The Chinese Sun Hazemeter Network (CSHNET) provides the necessary ground-based observation to validate and assess the applicability of MODIS aerosol optical depth (AOD) products over different ecological and geographi...The Chinese Sun Hazemeter Network (CSHNET) provides the necessary ground-based observation to validate and assess the applicability of MODIS aerosol optical depth (AOD) products over different ecological and geographic regions in China for the first time. The validation results show that the comprehensive utilization ratio and applicability of MODIS products varied very much over different regions and seasons from August 2004 to July 2005. On the Tibetan Plateau, the comprehensive utili- zation ratio of MODIS data was low: MODIS products only accounted for 16% of the ground-based observation; on average, 31% to 45% of MODIS products fell within the retrieval errors issued by NASA. A similar result was found in northern desert areas with the ratio of MODIS to observation ranging from 15% to 55%, with 7% to 39% of MODIS products within errors. In the remote northeast corner of China, low ratios of MODIS to observation were also found ranging from 14% to 46%, with 49% to 69% of MODIS within errors. The forested sites exhibited moderate ratios of MODIS to observation ranging from 46% to 65%, with 30% to 59% of MODIS within errors. This was similar to numbers observed at sites along eastern seashore of China and inland urban sites with the ratio of MODIS to observation between 63% to 75%, with 25% to 67% of MODIS within errors for sites along eastern seashore of China and 43% to 78%, with 35% to 75% of MODIS within errors for inland urban sites. The ratio of MODIS to observation over agricultural areas ranged from 61% to 89%; 59%-88% of MODIS fell within the retrieval errors. At homogeneous and well vegetated areas, the comprehensive utilization ratio of MODIS products was over 80% and above 70% of MODIS products fell within the retrieval errors in growing season.展开更多
结合2006年最新的气溶胶排放源资料,以NCEP/NCAR再分析资料为气象场,驱动大气化学传输模式MATCH(Model of Atmospheric Transport and Chemistry),模拟了2006年中国地区硫酸盐、黑碳和沙尘气溶胶的质量浓度分布及其季节变化。模拟的气...结合2006年最新的气溶胶排放源资料,以NCEP/NCAR再分析资料为气象场,驱动大气化学传输模式MATCH(Model of Atmospheric Transport and Chemistry),模拟了2006年中国地区硫酸盐、黑碳和沙尘气溶胶的质量浓度分布及其季节变化。模拟的气溶胶光学厚度(AOD)结果与CSHNET观测网数据比较分析后发现,基于21个观测站的61组月平均数据与相应模拟结果的相关系数为0.63。模拟结果表明:2006年中国地区硫酸盐气溶胶高值区主要分布在中国的四川盆地、华北及长江流域等工业较发达地区,而且具有明显的季节变化,四川盆地及长江以南地区,硫酸盐气溶胶1月份浓度高于7月份,长江以北的大部分地区,7月份浓度高于1月份;黑碳气溶胶主要分布在黄河、长江中下游地区及华南等地区,1月份浓度高于7月份;沙尘气溶胶主要分布在内蒙古中部沙漠地区,4月份浓度最高,7月份次之,其他月份较少。展开更多
利用2006年NCEP/NCAR再分析资料驱动大气化学传输模式MATCH(Model of Atmos-pheric Transport and Chemistry),模拟了中国地区气溶胶光学厚度的分布及其季节变化特征,并与MODIS(MODerate resolution Imaging Spectro-radiometer)卫星产...利用2006年NCEP/NCAR再分析资料驱动大气化学传输模式MATCH(Model of Atmos-pheric Transport and Chemistry),模拟了中国地区气溶胶光学厚度的分布及其季节变化特征,并与MODIS(MODerate resolution Imaging Spectro-radiometer)卫星产品MOD08_M3和中国太阳分光观测网CSHNET(the Chinese Sun Hazemeter Network)的观测资料进行了对比和验证。在此基础上,研究得出,2006年中国的华北、华中和华南地区是气溶胶光学厚度的高值区,青藏高原和东北地区是低值区。在中国的华北、华中、华南和西南等大部分地区,硫酸盐气溶胶产生的光学厚度所占的比重较大,其次为有机碳气溶胶,黑碳气溶胶和海盐气溶胶所占比重较小。展开更多
The Model of Atmospheric Transport and Chemistry (MATCH) developed by the US National Center for Atmospheric Research (NCAR) was used to calculate the aerosol optical thickness (AOT) over China in 2006, with emi...The Model of Atmospheric Transport and Chemistry (MATCH) developed by the US National Center for Atmospheric Research (NCAR) was used to calculate the aerosol optical thickness (AOT) over China in 2006, with emission source data of the Intercontinental Chemical Transport Experiment Phase B (INTEX-B) and NCEP/NCAR reanalysis data as inputs. The simulation results of AOT were then validated with obser- vational data from the Moderate Resolution Imaging Spectroradiometer (MODIS), Chinese Sun Hazemeter Network (CSHNET), Aerosol Robotics Network (AERONET), and China Aerosol Remote Sensing Network (CARSNET) at more than 30 stations over China. The comparison results indicated that the high values of AOT in the areas such as the Sichuan basin and East and South China and the low values of AOT over the Tibetan Plateau and Northwest and Northeast China were reasonably simulated by the MATCH. This model tended to underestimate the AOT values in high-aerosol-loading areas but overestimate the AOT val- ues in less polluted areas because there are still large uncertainties in the expression of emission sources, the description of the optical properties of aerosols, the treatment of cloud and precipitation, and the selection of grid resolution. The modeling results were consistent with the CSHNET, CARSNET, AERONET, and MODIS data in most parts of China, and the correlation coefficient of the monthly mean AOT between the model and the observation was 0.79 with CSHNET data at 23 stations, 0.51 with MODIS data, and 0.88 with data at 3 CARSNET stations and 2 other stations. All of them passed the significance test with c 〈 0.0001. The results demonstrated that the MATCH has the ability to simulate the characteristics of the AOT distribution and its seasonal variation over China.展开更多
基金Supported by the National Natural Science Foundation of China (Grants Nos. 40675073, 40525016 and 40520120071)the National Basic Research Program (973) of China (Grant No. 2007CB407303)
文摘The Chinese Sun Hazemeter Network (CSHNET) provides the necessary ground-based observation to validate and assess the applicability of MODIS aerosol optical depth (AOD) products over different ecological and geographic regions in China for the first time. The validation results show that the comprehensive utilization ratio and applicability of MODIS products varied very much over different regions and seasons from August 2004 to July 2005. On the Tibetan Plateau, the comprehensive utili- zation ratio of MODIS data was low: MODIS products only accounted for 16% of the ground-based observation; on average, 31% to 45% of MODIS products fell within the retrieval errors issued by NASA. A similar result was found in northern desert areas with the ratio of MODIS to observation ranging from 15% to 55%, with 7% to 39% of MODIS products within errors. In the remote northeast corner of China, low ratios of MODIS to observation were also found ranging from 14% to 46%, with 49% to 69% of MODIS within errors. The forested sites exhibited moderate ratios of MODIS to observation ranging from 46% to 65%, with 30% to 59% of MODIS within errors. This was similar to numbers observed at sites along eastern seashore of China and inland urban sites with the ratio of MODIS to observation between 63% to 75%, with 25% to 67% of MODIS within errors for sites along eastern seashore of China and 43% to 78%, with 35% to 75% of MODIS within errors for inland urban sites. The ratio of MODIS to observation over agricultural areas ranged from 61% to 89%; 59%-88% of MODIS fell within the retrieval errors. At homogeneous and well vegetated areas, the comprehensive utilization ratio of MODIS products was over 80% and above 70% of MODIS products fell within the retrieval errors in growing season.
文摘结合2006年最新的气溶胶排放源资料,以NCEP/NCAR再分析资料为气象场,驱动大气化学传输模式MATCH(Model of Atmospheric Transport and Chemistry),模拟了2006年中国地区硫酸盐、黑碳和沙尘气溶胶的质量浓度分布及其季节变化。模拟的气溶胶光学厚度(AOD)结果与CSHNET观测网数据比较分析后发现,基于21个观测站的61组月平均数据与相应模拟结果的相关系数为0.63。模拟结果表明:2006年中国地区硫酸盐气溶胶高值区主要分布在中国的四川盆地、华北及长江流域等工业较发达地区,而且具有明显的季节变化,四川盆地及长江以南地区,硫酸盐气溶胶1月份浓度高于7月份,长江以北的大部分地区,7月份浓度高于1月份;黑碳气溶胶主要分布在黄河、长江中下游地区及华南等地区,1月份浓度高于7月份;沙尘气溶胶主要分布在内蒙古中部沙漠地区,4月份浓度最高,7月份次之,其他月份较少。
文摘利用2006年NCEP/NCAR再分析资料驱动大气化学传输模式MATCH(Model of Atmos-pheric Transport and Chemistry),模拟了中国地区气溶胶光学厚度的分布及其季节变化特征,并与MODIS(MODerate resolution Imaging Spectro-radiometer)卫星产品MOD08_M3和中国太阳分光观测网CSHNET(the Chinese Sun Hazemeter Network)的观测资料进行了对比和验证。在此基础上,研究得出,2006年中国的华北、华中和华南地区是气溶胶光学厚度的高值区,青藏高原和东北地区是低值区。在中国的华北、华中、华南和西南等大部分地区,硫酸盐气溶胶产生的光学厚度所占的比重较大,其次为有机碳气溶胶,黑碳气溶胶和海盐气溶胶所占比重较小。
基金Supported by the National Basic Research and Development (973) Program of China (2012CB955303 and 2011CB403405)National Science and Technology Support Program of China (2007BAC03A01)+1 种基金Chinese Academy of Meteorological Sciences Basic Research Project (2012Y003)Tianjin Municipal Meteorological Bureau Research Program (201210)
文摘The Model of Atmospheric Transport and Chemistry (MATCH) developed by the US National Center for Atmospheric Research (NCAR) was used to calculate the aerosol optical thickness (AOT) over China in 2006, with emission source data of the Intercontinental Chemical Transport Experiment Phase B (INTEX-B) and NCEP/NCAR reanalysis data as inputs. The simulation results of AOT were then validated with obser- vational data from the Moderate Resolution Imaging Spectroradiometer (MODIS), Chinese Sun Hazemeter Network (CSHNET), Aerosol Robotics Network (AERONET), and China Aerosol Remote Sensing Network (CARSNET) at more than 30 stations over China. The comparison results indicated that the high values of AOT in the areas such as the Sichuan basin and East and South China and the low values of AOT over the Tibetan Plateau and Northwest and Northeast China were reasonably simulated by the MATCH. This model tended to underestimate the AOT values in high-aerosol-loading areas but overestimate the AOT val- ues in less polluted areas because there are still large uncertainties in the expression of emission sources, the description of the optical properties of aerosols, the treatment of cloud and precipitation, and the selection of grid resolution. The modeling results were consistent with the CSHNET, CARSNET, AERONET, and MODIS data in most parts of China, and the correlation coefficient of the monthly mean AOT between the model and the observation was 0.79 with CSHNET data at 23 stations, 0.51 with MODIS data, and 0.88 with data at 3 CARSNET stations and 2 other stations. All of them passed the significance test with c 〈 0.0001. The results demonstrated that the MATCH has the ability to simulate the characteristics of the AOT distribution and its seasonal variation over China.