We study odd–even high-order harmonic generation（HHG） from oriented asymmetric molecules He H2＋numerically and analytically. The variational method is used to improve the analytical description of the ground-state...We study odd–even high-order harmonic generation（HHG） from oriented asymmetric molecules He H2＋numerically and analytically. The variational method is used to improve the analytical description of the ground-state wave function for the asymmetric system, with which the ground-state-continuum-state transition dipole is evaluated. The comparison between the odd–even HHG spectra and the improved dipoles allows us to identify and clarify the complex generation mechanism of odd–even harmonics from asymmetric molecules, providing deep insights into the relation between the odd–even HHG and the asymmetric molecular orbital.展开更多
We experimentally and theoretically demonstrate that ＊~he property （odd or even） of generated harmonics can be selected by manipulating the macroscopic phase-matching conditions based on a three-color laser field. ...We experimentally and theoretically demonstrate that ＊~he property （odd or even） of generated harmonics can be selected by manipulating the macroscopic phase-matching conditions based on a three-color laser field. Only odd or even harmonics can be made dominant by changing the focal position and adjusting the gas pressure. These results indicate that the odd-even property of the generated harmonics can be controlled by using the mult i-color laser field with macroscopic phase-matching.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.11274090)the Fundamental Research Funds for the Central Universities,China(Grant No.SNNU.GK201403002)
文摘We study odd–even high-order harmonic generation（HHG） from oriented asymmetric molecules He H2＋numerically and analytically. The variational method is used to improve the analytical description of the ground-state wave function for the asymmetric system, with which the ground-state-continuum-state transition dipole is evaluated. The comparison between the odd–even HHG spectra and the improved dipoles allows us to identify and clarify the complex generation mechanism of odd–even harmonics from asymmetric molecules, providing deep insights into the relation between the odd–even HHG and the asymmetric molecular orbital.
基金supported by the National Natural Science Foundation of China(Nos.11127901,6122106460921004,11134010,11227902,11222439,11274325,61108012,and 11474223)the National 973 Program(No.2011CB808103)+1 种基金the Natural Science Foundation of Zhejiang(No.LY14F050008)the Open Fund of the State Key Laboratory of High Field Laser Physics
文摘We experimentally and theoretically demonstrate that ＊~he property （odd or even） of generated harmonics can be selected by manipulating the macroscopic phase-matching conditions based on a three-color laser field. Only odd or even harmonics can be made dominant by changing the focal position and adjusting the gas pressure. These results indicate that the odd-even property of the generated harmonics can be controlled by using the mult i-color laser field with macroscopic phase-matching.
