The skin heat loss(heat flow)of summer fabrics duringthe course of sweating--evaporating--drying is mea-sured by an apparatus specially made for the purpose.Itis pointed out that:the dynamic heat-moisture comfortcan b...The skin heat loss(heat flow)of summer fabrics duringthe course of sweating--evaporating--drying is mea-sured by an apparatus specially made for the purpose.Itis pointed out that:the dynamic heat-moisture comfortcan be described by evaporating rate or time required fordrying out of a certain amount of sweat.The evaporat-ing rate is influenced by the hygroscopic property andthickness of the fabric,the larger the hygroscopicity ofthe fabric with the same thickness,the smaller the evap-orating rate of the perspirated sweat.展开更多
The intention of this fundamental work is to explore the manipulation of a mixture of benzene,toluene and o-xylene separated from liquid-only transfer divided-wall column(LTS-DWC).First,two control structures are clea...The intention of this fundamental work is to explore the manipulation of a mixture of benzene,toluene and o-xylene separated from liquid-only transfer divided-wall column(LTS-DWC).First,two control structures are clearly proposed,including seven component control loops(CS1)and seven temperature control loops(CS2).However,two control structures can handle ±10% feed disturbances rather than larger feed disturbances.Subsequently,an equivalent four-column model by introducing withdraw ratio is developed to discuss the effect of two liquid-only side-stream on the overall reboiler duty.It is indicated that the second liquid-only side-stream withdraw ratio strongly affects the overall energy consumption.Hence,six-component control loops within the fixed second liquid-only side-stream withdraw ratio(CS3)is proposed and the purity of products returns to set value even as facing ±20% feed disturbances.Finally,based on the above results,it is established a temperature control structure(CS4)for controlling fixed second liquid-only side-stream withdraw ratio,which can cope with ±15% disturbances.Inspired by these findings,an insight into the dynamic control of LTS-DWC promotes the industrial implementation of DWC through new liquid-only side-stream configurations.展开更多
We present a quantum dynamics study on the isotope effects of hydro-gen transfer isomerization in the formic acid dimer,and this is achieved by multidimensional dy-namics calculations with an efficient quantum mechani...We present a quantum dynamics study on the isotope effects of hydro-gen transfer isomerization in the formic acid dimer,and this is achieved by multidimensional dy-namics calculations with an efficient quantum mechanical theoretical scheme developed by our group,on a full-dimensional neural network ab initio potential energy surface.The ground-state and fundamental tun-neling splittings for four deuterium isotopologues of formic acid dimer are considered,and the calculated results are in very good general agreement with the avail-able experimental measurements.Strong isotope effects are revealed,the mode-specific funda-mental excitation effects on the tunneling rate are evidently influenced by the deuterium sub-stitution of H atom with the substitution on the OH bond being more effective than on the CH bond.Our studies are helpful for acquiring a better understanding of isotope effects in the double-hydrogen transfer processes.展开更多
The selective aerobic oxidation of benzyl alcohol to benzaldehyde has attracted considerable attention because benzaldehyde is a high value-added product. The rate of this typical gas–liquid reaction is significantly...The selective aerobic oxidation of benzyl alcohol to benzaldehyde has attracted considerable attention because benzaldehyde is a high value-added product. The rate of this typical gas–liquid reaction is significantly affected by mass transfer. In this study, CoTPP-mediated(CoTPP: cobalt(II) mesotetraphenylporphyrin) selective benzyl alcohol oxidation with oxygen was conducted in a membrane microchannel(MMC) reactor and a bubble column(BC) reactor, respectively. We observed that 83% benzyl alcohol was converted within 6.5 min in the MMC reactor, but only less than 10% benzyl alcohol was converted in the BC reactor. Hydrodynamic characteristics and gas–liquid mass transfer performances were compared for the MMC and BC reactors. The MMC reactor was assumed to be a plug flow reactor,and the dimensionless variance was 0.29. Compared to the BC reactor, the gas–liquid mass transfer was intensified significantly in MMC reactor. It could be ascribed to the high gas holdup(2.9 times higher than that of BC reactor), liquid film mass transfer coefficient(8.2 times higher than that of BC reactor), and mass transfer coefficient per unit interfacial area(3.8 times higher than that of BC reactor). Moreover,the Hatta number for the MMC reactor reached up to 0.61, which was about 15 times higher than that of the BC reactor. The computational fluid dynamics calculations for mass fractions in both liquid and gas phases were consistent with the experimental data.展开更多
In this paper, by defining new state vectors and developing new transfer matrices of various elements mov- ing in space, the discrete time transfer matrix method of multi-rigid-flexible-body system is expanded to stud...In this paper, by defining new state vectors and developing new transfer matrices of various elements mov- ing in space, the discrete time transfer matrix method of multi-rigid-flexible-body system is expanded to study the dynamics of multibody system with flexible beams moving in space. Formulations and numerical example of a rigid- flexible-body three pendulums system moving in space are given to validate the method. Using the new method to study the dynamics of multi-rigid-flexible-body system mov- ing in space, the global dynamics equations of system are not needed, the orders of involved matrices of the system are very low and the computational speed is high, irrespec- tive of the size of the system. The new method is simple, straightforward, practical, and provides a powerful tool for multi-rigid-flexible-body system dynamics.展开更多
In machinery fault diagnosis,labeled data are always difficult or even impossible to obtain.Transfer learning can leverage related fault diagnosis knowledge from fully labeled source domain to enhance the fault diagno...In machinery fault diagnosis,labeled data are always difficult or even impossible to obtain.Transfer learning can leverage related fault diagnosis knowledge from fully labeled source domain to enhance the fault diagnosis performance in sparsely labeled or unlabeled target domain,which has been widely used for cross domain fault diagnosis.However,existing methods focus on either marginal distribution adaptation(MDA)or conditional distribution adaptation(CDA).In practice,marginal and conditional distributions discrepancies both have significant but different influences on the domain divergence.In this paper,a dynamic distribution adaptation based transfer network(DDATN)is proposed for cross domain bearing fault diagnosis.DDATN utilizes the proposed instance-weighted dynamic maximum mean discrepancy(IDMMD)for dynamic distribution adaptation(DDA),which can dynamically estimate the influences of marginal and conditional distribution and adapt target domain with source domain.The experimental evaluation on cross domain bearing fault diagnosis demonstrates that DDATN can outperformance the state-of-the-art cross domain fault diagnosis methods.展开更多
The dynamic stiffness method and Transfer method is applied to study the vibration characteristics of the Euler-Bernoulli pipe conveying fluid in this paper. According to the dynamics equation of the pipe conveying fl...The dynamic stiffness method and Transfer method is applied to study the vibration characteristics of the Euler-Bernoulli pipe conveying fluid in this paper. According to the dynamics equation of the pipe conveying fluid, the element dynamic stiffness is established. The vibration characteristic of the single-span pipe is analyzed under two kinds of boundary conditions. The results compared with the literature, which has a good consistency. Based on this method, natural frequency and the critical speed of the two types of multi-span pipe are deserved. This paper shows that the dynamic stiffness method and transfer matrix is an effective method to deal with the vibration problem of pipe conveying fluid.展开更多
In forecasting real time environmental factors,large data is needed to analyse the pattern behind the data values.Air pollution is a major threat towards developing countries and it is proliferating every year.Many me...In forecasting real time environmental factors,large data is needed to analyse the pattern behind the data values.Air pollution is a major threat towards developing countries and it is proliferating every year.Many methods in time ser-ies prediction and deep learning models to estimate the severity of air pollution.Each independent variable contributing towards pollution is necessary to analyse the trend behind the air pollution in that particular locality.This approach selects multivariate time series and coalesce a real time updatable autoregressive model to forecast Particulate matter(PM)PM2.5.To perform experimental analysis the data from the Central Pollution Control Board(CPCB)is used.Prediction is car-ried out for Chennai with seven locations and estimated PM’s using the weighted ensemble method.Proposed method for air pollution prediction unveiled effective and moored performance in long term prediction.Dynamic budge with high weighted k-models are used simultaneously and devising an ensemble helps to achieve stable forecasting.Computational time of ensemble decreases with paral-lel processing in each sub model.Weighted ensemble model shows high perfor-mance in long term prediction when compared to the traditional time series models like Vector Auto-Regression(VAR),Autoregressive Integrated with Mov-ing Average(ARIMA),Autoregressive Moving Average with Extended terms(ARMEX).Evaluation metrics like Root Mean Square Error(RMSE),Mean Absolute Error(MAE)and the time to achieve the time series are compared.展开更多
A mathematical model has been developed to describe the dynamic heat transfer in the clothing microclimate under transient wear conditions. This model is solved numerically by the implicit finite difference method. If...A mathematical model has been developed to describe the dynamic heat transfer in the clothing microclimate under transient wear conditions. This model is solved numerically by the implicit finite difference method. If the physical activity and ambient conditions are specified, the model can predict the thermoregulatory response of the body. Experimental measurements with garments made of fibers with different levels of hygroscopicity are compared with predictions by the model. There is good agreement between prediction and experiment for the temperature of the clothing microclimate.展开更多
Surface oxygen vacancies(OVs) with abundant localized electrons on bismuth-oxygen based photocatalysts are proved to have the ability to capture and activate CO_(2).However,the surface OVs are easily filled with oxyge...Surface oxygen vacancies(OVs) with abundant localized electrons on bismuth-oxygen based photocatalysts are proved to have the ability to capture and activate CO_(2).However,the surface OVs are easily filled with oxygen-containing species and destroyed,losing their effects as active sites and hindering the subsequent CO_(2)photoreduction.For realistic and sustainable CO_(2)photoreduction,constructing sustainable and stable surface OVs as active sites on photocatalysts is essential.This work shows the synthesis of interlayer stretched Bi_(2)O_(2)CO_(3) ultrathin nanosheets with tensile stress,which are beneficial to continuously generating light-induced dynamic OVs.With sufficient active sites,excellent,stable,and selective photoreduction of CO_(2)to CO under simulated solar light is achieved.The light-induced OVs can reduce the energy barrier of rate-determining step,resulting in the 100% product selectivity.The results presented herein demonstrate the effect of dynamic OVs induced by interlayer tensile strain on catalysts for the enhanced selective CO_(2)photoreduction process.展开更多
The hybrid dynamics of multi-rigid-body and multi-flexible-body system becomes the mainstream of multi-body dynamics.Currently there lacks a compact approach to model the hybrid dynamics,especially in modern machine t...The hybrid dynamics of multi-rigid-body and multi-flexible-body system becomes the mainstream of multi-body dynamics.Currently there lacks a compact approach to model the hybrid dynamics,especially in modern machine tool application,due to the difficulty of solving the hybrid equations or the limitation of current software when dealing with the hybrid dynamics.The extended transfer matrix method(E-TMM),which extends elements in three-dimensional space with higher matrixes,is proposed to simplify the modeling process of the hybrid dynamics.The E-TMM modeling approaches of 3 basic elements including 3D vibrant rigid body,joint and flexible body are studied in details.A parallel mill-turn tool spindle head unit driven by dual-linear motors is chosen as a plant to demonstrate the E-TMM modeling process.By using E-TMM,the spindle head unit is simplified as a topological network consisting of the three types of element,i.e.,3D vibrant rigid body,joint and flexible body,including 11 rigid bodies,14 joints and 1 3D-Timoshenko beam.Then the dynamic model of the system can be easily obtained by deducing the element-network by means of state vector transformation.The dynamic characteristics of the spindle head,such as natural frequencies,dynamic flexibility,etc.can be predicted by solving the obtained model.Experiment verification indicates that the E-TMM is valid with enough accuracy in the dynamic analysis of the parallel mill-turn tool spindle head.The E-TMM is capable of modeling the dynamics of machine tool structure with no requirements of deducing and solving the sophisticated differential equations.Moreover,the E-TMM provides a simple and elegant tool for hybrid dynamic analysis in future dynamic design of machine tools.展开更多
A numerical investigation is conducted to explore the evolution of a plasma discharge and its interaction with the fluid flow based on a self-consistent fluid model which couples the discharge dynamics with the fluid ...A numerical investigation is conducted to explore the evolution of a plasma discharge and its interaction with the fluid flow based on a self-consistent fluid model which couples the discharge dynamics with the fluid dynamics.The effects of the applied voltage on the distribution of velocity and temperature in initially static air are parainetrically studied.Furthermore,the spatial structure of plasma discharge and the resulting force contours in streamwise and normal directions are discussed in detail.The result shows that the plasma actuator produces a net force that should always be directed away from the exposed electrode,which results in an ionic wind pushing particles into a jet downstream of the actuator.When the energy added by the plasma is taken into account,the ambient air temperature is increased slightly around the electrode,but the velocity is almost not affected.Therefore it is unlikely that the induced flow is buoyancy driven.For the operating voltages considered in this paper,the maximum induced velocity is found to follow a power law,i.e.,it is proportional to the applied voltage to the 3.5 power.This promises an efficient application in the flow control with plasma actuators.展开更多
A sweating apparatus has been developed to permit simultaneous measurement for fabric temperature change and relative humidity change at outer still air layer of fabrics. In this paper, we compared the temperature and...A sweating apparatus has been developed to permit simultaneous measurement for fabric temperature change and relative humidity change at outer still air layer of fabrics. In this paper, we compared the temperature and relative humidity changes for silk fabrics with polyester fabrics and got GM(1,P) relation models respectively between maximum fabric temperature change, maximum relative humidity change at outer still air layer and relative fabric character parameters. Furthermore, by comparing the objective experiments with subjective wear trials, it is found that the amounts of the change rate of fabric temperature and relative humidity at outer still layer are the most important factors which influence clothing comfort in dynamic moisture transfer condition. The more the changes of temperature and R.H., the more the mugginess and the thermal sensation.展开更多
Following Tsai & Ma[1] and Tsai & Liu[2], a statistical and dynamical near-wall turbulent coherent structural model with separate consideration of two different portions:locally generated and upstream-transpo...Following Tsai & Ma[1] and Tsai & Liu[2], a statistical and dynamical near-wall turbulent coherent structural model with separate consideration of two different portions:locally generated and upstream-transported large eddies has been established.With this model, heat transfer in a fully developed open channel in the absence of pressure gradient is numerically simulated. Database of fluctuations of velocity and temperature has also been set. Numerical analysis shows the existence of high-low temperature streak caused by near-wall coherent structure and its swing in the lateral direction.Numerical results are in accordance with the computations and experimental results of other researchers.展开更多
From resolution of two-dimensional equation of heat in dynamic frequency regime, we have plotted evolution curves of temperature according to depth of material or in lateral direction. They will allow us to evaluate t...From resolution of two-dimensional equation of heat in dynamic frequency regime, we have plotted evolution curves of temperature according to depth of material or in lateral direction. They will allow us to evaluate thermal behavior of towed material. Aim of study is to use fibers as a thermal insulating material by proposing a method for determining effective thermal insulation layer in dynamic frequency regime.展开更多
This work reveals essential details of plasma-surface interaction in atmospheric air that are important for a wide range of applications, beginning from airflow control and up to the high-voltage insulation. The paper...This work reveals essential details of plasma-surface interaction in atmospheric air that are important for a wide range of applications, beginning from airflow control and up to the high-voltage insulation. The paper discusses experimental data characterizing dynamics of development and kinetics of energy coupling in surface dielectric barrier discharge (SDBD), atmospheric air plasmas sustained over dielectric surfaces, over a wide range of time scales. The experiments have been conducted using microsecond pulse voltage waveform of single and alternating polarities. Time-resolved discharge development and mechanisms of coupling with quiescent air are analyzed using nanosecond gate camera imaging, electrical measurements, and original surface charge sensors. The results demonstrate several new, critically important processes overlooked in previous studies. Specifically, it is shown that SDBD plasmas energy release may be significantly increased by using an optimized waveform.展开更多
In this paper the results of dynamic NMR studies on ethylmethylamino-tertiary-butyl-phenylborane (EMABPB) with or without light are reported. The NMR data were recorded on a Bruker 400 MHz NMR equipped with our custom...In this paper the results of dynamic NMR studies on ethylmethylamino-tertiary-butyl-phenylborane (EMABPB) with or without light are reported. The NMR data were recorded on a Bruker 400 MHz NMR equipped with our custom-made optical probe and with our custom-made 450 watts (W) monochromatic light sources. The molecular photochemistry including twisted intramolecular charge-transfer-excited-state (TICT) of the EMABPB in several solvents has been investigated. These results indicate that the aminoborane demonstrates multiple configurations in CD3Cl and CD2Cl2 resulting in the shifts of the signals of the alkyl groups on the nitrogen and boron. This indicates that there are some time-dependent changes at constant temperature over the irradiation interval. At ﹣60°C and the presence of light (λ = 265 nm), we observed a large change in the populations of the two sites, and this by itself indicates a modification in the rotation around the boron nitrogen bond in the excited state. By considering the existence of the TICT state, many important energy technologies may be developed with higher efficiency by controlling the back-electron transfer processes.展开更多
We investigate the dynamics of entanglement in the excitation transfer through a model consisting of three interacting molecules coupled to environments. It is shown that the entanglement can be further enhanced if th...We investigate the dynamics of entanglement in the excitation transfer through a model consisting of three interacting molecules coupled to environments. It is shown that the entanglement can be further enhanced if the distance between the molecules is oscillating. Our results demonstrate that the motional effect plays a constructive role on quantum entanglement in the dynamics of excitation transfer. This mechanism might provide a useful guideline for designing artificial systems to battle against decoherence.展开更多
To find the difference in dynamic characteristics between conventional monohull ship and wave penetrating catamaran (WPC), a WPC was taken as an object; its dynamic characteristics were computed by transfer matrix met...To find the difference in dynamic characteristics between conventional monohull ship and wave penetrating catamaran (WPC), a WPC was taken as an object; its dynamic characteristics were computed by transfer matrix method and finite element method respectively. According to the comparison of the nature frequency results and mode shape results, the fact that FEM method is more suitable to dynamic characteristics analysis of a WPC was pointed out, special features on dynamic characteristics of WPC were given, and some beneficial suggestions are proposed to optimize the strength of a WPC in design period.展开更多
文摘The skin heat loss(heat flow)of summer fabrics duringthe course of sweating--evaporating--drying is mea-sured by an apparatus specially made for the purpose.Itis pointed out that:the dynamic heat-moisture comfortcan be described by evaporating rate or time required fordrying out of a certain amount of sweat.The evaporat-ing rate is influenced by the hygroscopic property andthickness of the fabric,the larger the hygroscopicity ofthe fabric with the same thickness,the smaller the evap-orating rate of the perspirated sweat.
基金supported by National Natural Science Foundation of China(21908056)Shanghai Sailing Program(19YF1410800)Science and Technology Commission of Shanghai Municipality(19DZ2271100)。
文摘The intention of this fundamental work is to explore the manipulation of a mixture of benzene,toluene and o-xylene separated from liquid-only transfer divided-wall column(LTS-DWC).First,two control structures are clearly proposed,including seven component control loops(CS1)and seven temperature control loops(CS2).However,two control structures can handle ±10% feed disturbances rather than larger feed disturbances.Subsequently,an equivalent four-column model by introducing withdraw ratio is developed to discuss the effect of two liquid-only side-stream on the overall reboiler duty.It is indicated that the second liquid-only side-stream withdraw ratio strongly affects the overall energy consumption.Hence,six-component control loops within the fixed second liquid-only side-stream withdraw ratio(CS3)is proposed and the purity of products returns to set value even as facing ±20% feed disturbances.Finally,based on the above results,it is established a temperature control structure(CS4)for controlling fixed second liquid-only side-stream withdraw ratio,which can cope with ±15% disturbances.Inspired by these findings,an insight into the dynamic control of LTS-DWC promotes the industrial implementation of DWC through new liquid-only side-stream configurations.
基金supported by the National Natural Sci-ence Foundation of China(No.21973098 and No.22133003)the Beijing National Laboratory for Molecular SciencesJianwei Cao acknowledges the Youth Innovation Promotion Association CAS(No.2018045).
文摘We present a quantum dynamics study on the isotope effects of hydro-gen transfer isomerization in the formic acid dimer,and this is achieved by multidimensional dy-namics calculations with an efficient quantum mechanical theoretical scheme developed by our group,on a full-dimensional neural network ab initio potential energy surface.The ground-state and fundamental tun-neling splittings for four deuterium isotopologues of formic acid dimer are considered,and the calculated results are in very good general agreement with the avail-able experimental measurements.Strong isotope effects are revealed,the mode-specific funda-mental excitation effects on the tunneling rate are evidently influenced by the deuterium sub-stitution of H atom with the substitution on the OH bond being more effective than on the CH bond.Our studies are helpful for acquiring a better understanding of isotope effects in the double-hydrogen transfer processes.
基金financially supported by the National Key Research and Development Program of China (2020YFA0210900)the National Natural Science Foundation of China (21938001 and 21878344)+1 种基金Guangdong Provincial Key Research and Development Programme (2019B110206002)the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01C102)。
文摘The selective aerobic oxidation of benzyl alcohol to benzaldehyde has attracted considerable attention because benzaldehyde is a high value-added product. The rate of this typical gas–liquid reaction is significantly affected by mass transfer. In this study, CoTPP-mediated(CoTPP: cobalt(II) mesotetraphenylporphyrin) selective benzyl alcohol oxidation with oxygen was conducted in a membrane microchannel(MMC) reactor and a bubble column(BC) reactor, respectively. We observed that 83% benzyl alcohol was converted within 6.5 min in the MMC reactor, but only less than 10% benzyl alcohol was converted in the BC reactor. Hydrodynamic characteristics and gas–liquid mass transfer performances were compared for the MMC and BC reactors. The MMC reactor was assumed to be a plug flow reactor,and the dimensionless variance was 0.29. Compared to the BC reactor, the gas–liquid mass transfer was intensified significantly in MMC reactor. It could be ascribed to the high gas holdup(2.9 times higher than that of BC reactor), liquid film mass transfer coefficient(8.2 times higher than that of BC reactor), and mass transfer coefficient per unit interfacial area(3.8 times higher than that of BC reactor). Moreover,the Hatta number for the MMC reactor reached up to 0.61, which was about 15 times higher than that of the BC reactor. The computational fluid dynamics calculations for mass fractions in both liquid and gas phases were consistent with the experimental data.
基金supported by the Natural Science Foundation of China Government (10902051)the Natural Science Foundation of Jiangsu Province (BK2008046)the German Science Foundation
文摘In this paper, by defining new state vectors and developing new transfer matrices of various elements mov- ing in space, the discrete time transfer matrix method of multi-rigid-flexible-body system is expanded to study the dynamics of multibody system with flexible beams moving in space. Formulations and numerical example of a rigid- flexible-body three pendulums system moving in space are given to validate the method. Using the new method to study the dynamics of multi-rigid-flexible-body system mov- ing in space, the global dynamics equations of system are not needed, the orders of involved matrices of the system are very low and the computational speed is high, irrespec- tive of the size of the system. The new method is simple, straightforward, practical, and provides a powerful tool for multi-rigid-flexible-body system dynamics.
基金Supported by National Natural Science Foundation of China(Grant Nos.51875208,51475170)National Key Research and Development Program of China(Grant No.2018YFB1702400).
文摘In machinery fault diagnosis,labeled data are always difficult or even impossible to obtain.Transfer learning can leverage related fault diagnosis knowledge from fully labeled source domain to enhance the fault diagnosis performance in sparsely labeled or unlabeled target domain,which has been widely used for cross domain fault diagnosis.However,existing methods focus on either marginal distribution adaptation(MDA)or conditional distribution adaptation(CDA).In practice,marginal and conditional distributions discrepancies both have significant but different influences on the domain divergence.In this paper,a dynamic distribution adaptation based transfer network(DDATN)is proposed for cross domain bearing fault diagnosis.DDATN utilizes the proposed instance-weighted dynamic maximum mean discrepancy(IDMMD)for dynamic distribution adaptation(DDA),which can dynamically estimate the influences of marginal and conditional distribution and adapt target domain with source domain.The experimental evaluation on cross domain bearing fault diagnosis demonstrates that DDATN can outperformance the state-of-the-art cross domain fault diagnosis methods.
文摘The dynamic stiffness method and Transfer method is applied to study the vibration characteristics of the Euler-Bernoulli pipe conveying fluid in this paper. According to the dynamics equation of the pipe conveying fluid, the element dynamic stiffness is established. The vibration characteristic of the single-span pipe is analyzed under two kinds of boundary conditions. The results compared with the literature, which has a good consistency. Based on this method, natural frequency and the critical speed of the two types of multi-span pipe are deserved. This paper shows that the dynamic stiffness method and transfer matrix is an effective method to deal with the vibration problem of pipe conveying fluid.
文摘In forecasting real time environmental factors,large data is needed to analyse the pattern behind the data values.Air pollution is a major threat towards developing countries and it is proliferating every year.Many methods in time ser-ies prediction and deep learning models to estimate the severity of air pollution.Each independent variable contributing towards pollution is necessary to analyse the trend behind the air pollution in that particular locality.This approach selects multivariate time series and coalesce a real time updatable autoregressive model to forecast Particulate matter(PM)PM2.5.To perform experimental analysis the data from the Central Pollution Control Board(CPCB)is used.Prediction is car-ried out for Chennai with seven locations and estimated PM’s using the weighted ensemble method.Proposed method for air pollution prediction unveiled effective and moored performance in long term prediction.Dynamic budge with high weighted k-models are used simultaneously and devising an ensemble helps to achieve stable forecasting.Computational time of ensemble decreases with paral-lel processing in each sub model.Weighted ensemble model shows high perfor-mance in long term prediction when compared to the traditional time series models like Vector Auto-Regression(VAR),Autoregressive Integrated with Mov-ing Average(ARIMA),Autoregressive Moving Average with Extended terms(ARMEX).Evaluation metrics like Root Mean Square Error(RMSE),Mean Absolute Error(MAE)and the time to achieve the time series are compared.
文摘A mathematical model has been developed to describe the dynamic heat transfer in the clothing microclimate under transient wear conditions. This model is solved numerically by the implicit finite difference method. If the physical activity and ambient conditions are specified, the model can predict the thermoregulatory response of the body. Experimental measurements with garments made of fibers with different levels of hygroscopicity are compared with predictions by the model. There is good agreement between prediction and experiment for the temperature of the clothing microclimate.
基金supported by the National Natural Science Foundation of China (52200123, 22225606, 22261142663)。
文摘Surface oxygen vacancies(OVs) with abundant localized electrons on bismuth-oxygen based photocatalysts are proved to have the ability to capture and activate CO_(2).However,the surface OVs are easily filled with oxygen-containing species and destroyed,losing their effects as active sites and hindering the subsequent CO_(2)photoreduction.For realistic and sustainable CO_(2)photoreduction,constructing sustainable and stable surface OVs as active sites on photocatalysts is essential.This work shows the synthesis of interlayer stretched Bi_(2)O_(2)CO_(3) ultrathin nanosheets with tensile stress,which are beneficial to continuously generating light-induced dynamic OVs.With sufficient active sites,excellent,stable,and selective photoreduction of CO_(2)to CO under simulated solar light is achieved.The light-induced OVs can reduce the energy barrier of rate-determining step,resulting in the 100% product selectivity.The results presented herein demonstrate the effect of dynamic OVs induced by interlayer tensile strain on catalysts for the enhanced selective CO_(2)photoreduction process.
基金supported by National Key Technology R&D Program of China (Grant No. 2006BAF01B09)the Research Fund for Doctoral Program of Higher Education of China (Grant No. 200800060010)
文摘The hybrid dynamics of multi-rigid-body and multi-flexible-body system becomes the mainstream of multi-body dynamics.Currently there lacks a compact approach to model the hybrid dynamics,especially in modern machine tool application,due to the difficulty of solving the hybrid equations or the limitation of current software when dealing with the hybrid dynamics.The extended transfer matrix method(E-TMM),which extends elements in three-dimensional space with higher matrixes,is proposed to simplify the modeling process of the hybrid dynamics.The E-TMM modeling approaches of 3 basic elements including 3D vibrant rigid body,joint and flexible body are studied in details.A parallel mill-turn tool spindle head unit driven by dual-linear motors is chosen as a plant to demonstrate the E-TMM modeling process.By using E-TMM,the spindle head unit is simplified as a topological network consisting of the three types of element,i.e.,3D vibrant rigid body,joint and flexible body,including 11 rigid bodies,14 joints and 1 3D-Timoshenko beam.Then the dynamic model of the system can be easily obtained by deducing the element-network by means of state vector transformation.The dynamic characteristics of the spindle head,such as natural frequencies,dynamic flexibility,etc.can be predicted by solving the obtained model.Experiment verification indicates that the E-TMM is valid with enough accuracy in the dynamic analysis of the parallel mill-turn tool spindle head.The E-TMM is capable of modeling the dynamics of machine tool structure with no requirements of deducing and solving the sophisticated differential equations.Moreover,the E-TMM provides a simple and elegant tool for hybrid dynamic analysis in future dynamic design of machine tools.
基金supported by the Foundation for Innovative Research Groups of National Natural Science Foundation of China(No.51121004)National Natural Science Foundation of China(No.50976026)
文摘A numerical investigation is conducted to explore the evolution of a plasma discharge and its interaction with the fluid flow based on a self-consistent fluid model which couples the discharge dynamics with the fluid dynamics.The effects of the applied voltage on the distribution of velocity and temperature in initially static air are parainetrically studied.Furthermore,the spatial structure of plasma discharge and the resulting force contours in streamwise and normal directions are discussed in detail.The result shows that the plasma actuator produces a net force that should always be directed away from the exposed electrode,which results in an ionic wind pushing particles into a jet downstream of the actuator.When the energy added by the plasma is taken into account,the ambient air temperature is increased slightly around the electrode,but the velocity is almost not affected.Therefore it is unlikely that the induced flow is buoyancy driven.For the operating voltages considered in this paper,the maximum induced velocity is found to follow a power law,i.e.,it is proportional to the applied voltage to the 3.5 power.This promises an efficient application in the flow control with plasma actuators.
文摘A sweating apparatus has been developed to permit simultaneous measurement for fabric temperature change and relative humidity change at outer still air layer of fabrics. In this paper, we compared the temperature and relative humidity changes for silk fabrics with polyester fabrics and got GM(1,P) relation models respectively between maximum fabric temperature change, maximum relative humidity change at outer still air layer and relative fabric character parameters. Furthermore, by comparing the objective experiments with subjective wear trials, it is found that the amounts of the change rate of fabric temperature and relative humidity at outer still layer are the most important factors which influence clothing comfort in dynamic moisture transfer condition. The more the changes of temperature and R.H., the more the mugginess and the thermal sensation.
文摘Following Tsai & Ma[1] and Tsai & Liu[2], a statistical and dynamical near-wall turbulent coherent structural model with separate consideration of two different portions:locally generated and upstream-transported large eddies has been established.With this model, heat transfer in a fully developed open channel in the absence of pressure gradient is numerically simulated. Database of fluctuations of velocity and temperature has also been set. Numerical analysis shows the existence of high-low temperature streak caused by near-wall coherent structure and its swing in the lateral direction.Numerical results are in accordance with the computations and experimental results of other researchers.
文摘From resolution of two-dimensional equation of heat in dynamic frequency regime, we have plotted evolution curves of temperature according to depth of material or in lateral direction. They will allow us to evaluate thermal behavior of towed material. Aim of study is to use fibers as a thermal insulating material by proposing a method for determining effective thermal insulation layer in dynamic frequency regime.
文摘This work reveals essential details of plasma-surface interaction in atmospheric air that are important for a wide range of applications, beginning from airflow control and up to the high-voltage insulation. The paper discusses experimental data characterizing dynamics of development and kinetics of energy coupling in surface dielectric barrier discharge (SDBD), atmospheric air plasmas sustained over dielectric surfaces, over a wide range of time scales. The experiments have been conducted using microsecond pulse voltage waveform of single and alternating polarities. Time-resolved discharge development and mechanisms of coupling with quiescent air are analyzed using nanosecond gate camera imaging, electrical measurements, and original surface charge sensors. The results demonstrate several new, critically important processes overlooked in previous studies. Specifically, it is shown that SDBD plasmas energy release may be significantly increased by using an optimized waveform.
文摘In this paper the results of dynamic NMR studies on ethylmethylamino-tertiary-butyl-phenylborane (EMABPB) with or without light are reported. The NMR data were recorded on a Bruker 400 MHz NMR equipped with our custom-made optical probe and with our custom-made 450 watts (W) monochromatic light sources. The molecular photochemistry including twisted intramolecular charge-transfer-excited-state (TICT) of the EMABPB in several solvents has been investigated. These results indicate that the aminoborane demonstrates multiple configurations in CD3Cl and CD2Cl2 resulting in the shifts of the signals of the alkyl groups on the nitrogen and boron. This indicates that there are some time-dependent changes at constant temperature over the irradiation interval. At ﹣60°C and the presence of light (λ = 265 nm), we observed a large change in the populations of the two sites, and this by itself indicates a modification in the rotation around the boron nitrogen bond in the excited state. By considering the existence of the TICT state, many important energy technologies may be developed with higher efficiency by controlling the back-electron transfer processes.
基金Supported by the National Natural Science Foundation of China under Grant Nos 11374085,61073048 and 11274010the Specialized Research Fund for the Doctoral Program of Higher Education under Grant No 20113401110002+3 种基金the 211 Project of Anhui Universitythe Anhui Provincial Natural Science Foundation under Grant No 1408085MA20the Personnel Department of Anhui Provincethe 136 Foundation of Hefei Normal University under Grant No 2014136KJB04
文摘We investigate the dynamics of entanglement in the excitation transfer through a model consisting of three interacting molecules coupled to environments. It is shown that the entanglement can be further enhanced if the distance between the molecules is oscillating. Our results demonstrate that the motional effect plays a constructive role on quantum entanglement in the dynamics of excitation transfer. This mechanism might provide a useful guideline for designing artificial systems to battle against decoherence.
文摘To find the difference in dynamic characteristics between conventional monohull ship and wave penetrating catamaran (WPC), a WPC was taken as an object; its dynamic characteristics were computed by transfer matrix method and finite element method respectively. According to the comparison of the nature frequency results and mode shape results, the fact that FEM method is more suitable to dynamic characteristics analysis of a WPC was pointed out, special features on dynamic characteristics of WPC were given, and some beneficial suggestions are proposed to optimize the strength of a WPC in design period.