Nonlinear optical CsB3O5 single crystals have been grown successfully using NaF as a flux. The primary CsB3O5-NaF quasi-binary system has been investigated by X-ray diffraction and differential thermal analysis. There...Nonlinear optical CsB3O5 single crystals have been grown successfully using NaF as a flux. The primary CsB3O5-NaF quasi-binary system has been investigated by X-ray diffraction and differential thermal analysis. There is a single eutectic point, and the eutectic composition corresponds to 40mol% NaF with the temperature of 690.5 ℃ in CsB3O5-NaF system. Volatility of the CsB3O5-NaF system along the liquidus has been measured, and the volatiles of the solution were collected and detected by XRD method. Growth of CsB3O5 crystals was carried out by different composition of NaF in CsB3O5-NaF system, and the growth parameters were discussed. Simultaneously, the properties of grown crystals from NaF flux were characterized by transmission spectrum and scanning electron microscopy.展开更多
We report on the experimental investigation and theoretical analysis of a nanosecond pulse high power ultraviolet（UV） 278 nm laser by fourth-harmonic generation（FHG） of a 1112-nm Nd：YAG amplifier in LiB3O5（LBO）...We report on the experimental investigation and theoretical analysis of a nanosecond pulse high power ultraviolet（UV） 278 nm laser by fourth-harmonic generation（FHG） of a 1112-nm Nd：YAG amplifier in LiB3O5（LBO） and CsB3O5（CBO） crystals. The UV laser delivers a maximum average power of 10.3 W at 278 nm with peak power of 36.8 k W under input pump power of 41 W at 556 nm. This is, to the best of our knowledge, the highest output power at the specific UV wavelength of 278 nm. We also performed the theoretical investigation on the FHG with a model in the Gaussian approximation of both spatial and temporal profiles, especially accounting for the two-photon absorption effect in CBO crystal for the first time. The average output power, pulse width, and beam spatial distribution of the UV laser were simulated. The theoretical calculations are in close agreement with the experimental results.展开更多
基金This work was financially supported by the National Natural Science Foundation of China (No. 60378026)
文摘Nonlinear optical CsB3O5 single crystals have been grown successfully using NaF as a flux. The primary CsB3O5-NaF quasi-binary system has been investigated by X-ray diffraction and differential thermal analysis. There is a single eutectic point, and the eutectic composition corresponds to 40mol% NaF with the temperature of 690.5 ℃ in CsB3O5-NaF system. Volatility of the CsB3O5-NaF system along the liquidus has been measured, and the volatiles of the solution were collected and detected by XRD method. Growth of CsB3O5 crystals was carried out by different composition of NaF in CsB3O5-NaF system, and the growth parameters were discussed. Simultaneously, the properties of grown crystals from NaF flux were characterized by transmission spectrum and scanning electron microscopy.
基金Project supported by the National Natural Science Foundation Program of China(Grant Nos.11504389 and 61505226)the National Key Research Development Program of China(Grant Nos.2016YFB040203 and 61535013)the National Development Project for Major Scientific Research Facility of China(Grant No.ZDYZ2012-2)
文摘We report on the experimental investigation and theoretical analysis of a nanosecond pulse high power ultraviolet（UV） 278 nm laser by fourth-harmonic generation（FHG） of a 1112-nm Nd：YAG amplifier in LiB3O5（LBO） and CsB3O5（CBO） crystals. The UV laser delivers a maximum average power of 10.3 W at 278 nm with peak power of 36.8 k W under input pump power of 41 W at 556 nm. This is, to the best of our knowledge, the highest output power at the specific UV wavelength of 278 nm. We also performed the theoretical investigation on the FHG with a model in the Gaussian approximation of both spatial and temporal profiles, especially accounting for the two-photon absorption effect in CBO crystal for the first time. The average output power, pulse width, and beam spatial distribution of the UV laser were simulated. The theoretical calculations are in close agreement with the experimental results.
