The GECAM series of satellites utilizes LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals as sensitive materials for gamma-ray detectors(GRDs).To investigate the nonlinearity in the detection of low-energy gamma rays a...The GECAM series of satellites utilizes LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals as sensitive materials for gamma-ray detectors(GRDs).To investigate the nonlinearity in the detection of low-energy gamma rays and address the errors in the calibration of the E-C relationship,comprehensive tests and comparative studies of the three aforementioned crystals were conducted using Compton electrons,radioactive sources,and mono-energetic X-rays.The nonlinearity test results of the Compton electrons and X-rays demonstrated substantial differences,with all three crystals presenting a higher nonlinearity for X/-rays than for Compton electrons.Despite the LaBr_(3)(Ce)and LaBr_(3)(Ce,Sr)crystals having higher absolute light yields,they exhibited a noticeable nonlinear decrease in the light yield,especially at energies below 400 keV.The NaI(Tl)crystal demonstrated an"excess"light output in the 6-200 keV range,reaching a maximum"excess"of 9.2%at 30 keV in the X-ray testing and up to 15.5%at 14 keV during Compton electron testing,indicating a significant advantage in the detection of low-energy gamma rays.Furthermore,we explored the underlying causes of the observed nonlinearity in these crystals.This study not only elucidates the detector responses of GECAM,but also initiates a comprehensive investigation of the nonlinearity of domestically produced lanthanum bromide and sodium iodide crystals.展开更多
With respect to the gamma spectrum, the energy resolution improves with increase in energy. The counts of full energy peak change with energy, and this approximately complies with the Gaussian distribution. This study...With respect to the gamma spectrum, the energy resolution improves with increase in energy. The counts of full energy peak change with energy, and this approximately complies with the Gaussian distribution. This study mainly examines a method to deconvolve the LaBr_3:Ce gamma spectrum with a detector response matrix constructing algorithm based on energy resolution calibration.In the algorithm, the full width at half maximum(FWHM)of full energy peak was calculated by the cubic spline interpolation algorithm and calibrated by a square root of a quadratic function that changes with the energy. Additionally, the detector response matrix was constructed to deconvolve the gamma spectrum. Furthermore, an improved SNIP algorithm was proposed to eliminate the background. In the experiment, several independent peaks of ^(152)Eu,^(137)Cs, and ^(60)Co sources were detected by a LaBr_3:Ce scintillator that were selected to calibrate the energy resolution. The Boosted Gold algorithm was applied to deconvolve the gamma spectrum. The results showed that the peak position difference between the experiment and the deconvolution was within ± 2 channels and the relative error of peak area was approximately within 0.96–6.74%. Finally, a ^(133) Ba spectrum was deconvolved to verify the efficiency and accuracy of the algorithm in unfolding the overlapped peaks.展开更多
Usually, there are several methods, e.g. experiment, interpolation experiment-based, analytic function, and Monte-Carlo simulation, to calculate the response functions in LaBr3（Ce） detectors. In logging applications...Usually, there are several methods, e.g. experiment, interpolation experiment-based, analytic function, and Monte-Carlo simulation, to calculate the response functions in LaBr3（Ce） detectors. In logging applications, the experiment-based methods cannot be adopted because of their limitations. Analytic function has the advantage of fast calculating speed, but it is very difficult to take into account many effects that occur in practical applications. On the contrary, Monte-Carlo simulation can deal with physical and geometric configurations very tactfully. It has a distinct advantage for calculating the functions with complex configurations in borehole. A new application of LaBr3（Ce） detector is in natural gamma-rays borehole spectrometer for uranium well logging. Calculation of response functions must consider a series of physical and geometric factors under complex logging conditions, including earth formations and its relevant parameters, different energies, material and thickness of the casings, the fluid between the two tubes, and relative position of the LaBr3（Ce） crystal to steel ingot at the front of logging tube. The present work establishes Monte-Carlo simulation models for the above-mentioned situations, and then performs calculations for main gamma-rays from natural radio-elements series. The response functions can offer experimental directions for the design of borehole detection system, and provide technique basis and basic data for spectral analysis of natural gamma-rays, and for sonrceless calibration in uranium quantitative interpretation.展开更多
基金This work was supported by the National Key Research and Development Program(Nos.2022YFB3503600 and 2021YFA0718500)Strategic Priority Research Program of the Chinese Academy of Sciences(Nos.XDA15360102)National Natural Science Foundation of China(Nos.12273042 and 12075258).
文摘The GECAM series of satellites utilizes LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals as sensitive materials for gamma-ray detectors(GRDs).To investigate the nonlinearity in the detection of low-energy gamma rays and address the errors in the calibration of the E-C relationship,comprehensive tests and comparative studies of the three aforementioned crystals were conducted using Compton electrons,radioactive sources,and mono-energetic X-rays.The nonlinearity test results of the Compton electrons and X-rays demonstrated substantial differences,with all three crystals presenting a higher nonlinearity for X/-rays than for Compton electrons.Despite the LaBr_(3)(Ce)and LaBr_(3)(Ce,Sr)crystals having higher absolute light yields,they exhibited a noticeable nonlinear decrease in the light yield,especially at energies below 400 keV.The NaI(Tl)crystal demonstrated an"excess"light output in the 6-200 keV range,reaching a maximum"excess"of 9.2%at 30 keV in the X-ray testing and up to 15.5%at 14 keV during Compton electron testing,indicating a significant advantage in the detection of low-energy gamma rays.Furthermore,we explored the underlying causes of the observed nonlinearity in these crystals.This study not only elucidates the detector responses of GECAM,but also initiates a comprehensive investigation of the nonlinearity of domestically produced lanthanum bromide and sodium iodide crystals.
基金supported by the National Natural Science Foundation of China(Nos.41374130 and 41604154)
文摘With respect to the gamma spectrum, the energy resolution improves with increase in energy. The counts of full energy peak change with energy, and this approximately complies with the Gaussian distribution. This study mainly examines a method to deconvolve the LaBr_3:Ce gamma spectrum with a detector response matrix constructing algorithm based on energy resolution calibration.In the algorithm, the full width at half maximum(FWHM)of full energy peak was calculated by the cubic spline interpolation algorithm and calibrated by a square root of a quadratic function that changes with the energy. Additionally, the detector response matrix was constructed to deconvolve the gamma spectrum. Furthermore, an improved SNIP algorithm was proposed to eliminate the background. In the experiment, several independent peaks of ^(152)Eu,^(137)Cs, and ^(60)Co sources were detected by a LaBr_3:Ce scintillator that were selected to calibrate the energy resolution. The Boosted Gold algorithm was applied to deconvolve the gamma spectrum. The results showed that the peak position difference between the experiment and the deconvolution was within ± 2 channels and the relative error of peak area was approximately within 0.96–6.74%. Finally, a ^(133) Ba spectrum was deconvolved to verify the efficiency and accuracy of the algorithm in unfolding the overlapped peaks.
基金supported by Key Laboratory of Radioactive Geology and Exploration Technology Fundamental Science for National Defense(No. 2011RGET04)East China Institute of Technology, and National Natural Science Foundation of China (No. 41074078)
文摘Usually, there are several methods, e.g. experiment, interpolation experiment-based, analytic function, and Monte-Carlo simulation, to calculate the response functions in LaBr3（Ce） detectors. In logging applications, the experiment-based methods cannot be adopted because of their limitations. Analytic function has the advantage of fast calculating speed, but it is very difficult to take into account many effects that occur in practical applications. On the contrary, Monte-Carlo simulation can deal with physical and geometric configurations very tactfully. It has a distinct advantage for calculating the functions with complex configurations in borehole. A new application of LaBr3（Ce） detector is in natural gamma-rays borehole spectrometer for uranium well logging. Calculation of response functions must consider a series of physical and geometric factors under complex logging conditions, including earth formations and its relevant parameters, different energies, material and thickness of the casings, the fluid between the two tubes, and relative position of the LaBr3（Ce） crystal to steel ingot at the front of logging tube. The present work establishes Monte-Carlo simulation models for the above-mentioned situations, and then performs calculations for main gamma-rays from natural radio-elements series. The response functions can offer experimental directions for the design of borehole detection system, and provide technique basis and basic data for spectral analysis of natural gamma-rays, and for sonrceless calibration in uranium quantitative interpretation.
