With the increasing exploration and development of typical hydrocarbon-rich depressions,such as the Dongpu Depression,the exploitation difficulty of shallow formations is increasing.There is an urgent need to clarify ...With the increasing exploration and development of typical hydrocarbon-rich depressions,such as the Dongpu Depression,the exploitation difficulty of shallow formations is increasing.There is an urgent need to clarify the hydrocarbon generation mode and hydrocarbon generation histories in deep formations.In this study,a gold tube-autoclave closed system was used to simulate the hydrocarbon generation processes and establish the hydrocarbon generation mode of different types of kerogen.Then,constrained by the thermal history and hydrocarbon generation kinetics,hydrocarbon generation histories were modeled.The results show that hydrocarbon generation evolution can be divided into five stages,and the maturity of each stage is different.The hydrocarbon generation history of the source rocks of the Shahejie 3 Formation mainly dates from the early depositional period of the Shahejie 1 Formation to the middle depositional period of the Dongying Formation.Hydrocarbon generation history constrained by thermal history and hydrocarbon generation kinetics is more in line with actual geological conditions.Moreover,this research can provide important hydrocarbon generation parameters for deep oil and gas exploration and exploitation of the Shahejie 3 Formation in the Dongpu Depression.展开更多
A sample from the Jurassic Tamulangou Fm.and two comparison samples from the Cretaceous Fm.were used to document the hydrocarbon generation kinetics and phase behaviors at two heating rates using the confined gold tub...A sample from the Jurassic Tamulangou Fm.and two comparison samples from the Cretaceous Fm.were used to document the hydrocarbon generation kinetics and phase behaviors at two heating rates using the confined gold tube system.The results show that the different heating rates affect the reaction rates,paths and levels of organic matter evolution.The average activation energy and dominant frequency activation energy of liquid hydrocarbon are significantly lower than those of gaseous.Moreover,igneous intrusion had a positive effect on the blooming,enrichment and preservation of organic matter,promoting a Ro increase of 0.09%–1.07%in the Jurassic Tamulangou Fm.Two models were used to simulate the normal and abnormal evolution caused by thermal events combined hydrocarbon generation kinetic parameters.Thermal simulation analysis shows that oil generation was initially slow and then increased rapidly until a burial depth of 1500 m was reached at~128 Ma.The largest hydrocarbon expulsion began at~120 Ma,corresponding to a burial depth of 2450 m.The maximum cumulative yield is 510 mg/g TOC,and it is still in the peak period of hydrocarbon generation,which demonstrates a favorable potential for hydrocarbon exploration.展开更多
The Taoudeni Basin is a typical and steady intracratonic basin in Mauritania, northwest Africa. There are six sets of potential source rocks and five regional unconformable surfaces of the Infracambrian and Paleozoic ...The Taoudeni Basin is a typical and steady intracratonic basin in Mauritania, northwest Africa. There are six sets of potential source rocks and five regional unconformable surfaces of the Infracambrian and Paleozoic developed in the basin. We used seismic stratigraphic correlation to recover the denudation thickness of formations at a particular well location. Studies of the hydrocarbon generation history of the basin illustrate that hydrocarbon migration and accumulation occurred in the end of the Carboniferous, and after that, the whole basin suffered denudation for a long period of time. Because there is no thick Mesozoic overburden in the basin, the Silurian source rocks could not generate hydrocarbon in the Mesozoic era for the second time. Consequently, the prospects for successful hydrocarbon exploration in the basin are not good.展开更多
The hydrocarbon charge history of the Paleogene in the northern Dongpu Depression was analyzed in detail based on a comprehensive analysis of the generation and expulsion history of the major hydrocarbon source rocks,...The hydrocarbon charge history of the Paleogene in the northern Dongpu Depression was analyzed in detail based on a comprehensive analysis of the generation and expulsion history of the major hydrocarbon source rocks, fluorescence microscopic features and fluid inclusion petrography. There were two main stages of hydrocarbon generation and expulsion of oil from the major hydrocarbon source rocks. The first stage was the main hydrocarbon expulsion stage. The fluorescence microscopic features also indicated two stages of hydrocarbon accumulation. Carbonaceous bitumen, asphaltene bitumen and colloidal bitumen reflected an early hydrocarbon charge, whereas the oil bitumen reflected a second hydrocarbon charge. Hydrocarbon inclusions also indicate two distinct charges according to the diagenetic evolution sequence, inclusion petrography features combined with the homogenization temperature and reservoir burial history analysis. According to these comprehensive analysis results, the hydrocarbon charge history of the Paleogene reservoir in the northern Dongpu Depression was divided into two phases. The first phase was from the late Dongying depositional period of the Oligocene to the early uplift stages of the late Paleogene. The second phase was from the late Minghuazhen period of the Pliocene to the Quaternary. Reservoirs formed during the first period were widely distributed covering the entire area. In contrast,reservoirs formed during the second period were mainly distributed near the hydrocarbon generation sags. Vertically, it was characterized by a single phase in the upper layers and two phases in the lower layers of the Paleogene.展开更多
This work restored the erosion thickness of the top surface of each Cretaceous formations penetrated by the typical well in the Hari sag, and simulated the subsidence burial history of this well with software BasinMod...This work restored the erosion thickness of the top surface of each Cretaceous formations penetrated by the typical well in the Hari sag, and simulated the subsidence burial history of this well with software BasinMod. It is firstly pointed out that the tectonic subsidence evolution of the Hari sag since the Cretaceous can be divided into four phases: initial subsidence phase, rapid subsidence phase,uplift and erosion phase, and stable slow subsidence phase. A detailed reconstruction of the tectonothermal evolution and hydrocarbon generation histories of typical well was undertaken using the EASY R% model, which is constrained by vitrinite reflectance(R) and homogenization temperatures of fluid inclusions. In the rapid subsidence phase, the peak period of hydrocarbon generation was reached at c.a.105.59 Ma with the increasing thermal evolution degree. A concomitant rapid increase in paleotemperatures occurred and reached a maximum geothermal gradient of about 43-45℃/km. The main hydrocarbon generation period ensued around 105.59-80.00 Ma and the greatest buried depth of the Hari sag was reached at c.a. 80.00 Ma, when the maximum paleo-temperature was over 180℃.Subsequently, the sag entered an uplift and erosion phase followed by a stable slow subsidence phase during which the temperature gradient, thermal evolution, and hydrocarbon generation decreased gradually. The hydrocarbon accumulation period was discussed based on homogenization temperatures of inclusions and it is believed that two periods of rapid hydrocarbon accumulation events occurred during the Cretaceous rapid subsidence phase. The first accumulation period observed in the Bayingebi Formation(Kb) occurred primarily around 105.59-103.50 Ma with temperatures of 125-150℃. The second accumulation period observed in the Suhongtu Formation(Ks) occurred primarily around84.00-80.00 Ma with temperatures of 120-130℃. The second is the major accumulation period, and the accumulation mainly occurred in the Late Cretaceous. The hydrocarbon accumulation process was comprehensively controlled by tectono-thermal evolution and hydrocarbon generation history. During the rapid subsidence phase, the paleo temperature and geothermal gradient increased rapidly and resulted in increasing thermal evolution extending into the peak period of hydrocarbon generation,which is the key reason for hydrocarbon filling and accumulation.展开更多
基金funded by the National Major Science and Technology Projects of China(Grant No.2016ZX05006-004)the Sichuan Youth Science and Technology Foundation(Grant No.2016JQ0043)the National Natural Science Foundation of China(Grant No.41972144)
文摘With the increasing exploration and development of typical hydrocarbon-rich depressions,such as the Dongpu Depression,the exploitation difficulty of shallow formations is increasing.There is an urgent need to clarify the hydrocarbon generation mode and hydrocarbon generation histories in deep formations.In this study,a gold tube-autoclave closed system was used to simulate the hydrocarbon generation processes and establish the hydrocarbon generation mode of different types of kerogen.Then,constrained by the thermal history and hydrocarbon generation kinetics,hydrocarbon generation histories were modeled.The results show that hydrocarbon generation evolution can be divided into five stages,and the maturity of each stage is different.The hydrocarbon generation history of the source rocks of the Shahejie 3 Formation mainly dates from the early depositional period of the Shahejie 1 Formation to the middle depositional period of the Dongying Formation.Hydrocarbon generation history constrained by thermal history and hydrocarbon generation kinetics is more in line with actual geological conditions.Moreover,this research can provide important hydrocarbon generation parameters for deep oil and gas exploration and exploitation of the Shahejie 3 Formation in the Dongpu Depression.
基金supported by the National Natural Science Foundation of China(Grant No.42072119)Science and Technology Project of Petro China(Grant No.101017kt1604003x20)。
文摘A sample from the Jurassic Tamulangou Fm.and two comparison samples from the Cretaceous Fm.were used to document the hydrocarbon generation kinetics and phase behaviors at two heating rates using the confined gold tube system.The results show that the different heating rates affect the reaction rates,paths and levels of organic matter evolution.The average activation energy and dominant frequency activation energy of liquid hydrocarbon are significantly lower than those of gaseous.Moreover,igneous intrusion had a positive effect on the blooming,enrichment and preservation of organic matter,promoting a Ro increase of 0.09%–1.07%in the Jurassic Tamulangou Fm.Two models were used to simulate the normal and abnormal evolution caused by thermal events combined hydrocarbon generation kinetic parameters.Thermal simulation analysis shows that oil generation was initially slow and then increased rapidly until a burial depth of 1500 m was reached at~128 Ma.The largest hydrocarbon expulsion began at~120 Ma,corresponding to a burial depth of 2450 m.The maximum cumulative yield is 510 mg/g TOC,and it is still in the peak period of hydrocarbon generation,which demonstrates a favorable potential for hydrocarbon exploration.
文摘The Taoudeni Basin is a typical and steady intracratonic basin in Mauritania, northwest Africa. There are six sets of potential source rocks and five regional unconformable surfaces of the Infracambrian and Paleozoic developed in the basin. We used seismic stratigraphic correlation to recover the denudation thickness of formations at a particular well location. Studies of the hydrocarbon generation history of the basin illustrate that hydrocarbon migration and accumulation occurred in the end of the Carboniferous, and after that, the whole basin suffered denudation for a long period of time. Because there is no thick Mesozoic overburden in the basin, the Silurian source rocks could not generate hydrocarbon in the Mesozoic era for the second time. Consequently, the prospects for successful hydrocarbon exploration in the basin are not good.
基金supported by the Important National Science&Technology Specific Projects(Grant No.2011ZX05006-003/004)
文摘The hydrocarbon charge history of the Paleogene in the northern Dongpu Depression was analyzed in detail based on a comprehensive analysis of the generation and expulsion history of the major hydrocarbon source rocks, fluorescence microscopic features and fluid inclusion petrography. There were two main stages of hydrocarbon generation and expulsion of oil from the major hydrocarbon source rocks. The first stage was the main hydrocarbon expulsion stage. The fluorescence microscopic features also indicated two stages of hydrocarbon accumulation. Carbonaceous bitumen, asphaltene bitumen and colloidal bitumen reflected an early hydrocarbon charge, whereas the oil bitumen reflected a second hydrocarbon charge. Hydrocarbon inclusions also indicate two distinct charges according to the diagenetic evolution sequence, inclusion petrography features combined with the homogenization temperature and reservoir burial history analysis. According to these comprehensive analysis results, the hydrocarbon charge history of the Paleogene reservoir in the northern Dongpu Depression was divided into two phases. The first phase was from the late Dongying depositional period of the Oligocene to the early uplift stages of the late Paleogene. The second phase was from the late Minghuazhen period of the Pliocene to the Quaternary. Reservoirs formed during the first period were widely distributed covering the entire area. In contrast,reservoirs formed during the second period were mainly distributed near the hydrocarbon generation sags. Vertically, it was characterized by a single phase in the upper layers and two phases in the lower layers of the Paleogene.
基金supported by the project of "Constraints on Lithospheric Dynamic Evolution and Hydrocarbon Accumulation from Late Mesozoic Paleo-geothermal Field in Ordos and Qinshui Basins" (grant No. 41630312)the National Nature Science Foundation of China (grants No. 41372208 and 40534019)+1 种基金the Open Found of the State Key Laboratory of Ore Deposit Geochemistry, CAS (grant No. 201304)supported by international program for Ph.D. candidates, Sun Yat-Sen University
文摘This work restored the erosion thickness of the top surface of each Cretaceous formations penetrated by the typical well in the Hari sag, and simulated the subsidence burial history of this well with software BasinMod. It is firstly pointed out that the tectonic subsidence evolution of the Hari sag since the Cretaceous can be divided into four phases: initial subsidence phase, rapid subsidence phase,uplift and erosion phase, and stable slow subsidence phase. A detailed reconstruction of the tectonothermal evolution and hydrocarbon generation histories of typical well was undertaken using the EASY R% model, which is constrained by vitrinite reflectance(R) and homogenization temperatures of fluid inclusions. In the rapid subsidence phase, the peak period of hydrocarbon generation was reached at c.a.105.59 Ma with the increasing thermal evolution degree. A concomitant rapid increase in paleotemperatures occurred and reached a maximum geothermal gradient of about 43-45℃/km. The main hydrocarbon generation period ensued around 105.59-80.00 Ma and the greatest buried depth of the Hari sag was reached at c.a. 80.00 Ma, when the maximum paleo-temperature was over 180℃.Subsequently, the sag entered an uplift and erosion phase followed by a stable slow subsidence phase during which the temperature gradient, thermal evolution, and hydrocarbon generation decreased gradually. The hydrocarbon accumulation period was discussed based on homogenization temperatures of inclusions and it is believed that two periods of rapid hydrocarbon accumulation events occurred during the Cretaceous rapid subsidence phase. The first accumulation period observed in the Bayingebi Formation(Kb) occurred primarily around 105.59-103.50 Ma with temperatures of 125-150℃. The second accumulation period observed in the Suhongtu Formation(Ks) occurred primarily around84.00-80.00 Ma with temperatures of 120-130℃. The second is the major accumulation period, and the accumulation mainly occurred in the Late Cretaceous. The hydrocarbon accumulation process was comprehensively controlled by tectono-thermal evolution and hydrocarbon generation history. During the rapid subsidence phase, the paleo temperature and geothermal gradient increased rapidly and resulted in increasing thermal evolution extending into the peak period of hydrocarbon generation,which is the key reason for hydrocarbon filling and accumulation.