Atmospheric ammonia(NH_(3)) is a chemically active trace gas that plays an important role in the atmospheric environment and climate change. Satellite remote sensing is a powerful technique to monitor NH_(3) concentra...Atmospheric ammonia(NH_(3)) is a chemically active trace gas that plays an important role in the atmospheric environment and climate change. Satellite remote sensing is a powerful technique to monitor NH_(3) concentration based on the absorption lines of NH_(3) in the thermal infrared region. In this study, we establish a retrieval algorithm to derive the NH_(3)column from the Hyperspectral Infrared Atmospheric Sounder(HIRAS) onboard the Chinese Feng Yun(FY)-3D satellite and present the first atmospheric NH_(3) column global map observed by the HIRAS instrument. The HIRAS observations can well capture NH_(3) hotspots around the world, e.g., India, West Africa, and East China, where large NH_(3) emissions exist. The HIRAS NH_(3) columns are also compared to the space-based Infrared Atmospheric Sounding Interferometer(IASI)measurements, and we find that the two instruments observe a consistent NH_(3) global distribution, with correlation coefficient(R) values of 0.28–0.73. Finally, some remaining issues about the HIRAS NH_(3) retrieval are discussed.展开更多
文摘目前还没有基于国产卫星的1 km分辨率的全天候陆表温度(LST)产品,FY-3D卫星提供了中分辨率成像仪(MERSI)Ⅱ型1 km分辨率晴空LST产品与微波成像仪(MWRI)25 km全天候LST产品,因此可结合两者优势开展全天候1 km分辨率LST的融合研究。基于地理加权回归(GWR)方法,选择海拔、FY-3D归一化植被指数和归一化建筑指数等建立GWR模型对FY-3D/MWRI 25 km LST降尺度到1 km,并与MERSI 1 km LST进行融合;同时针对MWRI轨道间隙,利用前后1天融合后的云覆盖像元1 km LST进行补值,可以得到接近全天候下的1 km LST。基于以上融合算法,选择了中国区域多个典型日期FY-3D/MERSI和MWRI LST官网产品进行了融合试验,并利用公开发布的全天候1 km LST产品(TPDC LST)对FY-3D 1 km LST融合结果进行了评估。研究结果表明,基于GWR法的LST降尺度方法,可以有效避免传统微波LST降尺度方法中存在的“斑块”效应和局地温度偏低等问题;LST融合结果有值率从融合前的22.4%~36.9%可提高到融合后69.3%~80.7%,融合结果与TPDC LST的空间决定系数为0.503~0.787,均方根误差为3.6~5.8 K,其中晴空为2.6~4.9 K,云下为4.1~6.1 K;分析还表明目前官网产品FY-3D/MERSI和MWRI LST均存在缺值较多与精度偏低等问题,显示其存在较大改进潜力,这有利于进一步改进FY-3D LST融合质量。
基金supported by the Feng Yun Application Pioneering Project (FY-APP-2022.0502)the National Natural Science Foundation of China (Grant No. 42205140)。
文摘Atmospheric ammonia(NH_(3)) is a chemically active trace gas that plays an important role in the atmospheric environment and climate change. Satellite remote sensing is a powerful technique to monitor NH_(3) concentration based on the absorption lines of NH_(3) in the thermal infrared region. In this study, we establish a retrieval algorithm to derive the NH_(3)column from the Hyperspectral Infrared Atmospheric Sounder(HIRAS) onboard the Chinese Feng Yun(FY)-3D satellite and present the first atmospheric NH_(3) column global map observed by the HIRAS instrument. The HIRAS observations can well capture NH_(3) hotspots around the world, e.g., India, West Africa, and East China, where large NH_(3) emissions exist. The HIRAS NH_(3) columns are also compared to the space-based Infrared Atmospheric Sounding Interferometer(IASI)measurements, and we find that the two instruments observe a consistent NH_(3) global distribution, with correlation coefficient(R) values of 0.28–0.73. Finally, some remaining issues about the HIRAS NH_(3) retrieval are discussed.