As an exercise in model sensitivity, the Models-3 Community Multiscale Air Quality (CMAQ) modeling system with meteorological fields from the Regional Atmospheric Modeling System (RAMS) was applied to study the respon...As an exercise in model sensitivity, the Models-3 Community Multiscale Air Quality (CMAQ) modeling system with meteorological fields from the Regional Atmospheric Modeling System (RAMS) was applied to study the response of photochemical oxidants to systematic increases in anthropogenic volatile organic compounds (VOC) and nitrogen oxides (NO x) emissions in January 1997 over East Asia. Three simulations-one base case and two sensitivity simulations were carried out. Two sensitivity simulations were performed by assuming a 35% separate increase in anthropogenic VOC and NO x emissions comparing with the base case. Biogenic VOC emissions were held constant across the sensitivity simulations. To evaluate the model performance, ozone mixing ratios (O 3) from the base case simulation were compared with surface observations at five remote sites in Japan, and it was found that the model reproduces most of the important features in the observations. Monthly average O 3 concentrations in the daytime were examined to gain an understanding of how the increase in anthropogenic emissions affected the overall chemical system for each sensitivity simulation.展开更多
文摘As an exercise in model sensitivity, the Models-3 Community Multiscale Air Quality (CMAQ) modeling system with meteorological fields from the Regional Atmospheric Modeling System (RAMS) was applied to study the response of photochemical oxidants to systematic increases in anthropogenic volatile organic compounds (VOC) and nitrogen oxides (NO x) emissions in January 1997 over East Asia. Three simulations-one base case and two sensitivity simulations were carried out. Two sensitivity simulations were performed by assuming a 35% separate increase in anthropogenic VOC and NO x emissions comparing with the base case. Biogenic VOC emissions were held constant across the sensitivity simulations. To evaluate the model performance, ozone mixing ratios (O 3) from the base case simulation were compared with surface observations at five remote sites in Japan, and it was found that the model reproduces most of the important features in the observations. Monthly average O 3 concentrations in the daytime were examined to gain an understanding of how the increase in anthropogenic emissions affected the overall chemical system for each sensitivity simulation.
