In this study, three Danish sites having the longest (1990-2004) time-series of ozone measurements were analysed on inter-annual, monthly and diurnal cycle variability as well as elevated and lowered ozone concentrati...In this study, three Danish sites having the longest (1990-2004) time-series of ozone measurements were analysed on inter-annual, monthly and diurnal cycle variability as well as elevated and lowered ozone concentration events were identified. The atmospheric trajectory (HYSPLIT) and dispersion (HIRLAM + CAMx) models were employed to study dominating atmospheric transport patterns associated with elevated events and to evaluate spatio-temporal variability of ozone specific episode and typical seasonal patterns for Denmark. It was found that generally inter-annual variability has a positive trend, and events with low ozone concentration (≤10 μg/m3) continued to diminish. On a monthly scale, the highest and lowest mean concentrations are observed in May and November-December, respectively. The elevated concentrations (≥120 μg/m3) are observed during March-September. On a diurnal cycle, it is observed mostly during 13-16 of local time, and more frequent (ten-fold) compared with nighttime-early morning hours. For ozone elevated events, several sectors (or pathways of atmospheric transport) were identified depending on the sites’ positions, showing the largest (39%) number of such events associated with the north-western sector, and lowest (13% each)—southwestern and northern sectors. For each site, less than 60 events showed very high concentrations (≥180 μg/m3). Among 12 episodes, one longest elevated episode (19-21 Jun 2000) simultaneously registered at all sites and characterized by dominating transport from the south-southwestern sector, low wind speed, clear-sky, and multiple inversions was studied using modelling tools. For this episode, both measurements and modeling (trajectory and dispersion) results showed a relatively good agreement.展开更多
The impacts of the enhanced model's moist physics and horizontal resolution upon the QPFs (quantitative precipitation forecasts)are investigated by applying the HIRLAM(high resolution limited area model)to the sum...The impacts of the enhanced model's moist physics and horizontal resolution upon the QPFs (quantitative precipitation forecasts)are investigated by applying the HIRLAM(high resolution limited area model)to the summer heavy-rain cases in China.The performance of the control run, for which a 0.5°×0.5°grid spacing and a traditional“grid-box supersaturation removal+Kuo type convective paramerization”are used as the moist physics,is compared with that of the sensitivity runs with an enhanced model's moist physics(Sundqvist scheme)and an increased horizontal resolution(0.25°×0.25°),respectively.The results show: (1)The enhanced moist physics scheme(Sundqvist scheme),by introducing the cloud water content as an additional prognostic variable and taking into account briefly of the microphysics involved in the cloud-rain conversion,does bring improvements in the model's QPFs.Although the deteriorated QPFs also occur occasionally,the improvements are found in the majority of the cases,indicating the great potential for the improvement of QPFs by enhancing the model's moist physics. (2)By increasing the model's horizontal resolution from 0.5°×0.5°,which is already quite high compared with that of the conventional atmospheric soundings,to 0.25°×0.25°without the simultaneous enhancement in model physics and objective analysis,the improvements in QPFs are very limited.With higher resolution,although slight amelioration in locating the rainfall centers and in resolving some finer structures of precipitation pattern are made,the number of the mis- predicted fine structures in rainfall field increases with the enhanced model resolution as well.展开更多
文摘In this study, three Danish sites having the longest (1990-2004) time-series of ozone measurements were analysed on inter-annual, monthly and diurnal cycle variability as well as elevated and lowered ozone concentration events were identified. The atmospheric trajectory (HYSPLIT) and dispersion (HIRLAM + CAMx) models were employed to study dominating atmospheric transport patterns associated with elevated events and to evaluate spatio-temporal variability of ozone specific episode and typical seasonal patterns for Denmark. It was found that generally inter-annual variability has a positive trend, and events with low ozone concentration (≤10 μg/m3) continued to diminish. On a monthly scale, the highest and lowest mean concentrations are observed in May and November-December, respectively. The elevated concentrations (≥120 μg/m3) are observed during March-September. On a diurnal cycle, it is observed mostly during 13-16 of local time, and more frequent (ten-fold) compared with nighttime-early morning hours. For ozone elevated events, several sectors (or pathways of atmospheric transport) were identified depending on the sites’ positions, showing the largest (39%) number of such events associated with the north-western sector, and lowest (13% each)—southwestern and northern sectors. For each site, less than 60 events showed very high concentrations (≥180 μg/m3). Among 12 episodes, one longest elevated episode (19-21 Jun 2000) simultaneously registered at all sites and characterized by dominating transport from the south-southwestern sector, low wind speed, clear-sky, and multiple inversions was studied using modelling tools. For this episode, both measurements and modeling (trajectory and dispersion) results showed a relatively good agreement.
基金Financially supported by the Chinese State Education Committee's Research Foundation for scholars returning from abroad and by Danish Government's Danida Foundation.
文摘The impacts of the enhanced model's moist physics and horizontal resolution upon the QPFs (quantitative precipitation forecasts)are investigated by applying the HIRLAM(high resolution limited area model)to the summer heavy-rain cases in China.The performance of the control run, for which a 0.5°×0.5°grid spacing and a traditional“grid-box supersaturation removal+Kuo type convective paramerization”are used as the moist physics,is compared with that of the sensitivity runs with an enhanced model's moist physics(Sundqvist scheme)and an increased horizontal resolution(0.25°×0.25°),respectively.The results show: (1)The enhanced moist physics scheme(Sundqvist scheme),by introducing the cloud water content as an additional prognostic variable and taking into account briefly of the microphysics involved in the cloud-rain conversion,does bring improvements in the model's QPFs.Although the deteriorated QPFs also occur occasionally,the improvements are found in the majority of the cases,indicating the great potential for the improvement of QPFs by enhancing the model's moist physics. (2)By increasing the model's horizontal resolution from 0.5°×0.5°,which is already quite high compared with that of the conventional atmospheric soundings,to 0.25°×0.25°without the simultaneous enhancement in model physics and objective analysis,the improvements in QPFs are very limited.With higher resolution,although slight amelioration in locating the rainfall centers and in resolving some finer structures of precipitation pattern are made,the number of the mis- predicted fine structures in rainfall field increases with the enhanced model resolution as well.
