On 20 July 2021,northern Henan Province in China experienced catastrophic flooding as a result of an extremely intense rainstorm,with a record-breaking hourly rainfall of 201.9 mm during 0800–0900 UTC and daily accum...On 20 July 2021,northern Henan Province in China experienced catastrophic flooding as a result of an extremely intense rainstorm,with a record-breaking hourly rainfall of 201.9 mm during 0800–0900 UTC and daily accumulated rainfall in Zhengzhou City exceeding 600 mm(“Zhengzhou 7.20 rainstorm”for short).The multi-scale dynamical and thermodynamical mechanisms for this rainstorm are investigated based on station-observed and ERA-5 reanalysis datasets.The backward trajectory tracking shows that the warm,moist air from the northwestern Pacific was mainly transported toward Henan Province by confluent southeasterlies on the northern side of a strong typhoon In-Fa(2021),with the convergent southerlies associated with a weaker typhoon Cempaka(2021)concurrently transporting moisture northward from South China Sea,supporting the rainstorm.In the upper troposphere,two equatorward-intruding potential vorticity(PV)streamers within the planetary-scale wave train were located over northern Henan Province,forming significant divergent flow aloft to induce stronger ascending motion locally.Moreover,the converged moist air was also blocked by the mountains in western Henan Province and forced to rise so that a deep meso-β-scale convective vortex(MβCV)was induced over the west of Zhengzhou City.The PV budget analyses demonstrate that the MβCV development was attributed to the positive feedback between the rainfall-related diabatic heating and high-PV under the strong upward PV advection during the Zhengzhou 7.20 rainstorm.Importantly,the MβCV was forced by upper-level larger-scale westerlies becoming eastward-sloping,which allowed the mixtures of abundant raindrops and hydrometeors to ascend slantwise and accumulate just over Zhengzhou City,resulting in the record-breaking hourly rainfall locally.展开更多
A relatively independent and small-scale heavy rainfall event occurred to the south of a slow eastwardmoving meso-α-scale vortex. The analysis shows that a meso-β-scale system is heavily responsible for the intense ...A relatively independent and small-scale heavy rainfall event occurred to the south of a slow eastwardmoving meso-α-scale vortex. The analysis shows that a meso-β-scale system is heavily responsible for the intense precipitation. An attempt to simulate it met with some failures. In view of its small scale, short lifetime and relatively sparse observations at the initial time, an adjoint model was used to examine the sensitivity of the meso-β-scale vortex simulation with respect to initial conditions. The adjoint sensitivity indicates how small perturbations of initial model variables anywhere in the model domain can influence the central vorticity of the vortex. The largest sensitivity for both the wind and temperature perturbation is located below 700 hPa, especially at the low level. The largest sensitivity for the water vapor perturbation is located below 500 hPa, especially at the middle and low levels. The horizontal adjoint sensitivity for all variables is mainly located toward the upper reaches of the Yangtze River with respect to the simulated meso-β-scale system in Hunan and Jiangxi provinces with strong locality. The sensitivity shows that warm cyclonic perturbations in the upper reaches can have a great effect on the development of the meso-β-scale vortex. Based on adjoint sensitivity, forward sensitivity experiments were conducted to identify factors influencing the development of the meso-β-scale vortex and to explore ways of improving the prediction. A realistic prediction was achieved by using adjoint sensitivity to modify the initial conditions and implanting a warm cyclone at the initial time in the upper reaches of the river with respect to the meso-β-scale vortex, as is commonly done in tropical cyclone prediction.展开更多
Over the last decade, computational methods have been intensively applied to a variety of scientific researches and engineering designs. Although the computational fluid dynamics （CFD） method has played a dominant r...Over the last decade, computational methods have been intensively applied to a variety of scientific researches and engineering designs. Although the computational fluid dynamics （CFD） method has played a dominant role in studying and simulating transport phenomena involving fluid flow and heat and mass transfers, in recent years, other numerical methods for the simulations at meso- and micro-scales have also been actively applied to solve the physics of complex flow and fluid-interface interactions. This paper presents a review of recent advances in multi-scale computational simulation of biomimetics related fluid flow problems. The state-of-the-art numerical techniques, such as lattice Boltzmann method （LBM）, molecular dynamics （MD）, and conventional CFD, applied to different problems such as fish flow, electro-osmosis effect of earthworm motion, and self-cleaning hydrophobic surface, and the numerical approaches are introduced. The new challenging of modelling biomimetics problems in developing the physical conditions of self-clean hydrophobic surfaces is discussed.展开更多
A mei-yu front process in the lower reaches of the Yangtze River on 23 June 1999 was simulated by using the fifth-generation Pennsylvania State University-NCAR （PSU/NCAR） Mesoscale Model （MM5） with FDDA （Four Dim...A mei-yu front process in the lower reaches of the Yangtze River on 23 June 1999 was simulated by using the fifth-generation Pennsylvania State University-NCAR （PSU/NCAR） Mesoscale Model （MM5） with FDDA （Four Dimension Data Assimilation）. The analysis shows that seven weak small mesoscale vortexes of tens of kilometers, correspondent to surface low trough or mesoscale centers, in the planetary boundary layer （PBL） in the mei-yu front were heavily responsible for the heavy rainfall. Sometimes, several weak small-scale vortexes in the PBL could form a vortex group, some of which would weaken locally, and some would develop to be a meso-α-scale low vortex through combination. The initial dynamical triggering mechanism was related to two strong currents： one was the northeast flow in the PBL at the rear of the mei-yu front, the vortexes occurred exactly at the side of the northeast flow; and the other was the strong southwest low-level jet （LLJ） in front of the Mei-yu front, which moved to the upper of the vortexes. Consequently, there were notable horizontal and vertical wind shears to form positive vorticity in the center of the southwest LLJ. The development of mesoscale convergence in the PBL and divergence above, as well as the vertical positive vorticity column, were related to the small wind column above the nose-shaped velocity contours of the northeast flow embedding southwestward in the PBL, which intensified the horizontal wind shear and the positive vorticity column above the vortexes, baroclinicity and instability.展开更多
Recent advances in Global Positioning System （GPS） remote sensing technology allow for a direct estimation of the precipitable water vapor （PWV） from delayed signals transmitted by GPS satellites, which can be ass...Recent advances in Global Positioning System （GPS） remote sensing technology allow for a direct estimation of the precipitable water vapor （PWV） from delayed signals transmitted by GPS satellites, which can be assimilated into numerical models with four-dimensional variational （4DVAR） data assimilation. A mesoscale model and its 4DVAR system are used to access the impacts of assimilating GPS-PWV and hourly rainfall observations on the short-range prediction of a heavy rainfall event on 20 June 2002. The heavy precipitation was induced by a sequence of meso-β-scale convective systems （MCS） along the mei-yu front in China. The experiments with GPS-PWV assimilation cluster and also eliminated the erroneous rainfall successfully simulated the evolution of the observed MCS systems found in the experiment without 4DVAR assimilation. Experiments with hourly rainfall assimilation performed similarly both on the prediction of MCS initiation and the elimination of erroneous systems, however the MCS dissipated much sooner than it did in observations. It is found that the assimilation-induced moisture perturbation and mesoscale low-level jet are helpful for the MCS generation and development. It is also discovered that spurious gravity waves may post serious limitations for the current 4DVAR algorithm, which would degrade the assimilation efficiency, especially for rainfall data. Sensitivity experiments with different observations, assimilation windows and observation weightings suggest that assimilating GPS-PWV can be quite effective, even with the assimilation window as short as 1 h. On the other hand, assimilating rainfall observations requires extreme cautions on the selection of observation weightings and the control of spurious gravity waves.展开更多
The method of Adler was improved to prepare a series of 5,10,15,20-tetrakis(4-alkoxyphenyl)porphyrins and their complexes containing Fe3+, Mn3+, Pb2+, Co2+, Cu2+, Zn2+. Among them there were seven new compounds. All t...The method of Adler was improved to prepare a series of 5,10,15,20-tetrakis(4-alkoxyphenyl)porphyrins and their complexes containing Fe3+, Mn3+, Pb2+, Co2+, Cu2+, Zn2+. Among them there were seven new compounds. All these compounds were identified through 1H NMR, MS, IR, UV and Element analysis. The correlation between the structure of compounds and their 1H NMR, MS, IR, UV spectra was discussed and their specific spectra were explained. We found nine metalloporphyrins exhibited liquid crystal behaviour through DSC and polarized-light microscope. They had one to three mesophases and certain phase transition temperature, ?H and temperature range of L.C(?T).展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.42288101,and 42175076)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB40000000)the Open Research Fund Program of Plateau Atmosphere and Environment Key Laboratory of Sichuan Province(Project PAEKL-2022-K02).
文摘On 20 July 2021,northern Henan Province in China experienced catastrophic flooding as a result of an extremely intense rainstorm,with a record-breaking hourly rainfall of 201.9 mm during 0800–0900 UTC and daily accumulated rainfall in Zhengzhou City exceeding 600 mm(“Zhengzhou 7.20 rainstorm”for short).The multi-scale dynamical and thermodynamical mechanisms for this rainstorm are investigated based on station-observed and ERA-5 reanalysis datasets.The backward trajectory tracking shows that the warm,moist air from the northwestern Pacific was mainly transported toward Henan Province by confluent southeasterlies on the northern side of a strong typhoon In-Fa(2021),with the convergent southerlies associated with a weaker typhoon Cempaka(2021)concurrently transporting moisture northward from South China Sea,supporting the rainstorm.In the upper troposphere,two equatorward-intruding potential vorticity(PV)streamers within the planetary-scale wave train were located over northern Henan Province,forming significant divergent flow aloft to induce stronger ascending motion locally.Moreover,the converged moist air was also blocked by the mountains in western Henan Province and forced to rise so that a deep meso-β-scale convective vortex(MβCV)was induced over the west of Zhengzhou City.The PV budget analyses demonstrate that the MβCV development was attributed to the positive feedback between the rainfall-related diabatic heating and high-PV under the strong upward PV advection during the Zhengzhou 7.20 rainstorm.Importantly,the MβCV was forced by upper-level larger-scale westerlies becoming eastward-sloping,which allowed the mixtures of abundant raindrops and hydrometeors to ascend slantwise and accumulate just over Zhengzhou City,resulting in the record-breaking hourly rainfall locally.
基金This work was supported by the National Natural Science Foundation of China under Grant No.40075009 and 40505011.The authors would like to thank the computer center of the College of Science at Zhejiang University for computer support of the 0rigin2K.
文摘A relatively independent and small-scale heavy rainfall event occurred to the south of a slow eastwardmoving meso-α-scale vortex. The analysis shows that a meso-β-scale system is heavily responsible for the intense precipitation. An attempt to simulate it met with some failures. In view of its small scale, short lifetime and relatively sparse observations at the initial time, an adjoint model was used to examine the sensitivity of the meso-β-scale vortex simulation with respect to initial conditions. The adjoint sensitivity indicates how small perturbations of initial model variables anywhere in the model domain can influence the central vorticity of the vortex. The largest sensitivity for both the wind and temperature perturbation is located below 700 hPa, especially at the low level. The largest sensitivity for the water vapor perturbation is located below 500 hPa, especially at the middle and low levels. The horizontal adjoint sensitivity for all variables is mainly located toward the upper reaches of the Yangtze River with respect to the simulated meso-β-scale system in Hunan and Jiangxi provinces with strong locality. The sensitivity shows that warm cyclonic perturbations in the upper reaches can have a great effect on the development of the meso-β-scale vortex. Based on adjoint sensitivity, forward sensitivity experiments were conducted to identify factors influencing the development of the meso-β-scale vortex and to explore ways of improving the prediction. A realistic prediction was achieved by using adjoint sensitivity to modify the initial conditions and implanting a warm cyclone at the initial time in the upper reaches of the river with respect to the meso-β-scale vortex, as is commonly done in tropical cyclone prediction.
文摘Over the last decade, computational methods have been intensively applied to a variety of scientific researches and engineering designs. Although the computational fluid dynamics （CFD） method has played a dominant role in studying and simulating transport phenomena involving fluid flow and heat and mass transfers, in recent years, other numerical methods for the simulations at meso- and micro-scales have also been actively applied to solve the physics of complex flow and fluid-interface interactions. This paper presents a review of recent advances in multi-scale computational simulation of biomimetics related fluid flow problems. The state-of-the-art numerical techniques, such as lattice Boltzmann method （LBM）, molecular dynamics （MD）, and conventional CFD, applied to different problems such as fish flow, electro-osmosis effect of earthworm motion, and self-cleaning hydrophobic surface, and the numerical approaches are introduced. The new challenging of modelling biomimetics problems in developing the physical conditions of self-clean hydrophobic surfaces is discussed.
基金supported by the National Natural Science Foundation of China under Grant No.40505011.
文摘A mei-yu front process in the lower reaches of the Yangtze River on 23 June 1999 was simulated by using the fifth-generation Pennsylvania State University-NCAR （PSU/NCAR） Mesoscale Model （MM5） with FDDA （Four Dimension Data Assimilation）. The analysis shows that seven weak small mesoscale vortexes of tens of kilometers, correspondent to surface low trough or mesoscale centers, in the planetary boundary layer （PBL） in the mei-yu front were heavily responsible for the heavy rainfall. Sometimes, several weak small-scale vortexes in the PBL could form a vortex group, some of which would weaken locally, and some would develop to be a meso-α-scale low vortex through combination. The initial dynamical triggering mechanism was related to two strong currents： one was the northeast flow in the PBL at the rear of the mei-yu front, the vortexes occurred exactly at the side of the northeast flow; and the other was the strong southwest low-level jet （LLJ） in front of the Mei-yu front, which moved to the upper of the vortexes. Consequently, there were notable horizontal and vertical wind shears to form positive vorticity in the center of the southwest LLJ. The development of mesoscale convergence in the PBL and divergence above, as well as the vertical positive vorticity column, were related to the small wind column above the nose-shaped velocity contours of the northeast flow embedding southwestward in the PBL, which intensified the horizontal wind shear and the positive vorticity column above the vortexes, baroclinicity and instability.
文摘Recent advances in Global Positioning System （GPS） remote sensing technology allow for a direct estimation of the precipitable water vapor （PWV） from delayed signals transmitted by GPS satellites, which can be assimilated into numerical models with four-dimensional variational （4DVAR） data assimilation. A mesoscale model and its 4DVAR system are used to access the impacts of assimilating GPS-PWV and hourly rainfall observations on the short-range prediction of a heavy rainfall event on 20 June 2002. The heavy precipitation was induced by a sequence of meso-β-scale convective systems （MCS） along the mei-yu front in China. The experiments with GPS-PWV assimilation cluster and also eliminated the erroneous rainfall successfully simulated the evolution of the observed MCS systems found in the experiment without 4DVAR assimilation. Experiments with hourly rainfall assimilation performed similarly both on the prediction of MCS initiation and the elimination of erroneous systems, however the MCS dissipated much sooner than it did in observations. It is found that the assimilation-induced moisture perturbation and mesoscale low-level jet are helpful for the MCS generation and development. It is also discovered that spurious gravity waves may post serious limitations for the current 4DVAR algorithm, which would degrade the assimilation efficiency, especially for rainfall data. Sensitivity experiments with different observations, assimilation windows and observation weightings suggest that assimilating GPS-PWV can be quite effective, even with the assimilation window as short as 1 h. On the other hand, assimilating rainfall observations requires extreme cautions on the selection of observation weightings and the control of spurious gravity waves.
文摘The method of Adler was improved to prepare a series of 5,10,15,20-tetrakis(4-alkoxyphenyl)porphyrins and their complexes containing Fe3+, Mn3+, Pb2+, Co2+, Cu2+, Zn2+. Among them there were seven new compounds. All these compounds were identified through 1H NMR, MS, IR, UV and Element analysis. The correlation between the structure of compounds and their 1H NMR, MS, IR, UV spectra was discussed and their specific spectra were explained. We found nine metalloporphyrins exhibited liquid crystal behaviour through DSC and polarized-light microscope. They had one to three mesophases and certain phase transition temperature, ?H and temperature range of L.C(?T).
