Tree-ring width(RW),density,elemental com-position,and stable carbon and oxygen isotope(δ^(13)C,δ^(18)O)are widely used as proxies to assess climate change,ecology,and environmental pollution;however,a specific pret...Tree-ring width(RW),density,elemental com-position,and stable carbon and oxygen isotope(δ^(13)C,δ^(18)O)are widely used as proxies to assess climate change,ecology,and environmental pollution;however,a specific pretreat-ment has been needed for each proxy.Here,we developed a method by which each proxy can be measured in the same sample.First,the sample is polished for ring width meas-urement.After obtaining the ring width data,the sample is cut to form a 1-mm-thick wood plate.The sample is then mounted in a vertical sample holder,and gradually scanned by an X-ray beam.Simultaneously,the count rates of the fluorescent photons of elements(for chemical characteriza-tion)and a radiographic grayscale image(for wood density)are obtained,i.e.the density and the element content are obtained.Then,cellulose is isolated from the 1-mm wood plate by removal of lignin,and hemicellulose.After producing this cellulose plate,cellulose subsamples are separated by knife under the microscope for inter-annual and intra-annual stable carbon and oxygen isotope(δ^(13)C,δ^(18)O)analysis.Based on this method,RW,density,elemental composition,δ^(13)C,and δ^(18)O can be measured from the same sample,which reduces sample amount and treatment time,and is helpful for multi-proxy comparison and combination research.展开更多
Facing the complex variable high-temperature environment,electromagnetic wave(EMW)absorbing materials maintaining high stability and satisfying absorbing properties is essential.This study focused on the synthesis and...Facing the complex variable high-temperature environment,electromagnetic wave(EMW)absorbing materials maintaining high stability and satisfying absorbing properties is essential.This study focused on the synthesis and EMW absorbing performance evaluation of TiN/Fe_(2)N/C composite materials,which were prepared using electrostatic spinning followed by a high-temperature nitridation process.The TiN/Fe_(2)N/C fibers constructed a well-developed conductive network that generates considerable conduction loss.The heterogeneous interfaces between different components generated a significant level of interfacial polarization.Thanks to the synergistic effect of stable dielectric loss and optimized impedance matching,the TiN/Fe_(2)N/C composite materials demonstrated excellent and stable absorption performance across a wide temperature range(293-453 K).Moreover,TiN/Fe_(2)N/C-15 achieved a minimum reflection loss(RL)of−48.01 dB and an effective absorption bandwidth(EAB)of 3.64 GHz at 2.1 mm and 373 K.This work provides new insights into the development of high-efficiency and stabile EMW absorbing materials under complex variable high-temperature conditions.展开更多
The oceanic trace metals iron(Fe),nickel(Ni),copper(Cu),zinc(Zn),and cadmium(Cd)are crucial to marine phytoplankton growth and global carbon cycle,and the analysis of their stable isotopes can provide valuable insight...The oceanic trace metals iron(Fe),nickel(Ni),copper(Cu),zinc(Zn),and cadmium(Cd)are crucial to marine phytoplankton growth and global carbon cycle,and the analysis of their stable isotopes can provide valuable insights into their biogeochemical cycles within the ocean.However,the simultaneous isotopic analysis of multiple elements present in seawater is challenging because of their low concentrations,limited volumes of the test samples,and high salt matrix.In this study,we present the novel method developed for the simultaneous analysis of five isotope systems by 1 L seawater sample.In the developed method,the NOBIAS Chelate-PA1 resin was used to extract metals from seawater,the AG MP-1M anion-exchange resin to purify Cu,Fe,Zn,Cd,and the NOBIAS Chelate-PA1 resin to further extract Ni from the matrix elements.Finally,a multi-collector inductively coupled plasma mass spectroscope(MC-ICPMS)was employed for the isotopic measurements using a doublespike technique or sample-standard bracketing combined with internal normalization.This method exhibited low total procedural blanks(0.04 pg,0.04 pg,0.21 pg,0.15 pg,and 3 pg for Ni,Cu,Fe,Zn,and Cd,respectively)and high extraction efficiencies(100.5%±0.3%,100.2%±0.5%,97.8%±1.4%,99.9%±0.8%,and 100.1%±0.2%for Ni,Cu,Fe,Zn,and Cd,respectively).The external errors and external precisions of this method could be considered negligible.The proposed method was further tested on the seawater samples obtained from the whole vertical profile of a water column during the Chinese GEOTRACES GP09 cruise in the Northwest Pacific,and the results showed good agreement with previous related data.This innovative method will contribute to the advancement of isotope research and enhance our understanding of the marine biogeochemical cycling of Fe,Ni,Cu,Zn,and Cd.展开更多
针对滚动轴承在小样本条件下诊断准确率低和泛化性弱的问题,提出了一种基于注意力特征融合的深度稳定学习(Attention Feature Fusion and Deep Stable Learning,AFF-Stablenet)模型的故障诊断方法。该方法首先使用经验模态分解(Empirica...针对滚动轴承在小样本条件下诊断准确率低和泛化性弱的问题,提出了一种基于注意力特征融合的深度稳定学习(Attention Feature Fusion and Deep Stable Learning,AFF-Stablenet)模型的故障诊断方法。该方法首先使用经验模态分解(Empirical Mode Decompositim,EMD)将样本分解成多段频率的子信号,求取子信号与原始信号的互相关系数,选择系数较高的前三阶子信号;利用连续小波变换(Continuws Narelet Transorm,CWT)将子信号转换为时频图表示,通过注意力特征融合的方式将这些时频图特征进行融合;最后将融合特征输入到深度稳定学习(Stablenet)模型进行训练与预测。为验证模型的有效性,采用凯斯西储大学轴承数据集进行各组对比试验,都灵理工大学轴承数据集进行验证。实验结果表明,AFF-Stablenet模型在小样本情况下的泛化性和鲁棒性均强于其他对比模型,证明了模型的优越性。展开更多
Rechargeable magnesium batteries(RMBs)hold promise for offering higher volumetric energy density and safety features,attracting increasing research interest as the next post lithium-ion batteries.Developing high perfo...Rechargeable magnesium batteries(RMBs)hold promise for offering higher volumetric energy density and safety features,attracting increasing research interest as the next post lithium-ion batteries.Developing high performance cathode material by inducing multi-electron reaction process as well as maintaining structural stability is the key to the development and application of RMBs.Herein,multielectron reaction occurred in VS_(4)by simple W doping strategy.W doping induces valence of partial V as V^(2+)and V^(3+)in VS_(4)structure,and then stimulates electrochemical reaction involving multi-electrons in 0.5%W-V-S.The flower-like microsphere morphology as well as rich S vacancies is also modulated by W doping to neutralize structure change in such multi-electron reaction process.The fabricated 0.5%W-V-S delivers higher specific capacity(149.3 m A h g^(-1)at 50 m A g^(-1),which is 1.6 times higher than that of VS_(4)),superior rate capability(76 mA h g^(-1)at 1000 mA g^(-1)),and stable cycling performance(1500cycles with capacity retention ratio of 93.8%).Besides that,pesudocapaticance-like contribution analysis as well as galvanostatic intermittent titration technique(GITT)further confirms the enhanced Mg^(2+)storage kinetics during such multi-electron involved electrochemical reaction process.Such discovery provides new insights into the designing of multi-electron reaction process in cathode as well as neutralizing structural change during such reaction for realizing superior electrochemical performance in energy storage devices.展开更多
Analyses of stable isotopes(C,O,H)in tree rings are increasingly important cross-disciplinary programs.The rapid development in this field documented in an increasing number of publications requires a comprehensive re...Analyses of stable isotopes(C,O,H)in tree rings are increasingly important cross-disciplinary programs.The rapid development in this field documented in an increasing number of publications requires a comprehensive review.This study includes a bibliometric analysis-based review to better understand research trends in tree ring stable isotope research.Overall,1475 publications were selected from the Web of Science Core Collection for 1974-2023.The findings are that:(1)numbers of annual publications and citations increased since 1974.From 1974 to 1980,there were around two relevant publications per year.However,from 2020 to 2022,this rose sharply to 109 publications per year.Likewise,average article citations were less than four per year before 1990,but were around four per article per year after 2000;(2)the major subjects using tree ring stable isotopes include forestry,geosciences,and environmental sciences,contributing to 42.5%of the total during 1974-2023;(3)the top three most productive institutions are the Chinese Academy of Sciences(423),the Swiss Federal Institute for Forest,Snow and Landscape Research(227),and the University of Arizona(204).These achievements result from strong collaborations;(4)review papers,for example,(Dawson et al.,Annu Rev Ecol Syst 33:507-559,2002)and(McCarroll and Loader,Quat Sci Rev 23:771-801,2004),are among the most cited,with more than 1000 citations;(5)tree ring stable isotope studies mainly focus on climatology and ecology,with atmospheric CO_(2) one of the most popular topics.Since 2010,precipitation and drought have received increasing attention.Based on this analysis,the research stages,key findings,debated issues,limitations and direc-tions for future research are summarized.This study serves as an important attempt to understand the progress on the use of stable isotopes in tree rings,providing scientific guid-ance for young researchers in this field.展开更多
The purpose of software defect prediction is to identify defect-prone code modules to assist software quality assurance teams with the appropriate allocation of resources and labor.In previous software defect predicti...The purpose of software defect prediction is to identify defect-prone code modules to assist software quality assurance teams with the appropriate allocation of resources and labor.In previous software defect prediction studies,transfer learning was effective in solving the problem of inconsistent project data distribution.However,target projects often lack sufficient data,which affects the performance of the transfer learning model.In addition,the presence of uncorrelated features between projects can decrease the prediction accuracy of the transfer learning model.To address these problems,this article propose a software defect prediction method based on stable learning(SDP-SL)that combines code visualization techniques and residual networks.This method first transforms code files into code images using code visualization techniques and then constructs a defect prediction model based on these code images.During the model training process,target project data are not required as prior knowledge.Following the principles of stable learning,this paper dynamically adjusted the weights of source project samples to eliminate dependencies between features,thereby capturing the“invariance mechanism”within the data.This approach explores the genuine relationship between code defect features and labels,thereby enhancing defect prediction performance.To evaluate the performance of SDP-SL,this article conducted comparative experiments on 10 open-source projects in the PROMISE dataset.The experimental results demonstrated that in terms of the F-measure,the proposed SDP-SL method outperformed other within-project defect prediction methods by 2.11%-44.03%.In cross-project defect prediction,the SDP-SL method provided an improvement of 5.89%-25.46% in prediction performance compared to other cross-project defect prediction methods.Therefore,SDP-SL can effectively enhance within-and cross-project defect predictions.展开更多
Understanding the hydrogen and oxygen stable isotope composition and characteristics of different water bodies in soil-plant-atmosphere continuum is of significance for revealing regional hydrological processes and wa...Understanding the hydrogen and oxygen stable isotope composition and characteristics of different water bodies in soil-plant-atmosphere continuum is of significance for revealing regional hydrological processes and water cycle mechanisms.In this study,we analyzed the stable isotopic composition,relationship and indicative significance of precipitation,soil water(0~100 cm depth)and xylem water of Qinghai spruce(Picea crassifolia)forest in the eastern Qilian Mountains,and explored the circulation process among different water bodies.The results show that the stable isotopes of precipitation vary greatly during the entire observation period.The values ofδ2H andδ^(18)O in the precipitation in the warm season are richer than those in the cold season,and the slope and intercept of local meteoric water line(LMWL,δ2H=6.79δ18O+7.13)are both smaller than global meteoric water line(GMWL,δ2H=8.17δ18O+10.56).The stable isotopes of soil water at different depths underwent different degrees of evaporative fractionation,and theδ18O andδ2H of shallow soil water varied greatly,while the deep soil water tended to be similar.The topsoil(0~10 cm)can respond quickly to precipitation,and the response of the deep soil has a time lag.In the whole growing season,0~30 cm and 60~100 cm soil water are the main water sources of Qinghai spruce.The water source of Qinghai spruce was from all soil layers in May and September,mainly from the shallow soil layer(0~30 cm)in August and October,and mainly from the deep soil layer(60~100 cm)in June and July.展开更多
Zhanjiang Bay is a major aquaculture area in China with many types of mariculture products(such as oysters,fish,and shrimp).The culture area and shrimp output in Zhanjiang Bay are ranked first in China.We investigated...Zhanjiang Bay is a major aquaculture area in China with many types of mariculture products(such as oysters,fish,and shrimp).The culture area and shrimp output in Zhanjiang Bay are ranked first in China.We investigated the total organic carbon(TOC),total nitrogen(TN),TOC/TN ratio,and stable isotopes(δ^(13)C and δ^(15)N) of the fish and shrimp feed,fish and shrimp feces,and sedimentary organic matter(SOM) in and around different aquaculture areas of northeastern Zhanjiang B ay to study the impact of aquaculture activities on SOM.The average TOC contents of fish and shrimp feed were 39.20%±0.91% and 39.29%±0.21%,respectively.The average TOC content in the surface sediments of the oyster culture area,the mixed(fish and shrimp) culture area,and the cage fish farm area were 0.66%,0.88%±0.10%,and 0.58%±0.19%,respectively,which may indicate that mixed culture had a greater impact on SOM.The relatively high TOC and TN contents and relatively low TOC/TN ratios,and δ^(15)N values in the upper layer of the core sediment in the mixed culture area could also support the significant influence of mixed culture.The average δ^(13)C and δ^(15)N values of fish and shrimp feed were -20.6‰±2.2‰ and 1.8‰±1.2‰,respectively,which were different from the isotopic values of SOM in the study area.δ^(13)C and δ^(15)N values for SOM in different aquaculture areas were different from those of nearby reference stations,probably reflecting the influence of aquaculture.The δ^(13)C and δ^(15)N values in the oyster culture area(-25.9‰ and6.0‰,respectively) seemed to have reduced δ^(13)C and enriched δ^(15)N relative to those of the reference station(-24.6‰ and 5.8‰,respectively).This may reflect the influence of organic matter on oyster culture.The δ^(15)N value of the station in the mixed culture area(7.1‰±0.4‰) seemed to be relatively enriched in δ^(15)N relative to that of the reference station(6.6‰).Sedimentation and the subsequent degradation of organic matter from mixed cultures may have contributed to this phenomenon.The surface sediment at the cage fish farm area seemed to be affected by fish feces and primary production based on the indication of δ^(13)C and δ^(15)N values.The sediment core at the mixed culture region(NS6) had lower TOC/TN ratios and more positive δ^(13)C and δ^(15)N values than the sediment core at the oyster culture area,suggesting a higher proportionate contribution of marine organic matter in the mixed culture area.In summary,oyster culture,mixed culture,and cage fish culture in northeastern Zhanjiang Bay had a certain degree of impact on SOM,and mixed culture had more significant influences on SOM based on the high TOC contents and the significant vertical variations of TOC/TN ratio and δ^(15)N value in the sediment of this area.This study provides new insights into the impact of aquaculture activities on SOM content.展开更多
Understanding the relationship between forest management and water use efficiency(WUE)is important for evaluating forest adaptability to climate change.However,the effects of thinning and understory removal on WUE and...Understanding the relationship between forest management and water use efficiency(WUE)is important for evaluating forest adaptability to climate change.However,the effects of thinning and understory removal on WUE and its key controlling processes are not well understood,which limits our comprehension of the physiological mechanisms of various management practices.In this study,four forest management measures(no thinning:NT;understory removal:UR;light thinning:LT;and heavy thinning:HT)were carried out in Pinus massoniana plantations in a subtropical region of China.Photosynthetic capacity and needle stable carbon isotope composition(δ^(13)C)were measured to assess instantaneous water use efficiency(WUE_(inst))and long-term water use efficiency(WUE_(i)).Multiple regression models and structural equation modelling(SEM)identified the effects of soil properties and physiological performances on WUE_(inst)and WUE_(i).The results show that WUE_(inst)values among the four treatments were insignificant.However,compared with the NT stand(35.8μmol·mol^(-1)),WUE_(i)values significantly increased to 41.7μmol·mol^(-1)in the UR,50.1μmol·mol^(-1)in the LT and 46.6μmol·mol^(-1)in HT treatments,largely explained by photosynthetic capacity and soil water content.Understory removal did not change physiological performance(needle water potential and photosynthetic capacity).Thinning increased the net photosynthetic rate(A_n)but not stomatal conductance(g_s)or predawn needle water potential(ψ_(pd)),implying that the improvement in water use efficiency for thinned stands was largely driven by radiation interception than by soil water availability.In general,thinning may be an appropriate management measure to promote P.massoniana WUE to cope with seasonal droughts under future extreme climates.展开更多
Background,aim,and scope Stable isotope in water could respond sensitively to the variation of environment and be reserved in different geological archives,although they are scarce in the environment.And the methods d...Background,aim,and scope Stable isotope in water could respond sensitively to the variation of environment and be reserved in different geological archives,although they are scarce in the environment.And the methods derived from the stable isotope composition of water have been widely applied in researches on hydrometeorology,weather diagnosis,and paleoclimate reconstruction,which help well for understanding the water-cycle processes in one region.Here,it is aimed to explore the temporal changes of stable isotopes in precipitation from Adelaide,Australia and determine the influencing factors at different timescales.Materials and methods Based on the isotopic data of daily precipitation over four years collected in Adelaide,Australia,the variation characteristics of dailyδD,δ^(18)O,and dexcess in precipitation and its relationship with meteorological elements were analyzed.Results The results demonstrated the local meteoric water line(LMWL)in Adelaide,wasδD=6.38×δ^(18)O+6.68,with a gradient less than 8.There is a significant negative correlation between dailyδ^(18)O and precipitation amount or relative humidity at daily timescales in both the whole year and wither/summerhalf year(p<0.001),but a significant positive correlation between dailyδ^(18)O and temperature in the whole year and the winter half-year(p<0.001).Discussion The correlation coefficients betweenδ^(18)O and daily mean temperature didn’t show a significant positive correlation,which may be attributed to that the precipitation in Adelaide area in January was mainly influenced by strong convective weather,and the stable isotope values in precipitation were significantly negative.Furthermore,this propose was also evidenced by the results from dexcess of precipitation with larger value in the winter half-year than that in the summer half-year,which may be resulted from the precipitation events in winter are mostly influenced by oceanic water vapor,while the sources of water vapor in summer precipitation events are more complicated and influenced by strong convective weather.On the other hand,the slope and intercept of theδ^(18)O—P regression lines in the summer months(-0.41 and 0.50‰)are larger and smaller than those in the winter months(-0.22 and-2.15‰),respectively,indicating that the precipitation stable isotopes have a relatively stronger rainout effect in the summer months than in the winter months.Besides,the measured values ofδ^(18)O in daily precipitation have a good linear relationship with our simulated values ofδ^(18)O,demonstrating the established regression model could provide a reliable simulation for theδ^(18)O values in daily precipitation in Adelaide area.It’s worth noting that the precipitation events with low precipitation amount,low relative humidity and high temperature,usually had relatively small slope and intercept of MWL,implying that raindrops may be strongly affected by sub-cloud secondary evaporation in the falling process.Conclusions The variation ofδ^(18)O in daily precipitation from Adelaide region was controlled by different factors at different timescales.And the water vapor sources and the meteorological conditions of precipitation events(such as the degree of sub-cloud secondary evaporation)also played an important role on the variation ofδ^(18)O.Recommendations and perspectives Stable isotope in daily precipitation can provide more accurate information about water-cycle and atmosphere circulation,it is therefore necessary to continue to collect and analyze daily-scale precipitation data over a longer time span.The results of this study will provide the basis for the fields of hydrometeorology,meteorological diagnosis and paleoclimate reconstruction in Adelaide,Australia.展开更多
ZiZiphus jujuba,which is native to China,has become one of the main crops widely planted in the western Loess Plateau because of its drought and flood-tolerance,adaptability,and higher nutritional value of the fruit.T...ZiZiphus jujuba,which is native to China,has become one of the main crops widely planted in the western Loess Plateau because of its drought and flood-tolerance,adaptability,and higher nutritional value of the fruit.The irrigation water infiltration in Z.jujuba gardens is complex,and understanding its mechanisms is essential for efficient water use and sustainable agriculture.This knowledge helps ensure the long-term success of jujuba cultivation.This paper describes a field experiment that investigates the infiltration process of irrigation water from Z.jujuba garden and quantifies the contribution of irrigation water to soil water at different depths using the MixSIAR model.According to the FC(Field water holding Capacity)of Z.jujuba,irrigation experiments with three volumes of 80%FC,60%FC,and 40%FC are set up in this study.The study finds that water retention is better in Z.jujuba garden soils with a higher proportion of coarse gravel in the soil particle composition.Soil water content exhibits a gradient change after irrigation,with deeper wetting front transport depth observed with increased irrigation water.Additionally,there is correlation between soil temperature and soil water content.The soil water in Z.jujuba garden generally exhibits a preferential flow signal in the 0-40 cm range.Below 40 cm,a piston flow pattern dominates.The rate of soil water infiltration increases with the amount of irrigation water.In the 0-40 cm range of the soil vertical profile,irrigation water was the main contributor to soil water.Z.jujuba demonstrated flexibility in water uptake,primarily absorbing soil water at depths of 0-40 cm.For optimal growth of Z.jujuba at this stage,40%FC irrigation is recommended.The results are expected to be valuable future irrigation practices and land use planning for Z.jujuba garden in arid zones,supporting sustainable agricultural development and water management.展开更多
A mass flow matching model(MFMM)was established for studying the stable status of solution electrospinning.The study of the solution droplet status at the needle tip focused on various combinations of applied voltages...A mass flow matching model(MFMM)was established for studying the stable status of solution electrospinning.The study of the solution droplet status at the needle tip focused on various combinations of applied voltages and injection rates to figure out their influence on steadily fabricating polyvinyl alcohol(PVA)nanofibers prepared from PVA spinning solutions with two different mass fractions(10%and 16%).The results revealed that during the stable electrospinning,the influence resulted from the change of the injection rate approximately canceled out the impact brought by adjusting the applied voltage,leading to almost the same morphology as that of the PVA nanofibers.And the mass fraction of PVA in the spinning solution dominated the structure and the diameter distribution of the electrospun nanofibers.Under stable electrospinning conditions,the composite membrane was produced by depositing PVA nanofibers on the polyethylene terephthalate(PET)nonwoven substrate for an air filtration test.Furthermore,the prepared composite membrane exhibited a high air filtration efficiency(99.97%)and a low pressure drop(120 Pa)for 300-500 nm neutralized polystyrene latex(PSL)aerosol particles,demonstrating its potential as an alternative for a variety of commercial applications in air filtration.展开更多
Ultrathin and air-stable Li metal anodes hold great promise toward high-energy and high-safety Li metal batteries(LMBs).However,the application of LMBs is technically impeded by existing Li metal anodes with large thi...Ultrathin and air-stable Li metal anodes hold great promise toward high-energy and high-safety Li metal batteries(LMBs).However,the application of LMBs is technically impeded by existing Li metal anodes with large thickness,high reactivity,and poor performance.Here,we developed a novel and scalable approach for the construction of a 10-μm-thick flexible and air-stable Li metal anode by conformally encapsulating Li within a multifunctional VN film.Specifically,the highly lithiophilic VN layer guides a uniform deposition of Li,while abundant and multilevel pores arising from assembly of ultrathin nanosheets enable a spatially confined immersion of metallic Li,thus ensuring an ultrathin and sandwiched Li anode.More impressively,the strong hydrophobicity of VN surface can effectively improve the stability of anode to humid air,whereas the highly conductive framework greatly boosts charge transfer dynamics and enhances Li utilization and high-rate capability.Benefiting from such fascinating features,the constructed Li-VN anode exhibits ultrastable cycling stability in both ether(2500 h)and carbonate(900 h)electrolytes,respectively.Moreover,even exposed to ambient air for 12 h,the anode still can retain~78%capacity,demonstrating excellent air-defendable capability.This work affords a promising strategy for fabricating high-performance,high-safety,and low-cost LMBs.展开更多
In this paper,a stable two-sided matching(TSM)method considering the matching intention of agents under a hesitant fuzzy environment is proposed.The method uses a hesitant fuzzy element(HFE)as its basis.First,the HFE ...In this paper,a stable two-sided matching(TSM)method considering the matching intention of agents under a hesitant fuzzy environment is proposed.The method uses a hesitant fuzzy element(HFE)as its basis.First,the HFE preference matrix is transformed into the normalized HFE preference matrix.On this basis,the distance and the projection of the normalized HFEs on positive and negative ideal solutions are calculated.Then,the normalized HFEs are transformed into agent satisfactions.Considering the stable matching constraints,a multiobjective programming model with the objective of maximizing the satisfactions of two-sided agents is constructed.Based on the agent satisfaction matrix,the matching intention matrix of two-sided agents is built.According to the agent satisfaction matrix and matching intention matrix,the comprehensive satisfaction matrix is set up.Furthermore,the multiobjective programming model based on satisfactions is transformed into a multiobjective programming model based on comprehensive satisfactions.Using the G-S algorithm,the multiobjective programming model based on comprehensive satisfactions is solved,and then the best TSM scheme is obtained.Finally,a terminal distribution example is used to verify the feasibility and effectiveness of the proposed method.展开更多
基金supported the National Natural Science Foundation of China (42022059,41888101)the Strategic Priority Research Program of the Chinese Academy of Sciences,China (Grant No.XDB26020000)+1 种基金the Key Research Program of the Institute of Geology and Geophysics (CAS Grant IGGCAS-201905)the CAS Youth Interdisciplinary Team (JCTD-2021-05).
文摘Tree-ring width(RW),density,elemental com-position,and stable carbon and oxygen isotope(δ^(13)C,δ^(18)O)are widely used as proxies to assess climate change,ecology,and environmental pollution;however,a specific pretreat-ment has been needed for each proxy.Here,we developed a method by which each proxy can be measured in the same sample.First,the sample is polished for ring width meas-urement.After obtaining the ring width data,the sample is cut to form a 1-mm-thick wood plate.The sample is then mounted in a vertical sample holder,and gradually scanned by an X-ray beam.Simultaneously,the count rates of the fluorescent photons of elements(for chemical characteriza-tion)and a radiographic grayscale image(for wood density)are obtained,i.e.the density and the element content are obtained.Then,cellulose is isolated from the 1-mm wood plate by removal of lignin,and hemicellulose.After producing this cellulose plate,cellulose subsamples are separated by knife under the microscope for inter-annual and intra-annual stable carbon and oxygen isotope(δ^(13)C,δ^(18)O)analysis.Based on this method,RW,density,elemental composition,δ^(13)C,and δ^(18)O can be measured from the same sample,which reduces sample amount and treatment time,and is helpful for multi-proxy comparison and combination research.
基金financially supported by the Natural Science Foundation of Henan Province Youth Fund of China(No.242300421466)the Key Scientific Research Project Plan in Universities of Henan Province,China(No.23A430037)+1 种基金the Research Project of Xuchang University,China(No.2024ZD004)the College Students’Innovation and Entrepreneurship Training Program of China(No.202410480008).
文摘Facing the complex variable high-temperature environment,electromagnetic wave(EMW)absorbing materials maintaining high stability and satisfying absorbing properties is essential.This study focused on the synthesis and EMW absorbing performance evaluation of TiN/Fe_(2)N/C composite materials,which were prepared using electrostatic spinning followed by a high-temperature nitridation process.The TiN/Fe_(2)N/C fibers constructed a well-developed conductive network that generates considerable conduction loss.The heterogeneous interfaces between different components generated a significant level of interfacial polarization.Thanks to the synergistic effect of stable dielectric loss and optimized impedance matching,the TiN/Fe_(2)N/C composite materials demonstrated excellent and stable absorption performance across a wide temperature range(293-453 K).Moreover,TiN/Fe_(2)N/C-15 achieved a minimum reflection loss(RL)of−48.01 dB and an effective absorption bandwidth(EAB)of 3.64 GHz at 2.1 mm and 373 K.This work provides new insights into the development of high-efficiency and stabile EMW absorbing materials under complex variable high-temperature conditions.
基金The National Key Research and Development Program of China under contract No.2022YFE0136500the National Nature Science Foundation of China under contract Nos 41890801 and 42076227the Shanghai Pilot Program for Basic Research-Shanghai Jiao Tong University under contract No.21TQ1400201.
文摘The oceanic trace metals iron(Fe),nickel(Ni),copper(Cu),zinc(Zn),and cadmium(Cd)are crucial to marine phytoplankton growth and global carbon cycle,and the analysis of their stable isotopes can provide valuable insights into their biogeochemical cycles within the ocean.However,the simultaneous isotopic analysis of multiple elements present in seawater is challenging because of their low concentrations,limited volumes of the test samples,and high salt matrix.In this study,we present the novel method developed for the simultaneous analysis of five isotope systems by 1 L seawater sample.In the developed method,the NOBIAS Chelate-PA1 resin was used to extract metals from seawater,the AG MP-1M anion-exchange resin to purify Cu,Fe,Zn,Cd,and the NOBIAS Chelate-PA1 resin to further extract Ni from the matrix elements.Finally,a multi-collector inductively coupled plasma mass spectroscope(MC-ICPMS)was employed for the isotopic measurements using a doublespike technique or sample-standard bracketing combined with internal normalization.This method exhibited low total procedural blanks(0.04 pg,0.04 pg,0.21 pg,0.15 pg,and 3 pg for Ni,Cu,Fe,Zn,and Cd,respectively)and high extraction efficiencies(100.5%±0.3%,100.2%±0.5%,97.8%±1.4%,99.9%±0.8%,and 100.1%±0.2%for Ni,Cu,Fe,Zn,and Cd,respectively).The external errors and external precisions of this method could be considered negligible.The proposed method was further tested on the seawater samples obtained from the whole vertical profile of a water column during the Chinese GEOTRACES GP09 cruise in the Northwest Pacific,and the results showed good agreement with previous related data.This innovative method will contribute to the advancement of isotope research and enhance our understanding of the marine biogeochemical cycling of Fe,Ni,Cu,Zn,and Cd.
基金supported by the National Natural Science Foundation of China under Grant No.52072196,52002200,52102106,52202262,22379081,and 22379080Major Basic Research Program of the Natural Science Foundation of Shandong Province under Grant No.ZR2020ZD09+1 种基金the Natural Science Foundation of Shandong Province under Grant No.ZR2020QE063,ZR202108180009,ZR2023QE059the Postdoctoral Program in Qingdao under No.QDBSH20220202019。
文摘Rechargeable magnesium batteries(RMBs)hold promise for offering higher volumetric energy density and safety features,attracting increasing research interest as the next post lithium-ion batteries.Developing high performance cathode material by inducing multi-electron reaction process as well as maintaining structural stability is the key to the development and application of RMBs.Herein,multielectron reaction occurred in VS_(4)by simple W doping strategy.W doping induces valence of partial V as V^(2+)and V^(3+)in VS_(4)structure,and then stimulates electrochemical reaction involving multi-electrons in 0.5%W-V-S.The flower-like microsphere morphology as well as rich S vacancies is also modulated by W doping to neutralize structure change in such multi-electron reaction process.The fabricated 0.5%W-V-S delivers higher specific capacity(149.3 m A h g^(-1)at 50 m A g^(-1),which is 1.6 times higher than that of VS_(4)),superior rate capability(76 mA h g^(-1)at 1000 mA g^(-1)),and stable cycling performance(1500cycles with capacity retention ratio of 93.8%).Besides that,pesudocapaticance-like contribution analysis as well as galvanostatic intermittent titration technique(GITT)further confirms the enhanced Mg^(2+)storage kinetics during such multi-electron involved electrochemical reaction process.Such discovery provides new insights into the designing of multi-electron reaction process in cathode as well as neutralizing structural change during such reaction for realizing superior electrochemical performance in energy storage devices.
基金This study was supported by the National Natural Science Foundation of China(Grant Number:42007407,42022059)the Sino-German mobility program(M-0393)+1 种基金the Key Research Program of the Institute of Geology and Geophysics(CAS Grant IGGCAS-201905)the CAS Youth Interdisciplinary Team(JCTD-2021-05).
文摘Analyses of stable isotopes(C,O,H)in tree rings are increasingly important cross-disciplinary programs.The rapid development in this field documented in an increasing number of publications requires a comprehensive review.This study includes a bibliometric analysis-based review to better understand research trends in tree ring stable isotope research.Overall,1475 publications were selected from the Web of Science Core Collection for 1974-2023.The findings are that:(1)numbers of annual publications and citations increased since 1974.From 1974 to 1980,there were around two relevant publications per year.However,from 2020 to 2022,this rose sharply to 109 publications per year.Likewise,average article citations were less than four per year before 1990,but were around four per article per year after 2000;(2)the major subjects using tree ring stable isotopes include forestry,geosciences,and environmental sciences,contributing to 42.5%of the total during 1974-2023;(3)the top three most productive institutions are the Chinese Academy of Sciences(423),the Swiss Federal Institute for Forest,Snow and Landscape Research(227),and the University of Arizona(204).These achievements result from strong collaborations;(4)review papers,for example,(Dawson et al.,Annu Rev Ecol Syst 33:507-559,2002)and(McCarroll and Loader,Quat Sci Rev 23:771-801,2004),are among the most cited,with more than 1000 citations;(5)tree ring stable isotope studies mainly focus on climatology and ecology,with atmospheric CO_(2) one of the most popular topics.Since 2010,precipitation and drought have received increasing attention.Based on this analysis,the research stages,key findings,debated issues,limitations and direc-tions for future research are summarized.This study serves as an important attempt to understand the progress on the use of stable isotopes in tree rings,providing scientific guid-ance for young researchers in this field.
基金supported by the NationalNatural Science Foundation of China(Grant No.61867004)the Youth Fund of the National Natural Science Foundation of China(Grant No.41801288).
文摘The purpose of software defect prediction is to identify defect-prone code modules to assist software quality assurance teams with the appropriate allocation of resources and labor.In previous software defect prediction studies,transfer learning was effective in solving the problem of inconsistent project data distribution.However,target projects often lack sufficient data,which affects the performance of the transfer learning model.In addition,the presence of uncorrelated features between projects can decrease the prediction accuracy of the transfer learning model.To address these problems,this article propose a software defect prediction method based on stable learning(SDP-SL)that combines code visualization techniques and residual networks.This method first transforms code files into code images using code visualization techniques and then constructs a defect prediction model based on these code images.During the model training process,target project data are not required as prior knowledge.Following the principles of stable learning,this paper dynamically adjusted the weights of source project samples to eliminate dependencies between features,thereby capturing the“invariance mechanism”within the data.This approach explores the genuine relationship between code defect features and labels,thereby enhancing defect prediction performance.To evaluate the performance of SDP-SL,this article conducted comparative experiments on 10 open-source projects in the PROMISE dataset.The experimental results demonstrated that in terms of the F-measure,the proposed SDP-SL method outperformed other within-project defect prediction methods by 2.11%-44.03%.In cross-project defect prediction,the SDP-SL method provided an improvement of 5.89%-25.46% in prediction performance compared to other cross-project defect prediction methods.Therefore,SDP-SL can effectively enhance within-and cross-project defect predictions.
基金supported by the National Natural Science Foundation of China(Grant Nos.41761047,41861040 and 41861034).
文摘Understanding the hydrogen and oxygen stable isotope composition and characteristics of different water bodies in soil-plant-atmosphere continuum is of significance for revealing regional hydrological processes and water cycle mechanisms.In this study,we analyzed the stable isotopic composition,relationship and indicative significance of precipitation,soil water(0~100 cm depth)and xylem water of Qinghai spruce(Picea crassifolia)forest in the eastern Qilian Mountains,and explored the circulation process among different water bodies.The results show that the stable isotopes of precipitation vary greatly during the entire observation period.The values ofδ2H andδ^(18)O in the precipitation in the warm season are richer than those in the cold season,and the slope and intercept of local meteoric water line(LMWL,δ2H=6.79δ18O+7.13)are both smaller than global meteoric water line(GMWL,δ2H=8.17δ18O+10.56).The stable isotopes of soil water at different depths underwent different degrees of evaporative fractionation,and theδ18O andδ2H of shallow soil water varied greatly,while the deep soil water tended to be similar.The topsoil(0~10 cm)can respond quickly to precipitation,and the response of the deep soil has a time lag.In the whole growing season,0~30 cm and 60~100 cm soil water are the main water sources of Qinghai spruce.The water source of Qinghai spruce was from all soil layers in May and September,mainly from the shallow soil layer(0~30 cm)in August and October,and mainly from the deep soil layer(60~100 cm)in June and July.
基金The National Natural Science Foundation of China under contract No.42276047the Guangdong Basic and Applied Basic Research Foundation under contract Nos 2023A1515110473 and 2021A1515110172+1 种基金the Program for Scientific Research Start-up Funds of Guangdong Ocean University under contract No.R17058the National College Student Innovation and Entrepreneurship Training Program Project under contract No.202310566007。
文摘Zhanjiang Bay is a major aquaculture area in China with many types of mariculture products(such as oysters,fish,and shrimp).The culture area and shrimp output in Zhanjiang Bay are ranked first in China.We investigated the total organic carbon(TOC),total nitrogen(TN),TOC/TN ratio,and stable isotopes(δ^(13)C and δ^(15)N) of the fish and shrimp feed,fish and shrimp feces,and sedimentary organic matter(SOM) in and around different aquaculture areas of northeastern Zhanjiang B ay to study the impact of aquaculture activities on SOM.The average TOC contents of fish and shrimp feed were 39.20%±0.91% and 39.29%±0.21%,respectively.The average TOC content in the surface sediments of the oyster culture area,the mixed(fish and shrimp) culture area,and the cage fish farm area were 0.66%,0.88%±0.10%,and 0.58%±0.19%,respectively,which may indicate that mixed culture had a greater impact on SOM.The relatively high TOC and TN contents and relatively low TOC/TN ratios,and δ^(15)N values in the upper layer of the core sediment in the mixed culture area could also support the significant influence of mixed culture.The average δ^(13)C and δ^(15)N values of fish and shrimp feed were -20.6‰±2.2‰ and 1.8‰±1.2‰,respectively,which were different from the isotopic values of SOM in the study area.δ^(13)C and δ^(15)N values for SOM in different aquaculture areas were different from those of nearby reference stations,probably reflecting the influence of aquaculture.The δ^(13)C and δ^(15)N values in the oyster culture area(-25.9‰ and6.0‰,respectively) seemed to have reduced δ^(13)C and enriched δ^(15)N relative to those of the reference station(-24.6‰ and 5.8‰,respectively).This may reflect the influence of organic matter on oyster culture.The δ^(15)N value of the station in the mixed culture area(7.1‰±0.4‰) seemed to be relatively enriched in δ^(15)N relative to that of the reference station(6.6‰).Sedimentation and the subsequent degradation of organic matter from mixed cultures may have contributed to this phenomenon.The surface sediment at the cage fish farm area seemed to be affected by fish feces and primary production based on the indication of δ^(13)C and δ^(15)N values.The sediment core at the mixed culture region(NS6) had lower TOC/TN ratios and more positive δ^(13)C and δ^(15)N values than the sediment core at the oyster culture area,suggesting a higher proportionate contribution of marine organic matter in the mixed culture area.In summary,oyster culture,mixed culture,and cage fish culture in northeastern Zhanjiang Bay had a certain degree of impact on SOM,and mixed culture had more significant influences on SOM based on the high TOC contents and the significant vertical variations of TOC/TN ratio and δ^(15)N value in the sediment of this area.This study provides new insights into the impact of aquaculture activities on SOM content.
基金supported by the National Key Research and Development Program of China(2016YFD0600201)the National Nonprofit Institute Research Grant of CAF(CAFYBB2017ZB003)+1 种基金the National Natural Science Foundation of China(3187071631670720)。
文摘Understanding the relationship between forest management and water use efficiency(WUE)is important for evaluating forest adaptability to climate change.However,the effects of thinning and understory removal on WUE and its key controlling processes are not well understood,which limits our comprehension of the physiological mechanisms of various management practices.In this study,four forest management measures(no thinning:NT;understory removal:UR;light thinning:LT;and heavy thinning:HT)were carried out in Pinus massoniana plantations in a subtropical region of China.Photosynthetic capacity and needle stable carbon isotope composition(δ^(13)C)were measured to assess instantaneous water use efficiency(WUE_(inst))and long-term water use efficiency(WUE_(i)).Multiple regression models and structural equation modelling(SEM)identified the effects of soil properties and physiological performances on WUE_(inst)and WUE_(i).The results show that WUE_(inst)values among the four treatments were insignificant.However,compared with the NT stand(35.8μmol·mol^(-1)),WUE_(i)values significantly increased to 41.7μmol·mol^(-1)in the UR,50.1μmol·mol^(-1)in the LT and 46.6μmol·mol^(-1)in HT treatments,largely explained by photosynthetic capacity and soil water content.Understory removal did not change physiological performance(needle water potential and photosynthetic capacity).Thinning increased the net photosynthetic rate(A_n)but not stomatal conductance(g_s)or predawn needle water potential(ψ_(pd)),implying that the improvement in water use efficiency for thinned stands was largely driven by radiation interception than by soil water availability.In general,thinning may be an appropriate management measure to promote P.massoniana WUE to cope with seasonal droughts under future extreme climates.
文摘Background,aim,and scope Stable isotope in water could respond sensitively to the variation of environment and be reserved in different geological archives,although they are scarce in the environment.And the methods derived from the stable isotope composition of water have been widely applied in researches on hydrometeorology,weather diagnosis,and paleoclimate reconstruction,which help well for understanding the water-cycle processes in one region.Here,it is aimed to explore the temporal changes of stable isotopes in precipitation from Adelaide,Australia and determine the influencing factors at different timescales.Materials and methods Based on the isotopic data of daily precipitation over four years collected in Adelaide,Australia,the variation characteristics of dailyδD,δ^(18)O,and dexcess in precipitation and its relationship with meteorological elements were analyzed.Results The results demonstrated the local meteoric water line(LMWL)in Adelaide,wasδD=6.38×δ^(18)O+6.68,with a gradient less than 8.There is a significant negative correlation between dailyδ^(18)O and precipitation amount or relative humidity at daily timescales in both the whole year and wither/summerhalf year(p<0.001),but a significant positive correlation between dailyδ^(18)O and temperature in the whole year and the winter half-year(p<0.001).Discussion The correlation coefficients betweenδ^(18)O and daily mean temperature didn’t show a significant positive correlation,which may be attributed to that the precipitation in Adelaide area in January was mainly influenced by strong convective weather,and the stable isotope values in precipitation were significantly negative.Furthermore,this propose was also evidenced by the results from dexcess of precipitation with larger value in the winter half-year than that in the summer half-year,which may be resulted from the precipitation events in winter are mostly influenced by oceanic water vapor,while the sources of water vapor in summer precipitation events are more complicated and influenced by strong convective weather.On the other hand,the slope and intercept of theδ^(18)O—P regression lines in the summer months(-0.41 and 0.50‰)are larger and smaller than those in the winter months(-0.22 and-2.15‰),respectively,indicating that the precipitation stable isotopes have a relatively stronger rainout effect in the summer months than in the winter months.Besides,the measured values ofδ^(18)O in daily precipitation have a good linear relationship with our simulated values ofδ^(18)O,demonstrating the established regression model could provide a reliable simulation for theδ^(18)O values in daily precipitation in Adelaide area.It’s worth noting that the precipitation events with low precipitation amount,low relative humidity and high temperature,usually had relatively small slope and intercept of MWL,implying that raindrops may be strongly affected by sub-cloud secondary evaporation in the falling process.Conclusions The variation ofδ^(18)O in daily precipitation from Adelaide region was controlled by different factors at different timescales.And the water vapor sources and the meteorological conditions of precipitation events(such as the degree of sub-cloud secondary evaporation)also played an important role on the variation ofδ^(18)O.Recommendations and perspectives Stable isotope in daily precipitation can provide more accurate information about water-cycle and atmosphere circulation,it is therefore necessary to continue to collect and analyze daily-scale precipitation data over a longer time span.The results of this study will provide the basis for the fields of hydrometeorology,meteorological diagnosis and paleoclimate reconstruction in Adelaide,Australia.
基金funded by the National Natural Science Foundation of China(Grant No.42071047 and 41771035)the Basic Research Innovation Group Project of Gansu Province(Grant No.22JR5RA129).
文摘ZiZiphus jujuba,which is native to China,has become one of the main crops widely planted in the western Loess Plateau because of its drought and flood-tolerance,adaptability,and higher nutritional value of the fruit.The irrigation water infiltration in Z.jujuba gardens is complex,and understanding its mechanisms is essential for efficient water use and sustainable agriculture.This knowledge helps ensure the long-term success of jujuba cultivation.This paper describes a field experiment that investigates the infiltration process of irrigation water from Z.jujuba garden and quantifies the contribution of irrigation water to soil water at different depths using the MixSIAR model.According to the FC(Field water holding Capacity)of Z.jujuba,irrigation experiments with three volumes of 80%FC,60%FC,and 40%FC are set up in this study.The study finds that water retention is better in Z.jujuba garden soils with a higher proportion of coarse gravel in the soil particle composition.Soil water content exhibits a gradient change after irrigation,with deeper wetting front transport depth observed with increased irrigation water.Additionally,there is correlation between soil temperature and soil water content.The soil water in Z.jujuba garden generally exhibits a preferential flow signal in the 0-40 cm range.Below 40 cm,a piston flow pattern dominates.The rate of soil water infiltration increases with the amount of irrigation water.In the 0-40 cm range of the soil vertical profile,irrigation water was the main contributor to soil water.Z.jujuba demonstrated flexibility in water uptake,primarily absorbing soil water at depths of 0-40 cm.For optimal growth of Z.jujuba at this stage,40%FC irrigation is recommended.The results are expected to be valuable future irrigation practices and land use planning for Z.jujuba garden in arid zones,supporting sustainable agricultural development and water management.
文摘A mass flow matching model(MFMM)was established for studying the stable status of solution electrospinning.The study of the solution droplet status at the needle tip focused on various combinations of applied voltages and injection rates to figure out their influence on steadily fabricating polyvinyl alcohol(PVA)nanofibers prepared from PVA spinning solutions with two different mass fractions(10%and 16%).The results revealed that during the stable electrospinning,the influence resulted from the change of the injection rate approximately canceled out the impact brought by adjusting the applied voltage,leading to almost the same morphology as that of the PVA nanofibers.And the mass fraction of PVA in the spinning solution dominated the structure and the diameter distribution of the electrospun nanofibers.Under stable electrospinning conditions,the composite membrane was produced by depositing PVA nanofibers on the polyethylene terephthalate(PET)nonwoven substrate for an air filtration test.Furthermore,the prepared composite membrane exhibited a high air filtration efficiency(99.97%)and a low pressure drop(120 Pa)for 300-500 nm neutralized polystyrene latex(PSL)aerosol particles,demonstrating its potential as an alternative for a variety of commercial applications in air filtration.
基金financialy supported by National Natural Science Foundation of China(52002297,51974208,and 21875080)Wuhan Yellow Crane Talents ProgramNumerical calculation is supported by High-Performance Computing Center of Wuhan University of Science and Technology)
文摘Ultrathin and air-stable Li metal anodes hold great promise toward high-energy and high-safety Li metal batteries(LMBs).However,the application of LMBs is technically impeded by existing Li metal anodes with large thickness,high reactivity,and poor performance.Here,we developed a novel and scalable approach for the construction of a 10-μm-thick flexible and air-stable Li metal anode by conformally encapsulating Li within a multifunctional VN film.Specifically,the highly lithiophilic VN layer guides a uniform deposition of Li,while abundant and multilevel pores arising from assembly of ultrathin nanosheets enable a spatially confined immersion of metallic Li,thus ensuring an ultrathin and sandwiched Li anode.More impressively,the strong hydrophobicity of VN surface can effectively improve the stability of anode to humid air,whereas the highly conductive framework greatly boosts charge transfer dynamics and enhances Li utilization and high-rate capability.Benefiting from such fascinating features,the constructed Li-VN anode exhibits ultrastable cycling stability in both ether(2500 h)and carbonate(900 h)electrolytes,respectively.Moreover,even exposed to ambient air for 12 h,the anode still can retain~78%capacity,demonstrating excellent air-defendable capability.This work affords a promising strategy for fabricating high-performance,high-safety,and low-cost LMBs.
基金supported by the National Natural Science Foundation of China (Grant No.71861015)the Humanities and Social Science Foundation of the Ministry of Education of China (Grant No.18YJA630047)the Distinguished Young Scholar Talent of Jiangxi Province (Grant No.20192BCBL23008).
文摘In this paper,a stable two-sided matching(TSM)method considering the matching intention of agents under a hesitant fuzzy environment is proposed.The method uses a hesitant fuzzy element(HFE)as its basis.First,the HFE preference matrix is transformed into the normalized HFE preference matrix.On this basis,the distance and the projection of the normalized HFEs on positive and negative ideal solutions are calculated.Then,the normalized HFEs are transformed into agent satisfactions.Considering the stable matching constraints,a multiobjective programming model with the objective of maximizing the satisfactions of two-sided agents is constructed.Based on the agent satisfaction matrix,the matching intention matrix of two-sided agents is built.According to the agent satisfaction matrix and matching intention matrix,the comprehensive satisfaction matrix is set up.Furthermore,the multiobjective programming model based on satisfactions is transformed into a multiobjective programming model based on comprehensive satisfactions.Using the G-S algorithm,the multiobjective programming model based on comprehensive satisfactions is solved,and then the best TSM scheme is obtained.Finally,a terminal distribution example is used to verify the feasibility and effectiveness of the proposed method.