The quantum phase transition and the electronic transport in a triangular quantum dot system are investigated using the numerical renormalization group method.We concentrate on the interplay between the interdot capac...The quantum phase transition and the electronic transport in a triangular quantum dot system are investigated using the numerical renormalization group method.We concentrate on the interplay between the interdot capacitive coupling V and the interdot tunnel coupling t.For small t,three dots form a local spin doublet.As t increases,due to the competition between V and t,there exist two first-order transitions with phase sequence spin-doublet-magnetic frustration phase-orbital spin singlet.When t is absent,the evolutions of the total charge on the dots and the linear conductance are of the typical Coulomb-blockade features with increasing gate voltage.While for sufficient t,the antiferromagnetic spin correlation between dots is enhanced,and the conductance is strongly suppressed for the bonding state is almost doubly occupied.展开更多
Nanometer-scale Au quantum dots have been assembled on SiO2 by controlling the reaction of raw materials to form a citrate Au sol and an aminosilane/dithiol-treated patterned Si wafer. The detailed formation mechanism...Nanometer-scale Au quantum dots have been assembled on SiO2 by controlling the reaction of raw materials to form a citrate Au sol and an aminosilane/dithiol-treated patterned Si wafer. The detailed formation mechanism has been studied. Three gold colloidal particles (15 nm), aligned in a chain to form a one-dimensional current path, was bridged across an 80-nm gap between source and drain metal electrodes. The device exhibited a Coulomb blockade effect at 33 K.展开更多
To get a dielectric material with a high dielectric permittivity and suppressed dielectric loss,nano-Ag with a particle size of 20 nm and Ag@TiO_(2)core-shell particles with diameters of approximately 70-120 nm were e...To get a dielectric material with a high dielectric permittivity and suppressed dielectric loss,nano-Ag with a particle size of 20 nm and Ag@TiO_(2)core-shell particles with diameters of approximately 70-120 nm were embedded in polyvinylidene fluoride(PVDF)to fabricate nano-Ag/Ag@TiO_(2)/PVDF composites.After being modified by nano-Ag with 3 vol%optimal amount,the relative permittivity(ε_r)at 100 Hz of 50 vol%Ag@TiO_(2)/PVDF composites was 61,and the dielectric loss can be suppressed to 0.04,almost 96.4%lower than that of unmodified composites,and a higher frequency stability of bothε_r and loss has also been found.The underlying mechanism of the reduced loss was attributed to Maxwell-Wagner polarization and the Coulomb blockade effect caused by the introduction of a small amount of nano-Ag,which will block the movement of electrons between metal nanoparticles and composites.The space charge polarization and conductance loss are weakened at lower and higher Ag@TiO_(2)filling ratios,respectively,thus leading to a very low loss of the composites.展开更多
A method of fabricating Cu nanocrystals embedded in SiO2 dielectric film for nonvolatile memory applications by magnetron sputtering is introduced in this paper. The average size and distribution density of Cu nanocry...A method of fabricating Cu nanocrystals embedded in SiO2 dielectric film for nonvolatile memory applications by magnetron sputtering is introduced in this paper. The average size and distribution density of Cu nanocrystal grains are controlled by adjusting experimental parameters. The relationship between nanocrystal floating gate micro-structure and its charge storage capability is also discussed theoretically.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.10874132 and 11174228)the Doctoral Scientific Research Foundation of HUAT(Grant No.BK201407)One of the authors(Huang Hai-Ming)supported by the Scientific Research Items Foundation of Educational Committee of Hubei Province,China(Grant No.Q20131805)
文摘The quantum phase transition and the electronic transport in a triangular quantum dot system are investigated using the numerical renormalization group method.We concentrate on the interplay between the interdot capacitive coupling V and the interdot tunnel coupling t.For small t,three dots form a local spin doublet.As t increases,due to the competition between V and t,there exist two first-order transitions with phase sequence spin-doublet-magnetic frustration phase-orbital spin singlet.When t is absent,the evolutions of the total charge on the dots and the linear conductance are of the typical Coulomb-blockade features with increasing gate voltage.While for sufficient t,the antiferromagnetic spin correlation between dots is enhanced,and the conductance is strongly suppressed for the bonding state is almost doubly occupied.
文摘Nanometer-scale Au quantum dots have been assembled on SiO2 by controlling the reaction of raw materials to form a citrate Au sol and an aminosilane/dithiol-treated patterned Si wafer. The detailed formation mechanism has been studied. Three gold colloidal particles (15 nm), aligned in a chain to form a one-dimensional current path, was bridged across an 80-nm gap between source and drain metal electrodes. The device exhibited a Coulomb blockade effect at 33 K.
基金Funded by the National Natural Science Foundation of China(No.51772107)the Fundamental Research Funds for the Central Universities(No.2017KFYXJJ022)。
文摘To get a dielectric material with a high dielectric permittivity and suppressed dielectric loss,nano-Ag with a particle size of 20 nm and Ag@TiO_(2)core-shell particles with diameters of approximately 70-120 nm were embedded in polyvinylidene fluoride(PVDF)to fabricate nano-Ag/Ag@TiO_(2)/PVDF composites.After being modified by nano-Ag with 3 vol%optimal amount,the relative permittivity(ε_r)at 100 Hz of 50 vol%Ag@TiO_(2)/PVDF composites was 61,and the dielectric loss can be suppressed to 0.04,almost 96.4%lower than that of unmodified composites,and a higher frequency stability of bothε_r and loss has also been found.The underlying mechanism of the reduced loss was attributed to Maxwell-Wagner polarization and the Coulomb blockade effect caused by the introduction of a small amount of nano-Ag,which will block the movement of electrons between metal nanoparticles and composites.The space charge polarization and conductance loss are weakened at lower and higher Ag@TiO_(2)filling ratios,respectively,thus leading to a very low loss of the composites.
文摘A method of fabricating Cu nanocrystals embedded in SiO2 dielectric film for nonvolatile memory applications by magnetron sputtering is introduced in this paper. The average size and distribution density of Cu nanocrystal grains are controlled by adjusting experimental parameters. The relationship between nanocrystal floating gate micro-structure and its charge storage capability is also discussed theoretically.
