ITO (indium oxide doped with tin) thin films were deposited on glass substrates by using ITO pellet with a composition of w(In2O3)=90% and w(SnO2)=10% by electron beam evaporated with End-Hall ion source assiste...ITO (indium oxide doped with tin) thin films were deposited on glass substrates by using ITO pellet with a composition of w(In2O3)=90% and w(SnO2)=10% by electron beam evaporated with End-Hall ion source assisted without extra heating. The rate of deposition and flow rate of oxygen were measured and changed to obtain the best properties of ITO thin films. Furthermore, the post annealing process was done in vacuum at different annealing temperatures for 2 h and at 400℃ for different keeping time, respectively. The relation between optical, electrical properties and structure was discussed in detail.展开更多
A magnetic field produced by a current flowing through the plasma grid(PG) is one of the solutions to reduce the collisional loss of negative ions in a negative ion source, which reduces the electron temperature in fr...A magnetic field produced by a current flowing through the plasma grid(PG) is one of the solutions to reduce the collisional loss of negative ions in a negative ion source, which reduces the electron temperature in front of the PG. However, the magnetic field diffused into the driver has some influence on the plasma outflowing. In order to investigate the effect of changing this magnetic field on the outflowing of plasma from the driver, a circular ring(absorber) of high permeability iron has been introduced at the driver exit, which can reduce the magnetic field around it and improve plasma outflowing. With the application of the absorber, the electron density is increased by about 35%, and the extraction current measured from the extraction grid is increased from 1.02 A to 1.29 A. The results of the extraction experiment with cesium injection show that both the extraction grid(EG) current and H-current are increased when the absorber is introduced.展开更多
A new electron impact storage ion source has been designed for time of flight mass spectrometers with a high mass resolving power and high sensitivity. Because of the storage and compressing focus of the source, the o...A new electron impact storage ion source has been designed for time of flight mass spectrometers with a high mass resolving power and high sensitivity. Because of the storage and compressing focus of the source, the overall performance of the instrument has been improved greatly with a mass resolving power up to 3 500. The conditions of the second order of the focus are given and the storage ability is proved. The competer simulations and experiment results are given, too.展开更多
Neutral beam injection is one of the main plasma heating methods in nuclear fusion devices. In order to support the scientific study of the Experimental Advanced Superconducting Tokamak (EAST), a megawatt-level high...Neutral beam injection is one of the main plasma heating methods in nuclear fusion devices. In order to support the scientific study of the Experimental Advanced Superconducting Tokamak (EAST), a megawatt-level high current ion source is designed and manufactured in the ASIPP, and the progress and preliminary test results will be presented in this paper.展开更多
Long pulse operation of high power ion source is the requirement of fusion science research on neutral beam injector. A breakdown of accelerator column is drastically increased when operating with high beam energy and...Long pulse operation of high power ion source is the requirement of fusion science research on neutral beam injector. A breakdown of accelerator column is drastically increased when operating with high beam energy and long beam duration. To extend the pulse length, which was stopped with every breakdown so far, the beam re-starting technology was developed and utilized. As a result, the voltage drop of every power supply due to breakdown was recovered within a time of 90 ms and beam pulse length was extended much longer than the case before this improvement. The details of the beam re-starting technology and the preliminary results were presented in this manuscript.展开更多
A simple negative ion mobility spectrometer (IMS) is designed and used to investi- gate the factors that influence the number and efficiency of electrons generated by the needle-ring pulsed corona discharge electron...A simple negative ion mobility spectrometer (IMS) is designed and used to investi- gate the factors that influence the number and efficiency of electrons generated by the needle-ring pulsed corona discharge electron source. Simulation with Ansoft Maxwell 12 is carried out to analyze the electric field distribution within the IMS, and to offer the basis and foundation for analyzing the measurement results. The measurement results of the quantities of electrons show that when the drift electric field strength and the ring inner diameter rise, both the number of ef- fective electrons and the effective electron rate are increased. When the discharge voltage becomes stronger, the number of effective electrons goes up while the effective electron rate goes down. In light of the simulation results, mechanisms underlying the effects of drift electric field strength, ring inner diameter, and discharge voltage on the effective electron number and effective electron rate are discussed. These will make great sense for designing negative ion mode IMS using the needle-ring pulsed corona discharge as the electron source.展开更多
In order to study the key technology and physics of RF driven negative ion source for neutral beam injector in China, the Hefei utility negative ions test equipment with RF source was developed at Institute of Plasma ...In order to study the key technology and physics of RF driven negative ion source for neutral beam injector in China, the Hefei utility negative ions test equipment with RF source was developed at Institute of Plasma Physics, Chinese Academy of Sciences(ASIPP). Its negative ion source can be equipped with single or double RF drivers. There is a plasma expansion chamber with depth of 19 mm and an enhanced filter field. A three electrodes negative ion accelerator was employed to extract and accelerate the negative ions, which are plasma grid,extraction grid and ground grid. And there are several diagnostic tools for the plasma and beam parameters measurement. The characteristics of plasma generation, negative ion production and extraction were studied on the test equipment. The negative ion beam was extracted from the RF driven negative ion source for the first time. The detailed structure and main results are presented in this article.展开更多
As the key ion source component of nuclear fusion auxiliary heating devices, the radio frequency (RF) ion source is developed and applied gradually to offer a source plasma with the advantages of ease of control and...As the key ion source component of nuclear fusion auxiliary heating devices, the radio frequency (RF) ion source is developed and applied gradually to offer a source plasma with the advantages of ease of control and high reliability. In addition, it easily achieves long-pulse steady-state operation. During the process of the development and testing of the RF ion source, a lot of original experimental data will be generated. Therefore, it is necessary to develop a stable and reliable computer data acquisition and processing application system for realizing the functions of data acquisition, storage, access, and real-time monitoring. In this paper, the development of a data acquisition and processing application system for the RF ion source is presented. The hardware platform is based on the PXI system and the software is programmed on the LabVIEW development environment. The key technologies that are used for the implementation of this software programming mainly include the long-pulse data acquisition technology, multi- threading processing technology, transmission control communication protocol, and the Lempel-Ziv-Oberhumer data compression algorithm. Now, this design has been tested and applied on the RF ion source. The test results show that it can work reliably and steadily. With the help of this design, the stable plasma discharge data of the RF ion source are collected, stored, accessed, and monitored in real-time. It is shown that it has a very practical application significance for the RF experiments.展开更多
An experiment facility has been set up for the study of metal cluster compounds in our laboratory, which consists of a nano-electrospray ionization source, an ion transmission and focus system, and a reflectron time-o...An experiment facility has been set up for the study of metal cluster compounds in our laboratory, which consists of a nano-electrospray ionization source, an ion transmission and focus system, and a reflectron time-of-fight mass spectrometer. Taking advantage of the nano-electrospray ionization source, polyvalent ions are usually produced in the "ionization" process and the obtained mass resolution of the equipment is over 8000. The molecular ion peaks of metal cluster compounds [Au20(PPhpy2)10Cl2](SbF6)4, where PPhpy2=bis(2- pyridyl)phenylphosphine, and [AuaAg2(C)L6](BF4)4, where L=2-(diphenylphosphino)-5- methylpyridine, are distinguished in the respective mass spectrum, accompanied by some fragment ion peaks. In addition, the mass-to-charge ratios of the parent ions are determi- nated. Preliminary results suggest that the device is a powerful tool for the study of metal cluster compounds. It turns out that the information obtained by the instrumentation serves as an essential supplement to single crystal X-ray diffraction for structure characterization of metal cluster compounds.展开更多
[Objective] The present study was conducted to explore the effects of dif- ferent nitrogen sources and metal ions on the biogas production process and biogas yield by fermentation of corn stalk powder using self-desig...[Objective] The present study was conducted to explore the effects of dif- ferent nitrogen sources and metal ions on the biogas production process and biogas yield by fermentation of corn stalk powder using self-designed anaerobic fermenta- tion system. [Method] The biogas produced during fermentation was collected by water displacement, and measured by ignition. [Result] Ammonium bicarbonate, urea and yeast extract powder all increased biogas yield. Among them, ammonium bi- carbonate was the best nitrogen source. Ammonium dihydrogen phosphate showed an inhibitory effect on biogas production. Biogas yield was significantly increased by adding NaCl, KCl, MgCl2 or CaCl2, among which, NaCl had the best effect. [Conclu- sion] It is not conducive to the growth and development of methanogenic flora in the production of biogas using corn stalks as the only material in fermentation. The biogas yield can be increased by adding exogenous nitrogen, which reduces the carbon to nitrogen (C:N) ratio of fermentation materials. The biogas yield can be significantly increased by adding appropriate types and amount of electrolytes, with appropriate C:N ratio. The methanogenic flora is more tolerant to NaCl and KCl than to MgCl2 and CaCl2. Moreover, NaCl can not only significantly increase the biogas production, but also shorten startup period of methanogenic flora, thereby shortening the gas producing cycle.展开更多
Collinear laser spectroscopy is a powerful tool for studying the nuclear spins,electromagnetic moments,and charge radii of exotic nuclei.To study the nuclear properties of unstable nuclei at the Beijing Radioactive Io...Collinear laser spectroscopy is a powerful tool for studying the nuclear spins,electromagnetic moments,and charge radii of exotic nuclei.To study the nuclear properties of unstable nuclei at the Beijing Radioactive Ion-beam Facility(BRIF)and the future High Intensity Heavy-ion Accelerator Facility(HIAF),we developed a collinear laser spectroscopy apparatus integrated with an offline laser ablation ion source and a laser system.The overall performance of this state-of-the-art technique was evaluated,and the system was commissioned using a bunched stable ion beam.The high-resolution optical spectra for the 4s ^(2)S_(1/2)→4p^(2)P_(3/2)(D2)ionic transition of ^(40;42;44;48)Ca isotopes were successfully measured.The extracted isotope shifts relative to ^(40)Ca showed excellent agreement with the literature values.This system is now ready for use at radioactive ion beam facilities such as the BRIF and paves the way for the further development of higher-sensitivity collinear resonance ionization spectroscopy techniques.展开更多
The ion source of the electron cyclotron resonance ion thruster (ECRIT) extracts ions from its ECR plasma to generate thrust, and has the property of low gas consumption (2 seem, standard-state cubic centimeter per...The ion source of the electron cyclotron resonance ion thruster (ECRIT) extracts ions from its ECR plasma to generate thrust, and has the property of low gas consumption (2 seem, standard-state cubic centimeter per minute) and high durability. Due to the indispensable effects of the primary electron in gas discharge, it is important to experimentally clarify the electron energy structure within the ion source of the ECRIT through analyzing the electron energy distribution function (EEDF) of the plasma inside the thruster. In this article the Langmuir probe diagnosing method was used to diagnose the EEDF, from which the effective electron temperature, plasma density and the electron energy probability function (EEPF) were deduced. The experimental results show that the magnetic field influences the curves of EEDF and EEPF and make the effective plasma parameter nonuniform. The diagnosed electron temperature and density from sample points increased from 4 eV/2 ×10^16 m-3 to 10 eV/4×10^16 m-3 with increasing distances from both the axis and the screen grid of the ion source. Electron temperature and density peaking near the wall coincided with the discharge process. However, a double Maxwellian electron distribution was unexpectedly observed at the position near the axis of the ion source and about 30 mm from the screen grid. Besides, the double Maxwellian electron distribution was more likely to emerge at high power and a low gas flow rate. These phenomena were believed to relate to the arrangements of the gas inlets and the magnetic field where the double Maxwellian electron distribution exits. The results of this research may enhance the understanding of the plasma generation process in the ion source of this type and help to improve its performance.展开更多
The proposed heavy ion inertial fusion(HIF)scenarios require ampere class low charge state ion beams of heavy species.The laser ion source(LIS)is recognized as one of the promising candidates of ion beam providers,sin...The proposed heavy ion inertial fusion(HIF)scenarios require ampere class low charge state ion beams of heavy species.The laser ion source(LIS)is recognized as one of the promising candidates of ion beam providers,since it can deliver high brightness heavy ion beams to accelerators.The design of LIS for the HIF depends on the accelerator structure and accelerator complex following the source.In this article,we discuss the specifications and design of an appropriate LIS assuming two major types of the accelerators:radio frequency(RF)high quality factor cavity type and non-resonant induction core type.We believe that a properly designed LIS would satisfy the requirements of both types,while some issues need to be verified experimentally.展开更多
Parameters of hydrogen plasma in a miniature Penning discharge ion source, including the electron temperature and the electron density, were measured by using double probes. The results indicate that the electron dens...Parameters of hydrogen plasma in a miniature Penning discharge ion source, including the electron temperature and the electron density, were measured by using double probes. The results indicate that the electron density increases and the electron temperature decreases with the increase in gas pressure and the discharge current. The electron temperature is about 5 - 9 eV and the electron density is 6.0× 10^13 ~ 1.2 × 10^14 m^-3 while the discharge current is in a range of 50 - 120 μA.展开更多
A practical 2.45-GHz microwave-driven Cs-free H^- source was improved based on the experimental H^- source at Peking University(PKU). Several structural improvements were implemented to meet the practical requiremen...A practical 2.45-GHz microwave-driven Cs-free H^- source was improved based on the experimental H^- source at Peking University(PKU). Several structural improvements were implemented to meet the practical requirements of Xi'an Proton Application Facility(XiPaf). Firstly, the plasma chamber size was optimized to enhance the plasma intensity and stability. Secondly, the filter magnetic field and electron deflecting magnetic field were enhanced to reduce co-extracted electrons. Thirdly, a new two-electrode extraction system with farther electrode gap and enhanced water cooling ability to diminish spark and sputter during beam extraction was applied. At last, the direct H^- current measuring method was adopted by the arrangement of a new pair of bending magnets before Faraday cup(FC) to remove residual electrons. With these improvements, electron cyclotron resonance(ECR) magnetic field optimization experiments and operation parameter variation experiments were carried out on the H^- ion source and a maximum 8.5-mA pure H^- beam was extracted at 50 kV with the time structure of 100 Hz/0.3 ms. The root-mean-square(RMS) emittance of the beam is 0.25 Π·mm·mrad. This improved H^- source and extraction system were maintenance-free for more than 200 hours in operation.展开更多
The bond length of ^4HeH^+ resulting from collision-induced destruction is measured at 1.4420 MeV using the Coulomb Explosion Technique. The measured bond length of ^4HeH^+ is 0.094±0.003nm. The bond length of ...The bond length of ^4HeH^+ resulting from collision-induced destruction is measured at 1.4420 MeV using the Coulomb Explosion Technique. The measured bond length of ^4HeH^+ is 0.094±0.003nm. The bond length of ^4HeH^+ obtained with our radio frequency (RF) ion source is larger than that obtained with a duoplasmatron ion source at Argonne National Laboratory (ANL), but the bond lengths of H^+2 and H^+3obtained separately by ANL and by us with the two different ion sources are consistent with each other, which implies that there exists an ion source effect on the bond length of ^4HeH^+. The main reason why the 4^4HeH^+ bond lengths obtained by the two different ion sources are different is also discussed.展开更多
An electron cyclotron resonance ion source model that uses a coaxial antenna to inject the RF power was simulated, and the corresponding hydrogen plasma densities of the ion source were calculated at different magneti...An electron cyclotron resonance ion source model that uses a coaxial antenna to inject the RF power was simulated, and the corresponding hydrogen plasma densities of the ion source were calculated at different magnetic field distributions via a fluid model. The results show that most of the microwave power is absorbed around the resonance surface near the antenna when the plasma density is below the cutoff density of 7.4 × 10^(16) m^(-3) for 2.45 GHz microwaves, and the simulation results also show that the plasma density is strongly influenced by the position and shape of the resonance surface, where a larger resonance surface would improve the plasma density.展开更多
Through diagnosing the plasma density and calculating the intensity of microwave electric field,four 10 cm electron cyclotron resonance(ECR)ion sources with different magnetic field structures are studied to reveal th...Through diagnosing the plasma density and calculating the intensity of microwave electric field,four 10 cm electron cyclotron resonance(ECR)ion sources with different magnetic field structures are studied to reveal the inside interaction between the plasma,magnetic field and microwave electric field.From the diagnosing result it can be found that the plasma density distribution is controlled by the plasma generation and electron loss volumes associated with the magnetic field and microwave power level.Based on the cold plasma hypothesis and diagnosing result,the microwave electric field intensity distribution in the plasma is calculated.The result shows that the plasma will significantly change the distribution of the microwave electric field intensity to form a bow shape.From the boundary region of the shape to the center,the electric field intensity varies from higher to lower and the diagnosed density inversely changes.If the bow and its inside lower electric field intensity region are close to the screen grid,the performance of ion beam extracting will be better.The study can provide useful information for the creating of 10 cm ECR ion source and understanding its mechanism.展开更多
The arc regulation method is applied to the high-current ion source for high-power hydrogen ion beam extraction for the first time. The characteristics of the arc and beam, including the probe ion saturation current, ...The arc regulation method is applied to the high-current ion source for high-power hydrogen ion beam extraction for the first time. The characteristics of the arc and beam, including the probe ion saturation current, the arc power and the beam current, are studied with feedback control. The results show that the arc regulation method can be successfully applied to ion beam extraction. This lays a sound foundation for the testing of a new ion source and the operation of a conditioned ion source for neutral beam injector devices.展开更多
An ionic liquid ion source(ILIS)is a kind of high brightness ion source capable of providing high-speed positive or negative ion beams.This paper presents a miniaturized ILIS based on an array of porous metal strips.T...An ionic liquid ion source(ILIS)is a kind of high brightness ion source capable of providing high-speed positive or negative ion beams.This paper presents a miniaturized ILIS based on an array of porous metal strips.The porous emitter array,integrated with seven 10 mm long strips,is fabricated using wire electrical discharge machining(WEDM)combined with electrochemical etching.The assembled ILIS is 30 mm×30 mm×17.5 mm in size and weighs less than 25 g.A series of experiments,including anⅠ-Ⅴcharacteristic test,a retarding potential analyzer(RPA)test,and a spatial plume distribution test,have been conducted in vacuo to characterize the performance of the ILIS.Results show that the emitted current is up to about 800μA and ion transparency is as high as 94%.Besides,RPA curves reveal that the total fragmentation rate of the emitted particles accounts for 48.8%in positive mode and 59.8%in negative mode.Further,with the increase in applied acceleration voltage,the voltage loss rises while the energy efficiency decreases.It is also found that the plume perpendicular to the strips has a higher divergence than the one parallel to the strips.A numerical simulation by COMSOL reveals that the electric field distribution between the two electrodes results in such a spatial plume profile.展开更多
文摘ITO (indium oxide doped with tin) thin films were deposited on glass substrates by using ITO pellet with a composition of w(In2O3)=90% and w(SnO2)=10% by electron beam evaporated with End-Hall ion source assisted without extra heating. The rate of deposition and flow rate of oxygen were measured and changed to obtain the best properties of ITO thin films. Furthermore, the post annealing process was done in vacuum at different annealing temperatures for 2 h and at 400℃ for different keeping time, respectively. The relation between optical, electrical properties and structure was discussed in detail.
基金supported by the Comprehensive Research Facility for Fusion Technology Program of China(No.2018-000052-73-01-001228)National Natural Science Foundation of China(No.11975264)。
文摘A magnetic field produced by a current flowing through the plasma grid(PG) is one of the solutions to reduce the collisional loss of negative ions in a negative ion source, which reduces the electron temperature in front of the PG. However, the magnetic field diffused into the driver has some influence on the plasma outflowing. In order to investigate the effect of changing this magnetic field on the outflowing of plasma from the driver, a circular ring(absorber) of high permeability iron has been introduced at the driver exit, which can reduce the magnetic field around it and improve plasma outflowing. With the application of the absorber, the electron density is increased by about 35%, and the extraction current measured from the extraction grid is increased from 1.02 A to 1.29 A. The results of the extraction experiment with cesium injection show that both the extraction grid(EG) current and H-current are increased when the absorber is introduced.
文摘A new electron impact storage ion source has been designed for time of flight mass spectrometers with a high mass resolving power and high sensitivity. Because of the storage and compressing focus of the source, the overall performance of the instrument has been improved greatly with a mass resolving power up to 3 500. The conditions of the second order of the focus are given and the storage ability is proved. The competer simulations and experiment results are given, too.
基金supported by National Natural Science Foundation of China (Nos.10875146,11075183)the Knowledge Innovation Program of the Chinese Academy of Sciences (study of the physical characteristic of arc power feedback control for the high current ion source)
文摘Neutral beam injection is one of the main plasma heating methods in nuclear fusion devices. In order to support the scientific study of the Experimental Advanced Superconducting Tokamak (EAST), a megawatt-level high current ion source is designed and manufactured in the ASIPP, and the progress and preliminary test results will be presented in this paper.
基金supported by National Natural Science Foundation of China(Nos.11675215,11575240)the Key Program of Research and Development of Hefei Science Center,CAS(No.2016HSC-KPRD002)the National Key R&D Program of China(No.2017YFE300101)
文摘Long pulse operation of high power ion source is the requirement of fusion science research on neutral beam injector. A breakdown of accelerator column is drastically increased when operating with high beam energy and long beam duration. To extend the pulse length, which was stopped with every breakdown so far, the beam re-starting technology was developed and utilized. As a result, the voltage drop of every power supply due to breakdown was recovered within a time of 90 ms and beam pulse length was extended much longer than the case before this improvement. The details of the beam re-starting technology and the preliminary results were presented in this manuscript.
基金supported by National Natural Science Foundation of China(No.51077062)
文摘A simple negative ion mobility spectrometer (IMS) is designed and used to investi- gate the factors that influence the number and efficiency of electrons generated by the needle-ring pulsed corona discharge electron source. Simulation with Ansoft Maxwell 12 is carried out to analyze the electric field distribution within the IMS, and to offer the basis and foundation for analyzing the measurement results. The measurement results of the quantities of electrons show that when the drift electric field strength and the ring inner diameter rise, both the number of ef- fective electrons and the effective electron rate are increased. When the discharge voltage becomes stronger, the number of effective electrons goes up while the effective electron rate goes down. In light of the simulation results, mechanisms underlying the effects of drift electric field strength, ring inner diameter, and discharge voltage on the effective electron number and effective electron rate are discussed. These will make great sense for designing negative ion mode IMS using the needle-ring pulsed corona discharge as the electron source.
基金supported by the Key Program of Research and Development of Hefei Science Center,CAS(No.2016HSCKPRD002)National Natural Science Foundation of China(Nos.11505224,11505225,11575240,11675215,11675216)
文摘In order to study the key technology and physics of RF driven negative ion source for neutral beam injector in China, the Hefei utility negative ions test equipment with RF source was developed at Institute of Plasma Physics, Chinese Academy of Sciences(ASIPP). Its negative ion source can be equipped with single or double RF drivers. There is a plasma expansion chamber with depth of 19 mm and an enhanced filter field. A three electrodes negative ion accelerator was employed to extract and accelerate the negative ions, which are plasma grid,extraction grid and ground grid. And there are several diagnostic tools for the plasma and beam parameters measurement. The characteristics of plasma generation, negative ion production and extraction were studied on the test equipment. The negative ion beam was extracted from the RF driven negative ion source for the first time. The detailed structure and main results are presented in this article.
基金the NBI team and the partial support of National Natural Science Foundation of China (No. 61363019)National Natural Science Foundation of Qinghai Province (No. 2014-ZJ-718)
文摘As the key ion source component of nuclear fusion auxiliary heating devices, the radio frequency (RF) ion source is developed and applied gradually to offer a source plasma with the advantages of ease of control and high reliability. In addition, it easily achieves long-pulse steady-state operation. During the process of the development and testing of the RF ion source, a lot of original experimental data will be generated. Therefore, it is necessary to develop a stable and reliable computer data acquisition and processing application system for realizing the functions of data acquisition, storage, access, and real-time monitoring. In this paper, the development of a data acquisition and processing application system for the RF ion source is presented. The hardware platform is based on the PXI system and the software is programmed on the LabVIEW development environment. The key technologies that are used for the implementation of this software programming mainly include the long-pulse data acquisition technology, multi- threading processing technology, transmission control communication protocol, and the Lempel-Ziv-Oberhumer data compression algorithm. Now, this design has been tested and applied on the RF ion source. The test results show that it can work reliably and steadily. With the help of this design, the stable plasma discharge data of the RF ion source are collected, stored, accessed, and monitored in real-time. It is shown that it has a very practical application significance for the RF experiments.
文摘An experiment facility has been set up for the study of metal cluster compounds in our laboratory, which consists of a nano-electrospray ionization source, an ion transmission and focus system, and a reflectron time-of-fight mass spectrometer. Taking advantage of the nano-electrospray ionization source, polyvalent ions are usually produced in the "ionization" process and the obtained mass resolution of the equipment is over 8000. The molecular ion peaks of metal cluster compounds [Au20(PPhpy2)10Cl2](SbF6)4, where PPhpy2=bis(2- pyridyl)phenylphosphine, and [AuaAg2(C)L6](BF4)4, where L=2-(diphenylphosphino)-5- methylpyridine, are distinguished in the respective mass spectrum, accompanied by some fragment ion peaks. In addition, the mass-to-charge ratios of the parent ions are determi- nated. Preliminary results suggest that the device is a powerful tool for the study of metal cluster compounds. It turns out that the information obtained by the instrumentation serves as an essential supplement to single crystal X-ray diffraction for structure characterization of metal cluster compounds.
基金Supported by Innovation and Entrepreneurship Training Program for Undergraduates of Yanbian University (ydbksky2015216)~~
文摘[Objective] The present study was conducted to explore the effects of dif- ferent nitrogen sources and metal ions on the biogas production process and biogas yield by fermentation of corn stalk powder using self-designed anaerobic fermenta- tion system. [Method] The biogas produced during fermentation was collected by water displacement, and measured by ignition. [Result] Ammonium bicarbonate, urea and yeast extract powder all increased biogas yield. Among them, ammonium bi- carbonate was the best nitrogen source. Ammonium dihydrogen phosphate showed an inhibitory effect on biogas production. Biogas yield was significantly increased by adding NaCl, KCl, MgCl2 or CaCl2, among which, NaCl had the best effect. [Conclu- sion] It is not conducive to the growth and development of methanogenic flora in the production of biogas using corn stalks as the only material in fermentation. The biogas yield can be increased by adding exogenous nitrogen, which reduces the carbon to nitrogen (C:N) ratio of fermentation materials. The biogas yield can be significantly increased by adding appropriate types and amount of electrolytes, with appropriate C:N ratio. The methanogenic flora is more tolerant to NaCl and KCl than to MgCl2 and CaCl2. Moreover, NaCl can not only significantly increase the biogas production, but also shorten startup period of methanogenic flora, thereby shortening the gas producing cycle.
基金supported by the National Natural Science Foundation of China(Nos.12027809,U1967201,11875073,11875074 and 11961141003)National Key R&D Program of China(No.2018YFA0404403)+1 种基金China National Nuclear Corporation(No.FA18000201)the State Key Laboratory of Nuclear Physics and Technology,Peking University(No.NPT2019ZZ02).
文摘Collinear laser spectroscopy is a powerful tool for studying the nuclear spins,electromagnetic moments,and charge radii of exotic nuclei.To study the nuclear properties of unstable nuclei at the Beijing Radioactive Ion-beam Facility(BRIF)and the future High Intensity Heavy-ion Accelerator Facility(HIAF),we developed a collinear laser spectroscopy apparatus integrated with an offline laser ablation ion source and a laser system.The overall performance of this state-of-the-art technique was evaluated,and the system was commissioned using a bunched stable ion beam.The high-resolution optical spectra for the 4s ^(2)S_(1/2)→4p^(2)P_(3/2)(D2)ionic transition of ^(40;42;44;48)Ca isotopes were successfully measured.The extracted isotope shifts relative to ^(40)Ca showed excellent agreement with the literature values.This system is now ready for use at radioactive ion beam facilities such as the BRIF and paves the way for the further development of higher-sensitivity collinear resonance ionization spectroscopy techniques.
基金supported by National Natural Science Foundation of China(No.11475137)
文摘The ion source of the electron cyclotron resonance ion thruster (ECRIT) extracts ions from its ECR plasma to generate thrust, and has the property of low gas consumption (2 seem, standard-state cubic centimeter per minute) and high durability. Due to the indispensable effects of the primary electron in gas discharge, it is important to experimentally clarify the electron energy structure within the ion source of the ECRIT through analyzing the electron energy distribution function (EEDF) of the plasma inside the thruster. In this article the Langmuir probe diagnosing method was used to diagnose the EEDF, from which the effective electron temperature, plasma density and the electron energy probability function (EEPF) were deduced. The experimental results show that the magnetic field influences the curves of EEDF and EEPF and make the effective plasma parameter nonuniform. The diagnosed electron temperature and density from sample points increased from 4 eV/2 ×10^16 m-3 to 10 eV/4×10^16 m-3 with increasing distances from both the axis and the screen grid of the ion source. Electron temperature and density peaking near the wall coincided with the discharge process. However, a double Maxwellian electron distribution was unexpectedly observed at the position near the axis of the ion source and about 30 mm from the screen grid. Besides, the double Maxwellian electron distribution was more likely to emerge at high power and a low gas flow rate. These phenomena were believed to relate to the arrangements of the gas inlets and the magnetic field where the double Maxwellian electron distribution exits. The results of this research may enhance the understanding of the plasma generation process in the ion source of this type and help to improve its performance.
基金This work was performed under contract DE-AC02-98CH1-886 with the auspices of the DoE and National Aeronautics and Space Administration.
文摘The proposed heavy ion inertial fusion(HIF)scenarios require ampere class low charge state ion beams of heavy species.The laser ion source(LIS)is recognized as one of the promising candidates of ion beam providers,since it can deliver high brightness heavy ion beams to accelerators.The design of LIS for the HIF depends on the accelerator structure and accelerator complex following the source.In this article,we discuss the specifications and design of an appropriate LIS assuming two major types of the accelerators:radio frequency(RF)high quality factor cavity type and non-resonant induction core type.We believe that a properly designed LIS would satisfy the requirements of both types,while some issues need to be verified experimentally.
文摘Parameters of hydrogen plasma in a miniature Penning discharge ion source, including the electron temperature and the electron density, were measured by using double probes. The results indicate that the electron density increases and the electron temperature decreases with the increase in gas pressure and the discharge current. The electron temperature is about 5 - 9 eV and the electron density is 6.0× 10^13 ~ 1.2 × 10^14 m^-3 while the discharge current is in a range of 50 - 120 μA.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11775007 and 11575013)
文摘A practical 2.45-GHz microwave-driven Cs-free H^- source was improved based on the experimental H^- source at Peking University(PKU). Several structural improvements were implemented to meet the practical requirements of Xi'an Proton Application Facility(XiPaf). Firstly, the plasma chamber size was optimized to enhance the plasma intensity and stability. Secondly, the filter magnetic field and electron deflecting magnetic field were enhanced to reduce co-extracted electrons. Thirdly, a new two-electrode extraction system with farther electrode gap and enhanced water cooling ability to diminish spark and sputter during beam extraction was applied. At last, the direct H^- current measuring method was adopted by the arrangement of a new pair of bending magnets before Faraday cup(FC) to remove residual electrons. With these improvements, electron cyclotron resonance(ECR) magnetic field optimization experiments and operation parameter variation experiments were carried out on the H^- ion source and a maximum 8.5-mA pure H^- beam was extracted at 50 kV with the time structure of 100 Hz/0.3 ms. The root-mean-square(RMS) emittance of the beam is 0.25 Π·mm·mrad. This improved H^- source and extraction system were maintenance-free for more than 200 hours in operation.
基金Project supported by the National Natural Science Foundation of China (Grant Nos 10175041 and 10375040).
文摘The bond length of ^4HeH^+ resulting from collision-induced destruction is measured at 1.4420 MeV using the Coulomb Explosion Technique. The measured bond length of ^4HeH^+ is 0.094±0.003nm. The bond length of ^4HeH^+ obtained with our radio frequency (RF) ion source is larger than that obtained with a duoplasmatron ion source at Argonne National Laboratory (ANL), but the bond lengths of H^+2 and H^+3obtained separately by ANL and by us with the two different ion sources are consistent with each other, which implies that there exists an ion source effect on the bond length of ^4HeH^+. The main reason why the 4^4HeH^+ bond lengths obtained by the two different ion sources are different is also discussed.
文摘An electron cyclotron resonance ion source model that uses a coaxial antenna to inject the RF power was simulated, and the corresponding hydrogen plasma densities of the ion source were calculated at different magnetic field distributions via a fluid model. The results show that most of the microwave power is absorbed around the resonance surface near the antenna when the plasma density is below the cutoff density of 7.4 × 10^(16) m^(-3) for 2.45 GHz microwaves, and the simulation results also show that the plasma density is strongly influenced by the position and shape of the resonance surface, where a larger resonance surface would improve the plasma density.
基金the National Natural Science Foundation of China(Grant No.11875222)。
文摘Through diagnosing the plasma density and calculating the intensity of microwave electric field,four 10 cm electron cyclotron resonance(ECR)ion sources with different magnetic field structures are studied to reveal the inside interaction between the plasma,magnetic field and microwave electric field.From the diagnosing result it can be found that the plasma density distribution is controlled by the plasma generation and electron loss volumes associated with the magnetic field and microwave power level.Based on the cold plasma hypothesis and diagnosing result,the microwave electric field intensity distribution in the plasma is calculated.The result shows that the plasma will significantly change the distribution of the microwave electric field intensity to form a bow shape.From the boundary region of the shape to the center,the electric field intensity varies from higher to lower and the diagnosed density inversely changes.If the bow and its inside lower electric field intensity region are close to the screen grid,the performance of ion beam extracting will be better.The study can provide useful information for the creating of 10 cm ECR ion source and understanding its mechanism.
基金supported by the National Magnetic Confinement Fusion Science Program of China(No.2013GB101000)partly supported by National Natural Science Foundation of China(No.11075183)the Knowledge Innovation Program of the Chinese Academy of Sciences(Study of the physical characteristics of arc power feedback control for the high current ion source)
文摘The arc regulation method is applied to the high-current ion source for high-power hydrogen ion beam extraction for the first time. The characteristics of the arc and beam, including the probe ion saturation current, the arc power and the beam current, are studied with feedback control. The results show that the arc regulation method can be successfully applied to ion beam extraction. This lays a sound foundation for the testing of a new ion source and the operation of a conditioned ion source for neutral beam injector devices.
基金supported by National Natural Science Foundation of China(No.52075334)。
文摘An ionic liquid ion source(ILIS)is a kind of high brightness ion source capable of providing high-speed positive or negative ion beams.This paper presents a miniaturized ILIS based on an array of porous metal strips.The porous emitter array,integrated with seven 10 mm long strips,is fabricated using wire electrical discharge machining(WEDM)combined with electrochemical etching.The assembled ILIS is 30 mm×30 mm×17.5 mm in size and weighs less than 25 g.A series of experiments,including anⅠ-Ⅴcharacteristic test,a retarding potential analyzer(RPA)test,and a spatial plume distribution test,have been conducted in vacuo to characterize the performance of the ILIS.Results show that the emitted current is up to about 800μA and ion transparency is as high as 94%.Besides,RPA curves reveal that the total fragmentation rate of the emitted particles accounts for 48.8%in positive mode and 59.8%in negative mode.Further,with the increase in applied acceleration voltage,the voltage loss rises while the energy efficiency decreases.It is also found that the plume perpendicular to the strips has a higher divergence than the one parallel to the strips.A numerical simulation by COMSOL reveals that the electric field distribution between the two electrodes results in such a spatial plume profile.