Manure odor, which results in the increasing complaints and lawsuits, has increased the tension among swine producers and surrounding residents. The effects of Lactobacillus plantarum and different rates of soluble ca...Manure odor, which results in the increasing complaints and lawsuits, has increased the tension among swine producers and surrounding residents. The effects of Lactobacillus plantarum and different rates of soluble carbohydrates additions to swine manure on odorous compounds, chemical compounds and indigenous flora were evaluated. Additions were calculated on dried manure weight basis. Variables monitored included ammonia （NH3）, hydrogen sulfide （H2S）, odor offensiveness, pH, ammonium nitrogen（NH4^＋-N）, volatile fatty acids （VFAs）, urease and indigenous flora. The results indicated that the combination of L. plantarum and soluble carbohydrates dramatically reduced manure pH. Lower pH resulted in the reduction of NH3 volatilization （34.6%-92.4%, P〈0.01）, the increases of H2S （P〈 0.05） and NH4^＋-N （5.3%-17.5%, P〈0.05）. In addition, L. plantarum and soluble carbohydrates additions significantly reduced odor offensiveness, those VFAs related to malodor indicators（valeric acids, 12.3%-47.7%, P〈 0.05; iso-valeric, 3.5%-23.8%） and the main microorganisms responsible for odor production, with the number of Eubacteria in swine manure reducing by 4.9%, 11.6%, 17.4%, 34.1% and 32.2% respectively.展开更多
P omegranate(Punica granatum L.)has attracted considerable attention in world markets due to its valuable nutrients and highly appreciated sensory properties.The aroma profiles of 4 varieties of pomegranate juice,incl...P omegranate(Punica granatum L.)has attracted considerable attention in world markets due to its valuable nutrients and highly appreciated sensory properties.The aroma profiles of 4 varieties of pomegranate juice,including Dahongtian(DP),Jingpitian(JP),Luyudan(LP),and Tianhonngdan(TP),were investigated via gas chromatography-mass spectrometry(GC-MS)and gas chromatography-olfactometry(GC-O)analyses.A total of 43 volatile compounds were identified by using GC-MS.Among these compounds,16 were considered as potential aroma-active compounds as detected by GC-O.These compounds belonged to the classes of terpinenes,alcohols,and aldehydes.Eleven volatile compounds were defined as the main contributors to the overall aroma of pomegranate juice due to their high odor activity values(OAVs≥1).Aroma recombination and omission tests confirmed thatβ-myrcene,1-hexanol,and(Z)-3-hexen-1-ol were the key aroma compounds,and limonene,1-octen-3-ol,linalool,and hexanal were important aroma-active compounds in DP samples.展开更多
Three treatments were tested to investigate the release concentrations of volatile organic compounds （VOCs） during the bio-drying of municipal solid waste （MSW） by the aerobic and combined hydrolytic-aerobic proce...Three treatments were tested to investigate the release concentrations of volatile organic compounds （VOCs） during the bio-drying of municipal solid waste （MSW） by the aerobic and combined hydrolytic-aerobic processes.Results showed that VOCs were largely released in the first 4 days of bio-drying and the dominant components were：dimethyl disulfide,dimethyl sulfide,benzene,2-butanone,limonene and methylene chloride.Thus,the combined hydrolytic-aerobic process was suggested for MSW bio-drying due to fewer aeration quantities in this phase when compared with the aerobic process,and the treatment strategies should base on the key properties of these prominent components.Malodorous sulfur compounds and terpenes were mainly released in the early phase of bio-drying,whereas,two peaks of release concentrations appeared for aromatics and ketones during bio-drying.Notably,for the combined hydrolytic-aerobic processes there were also high concentrations of released aromatics in the shift from hydrolytic to aerobic stages.High concentrations of released chlorinateds were observed in the later phase.For the VOCs produced during MSW bio-drying,i.e.,malodorous sulfur compounds,terpenes and chlorinateds,their release concentrations were mainly determined by production rates;for the VOCs presented initially in MSW,such as aromatics,their transfer and transport in MSW mainly determined the release concentrations.展开更多
Volatile organic compounds(VOCs) emitted from stool are the components of the smell of stool representing the end products of microbial activity and metabolism that can be used to diagnose disease. Despite the abundan...Volatile organic compounds(VOCs) emitted from stool are the components of the smell of stool representing the end products of microbial activity and metabolism that can be used to diagnose disease. Despite the abundance of hydrogen, carbon dioxide, and methane that have already been identified in human flatus, the small portion of trace gases making up the VOCs emitted from stool include organic acids, alcohols, esters, heterocyclic compounds, aldehydes, ketones, and alkanes, among others. These are the gases that vary among individuals in sickness and in health, in dietary changes, and in gut microbial activity. Electronic nose devices are analytical and pattern recognition platforms that can utilize mass spectrometry or electrochemical sensors to detect these VOCs in gas samples. When paired with machine-learning and pattern recognition algorithms, this can identify patterns of VOCs, and thus patterns of smell, that can be used to identify disease states. In this review, we provide a clinical background of VOC identification, electronic nose development, and review gastroenterology applications toward diagnosing disease by the volatile headspace analysis of stool.展开更多
In this study, the amounts of odorous carbonyl compounds （OCCs） including acetaldehyde （Acet-A）, propionaldehyde （Pron-A）, butylaldehyde （Buty-A）, iso-valeric aldehyde （Iso-Vale-A） and n-valeric aldehyde （N...In this study, the amounts of odorous carbonyl compounds （OCCs） including acetaldehyde （Acet-A）, propionaldehyde （Pron-A）, butylaldehyde （Buty-A）, iso-valeric aldehyde （Iso-Vale-A） and n-valeric aldehyde （N-Vale-A） emitted from a fishery industrial complex near the exhibition facilities of ＂Expo 2012 Yeosu Korea＂ were measured. Acet-A was found to be the most abundant OCC, and the total concentrations of the OCCs were the highest in the summer. However, due to vehicular exhaust and photochemical reactions, the concentrations of some of the OCCs presented their highest levels in the fall. A significant correlation between Acet-A and Buty-A was found at the major fishery facilities （r = 0.816, p = 1.87E-15, n = 60） and at the border areas （r = 0.809, p = 3.40E-12, n = 48） of this fishery industrial complex. The concentrations of OCCs at the border areas were not worse than those at the urban areas in other places, indicating that the concentrations of ambient OCCs at the border areas were not greatly influenced by manmade activities.展开更多
Source separation sanitation systems have attracted more and more attention recently.However, separate urine collection and treatment could induce odor issues, especially in large scale application. In order to avoid ...Source separation sanitation systems have attracted more and more attention recently.However, separate urine collection and treatment could induce odor issues, especially in large scale application. In order to avoid such issues, it is necessary to monitor the odor related compounds that might be generated during urine storage. This study investigated the odorous compounds that emitted from source-separated human urine under different hydrolysis conditions. Batch experiments were conducted to investigate the effect of temperature, stale/fresh urine ratio and urine dilution on odor emissions. It was found that ammonia, dimethyl disulfide, allyl methyl sulfide and 4-heptanone were the main odorous compounds generated from human urine, with headspace concentrations hundreds of times higher than their respective odor thresholds. Furthermore, the high temperature accelerated urine hydrolysis and liquid–gas mass transfer, resulting a remarkable increase of odor emissions from the urine solution. The addition of stale urine enhanced urine hydrolysis and expedited odor emissions. On the contrary, diluted urine emitted less odorous compounds ascribed to reduced concentrations of odorant precursors. In addition,this study quantified the odor emissions and revealed the constraints of urine source separation in real-world applications. To address the odor issue, several control strategies are recommended for odor mitigation or elimination from an engineering perspective.展开更多
文摘Manure odor, which results in the increasing complaints and lawsuits, has increased the tension among swine producers and surrounding residents. The effects of Lactobacillus plantarum and different rates of soluble carbohydrates additions to swine manure on odorous compounds, chemical compounds and indigenous flora were evaluated. Additions were calculated on dried manure weight basis. Variables monitored included ammonia （NH3）, hydrogen sulfide （H2S）, odor offensiveness, pH, ammonium nitrogen（NH4^＋-N）, volatile fatty acids （VFAs）, urease and indigenous flora. The results indicated that the combination of L. plantarum and soluble carbohydrates dramatically reduced manure pH. Lower pH resulted in the reduction of NH3 volatilization （34.6%-92.4%, P〈0.01）, the increases of H2S （P〈 0.05） and NH4^＋-N （5.3%-17.5%, P〈0.05）. In addition, L. plantarum and soluble carbohydrates additions significantly reduced odor offensiveness, those VFAs related to malodor indicators（valeric acids, 12.3%-47.7%, P〈 0.05; iso-valeric, 3.5%-23.8%） and the main microorganisms responsible for odor production, with the number of Eubacteria in swine manure reducing by 4.9%, 11.6%, 17.4%, 34.1% and 32.2% respectively.
基金funded by Shaanxi Natural Science Foundation (2019JQ-665)Xi’an Agricultural Science and Technology Project (20NYYF0021)supported by the Open Project Program of Beijing Key Laboratory of Flavor Chemistry, Beijing Technology and Business University (BTBU), Beijing 100048, China (SPFW2020YB12)
文摘P omegranate(Punica granatum L.)has attracted considerable attention in world markets due to its valuable nutrients and highly appreciated sensory properties.The aroma profiles of 4 varieties of pomegranate juice,including Dahongtian(DP),Jingpitian(JP),Luyudan(LP),and Tianhonngdan(TP),were investigated via gas chromatography-mass spectrometry(GC-MS)and gas chromatography-olfactometry(GC-O)analyses.A total of 43 volatile compounds were identified by using GC-MS.Among these compounds,16 were considered as potential aroma-active compounds as detected by GC-O.These compounds belonged to the classes of terpinenes,alcohols,and aldehydes.Eleven volatile compounds were defined as the main contributors to the overall aroma of pomegranate juice due to their high odor activity values(OAVs≥1).Aroma recombination and omission tests confirmed thatβ-myrcene,1-hexanol,and(Z)-3-hexen-1-ol were the key aroma compounds,and limonene,1-octen-3-ol,linalool,and hexanal were important aroma-active compounds in DP samples.
基金financially supported by the National Key Technology R&D Program of China (No.2006BAC06B04,2008BAJ08B13)
文摘Three treatments were tested to investigate the release concentrations of volatile organic compounds （VOCs） during the bio-drying of municipal solid waste （MSW） by the aerobic and combined hydrolytic-aerobic processes.Results showed that VOCs were largely released in the first 4 days of bio-drying and the dominant components were：dimethyl disulfide,dimethyl sulfide,benzene,2-butanone,limonene and methylene chloride.Thus,the combined hydrolytic-aerobic process was suggested for MSW bio-drying due to fewer aeration quantities in this phase when compared with the aerobic process,and the treatment strategies should base on the key properties of these prominent components.Malodorous sulfur compounds and terpenes were mainly released in the early phase of bio-drying,whereas,two peaks of release concentrations appeared for aromatics and ketones during bio-drying.Notably,for the combined hydrolytic-aerobic processes there were also high concentrations of released aromatics in the shift from hydrolytic to aerobic stages.High concentrations of released chlorinateds were observed in the later phase.For the VOCs produced during MSW bio-drying,i.e.,malodorous sulfur compounds,terpenes and chlorinateds,their release concentrations were mainly determined by production rates;for the VOCs presented initially in MSW,such as aromatics,their transfer and transport in MSW mainly determined the release concentrations.
基金Supported by National Institute of Health GrantsNo.P30 CA015083+2 种基金No.U01 CA182940No.U54 CA163004Kathy and Russ Van Cleve Endowment for Gastroenterology Research(all to Wang KK)
文摘Volatile organic compounds(VOCs) emitted from stool are the components of the smell of stool representing the end products of microbial activity and metabolism that can be used to diagnose disease. Despite the abundance of hydrogen, carbon dioxide, and methane that have already been identified in human flatus, the small portion of trace gases making up the VOCs emitted from stool include organic acids, alcohols, esters, heterocyclic compounds, aldehydes, ketones, and alkanes, among others. These are the gases that vary among individuals in sickness and in health, in dietary changes, and in gut microbial activity. Electronic nose devices are analytical and pattern recognition platforms that can utilize mass spectrometry or electrochemical sensors to detect these VOCs in gas samples. When paired with machine-learning and pattern recognition algorithms, this can identify patterns of VOCs, and thus patterns of smell, that can be used to identify disease states. In this review, we provide a clinical background of VOC identification, electronic nose development, and review gastroenterology applications toward diagnosing disease by the volatile headspace analysis of stool.
基金support of this research program from the Jeonnam Green Environment Center (JNGEC),Korea
文摘In this study, the amounts of odorous carbonyl compounds （OCCs） including acetaldehyde （Acet-A）, propionaldehyde （Pron-A）, butylaldehyde （Buty-A）, iso-valeric aldehyde （Iso-Vale-A） and n-valeric aldehyde （N-Vale-A） emitted from a fishery industrial complex near the exhibition facilities of ＂Expo 2012 Yeosu Korea＂ were measured. Acet-A was found to be the most abundant OCC, and the total concentrations of the OCCs were the highest in the summer. However, due to vehicular exhaust and photochemical reactions, the concentrations of some of the OCCs presented their highest levels in the fall. A significant correlation between Acet-A and Buty-A was found at the major fishery facilities （r = 0.816, p = 1.87E-15, n = 60） and at the border areas （r = 0.809, p = 3.40E-12, n = 48） of this fishery industrial complex. The concentrations of OCCs at the border areas were not worse than those at the urban areas in other places, indicating that the concentrations of ambient OCCs at the border areas were not greatly influenced by manmade activities.
基金supported by the National Research Foundation,Singaporeprogram number NRF-CRP5-2009-02,for the School of Civil and Environmental Engineering/Residues and Resource Reclamation Centre,Nanyang Technological University,Singapore
文摘Source separation sanitation systems have attracted more and more attention recently.However, separate urine collection and treatment could induce odor issues, especially in large scale application. In order to avoid such issues, it is necessary to monitor the odor related compounds that might be generated during urine storage. This study investigated the odorous compounds that emitted from source-separated human urine under different hydrolysis conditions. Batch experiments were conducted to investigate the effect of temperature, stale/fresh urine ratio and urine dilution on odor emissions. It was found that ammonia, dimethyl disulfide, allyl methyl sulfide and 4-heptanone were the main odorous compounds generated from human urine, with headspace concentrations hundreds of times higher than their respective odor thresholds. Furthermore, the high temperature accelerated urine hydrolysis and liquid–gas mass transfer, resulting a remarkable increase of odor emissions from the urine solution. The addition of stale urine enhanced urine hydrolysis and expedited odor emissions. On the contrary, diluted urine emitted less odorous compounds ascribed to reduced concentrations of odorant precursors. In addition,this study quantified the odor emissions and revealed the constraints of urine source separation in real-world applications. To address the odor issue, several control strategies are recommended for odor mitigation or elimination from an engineering perspective.
