In this study, a regional air quality model system （RAQMS） was applied to investigate the spatial distributions and seasonal variations of atmospheric aerosols in 2006 over East Asia. Model validations demonstrated ...In this study, a regional air quality model system （RAQMS） was applied to investigate the spatial distributions and seasonal variations of atmospheric aerosols in 2006 over East Asia. Model validations demonstrated that RAQMS was able to reproduce the evolution processes of aerosol components reasonably well. Ground-level PM10 （particles with aerodynamic diameter ≤10 μm） concentrations were highest in spring and lowest in summer and were characterized by three maximum centers： the Taklimakan Desert （-1000 μg m^-3）, the Gobi Desert （-400 μg m^-3）, and the Huabei Plain （- 300 μg m^-3） of China. Vertically, high PM10 concentrations ranging from 100 μg m-3 to 250 μg m-3 occurred from the surface to an altitude of 6000 m at 30°-45°N in spring. In winter, the vertical gradient was so large that most aerosols were restricted in the boundary layer. Both sulfate and ammonium reached their highest concentrations in autumn, while nitrate reached its maximum level in winter. Black carbon and organic carbon aerosol concentrations reached maximums in winter. Soil dust were strongest in spring, whereas sea salt exerted the strongest influence on the coastal regions of eastern China in summer. The estimated burden of anthropogenic aerosols was largest in winter （1621 Gg） and smallest in summer （1040 Gg）. The sulfate burden accounted for -42% of the total anthropogenic aerosol burden. The dust burden was about twice the anthropogenic aerosol burden, implying the potentially important impacts of the natural aerosols on air quality and climate over East Asia.展开更多
A regional climate model （RegCM3）, coupled with an online dust module, is used to simulate the spatio-temporal distribution and emission flux of dust aerosol （smaller than 20 Wn in diameter） over East Asia in the ...A regional climate model （RegCM3）, coupled with an online dust module, is used to simulate the spatio-temporal distribution and emission flux of dust aerosol （smaller than 20 Wn in diameter） over East Asia in the period from 2000 to 2009. The model perfor- mance is firstly evaluated against available observations. Simulation results show that the model can capture the characteristics of spa- tio-temporal distribution of dust aerosol very well over East Asia. There always exist two extremes of dust aerosol optical depth （AOD） and column burden （CB）, one is in the Taklimakan Desert of Xinjiang Uygur Autonomous Region, China, and the other is in the Ba- dain Jaran Desert of Inner Mongolian Autonomous Region, China. The maximum value of CB appears in spring, secondary maxi- mum in winter and minimum in autumn. To the east of 110°E, dust is transported eastward from a maximum center at a height of 700 hPa over the East Asian continent. Dust emission sources are mainly located in the Taklimakan Desert, Badain Jaran Desert, North Qinghai-Tibetan Plateau and Southwest Mongolia. There is also an obvious seasonal variation of dust emission flux （EF）. Annual mean dust EF is 1,015.34 mg/（m2.d）, of which 62.4% and 2.3% are re-deposited onto the East Asian continent through a dry and wet deposition process, respectively, and the remaining 35.3% is injected into the atmosphere or subject to long-range transport.展开更多
The International Centre for Theoretical Physics(ICTP,Italy) Regional Climate Model version 3.0(RegCM3) is used to simulate spatio-temporal distribution characteristics and radiative forcing(RF) of organic carbon(OC) ...The International Centre for Theoretical Physics(ICTP,Italy) Regional Climate Model version 3.0(RegCM3) is used to simulate spatio-temporal distribution characteristics and radiative forcing(RF) of organic carbon(OC) aerosols in and around China.The preliminary simulation results show that OC aerosols are mostly concentrated in the area to the south of Yellow River and east of Tibetan Plateau.There is a decreasing trend of column burden of OC aerosols from south to north in China.The maximum value of column burden of OC aerosols is above 3 mg/m2 and located in the central and southern China,southeastern Tibet,and southwestern China's Yunnan,Guizhou,Sichuan provinces.The simulation on the seasonal variation shows that the maximum value of column burden of OC aerosols appears in winter and the secondary value is in spring and the minimum in summer.The RF of OC aerosols which varies seasonally is negative at the top of the atmosphere(TOA) and surface.The spatio-temporal characteristics of the RF of OC aerosols are basically consistent with that of IPCC,implying the high accuracy of the parameterization scheme for OC aerosols in RegCM3.展开更多
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences (Grant No. KZCX2-YW-Q11-03)the "Strategic Priority Research Program" of the Chinese Academy of Sciences (Grant No. XDA05100502)+2 种基金the National 973 Project of China (Grant No. 2010CB950804)the National Natural Science Foundation of China (GrantNo. 41075106)the Hundred Talents Program of the Chinese Academy of Sciences
文摘In this study, a regional air quality model system （RAQMS） was applied to investigate the spatial distributions and seasonal variations of atmospheric aerosols in 2006 over East Asia. Model validations demonstrated that RAQMS was able to reproduce the evolution processes of aerosol components reasonably well. Ground-level PM10 （particles with aerodynamic diameter ≤10 μm） concentrations were highest in spring and lowest in summer and were characterized by three maximum centers： the Taklimakan Desert （-1000 μg m^-3）, the Gobi Desert （-400 μg m^-3）, and the Huabei Plain （- 300 μg m^-3） of China. Vertically, high PM10 concentrations ranging from 100 μg m-3 to 250 μg m-3 occurred from the surface to an altitude of 6000 m at 30°-45°N in spring. In winter, the vertical gradient was so large that most aerosols were restricted in the boundary layer. Both sulfate and ammonium reached their highest concentrations in autumn, while nitrate reached its maximum level in winter. Black carbon and organic carbon aerosol concentrations reached maximums in winter. Soil dust were strongest in spring, whereas sea salt exerted the strongest influence on the coastal regions of eastern China in summer. The estimated burden of anthropogenic aerosols was largest in winter （1621 Gg） and smallest in summer （1040 Gg）. The sulfate burden accounted for -42% of the total anthropogenic aerosol burden. The dust burden was about twice the anthropogenic aerosol burden, implying the potentially important impacts of the natural aerosols on air quality and climate over East Asia.
基金supported by the National Basic Research Program of China(Grant No.2011CB403202)
文摘A regional climate model （RegCM3）, coupled with an online dust module, is used to simulate the spatio-temporal distribution and emission flux of dust aerosol （smaller than 20 Wn in diameter） over East Asia in the period from 2000 to 2009. The model perfor- mance is firstly evaluated against available observations. Simulation results show that the model can capture the characteristics of spa- tio-temporal distribution of dust aerosol very well over East Asia. There always exist two extremes of dust aerosol optical depth （AOD） and column burden （CB）, one is in the Taklimakan Desert of Xinjiang Uygur Autonomous Region, China, and the other is in the Ba- dain Jaran Desert of Inner Mongolian Autonomous Region, China. The maximum value of CB appears in spring, secondary maxi- mum in winter and minimum in autumn. To the east of 110°E, dust is transported eastward from a maximum center at a height of 700 hPa over the East Asian continent. Dust emission sources are mainly located in the Taklimakan Desert, Badain Jaran Desert, North Qinghai-Tibetan Plateau and Southwest Mongolia. There is also an obvious seasonal variation of dust emission flux （EF）. Annual mean dust EF is 1,015.34 mg/（m2.d）, of which 62.4% and 2.3% are re-deposited onto the East Asian continent through a dry and wet deposition process, respectively, and the remaining 35.3% is injected into the atmosphere or subject to long-range transport.
基金National Fundamental Research Program of China (2011CB403202)National Natural Science Foundation of China (40675040)
文摘The International Centre for Theoretical Physics(ICTP,Italy) Regional Climate Model version 3.0(RegCM3) is used to simulate spatio-temporal distribution characteristics and radiative forcing(RF) of organic carbon(OC) aerosols in and around China.The preliminary simulation results show that OC aerosols are mostly concentrated in the area to the south of Yellow River and east of Tibetan Plateau.There is a decreasing trend of column burden of OC aerosols from south to north in China.The maximum value of column burden of OC aerosols is above 3 mg/m2 and located in the central and southern China,southeastern Tibet,and southwestern China's Yunnan,Guizhou,Sichuan provinces.The simulation on the seasonal variation shows that the maximum value of column burden of OC aerosols appears in winter and the secondary value is in spring and the minimum in summer.The RF of OC aerosols which varies seasonally is negative at the top of the atmosphere(TOA) and surface.The spatio-temporal characteristics of the RF of OC aerosols are basically consistent with that of IPCC,implying the high accuracy of the parameterization scheme for OC aerosols in RegCM3.
