)over metal oxides sorbents is an effective way.Thus,the search for a highly reactive and utilized sorbent for NF_(3)destruction is in great demand.In this work,AlOOH supported on carbon-sphere(AlOOH/CS)as precursors were synthesized hydrothermally and heat-treated to prepare the Al_(2)O_(3)sorbents.The influence of AlOOH/CS hydrothermal temperatures on the reactivity of derived Al_(2)O_(3)sorbents for NF_(3)destruction was investigated,and it is shown that the Al2O3 from AlOOH/CS hydro-thermalized at 120℃is superior to others.Subsequently,the optimized Al_(2)O_(3)was covered by Mn(OH)x to prepare Mn/Al_(2)O_(3)sorbents via changing hydrothermal temperatures and Mn loadings.The results show that the Mn/Al_(2)O_(3)sorbents are more utilized than bare Al_(2)O_(3)in NF_(3)destructive sorption due to the promotional effect of Mn_(2)O_(3)as surface layer on the fluorination of Al_(2)O_(3)as substrate,especially the optimal 5%Mn/Al2O3(160℃)exhibits a utilization percentage as high as 90.4%,and remarkably exceeds all the sorbents reported so far.These findings are beneficial to develop more efficient sorbents for the destruction of NF_(3). 展开更多
关键词 Greenhouse gas NF_(3)destructive sorption Sorbents Al_(2)O_(3) Mn/Al_(2)O_(3) REACTIVITY
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PRP点注联合CO_2点阵激光治疗烧伤后增生瘢痕的效果观察
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作者 邓婉斯 李宁静 翁学君 《中文科技期刊数据库(引文版)医药卫生》 2024年第10期0025-0028,共4页
观察自体富小板血浆(PRP)点注技术与CO_2点阵激光技术联合治疗烧伤后增生瘢痕的临床疗效和安全性。方法 将在本院烧伤整形科就诊的烧伤后并发瘢痕增生患者列为本次研究对象,依据访谈和研究知情同意书签署结果将知情同意参与本次研究的3... 观察自体富小板血浆(PRP)点注技术与CO_2点阵激光技术联合治疗烧伤后增生瘢痕的临床疗效和安全性。方法 将在本院烧伤整形科就诊的烧伤后并发瘢痕增生患者列为本次研究对象,依据访谈和研究知情同意书签署结果将知情同意参与本次研究的30例患者纳为观察组,并选择未参与本研究,接受常规治疗的30例患者作为对照组。对照组按照瘢痕增生常规给予CO_2点阵激光治疗;观察组采用自体PRP微针点注技术联合CO_2点阵激光治疗。每2个月治疗一次,连续治疗3次为一疗程,观察并记录治疗前后两组的皮损治疗效果、温哥华瘢痕量表(VSS)评分以及治疗过程中的不良反应发生率。结果 观察组统计共90.00%的治疗有效率高于对照组统计66.67%的治疗有效率,组间统计学差异明显(P<0.05);两组到诊时的首次VSS测试结果,平均得分相近(P>0.05),一疗程后,两组的VSS评分均有明显下降,观察组的下降幅度大于对照组(P<0.01);治疗过程中,观察组的不良反应发生率明显低于对照组(P<0.05)。结论 自体PRP点注技术联合CO_2点阵激光治疗烧伤后瘢痕增生,不仅疗效显著,且安全性高,还能有效改善VSS评分,值得临床推广用。 展开更多
关键词 PRP CO_2点阵激光 瘢痕增生 疗效 不良反应
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氨基功能化介孔氧化硅材料的合成及其CO_2吸附性能的研究进展 被引量:3
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作者 郝仕油 肖强 +2 位作者 钟依均 朱伟东 杨辉 《材料科学与工程学报》 CAS CSCD 北大核心 2011年第1期143-148,共6页
本文综述了近年来氨基功能化介孔氧化硅材料的合成及其对CO2吸附性能的研究进展,重点介绍了氨基功能化MCM-41、MCM-48、SBA-15和以阴离子表面活性剂为模板剂合成氨基功能化介孔氧化硅的研究情况。同时本文对嫁接法和直接合成法在介孔氧... 本文综述了近年来氨基功能化介孔氧化硅材料的合成及其对CO2吸附性能的研究进展,重点介绍了氨基功能化MCM-41、MCM-48、SBA-15和以阴离子表面活性剂为模板剂合成氨基功能化介孔氧化硅的研究情况。同时本文对嫁接法和直接合成法在介孔氧化硅表面功能化中的优缺点进行了讨论。在研究展望部分,提出了氨基功能化介孔氧化硅在CO2吸附方面的研究方向。 展开更多
关键词 介孔氧化硅 表面改性 CO2吸附 氨基功能化
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加气灌溉对番茄地土壤CO_2排放的调控效应 被引量:12
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作者 陈慧 侯会静 +2 位作者 蔡焕杰 朱艳 王超 《中国农业科学》 CAS CSCD 北大核心 2016年第17期3380-3390,共11页
【目的】CO_2是大气中最重要的温室气体,对全球变暖起到重要作用。加气灌溉通过改善土壤通气状态,提高作物产量、品质及水分利用效率等已被大量研究证实,然而加气灌溉引起的土壤环境效应研究较少,且通过静态箱法系统地研究加气灌溉对设... 【目的】CO_2是大气中最重要的温室气体,对全球变暖起到重要作用。加气灌溉通过改善土壤通气状态,提高作物产量、品质及水分利用效率等已被大量研究证实,然而加气灌溉引起的土壤环境效应研究较少,且通过静态箱法系统地研究加气灌溉对设施菜地土壤CO_2排放影响的研究尚未见报道。因此,分析加气灌溉对土壤CO_2排放的影响,对评估加气灌溉技术的农田生态效应具有重要作用。【方法】供试番茄品种为‘飞越’,通过温室小区试验利用文丘里计作为加气设备,通过地下滴灌系统实现水气结合的加气灌溉方式。采用静态箱-气相色谱法对温室番茄地土壤CO_2排放进行原位观测,研究加气灌溉对土壤CO_2排放的调控效应。试验按灌水量(充分灌溉、亏缺灌溉)和加气(加气、不加气)的双因素设计,设置4个处理,分别为:加气亏缺灌溉(AI1)、不加气亏缺灌溉(CK1)、加气充分灌溉(AI2)和不加气充分灌溉(CK2),每个处理3个重复。研究加气和充分灌溉较不加气和亏缺灌溉对温室番茄地土壤CO_2排放、土壤水分、土壤温度和土壤有机碳的影响。【结果】番茄整个生育期,不同加气灌溉模式下土壤CO_2排放通量随移植后天数增加呈波动性变化,总体呈现先增加后减小的趋势,峰值均出现在番茄开花坐果期。加气和充分灌溉处理较对应的不加气和亏缺灌溉处理增加了番茄整个生育期土壤CO_2平均排放通量和排放量,但差异不显著(P>0.05)。AI1、CK1、AI2和CK2处理土壤CO_2平均排放通量分别为229.31、193.66、259.10和224.76 mg·m^(-2)·h^(-1),且以AI2处理土壤CO_2排放量最大(6 383.43 kg·hm^(-2)),分别是AI1、CK1和CK2处理的1.12、1.32和1.13倍。此外,不同加气灌溉模式下土壤充水孔隙率(WFPS)在番茄整个生育期内大致呈下降的趋势;土壤温度(T)大致呈上升的趋势,且同一时刻处理间土壤温度差异较小;而土壤有机碳(SOC)含量呈波动性变化且番茄整个生育期SOC含量变化幅度较小。加气灌溉较对应的不加气灌溉降低了T和WFPS,增加了SOC含量,但差异均不显著(P>0.05);充分灌溉较对应的亏缺灌溉增加了WFPS和SOC,但不显著,对T的影响不一。此外,经相关性分析可知,土壤CO_2排放通量与土壤充水孔隙率呈负相关,与土壤温度和有机碳呈正相关,但相关性均不显著(P>0.05)。【结论】通过温室小区试验得出,加气灌溉增加了土壤CO_2排放,但不显著(P>0.05)。研究结果为评估加气灌溉技术的农田生态效应和设施菜地温室气体减排提供了一定的参考和科学依据。 展开更多
关键词 加气灌溉 CO_2 排放 土壤 番茄 有机碳
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大气CO_2浓度倍增对宁夏枸杞生长的影响 被引量:11
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作者 曹兵 宋培建 +2 位作者 康建宏 侯晶东 宋丽华 《林业科学》 EI CAS CSCD 北大核心 2011年第7期193-198,共6页
以大气CO_2浓度和温度升高为主要特征的全球气候变化对农业生态系统、森林生态系统产生显著的影响。自20世纪90年代以来,气候变化,特别是大气CO_2浓度升高对植物的生理影响及植物的响应已成为一个重要的生理生态学研究热点问题(张晶晶... 以大气CO_2浓度和温度升高为主要特征的全球气候变化对农业生态系统、森林生态系统产生显著的影响。自20世纪90年代以来,气候变化,特别是大气CO_2浓度升高对植物的生理影响及植物的响应已成为一个重要的生理生态学研究热点问题(张晶晶等,2006;邓可洪等,2006;贾夏等,2005; 展开更多
关键词 宁夏枸杞 CO_2浓度升高 生长 活性成分含量
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Effect of Allelochemicals of Chinese-fir root extracted by supercritical CO_2 extraction on Chinese fir 被引量:9
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作者 林思祖 曹光球 +1 位作者 杜玲 王爱萍 《Journal of Forestry Research》 SCIE CAS CSCD 2003年第2期122-126,共5页
Allelochemicals of Chinese-fir root was extracted by technology ofsupercritical CO_2 extraction under orthogonal experiment design, and it was used to analyzeallelopathic activity of Chinese-fir through bioassay of se... Allelochemicals of Chinese-fir root was extracted by technology ofsupercritical CO_2 extraction under orthogonal experiment design, and it was used to analyzeallelopathic activity of Chinese-fir through bioassay of seed germination. The results showed thatas to the available rate of allelochemicals, the pressure and temperature of extraction were themost important factors. The allelochemicals of Chinese-fir root extracted by pure CO_2 and ethanolmixed with CO_2 have different allelopathic activities to seed germination, and the allelochemicalsextracted by ethanol mixed with CO_2 had stronger inhibitory effects on seed germination than thatextracted by pure CO_2. 展开更多
关键词 chinese fir autointoxication supercritical CO_2 extraction BIOASSAY SEEDGERMINATION
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火力发电企业CO_2排放量和减排分析 被引量:22
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作者 于海琴 李进 +3 位作者 安洪光 魏庆朝 田秀君 陈蕊 《北京交通大学学报》 CAS CSCD 北大核心 2010年第3期101-105,共5页
分析了电力企业CO2排放量的计算模式,提出IPCC排放因子计算模式、实测方法、物料衡算方法和宏观模型方法,并就影响排放因子的因素进行校核,提出电力生产低碳发展静脉循环经济模式下的捕获和资源化应用CCU减排思路.
关键词 火力发电 CO_2排放量 计算模式 排放因子 静脉低碳模式
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凋落茶叶对华中地区酸化茶园土壤N_2O与CO_2排放的影响 被引量:10
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作者 田亚男 何志龙 +2 位作者 吕昭琪 夏文建 林杉 《农业环境科学学报》 CAS CSCD 北大核心 2016年第8期1625-1632,共8页
采用室内培养试验方法,研究了凋落茶叶添加(0、5、10 g·kg-1和20 g·kg^(-1))对酸化茶园土壤N_2O和CO_2排放特征的影响。结果表明:4种添加水平下,N_2O和CO_2排放通量分别为0.24~3.92μg·kg^(-1)·h^(-1)和0.33~1.84 m... 采用室内培养试验方法,研究了凋落茶叶添加(0、5、10 g·kg-1和20 g·kg^(-1))对酸化茶园土壤N_2O和CO_2排放特征的影响。结果表明:4种添加水平下,N_2O和CO_2排放通量分别为0.24~3.92μg·kg^(-1)·h^(-1)和0.33~1.84 mg·kg^(-1)·h^(-1);凋落茶叶的添加显著促进了酸化茶园土壤N_2O和CO_2排放(P<0.05),且两种气体的排放通量随着凋落茶叶添加量的增加而增加;凋落茶叶显著提高了酸化土壤pH值(P<0.05),且添加量越多,pH值变幅越大,其一定程度上改善了茶园土壤酸化现象。茶园土壤铵态氮与N_2O排放通量呈极显著相关,而硝态氮与N_2O排放通量未呈显著相关性。土壤可溶性有机碳含量与N_2O和CO_2排放通量均呈极显著相关关系。茶园土壤N_2O排放通量和CO_2排放通量呈极显著正相关。研究结果有助于阐明凋落茶叶对茶园土壤温室气体排放的作用规律,且对了解茶园生态系统碳氮循环有一定的理论意义。 展开更多
关键词 凋落茶叶 酸化茶园 N_2O排放 CO_2排放 PH值
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低压电场驱动下膜分离CO_2的研究 被引量:7
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作者 陈一民 谢凯 +2 位作者 盘毅 许静 雍成纲 《国防科技大学学报》 EI CAS CSCD 2000年第4期38-40,56,共4页
以离子交换膜为基础 ,进行预处理和化学改性。研究了不同预处理条件、化学改性方法及低压电场的电压对离子交换膜的CO2 分离效率的影响。结果表明 ,改进处理条件、施加低压电场及在膜中加入亲水物质可明显地增加离子交换膜的二氧化碳通量。
关键词 CO_2 通量 离子交换膜
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CO_2浓度升高和施氮对冬小麦花前贮存碳氮转运的影响 被引量:19
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作者 许育彬 沈玉芳 李世清 《作物学报》 CAS CSCD 北大核心 2011年第8期1465-1474,共10页
为探讨大气CO2浓度升高对冬小麦花前贮存碳氮转运的影响及氮素营养的调节作用,以小偃22和小偃6号为材料,于2007-2009连续2个生长季,利用开顶式气室进行盆栽试验,对背景CO2浓度(375μLL-1)和高CO2浓度(2007-2008年度680μLL-1,2008-2009... 为探讨大气CO2浓度升高对冬小麦花前贮存碳氮转运的影响及氮素营养的调节作用,以小偃22和小偃6号为材料,于2007-2009连续2个生长季,利用开顶式气室进行盆栽试验,对背景CO2浓度(375μLL-1)和高CO2浓度(2007-2008年度680μLL-1,2008-2009年度750μLL-1)条件下不同施氮处理的干物质和氮素在籽粒、花前地上部中的累积以及花后营养器官的转运进行了评价。2007—2008年度设4个施氮水平,分别是0、0.1、0.2和0.3gkg-1土;2008—2009年度设3个施氮水平,分别是0、0.15和0.30gkg-1土。结果表明,施氮和CO2浓度升高促进了干物质和氮素在籽粒和花前营养器官的积累,增加了花前营养器官和地上部贮存干物质和氮素向籽粒的转运量,适量施氮提高了CO2浓度升高对花前营养器官干物质和氮素累积以及花后向籽粒转运的正向效应。与背景CO2浓度相比,高CO2浓度提高了花前营养器官和地上部干物质对籽粒产量的贡献率和转运率,但CO2浓度升高对花前氮素的贡献率和转运率的影响因年份和品种而异。CO2浓度升高后,2007-2008年度各营养器官和地上部,以及2008-2009年度茎鞘和穗的氮素贡献率和转运率均增加,但2008-2009年度2个品种叶片和地上部氮素贡献率在施氮时均显著降低,小偃22叶片和地上部氮素转运率在各施氮水平下以及小偃6号地上部氮素转运率在0.13gkg-1土施氮水平下均明显增加。适量施氮也在大多数情况下增强了CO2浓度升高对营养器官干物质和氮素的贡献率和转运率的正向效应。说明CO2浓度升高后小麦产量和氮素积累增加与其促进花前干物质和氮素积累及花后向籽粒的转运密切相关。 展开更多
关键词 冬小麦 CO_2浓度 施氮 产量 物质积累和转运
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北京山区辽东栎林土壤释放CO_2的模拟实验研究 被引量:57
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作者 蒋高明 黄银晓 《生态学报》 CAS CSCD 北大核心 1997年第5期477-482,共6页
模拟北京山区辽东栎林群落,对该类型土壤释放CO2过程进行了连续3a的实验研究,结果表明:辽东栎林土壤呼吸强度平均为5.92±1.32μmolCO2m-2s-1,在不同月份中,以8月份最高,10月最低,依次为8月>... 模拟北京山区辽东栎林群落,对该类型土壤释放CO2过程进行了连续3a的实验研究,结果表明:辽东栎林土壤呼吸强度平均为5.92±1.32μmolCO2m-2s-1,在不同月份中,以8月份最高,10月最低,依次为8月>7月>6月>9月>10月(P<0.05);13:00为土壤日呼吸的最高峰。温度为影响土壤呼吸的主要因子,二者存在极显著相关关系(r=0.5668,p<0.001,n=94)。据3a观测的土壤呼吸日平均值计算得出,模拟辽东栎林土壤释放CO2的通量估计范围为171.5~275.1kgCO2hm-2d-1,平均为223.3kgCO2hm-2d-1。 展开更多
关键词 辽东栎林 土壤呼吸 CO_2 模拟实验
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Cl^-含量对J55钢CO_2腐蚀行为的影响 被引量:26
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作者 张雷 国大鹏 路民旭 《中国腐蚀与防护学报》 CAS CSCD 北大核心 2009年第1期64-68,共5页
利用高温高压模拟实验、微观形貌观察和电化学测试研究了介质中Cl^-含量对J55钢CO_2腐蚀行为的影响。结果表明,在研究范围内(Cl^-含量为0~200 g/L),随Cl^-含量的增加,J55钢均匀腐蚀速率减小,腐蚀产物膜变得更加致密,对基体保护能力增强... 利用高温高压模拟实验、微观形貌观察和电化学测试研究了介质中Cl^-含量对J55钢CO_2腐蚀行为的影响。结果表明,在研究范围内(Cl^-含量为0~200 g/L),随Cl^-含量的增加,J55钢均匀腐蚀速率减小,腐蚀产物膜变得更加致密,对基体保护能力增强,且无明显局部腐蚀。Cl^-含量的变化没有改变电极反应活化控制步骤,但随含量增加,溶液的pH值降低,同时更多Cl^-占据阴极活性点,阻滞了阴极反应,提高了腐蚀电位。Cl^-含量较低时电化学阻抗谱呈现三个时间常数,随Cl^-含量增加,中低频区感抗弧逐渐消失,金属表面被完整的腐蚀产物膜覆盖。 展开更多
关键词 Cl^- CO_2腐蚀 J55钢 极化曲线 电化学阻抗
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O_2/CO_2煤粉燃烧时细灰颗粒中痕量元素分布特性的实验研究 被引量:7
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作者 李意 盛昌栋 +2 位作者 刘小伟 姚洪 徐明厚 《工程热物理学报》 EI CAS CSCD 北大核心 2008年第7期1236-1238,共3页
通过三个煤种在沉降炉中的燃烧实验,采用X-射线荧光光谱仪对实验收集的细灰颗粒物的元素组成进行定量测定,研究了O_2/CO_2煤粉燃烧对痕量元素行为的影响。结果表明,与O_2/N_2燃烧相比,O_2/CO_2燃烧对LPI颗粒物中Cu、Zn和Mn元素的分布形... 通过三个煤种在沉降炉中的燃烧实验,采用X-射线荧光光谱仪对实验收集的细灰颗粒物的元素组成进行定量测定,研究了O_2/CO_2煤粉燃烧对痕量元素行为的影响。结果表明,与O_2/N_2燃烧相比,O_2/CO_2燃烧对LPI颗粒物中Cu、Zn和Mn元素的分布形式没有影响,但显著增加了Cu、Zn元素在亚微米颗粒中的富集程度,Mn元素在细灰颗粒上没有出现富集,但O_2/CO_2燃烧时Mn在亚微米和超微米颗粒中的含量均显著减少。 展开更多
关键词 煤粉 O_2/CO_2燃烧 痕量元素 细灰颗粒
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