Research on the underwater target scattering can provide important theoretical support for target detection. The scattering model of cylindrical shell is established in this paper. It is found that the forward target ...Research on the underwater target scattering can provide important theoretical support for target detection. The scattering model of cylindrical shell is established in this paper. It is found that the forward target strength is much stronger and varies with angles of incident wave less significantly than backward target strength. The received forward signal strength fluctuates with the target moving due to the interference between direct signal and scattering signal, which is most significant when the target approaches the baseline. An experiment is carried out in an anechoic tank to validate the scattering model. The method of acquisiting forward scattering in the tank is proposed. The forward and the backward target strengths are achieved by using the pulse compression technology, and they axe about 3dB less than the modeling results. The forward scattering phenomena of quiescent and moving targets are measured, which are similar to modeling results with different target types.展开更多
A new forward scattering bistatic radar motion compensation method based on spectral analysis and minimum waveform entropy is proposed. In order to demonstrate effectiveness of the presented method and ground vehicles...A new forward scattering bistatic radar motion compensation method based on spectral analysis and minimum waveform entropy is proposed. In order to demonstrate effectiveness of the presented method and ground vehicles imaging function of forward scattering radar, a simple bistatic forward scattering radar experiment system is set up on both sides of a road to collection ground vehicles experimental data. Finally, experimental ground vehicles imaging results confirm validity of the proposed motion compensation method and the experimental imaging results are identical with computer simulation results in the same parameter and condition.展开更多
A novel temperature and salinity discriminative sensing method based on forward Brillouin scattering(FBS)in 1060-XP single-mode fiber(SMF)is proposed.The measured frequency shifts corresponding to different radial aco...A novel temperature and salinity discriminative sensing method based on forward Brillouin scattering(FBS)in 1060-XP single-mode fiber(SMF)is proposed.The measured frequency shifts corresponding to different radial acoustic modes in 1060-XP SMF show different sensitivities to temperature and salinity.Based on the new phenomenon that different radial acoustic modes have different frequency shift-temperature and frequency shift-salinity coefficients,we propose a novel method for simultaneously measuring temperature and salinity by measuring the frequency shift changes of two FBS scattering peaks.In a proof-of-concept experiment,the temperature and salinity measurement errors are 0.12℃and 0.29%,respectively.The proposed method for simultaneously measuring temperature and salinity has the potential applications such as ocean surveying,food manufacturing and pharmaceutical engineering.展开更多
The application scope of the forward scatter radar(FSR)based on the Global Navigation Satellite System(GNSS)can be expanded by improving the detection capability.Firstly,the forward-scatter signal model when the targe...The application scope of the forward scatter radar(FSR)based on the Global Navigation Satellite System(GNSS)can be expanded by improving the detection capability.Firstly,the forward-scatter signal model when the target crosses the baseline is constructed.Then,the detection method of the for-ward-scatter signal based on the Rényi entropy of time-fre-quency distribution is proposed and the detection performance with different time-frequency distributions is compared.Simula-tion results show that the method based on the smooth pseudo Wigner-Ville distribution(SPWVD)can achieve the best perfor-mance.Next,combined with the geometry of FSR,the influence on detection performance of the relative distance between the target and the baseline is analyzed.Finally,the proposed method is validated by the anechoic chamber measurements and the results show that the detection ability has a 10 dB improvement compared with the common constant false alarm rate(CFAR)detection.展开更多
Forward scattering micro radar is used for situation awareness; its operational range is relatively short because of the battery power and local horizon, the free space propagation model is not appropriate. The ground...Forward scattering micro radar is used for situation awareness; its operational range is relatively short because of the battery power and local horizon, the free space propagation model is not appropriate. The ground moving targets, such as humans, cars and tanks, have only comparable size with the transmitted signal wavelength; the point target model and the linear change of observation angle are not applicable. In this paper, the signal model of ground moving target is developed based on the case of forward scattering micro radar, considering the two-ray propagation model and area target model, and nonlinear change of observation angle as well as high order phase error. Furthermore, the analytical form of the received power from moving target has been obtained. Using the simulated forward scattering radar cross section, the received power of theoretical calculation is near to that of measured data. In addition, the simulated signal model of ground moving target is perfectly matched with the experimented data. All these results show the correctness of analytical calculation completely.展开更多
The aberration in the received acoustic field and the Doppler shift in the forward scattered field are simultaneously induced when a submerged target crosses the source–receiver line. Formulations for the two variati...The aberration in the received acoustic field and the Doppler shift in the forward scattered field are simultaneously induced when a submerged target crosses the source–receiver line. Formulations for the two variations are developed upon an ideal forward scattering configuration. Both the field aberration and the Doppler shift are expressed as functions of the same argument — the target motion time. An experimental validation was carried out in a tank, in which the continuous wave was transmitted. The field aberration and the Doppler shift were extracted from the collected data by the simple Hilbert transform and a hybrid technique, respectively. The measured aberration and Doppler shift agree with the theoretical results.Simultaneous detection outputs are beneficial to enhance the reliability on target detection by providing both the aberrations in the received acoustic field and the Doppler shift in the forward scattered field.展开更多
We present the application of the theory of Pade approximants to extending the perturbative solutions of acoustic wave equation for a three dimensional vertically varying medium with one interface.These type of soluti...We present the application of the theory of Pade approximants to extending the perturbative solutions of acoustic wave equation for a three dimensional vertically varying medium with one interface.These type of solutions have limited convergence properties depending on either the degree of contrast between the actual and the reference medium or the angle of incidence of a plane wave component.We show that the sequence of Pade approximants to the partial sums in the forward scattering series for the 3D wave equation is convergent for any contrast and any incidence angle.This allows the construction of any reflected waves including phase-shifted post-critical plane waves and,for a point-source problem,refracted events or headwaves,and it also provides interesting interpretations of these solutions in the scattering theory formalism.展开更多
Distributed fiber sensors based on forward stimulated Brillouin scattering(F-SBS)have attracted special attention because of their capability to detect the acoustic impedance of liquid material outside fiber.However,t...Distributed fiber sensors based on forward stimulated Brillouin scattering(F-SBS)have attracted special attention because of their capability to detect the acoustic impedance of liquid material outside fiber.However,the reported results were based on the extraction of a 1st-order local spectrum,causing the sensing distance to be restricted by pump depletion.Here,a novel post-processing technique was proposed for distributed acoustic impedance sensing by extracting the 2nd-order local spectrum,which is beneficial for improving the sensing signal-to-noise ratio(SNR)significantly,since its pulse energy penetrates into the fiber more deeply.As a proof-of-concept,distributed acoustic impedance sensing along~1630 m fiber under moderate spatial resolution of~20 m was demonstrated.展开更多
I found that when the Debye theory calculates the far-field scattered light intensity of bubbles, the forward scattered light intensity is quite different from the result calculated by the Mie theory due to the conver...I found that when the Debye theory calculates the far-field scattered light intensity of bubbles, the forward scattered light intensity is quite different from the result calculated by the Mie theory due to the convergence problem, so the expression of the Debye coefficient has been revised. I derived the Debye reflectance and transmittance according to the physical meaning of Debye theory and compared them with Fresnel’s formula. I modified the Debye coefficient expressions for bubbles based on the differences between the Debye reflectance and transmittance from the Fresnel formula. Finally, compared with the far-field scattered light intensity calculated by the original Debye theory, the far-field scattered light intensity calculated based on the modified Debye coefficient can obtain more accurate forward scattered light intensity with fewer sub-waves.展开更多
The reaction dynamics of the fluorine atom with vibrationally excited D2(v=1, v=0) was investigated using the crossed beam method. The scheme of stimulated Raman pumping was employed for preparation of vibrationally e...The reaction dynamics of the fluorine atom with vibrationally excited D2(v=1, v=0) was investigated using the crossed beam method. The scheme of stimulated Raman pumping was employed for preparation of vibrationally excited D2 molecules. Contribution from the reaction of spin-orbit excited F*(2P1/2) with vibrationally excited D2 was not found. Reaction of spin-orbit ground F(2P3/2) with vibrationally excited D2 was measured and DF products populated in v'=2, 3, 4, 5 were observed. Compared with the vibrationally ground reaction, DF products from the vibrationally excited reaction of F(2P3/2)+D2(v=1, j=0) are rotationally “hotter”. Differential cross sections at four collision energies, ranging from 0.32 kcal/mol to 2.62 kcal/mol, were obtained. Backward scattering dominates for DF products in all vibrational levels at the lowest collision energy of 0.32 kcal/mol. As the collision energy increases, angular distribution of DF products gradually shifts from backward to sideway. The collision-energy dependence of differential cross section of DF(v’=5) at forward direction was also measured. Forward-scattered signal of DF(v'=5) appears at the collision energy of 1.0 kcal/mol, and becomes dominated at 2.62 kcal/mol.展开更多
The H+H2 reaction is the simplest chemical reaction system and has long been the prototype model in the study of reaction dynamics. Here we report a high resolution experimental investigation of the state-to-state rea...The H+H2 reaction is the simplest chemical reaction system and has long been the prototype model in the study of reaction dynamics. Here we report a high resolution experimental investigation of the state-to-state reaction dynamics in the H+HD→H2+D reaction by using the crossed molecular beams method and velocity map ion imaging technique at the collision energy of 1.17 eV. D atom products in this reaction were probed by the near threshold 1+1'(vacuum ultraviolet+ultraviolet) laser ionization scheme. The ion image with both high angular and energy resolution were acquired. State-to-state differential cross sections was accurately derived. Fast forward scattering oscillations, relating with interference effects in the scattering process, were clearly observed for H2 products at H2(v'=0,j'=1) and H2(v'=0,j'=3) rovibrational levels. This study further demonstrates the importance of measuring high-resolution differential cross sections in the study of state-to-state reaction dynamics in the gas phase.展开更多
We propose the trench-assisted multimode fiber(TA-OM4)as a novel sensing fiber in forward Brillouin scattering(FBS)-based temperature sensor,due to its higher temperature sensitivity,better bending resistance and lowe...We propose the trench-assisted multimode fiber(TA-OM4)as a novel sensing fiber in forward Brillouin scattering(FBS)-based temperature sensor,due to its higher temperature sensitivity,better bending resistance and lower propagation loss,compared with the single mode fiber(SMF)and other sensing fibers.The FBS effect and acousto-optic interaction in TA-OM4 are the first time to be demonstrated and characterized at 1550 nm theoretically and experimentally.A 2.0 km long TA-OM4 is put into an oven to measure its temperature sensitivity,which can reach up to 80.3 kHz/℃,exceeding 53%of SMF(52.4 kHz/℃).The simulated and experimental results verify that the TA-OM4 may be a good candidate as the sensing fiber for the FBS-based temperature sensor.展开更多
A new algorithm of the relaxation method is developed for the inversion of forward scattered light to obtain the size distribution of spherical particles. Numerical tests are performed for a laser particle analyzer us...A new algorithm of the relaxation method is developed for the inversion of forward scattered light to obtain the size distribution of spherical particles. Numerical tests are performed for a laser particle analyzer using the Mie theory and the diffraction approximation. The algorithm efficiency, in the presence of experimental noises, is studied. The results show that the technique is fast in convergence, stable against random noise and insensitive to the distribution of particles and the initial trial distribution.展开更多
The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unav...The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unavoidable in online measurements, we present in this work a multiple scattering calculation method, in which a layer model is employed. The three-dimensional particle system is divided into a pile of layers the number of which is automatically determined, depending on the obscuration of the particle system. The calculation is found to be fast, reasonable and reliable.展开更多
The basic principles of target detection by forward acoustic scattering are presented.A direct blast suppression approach based on adaptive filtering(DBS-AF) is proposed to suppress the direct blast.The DBS-AF techniq...The basic principles of target detection by forward acoustic scattering are presented.A direct blast suppression approach based on adaptive filtering(DBS-AF) is proposed to suppress the direct blast.The DBS-AF technique is extended to the linear frequency modulation(LFM) signal,where the envelope of the signal is regarded as a 'general waveform' and imported into the adaptive filter.Application of the DBS-AF method to the data collected from a lake trial yields an output detection curve,in which the direct blast is mapped to the background while the acoustic field aberration is represented by the peak value fluctuation.The inhibitory effect in single hydrophone is approximately- 5 dB,and is then enhanced by exploiting the mean value removal approach as a preprocessing technique.The direct blast is further suppressed to a level of-10 dB by making full use of multichannel receptions.The main factors affecting the algorithm performance are as follows:the fluctuation degree of the receptions during the weighting vector training period and the power ratio of the forward scattered wave to the direct blast when the target is present.展开更多
Transparent electrodes made of silver nanowires (Ag NWs) exhibit a higher flexibility than conventional indium tin oxide electrodes.For this reason,Ag NWs may find applications in future flexible electronic and opto...Transparent electrodes made of silver nanowires (Ag NWs) exhibit a higher flexibility than conventional indium tin oxide electrodes.For this reason,Ag NWs may find applications in future flexible electronic and optoelectronic devices.However,different optoelectronic devices have different specific requirements for Ag NWs.For example,the optical transmittance haze is an important but rarely studied aspect of Ag NW films.In this study,the optical transmittance and optical scattering of long (5-50 μm,L-NWs) and short (1-20 μm,S-NWs) Ag NW films were investigated.The L-NWs exhibited better optical transmission than the S-NWs,whereas the S-NWs exhibited better light-scattering properties than the L-NWs.Our results indicate that the L-NWs are suitable for touch-screen displays,whereas the S-NWs are better suited as transparent conductive films for solar cells.We analyzed the scattering ratio of forward-scattered light to backscattered light for both the L-NWs and S-NWs and discovered that the mesh size affected the scattering ratio.For longer wavelengths,a larger mesh yielded a higher backscattering ratio,whereas a smaller mesh yielded a lower backscattering ratio.We formulated an equation for calculating the reflection haze using the total reflection (Ag NWs/glass),R and the reflection of glass,R0.The reflection haze of the S-NWs and L-NWs exhibited different trends in the visible-near-infrared region.An omnidirectional scattering model for the Ag NWs was used to evaluate the Ag NW scattering properties.The results of this study have great significance for the evaluation of the performance of Ag NWs in optoelectronic devices.展开更多
In the field of geophysics,although the first-order Rytov approximation is widely used,the higher-order approximation is seldom discussed.From both theo-retical analysis and numerical tests,the accumulated phase error...In the field of geophysics,although the first-order Rytov approximation is widely used,the higher-order approximation is seldom discussed.From both theo-retical analysis and numerical tests,the accumulated phase error introduced in the first-order Rytov approximation cannot be neglected in the presence of strong velocity perturbation.In this paper,we are focused on improving the phase accuracy of forward scattered wavefield,especially for the large-scale and strong velocity pertur-bation case.We develop an equivalent source method which can update the imaginary part of the complex phase iteratively,and the higher-order scattered wavefield can be approximated by multiplying the incident wavefield by the exponent of the imaginary part of the complex phase.Although the convergence of the proposed method has not been proved mathematically,numerical examples demonstrate that our method can produce an improved accuracy for traveltime(phase)prediction,even for strong perturbation media.However,due to the neglect of the real part of the complex phase,the amplitude change of the scattered wavefield cannot be recovered.Furthermore,in the presence of multi-arrivals phenomenon,the equivalent scattering source should be handled carefully due to the multi-directions of the wavefield.Further investigations should be done to improve the applicability of the proposed method.展开更多
Forward-scattering efficiency (FSE) is first proposed when an Ag nanoparticle serves as the light-trapping structure for thin-film (TF) solar cells because the Ag nanoparticle’s light-trapping efficiency lies on ...Forward-scattering efficiency (FSE) is first proposed when an Ag nanoparticle serves as the light-trapping structure for thin-film (TF) solar cells because the Ag nanoparticle’s light-trapping efficiency lies on the light-scattering direction of metal nanoparticles.Based on FSE analysis of Ag nanoparticles with radii of 53 and 88 nm,the forward-scattering spectra and light-trapping efficiencies are calculated.The contributions of dipole and quadrupole modes to light-trapping effect are also analyzed quantitatively.When the surface coverage of Ag nanoparticles is 5%,light-trapping efficiencies are 15.5% and 32.3%,respectively,for 53and 88-nm Ag nanoparticles.Results indicate that the plasmon quadrupole mode resonance of Ag nanoparticles could further enhance the light-trapping effect for TF solar cells.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant No. 10774119)the program for New Century Excellent Talents in University,China (Grant No. NCET-08-0455)+2 种基金the Natural Science Foundation of Shaanxi province,China(Grant No. SJ08F07)the Foundation of National Laboratory of Acousticsthe Northwestern Polytechnical University NPU Foundation for Fundamental Research,China (Grant No. 2007004)
文摘Research on the underwater target scattering can provide important theoretical support for target detection. The scattering model of cylindrical shell is established in this paper. It is found that the forward target strength is much stronger and varies with angles of incident wave less significantly than backward target strength. The received forward signal strength fluctuates with the target moving due to the interference between direct signal and scattering signal, which is most significant when the target approaches the baseline. An experiment is carried out in an anechoic tank to validate the scattering model. The method of acquisiting forward scattering in the tank is proposed. The forward and the backward target strengths are achieved by using the pulse compression technology, and they axe about 3dB less than the modeling results. The forward scattering phenomena of quiescent and moving targets are measured, which are similar to modeling results with different target types.
基金supported by the National Natural Science Foundation of China (60901068)
文摘A new forward scattering bistatic radar motion compensation method based on spectral analysis and minimum waveform entropy is proposed. In order to demonstrate effectiveness of the presented method and ground vehicles imaging function of forward scattering radar, a simple bistatic forward scattering radar experiment system is set up on both sides of a road to collection ground vehicles experimental data. Finally, experimental ground vehicles imaging results confirm validity of the proposed motion compensation method and the experimental imaging results are identical with computer simulation results in the same parameter and condition.
基金supported by the Na-tional Natural Science Foundation of China(Nos.62175105,61875086)Fundamental Research Funds for the Cen-tral Universities of China(No.ILB240041A24)。
文摘A novel temperature and salinity discriminative sensing method based on forward Brillouin scattering(FBS)in 1060-XP single-mode fiber(SMF)is proposed.The measured frequency shifts corresponding to different radial acoustic modes in 1060-XP SMF show different sensitivities to temperature and salinity.Based on the new phenomenon that different radial acoustic modes have different frequency shift-temperature and frequency shift-salinity coefficients,we propose a novel method for simultaneously measuring temperature and salinity by measuring the frequency shift changes of two FBS scattering peaks.In a proof-of-concept experiment,the temperature and salinity measurement errors are 0.12℃and 0.29%,respectively.The proposed method for simultaneously measuring temperature and salinity has the potential applications such as ocean surveying,food manufacturing and pharmaceutical engineering.
基金This work was supported by the National Natural Science Foundation of China(62071475,61890541,62171447).
文摘The application scope of the forward scatter radar(FSR)based on the Global Navigation Satellite System(GNSS)can be expanded by improving the detection capability.Firstly,the forward-scatter signal model when the target crosses the baseline is constructed.Then,the detection method of the for-ward-scatter signal based on the Rényi entropy of time-fre-quency distribution is proposed and the detection performance with different time-frequency distributions is compared.Simula-tion results show that the method based on the smooth pseudo Wigner-Ville distribution(SPWVD)can achieve the best perfor-mance.Next,combined with the geometry of FSR,the influence on detection performance of the relative distance between the target and the baseline is analyzed.Finally,the proposed method is validated by the anechoic chamber measurements and the results show that the detection ability has a 10 dB improvement compared with the common constant false alarm rate(CFAR)detection.
基金the Electro-Magnetic Remote Sensing Defence Technology Centre (EMRS DTC)established by the UK Ministry of Defence (Grant No. 1-27)+1 种基金the Program for New Century Excellent Talents in University (Grant No. NCET-06-0162)the National Natural Science Foundation of China (Grant Nos. 60890071-17, 60890072-13, 60890073)
文摘Forward scattering micro radar is used for situation awareness; its operational range is relatively short because of the battery power and local horizon, the free space propagation model is not appropriate. The ground moving targets, such as humans, cars and tanks, have only comparable size with the transmitted signal wavelength; the point target model and the linear change of observation angle are not applicable. In this paper, the signal model of ground moving target is developed based on the case of forward scattering micro radar, considering the two-ray propagation model and area target model, and nonlinear change of observation angle as well as high order phase error. Furthermore, the analytical form of the received power from moving target has been obtained. Using the simulated forward scattering radar cross section, the received power of theoretical calculation is near to that of measured data. In addition, the simulated signal model of ground moving target is perfectly matched with the experimented data. All these results show the correctness of analytical calculation completely.
基金supported by the National Natural Science Foundation of China(Grant Nos.11174235 and 61571366)
文摘The aberration in the received acoustic field and the Doppler shift in the forward scattered field are simultaneously induced when a submerged target crosses the source–receiver line. Formulations for the two variations are developed upon an ideal forward scattering configuration. Both the field aberration and the Doppler shift are expressed as functions of the same argument — the target motion time. An experimental validation was carried out in a tank, in which the continuous wave was transmitted. The field aberration and the Doppler shift were extracted from the collected data by the simple Hilbert transform and a hybrid technique, respectively. The measured aberration and Doppler shift agree with the theoretical results.Simultaneous detection outputs are beneficial to enhance the reliability on target detection by providing both the aberrations in the received acoustic field and the Doppler shift in the forward scattered field.
基金the NSF-CMG award number DMS-0327778the DOE Basic Sciences award number DE-FG02-05ER15697.
文摘We present the application of the theory of Pade approximants to extending the perturbative solutions of acoustic wave equation for a three dimensional vertically varying medium with one interface.These type of solutions have limited convergence properties depending on either the degree of contrast between the actual and the reference medium or the angle of incidence of a plane wave component.We show that the sequence of Pade approximants to the partial sums in the forward scattering series for the 3D wave equation is convergent for any contrast and any incidence angle.This allows the construction of any reflected waves including phase-shifted post-critical plane waves and,for a point-source problem,refracted events or headwaves,and it also provides interesting interpretations of these solutions in the scattering theory formalism.
基金Project supported by the Sichuan Science and Technology Program(Grant No.2019YJ0530)Scientific Research Fund of Sichuan Provincial Education Department,China(Grant No.18ZA0401)the National Natural Science Foundation of China(Grant No.61205079).
文摘Distributed fiber sensors based on forward stimulated Brillouin scattering(F-SBS)have attracted special attention because of their capability to detect the acoustic impedance of liquid material outside fiber.However,the reported results were based on the extraction of a 1st-order local spectrum,causing the sensing distance to be restricted by pump depletion.Here,a novel post-processing technique was proposed for distributed acoustic impedance sensing by extracting the 2nd-order local spectrum,which is beneficial for improving the sensing signal-to-noise ratio(SNR)significantly,since its pulse energy penetrates into the fiber more deeply.As a proof-of-concept,distributed acoustic impedance sensing along~1630 m fiber under moderate spatial resolution of~20 m was demonstrated.
文摘I found that when the Debye theory calculates the far-field scattered light intensity of bubbles, the forward scattered light intensity is quite different from the result calculated by the Mie theory due to the convergence problem, so the expression of the Debye coefficient has been revised. I derived the Debye reflectance and transmittance according to the physical meaning of Debye theory and compared them with Fresnel’s formula. I modified the Debye coefficient expressions for bubbles based on the differences between the Debye reflectance and transmittance from the Fresnel formula. Finally, compared with the far-field scattered light intensity calculated by the original Debye theory, the far-field scattered light intensity calculated based on the modified Debye coefficient can obtain more accurate forward scattered light intensity with fewer sub-waves.
基金supported by the Ministry of Science and Technology (No.2017YFF0104500)the Chinese Academy of Sciences (No.XDB17000000)the National Natural Science Foundation of China (No.21573226, No.21822305)
文摘The reaction dynamics of the fluorine atom with vibrationally excited D2(v=1, v=0) was investigated using the crossed beam method. The scheme of stimulated Raman pumping was employed for preparation of vibrationally excited D2 molecules. Contribution from the reaction of spin-orbit excited F*(2P1/2) with vibrationally excited D2 was not found. Reaction of spin-orbit ground F(2P3/2) with vibrationally excited D2 was measured and DF products populated in v'=2, 3, 4, 5 were observed. Compared with the vibrationally ground reaction, DF products from the vibrationally excited reaction of F(2P3/2)+D2(v=1, j=0) are rotationally “hotter”. Differential cross sections at four collision energies, ranging from 0.32 kcal/mol to 2.62 kcal/mol, were obtained. Backward scattering dominates for DF products in all vibrational levels at the lowest collision energy of 0.32 kcal/mol. As the collision energy increases, angular distribution of DF products gradually shifts from backward to sideway. The collision-energy dependence of differential cross section of DF(v’=5) at forward direction was also measured. Forward-scattered signal of DF(v'=5) appears at the collision energy of 1.0 kcal/mol, and becomes dominated at 2.62 kcal/mol.
基金supported by the National Key R&D Program of China (No.2016YFF0200500)the National Natural Science Foundation of China (No.21473173, No.21590802, No.21403207, No.21503206)the Strategic Priority Research Program of Chinese Academy of Sciences (No.XDB17000000)
文摘The H+H2 reaction is the simplest chemical reaction system and has long been the prototype model in the study of reaction dynamics. Here we report a high resolution experimental investigation of the state-to-state reaction dynamics in the H+HD→H2+D reaction by using the crossed molecular beams method and velocity map ion imaging technique at the collision energy of 1.17 eV. D atom products in this reaction were probed by the near threshold 1+1'(vacuum ultraviolet+ultraviolet) laser ionization scheme. The ion image with both high angular and energy resolution were acquired. State-to-state differential cross sections was accurately derived. Fast forward scattering oscillations, relating with interference effects in the scattering process, were clearly observed for H2 products at H2(v'=0,j'=1) and H2(v'=0,j'=3) rovibrational levels. This study further demonstrates the importance of measuring high-resolution differential cross sections in the study of state-to-state reaction dynamics in the gas phase.
基金supported in part by the National Natural Foundation of China(Nos. 61875086, 61377086)the Aerospace Science Foundation of China (No.2016ZD52042)Nanjing University of Aeronautics and Astronautics Ph. D. short-term visiting scholar project (No.190901DF08)
文摘We propose the trench-assisted multimode fiber(TA-OM4)as a novel sensing fiber in forward Brillouin scattering(FBS)-based temperature sensor,due to its higher temperature sensitivity,better bending resistance and lower propagation loss,compared with the single mode fiber(SMF)and other sensing fibers.The FBS effect and acousto-optic interaction in TA-OM4 are the first time to be demonstrated and characterized at 1550 nm theoretically and experimentally.A 2.0 km long TA-OM4 is put into an oven to measure its temperature sensitivity,which can reach up to 80.3 kHz/℃,exceeding 53%of SMF(52.4 kHz/℃).The simulated and experimental results verify that the TA-OM4 may be a good candidate as the sensing fiber for the FBS-based temperature sensor.
基金supported by National Natural Science Foundation of China(NSFC 50376041)the Shu Guang Project of Shanghai Educational Development Foundation(04SG49)the DFG projects(grant Ri 533/7-1 and Ri 533/7-2)
文摘A new algorithm of the relaxation method is developed for the inversion of forward scattered light to obtain the size distribution of spherical particles. Numerical tests are performed for a laser particle analyzer using the Mie theory and the diffraction approximation. The algorithm efficiency, in the presence of experimental noises, is studied. The results show that the technique is fast in convergence, stable against random noise and insensitive to the distribution of particles and the initial trial distribution.
基金support from the National Natural Science Foundation of China (No. 50876069)the Ministry of Education of the People’s Republic of China (No.208041)from the Shanghai Municipal Education Commis-sion (No. 07ZZ88)
文摘The optical measurement technique based on Mie scattering has been applied to various areas, in which single scattering at low particle concentration is assumed. Nevertheless, since multiple scattering is usually unavoidable in online measurements, we present in this work a multiple scattering calculation method, in which a layer model is employed. The three-dimensional particle system is divided into a pile of layers the number of which is automatically determined, depending on the obscuration of the particle system. The calculation is found to be fast, reasonable and reliable.
基金supported by the National Natural Science Foundation of China(11174235,61571366)
文摘The basic principles of target detection by forward acoustic scattering are presented.A direct blast suppression approach based on adaptive filtering(DBS-AF) is proposed to suppress the direct blast.The DBS-AF technique is extended to the linear frequency modulation(LFM) signal,where the envelope of the signal is regarded as a 'general waveform' and imported into the adaptive filter.Application of the DBS-AF method to the data collected from a lake trial yields an output detection curve,in which the direct blast is mapped to the background while the acoustic field aberration is represented by the peak value fluctuation.The inhibitory effect in single hydrophone is approximately- 5 dB,and is then enhanced by exploiting the mean value removal approach as a preprocessing technique.The direct blast is further suppressed to a level of-10 dB by making full use of multichannel receptions.The main factors affecting the algorithm performance are as follows:the fluctuation degree of the receptions during the weighting vector training period and the power ratio of the forward scattered wave to the direct blast when the target is present.
基金This work was supported from the National Natural Science Foundation of China (Nos. 11604298 and 61377031) and Scientific Research Foundation (Nos. Q1444 and 1539) of Zhejiang Ocean University.
文摘Transparent electrodes made of silver nanowires (Ag NWs) exhibit a higher flexibility than conventional indium tin oxide electrodes.For this reason,Ag NWs may find applications in future flexible electronic and optoelectronic devices.However,different optoelectronic devices have different specific requirements for Ag NWs.For example,the optical transmittance haze is an important but rarely studied aspect of Ag NW films.In this study,the optical transmittance and optical scattering of long (5-50 μm,L-NWs) and short (1-20 μm,S-NWs) Ag NW films were investigated.The L-NWs exhibited better optical transmission than the S-NWs,whereas the S-NWs exhibited better light-scattering properties than the L-NWs.Our results indicate that the L-NWs are suitable for touch-screen displays,whereas the S-NWs are better suited as transparent conductive films for solar cells.We analyzed the scattering ratio of forward-scattered light to backscattered light for both the L-NWs and S-NWs and discovered that the mesh size affected the scattering ratio.For longer wavelengths,a larger mesh yielded a higher backscattering ratio,whereas a smaller mesh yielded a lower backscattering ratio.We formulated an equation for calculating the reflection haze using the total reflection (Ag NWs/glass),R and the reflection of glass,R0.The reflection haze of the S-NWs and L-NWs exhibited different trends in the visible-near-infrared region.An omnidirectional scattering model for the Ag NWs was used to evaluate the Ag NW scattering properties.The results of this study have great significance for the evaluation of the performance of Ag NWs in optoelectronic devices.
基金supported by National Natural Science Foundation of China(41604091,41704111,41774126)the great and special project(2016ZX05024-001,2016ZX05006-002).
文摘In the field of geophysics,although the first-order Rytov approximation is widely used,the higher-order approximation is seldom discussed.From both theo-retical analysis and numerical tests,the accumulated phase error introduced in the first-order Rytov approximation cannot be neglected in the presence of strong velocity perturbation.In this paper,we are focused on improving the phase accuracy of forward scattered wavefield,especially for the large-scale and strong velocity pertur-bation case.We develop an equivalent source method which can update the imaginary part of the complex phase iteratively,and the higher-order scattered wavefield can be approximated by multiplying the incident wavefield by the exponent of the imaginary part of the complex phase.Although the convergence of the proposed method has not been proved mathematically,numerical examples demonstrate that our method can produce an improved accuracy for traveltime(phase)prediction,even for strong perturbation media.However,due to the neglect of the real part of the complex phase,the amplitude change of the scattered wavefield cannot be recovered.Furthermore,in the presence of multi-arrivals phenomenon,the equivalent scattering source should be handled carefully due to the multi-directions of the wavefield.Further investigations should be done to improve the applicability of the proposed method.
基金supported by the Natural Science Foundation of Beijing (No.2102042)the National Natural Science Foundation of China (No.20876040)the Fundamental Research Funds for the Central Universities (No.10QG24)
文摘Forward-scattering efficiency (FSE) is first proposed when an Ag nanoparticle serves as the light-trapping structure for thin-film (TF) solar cells because the Ag nanoparticle’s light-trapping efficiency lies on the light-scattering direction of metal nanoparticles.Based on FSE analysis of Ag nanoparticles with radii of 53 and 88 nm,the forward-scattering spectra and light-trapping efficiencies are calculated.The contributions of dipole and quadrupole modes to light-trapping effect are also analyzed quantitatively.When the surface coverage of Ag nanoparticles is 5%,light-trapping efficiencies are 15.5% and 32.3%,respectively,for 53and 88-nm Ag nanoparticles.Results indicate that the plasmon quadrupole mode resonance of Ag nanoparticles could further enhance the light-trapping effect for TF solar cells.