Employing both the Dirac R-matrix and the relativistic distorted wave with independent process and isolated reso- nance approaches, we report resonance enhanced electron impact excitation data (specifically, effectiv...Employing both the Dirac R-matrix and the relativistic distorted wave with independent process and isolated reso- nance approaches, we report resonance enhanced electron impact excitation data (specifically, effective collision strengths) among the lowest 41 levels from the n = 3 configurations of Cu XV. The results show that the latter approach can obtain resonance contributions reasonably well for most excitations of Cu XV, though a comparison between the two approaches shows that the close-coupling effects are truly significant for rather weak excitations, especially for two-electron excitations from the 3s3p4 to 3s23p23d configuration. Resonance contributions are significant (more than two orders of magnitude) for many excitations and dramatically influence the line intensity ratios associated with density diagnostics.展开更多
Earth's Coriolis force profoundly alters the eigen frequencies, eigen functions, and excitation of rotational normal modes. Some rotational modes of the solid mantle-fluid outer core-solid inner core Earth system are...Earth's Coriolis force profoundly alters the eigen frequencies, eigen functions, and excitation of rotational normal modes. Some rotational modes of the solid mantle-fluid outer core-solid inner core Earth system are confirmed observationally and some remain elusive. Here we bring together from literature assertions about an excited resonance system in terms of the Green's function and temporal convolution. We raise caveats against taking the face values of the oscillational motion which have been "masqueraded" by the convolution, necessitating deconvolution for retrieving the excitation function which reflects the true variability. Lastly we exemplify successful applications of the deconvolution in estimating resonance complex frequencies.展开更多
We apply the reductive perturbation method to the simple electrostatic ion-temperature-gradient mode in an advanced fluid description. The fluid resonance turns out to play a major role for the excitation of zonal flo...We apply the reductive perturbation method to the simple electrostatic ion-temperature-gradient mode in an advanced fluid description. The fluid resonance turns out to play a major role for the excitation of zonal flows. This is the mechanism recently found to lead to the low-to-high (L-H) mode transition and to the nonlinear Dimits upshift in transport code simulations. It is important that we have taken the nonlinear temperature dynamics from the Reynolds stress as the convected diamagnetic flow. This has turned out to be the most relevant effect as found in transport simulations of the L-H transition, internal transport barriers and Dimits shift. This is the first time that an analytical method is applied to a system which numerically has been found to give the right experimental dynamics.展开更多
The creation and relaxation of double K-hole states 1s^(0)2s^(2)2p^(6)np(n≥3)of Ne^(1+)in the interaction with ultraintense ultrafast x-ray pulses are theoretically investigated.The x-ray photon energies are selected...The creation and relaxation of double K-hole states 1s^(0)2s^(2)2p^(6)np(n≥3)of Ne^(1+)in the interaction with ultraintense ultrafast x-ray pulses are theoretically investigated.The x-ray photon energies are selected so that x-rays first photoionize1s^(22)s^(22)p^(6) of a neon atom to create a single K-hole state of 1s2s^(22)p^(6) of Ne^(1+),which is further excited resonantly to double K-hole states of ls^(0)2s^(2)2p^(6)np(n≥3).A time-dependent rate equation is used to investigate the creation and relaxation processes of 1s^(0)2s^(2)2p^(6)np,where the primary microscopic atomic processes including photoexcitation,spontaneous radiation,photoionization and Auger decay are considered.The calculated Auger electron energy spectra are compared with recent experimental results,which shows good agreement.The relative intensity of Auger electrons is very sensitive to the photon energy and bandwidth of x-ray pulses,which could be used as a diagnostic tool for x-ray free electron laser and atom experiments.展开更多
A vibration-based energy harvester is essentially a resonator working in a limited frequency range.To increase the working frequency range is a challenging problem.This paper reveals a novel possibility for enhancing ...A vibration-based energy harvester is essentially a resonator working in a limited frequency range.To increase the working frequency range is a challenging problem.This paper reveals a novel possibility for enhancing energy harvesting via internal resonance.An internal resonance energy harvester is proposed.The excitation is successively assumed as the Gaussian white noise,the colored noise defined by a second-order filter,the narrow-band noise,and exponentially correlated noise.The corresponding averaged root-meansquare output voltages are computed.Numerical results demonstrate that the internal resonance increases the operating bandwidth and the output voltage.展开更多
The relativistic configuration interaction method is employed to calculate the dielectronic recombination(DR) cross sections of helium-like krypton via the 1s2lnl '(n = 2,3,...,15) resonances.Then,the resonant tr...The relativistic configuration interaction method is employed to calculate the dielectronic recombination(DR) cross sections of helium-like krypton via the 1s2lnl '(n = 2,3,...,15) resonances.Then,the resonant transfer excitation(RTE) processes of Kr 34+ colliding with H,He,H 2,and CH x(x = 0-4) targets are investigated under the impulse approximation.The needed Compton profiles of targets are obtained from the Hartree-Fock wave functions.The RTE cross sections are strongly dependent on DR resonant energies and strengths,and the electron momentum distributions of the target.For H 2 and H targets,the ratio of their RTE cross sections changes from 1.85 for the 1s2l2l ' to 1.88 for other resonances,which demonstrates the weak molecular effects on the Compton profiles of H 2.For CH x(x = 0-4) targets,the main contribution to the RTE cross section comes from the carbon atom since carbon carries 6 electrons;as the number of hydrogen increases in CH x,the RTE cross section almost increases by the same value,displaying the strong separate atom character for the hydrogen.However,further comparison of the individual orbital contributions of C(2p,2s,1s) and CH 4(1t 2,2a 1,1a 1) to the RTE cross sections shows that the molecular effects induce differences of about 25.1%,19.9%,and 0.2% between 2p-1t 2,2s-2a 1,and 1s-1a 1 orbitals,respectively.展开更多
This paper proposes a novel one-colour Xe-Kr laser induced collisional ionization system. Considering the level scheme of the system, it finds that the initial state of the reaction--the four 4f levels with even J of ...This paper proposes a novel one-colour Xe-Kr laser induced collisional ionization system. Considering the level scheme of the system, it finds that the initial state of the reaction--the four 4f levels with even J of Xe-can be prepared through method of four-photon resonant excitation by dye laser with wavelength of -440 nm. Absorption of an additional photon (the transfer laser) of the same wavelength will complete the laser induced collisional ionization process. The resonance enhanced ionization spectrum of Xe by four laser photons at -440nm is measured through time-of-flight mass spectrometry, this aims at the preparation of the initial state of the system proposed. The Stark broadening of the measured spectrum is observed and consistent with the previous study. Analysis of the measured resonance ionization spectrum implies the feasibility of -440 nm four-photon resonant excitation of the initial 4f state of the Xe Kr system proposed in this paper, which prepares for a further experiment of laser induced collisional ionization.展开更多
Coherent electronic dynamics are of great significance in photo-induced processes and molecular magnetism.We theoretically investigate electronic dynamics of triatomic molecule H_(3)^(2+) by circularly polarized pulse...Coherent electronic dynamics are of great significance in photo-induced processes and molecular magnetism.We theoretically investigate electronic dynamics of triatomic molecule H_(3)^(2+) by circularly polarized pulses,including electron density distributions,induced electronic currents,and ultrafast magnetic field generation.By comparing the results of the coherent resonant excitation and direct ionization,we found that for the coherent resonant excitation,the electron is localized and the coherent electron wave packet moves periodically between three protons,which can be attributed to the coherent superposition of the ground A′state and excited E+state.Whereas,for the direct single-photon ionization,the induced electronic currents mainly come from the free electron in the continuum state.It is found that there are differences in the intensity,phase,and frequency of the induced current and the generated magnetic field.The scheme allows one to control the induced electronic current and the ultrafast magnetic field generation.展开更多
We investigate the dissociation dynamics of core-excited O_(2)molecules using a high-resolution energy-resolved electron-ion coincidence experimental setup.The excited cationic states with two valence holes and one Ry...We investigate the dissociation dynamics of core-excited O_(2)molecules using a high-resolution energy-resolved electron-ion coincidence experimental setup.The excited cationic states with two valence holes and one Rydberg electron are created after spectator Auger decay induced by O 1s→(^(4)Σ_(u)^(-))3sσcore excitation in O_(2).From the energy correlation between the kinetic energy of the Auger electron and the ion kinetic energy release,we distinguish several dissociation channels.Rather complex dissociation channels of the spectator Auger final states are disclosed,which can be explained by the increased number of the crossing point due to the existence of Rydberg electron.The quantum system will evolve into different dissociation limits at each crossing point between the potential energy curves.展开更多
The influence of air gaps on the response of transmission for a transverse-electric mode parallel-plate waveguide(TE-PPWG) with a single cavity and double cavities has been studied experimentally. As the air gap is ...The influence of air gaps on the response of transmission for a transverse-electric mode parallel-plate waveguide(TE-PPWG) with a single cavity and double cavities has been studied experimentally. As the air gap is larger than the resonant wavelength of high order cavity mode in the single deep grooved waveguide, only the fundamental cavity mode can be excited and single resonance can be observed in the transmission spectrum. Based on above observations, a tunable multiband terahertz(THz)notch filter has been proposed and the variation of air gap has turned out to be an effective method to select the band number. Experimental data and simulated results verify this band number tunability. This mechanical control mechanism for electromagnetic induced transparency(EIT) will open a door to design the tunable THz devices.展开更多
The phonon-assisted process of energy transfer aiming at exploring the newly emerging frontier between biology and physics is an issue of central interest.This article shows the important role of the intramolecular vi...The phonon-assisted process of energy transfer aiming at exploring the newly emerging frontier between biology and physics is an issue of central interest.This article shows the important role of the intramolecular vibrational modes for excitation energy transfer in the photosynthetic systems.Based on a dimer system consisting of a donor and an acceptor modeled by two two-level systems,in which one of them is coupled to a high-energy vibrational mode,we derive an effective Hamiltonian describing the vibration-assisted coherent energy transfer process in the polaron frame.The effective Hamiltonian reveals in the case that the vibrational mode dynamically matches the energy detuning between the donor and the acceptor,the original detuned energy transfer becomes resonant energy transfer.In addition,the population dynamics and coherence dynamics of the dimer system with and without vibration-assistance are investigated numerically.It is found that,the energy transfer efficiency and the transfer time depend heavily on the interaction strength of the donor and the high-energy vibrational mode,as well as the vibrational frequency.The numerical results also indicate that the initial state and dissipation rate of the vibrational mode have little influence on the dynamics of the dimer system.Results obtained in this article are not only helpful to understand the natural photosynthesis,but also offer an optimal design principle for artificial photosynthesis.展开更多
Based on excitation-resonance mass testing principle, a proper experiment testing system is designed for annular parts. The dynamics characters of the axis sleeve, which is made of a new Mn-Cu alloy and used as a vibr...Based on excitation-resonance mass testing principle, a proper experiment testing system is designed for annular parts. The dynamics characters of the axis sleeve, which is made of a new Mn-Cu alloy and used as a vibration reductor in high acceleration rotary testing machine for fusee, is investigated. The relationship between stiffness coefficient and utilizing frequency is obtained, and the simplified dynamics model of crystal is established From the viewpoint of crystal microstructure of the Mn-Cu alloy, the experiment result is analyzed by the viscoelastic theory, and the characters of stress and strain in the condition of high frequency are discussed. The results indicate that the Mn-Cu alloy annular parts are fit to be used on the high accleration rotary testing machine for fusee.展开更多
In this paper, the coupled extension and thickness- twist vibrations are studied for AT-cut quartz plates under Lateral Field Excitation (LFE) with variations along the x1- direction. Mindlin's two-dimensional equa...In this paper, the coupled extension and thickness- twist vibrations are studied for AT-cut quartz plates under Lateral Field Excitation (LFE) with variations along the x1- direction. Mindlin's two-dimensional equations are used for anisotropic crystal plates. Both free and electrically forced vibrations are considered. Important vibration characteristics are obtained, including dispersion relations, frequency spectra, and motional capacitances. It is shown that, to avoid the effects of the couplings between extension and thickness-twist vibrations, a series of discrete values of the length/thickness ratio of the crystal plate need to be excluded. The results are of fundamental significance for the design of LFE resonators and sensors.展开更多
Spectra of autoionizing states of the Sm atom in an energy region between 45948.9 cm^-1 and 46943.6 cm^-1 are systematically investigated by a three-color multi-step resonant excitation scheme with three different exc...Spectra of autoionizing states of the Sm atom in an energy region between 45948.9 cm^-1 and 46943.6 cm^-1 are systematically investigated by a three-color multi-step resonant excitation scheme with three different excitation paths.The three intermediate states,4f 66s7s 7F3,4f 66s7s 7F4,and 4f 66s7s 9F5 are employed for the three paths,respectively.Based on precise calibration of wavelength,the level energies of 112 autoionizing states are determined with the line widths and the relative line intensities of the related transitions.The possible influence of configuration interaction on the line shape of autoionizing state is also discussed.In addition,a unique value of J,the total angular momentum,is assigned to all detected states by comparing the three spectra obtained with the different excitation paths.展开更多
Thermal emission is often presented as a typical incoherent process. Incorporating periodic structures on the tungsten surface offers the possibility to obtain coherent thermal emission sources. Here we illustrate gra...Thermal emission is often presented as a typical incoherent process. Incorporating periodic structures on the tungsten surface offers the possibility to obtain coherent thermal emission sources. Here we illustrate grating as an example to examine the influence of the geometric parameters on the thermal emission properties. It is found that for very shallow gratings, only surface plasmon polariton(SPP) modes can be excited and the emission efficiency is closely related with the filling factor. When the ratio of the depth to period of the grating is in the range from 1/20 to 1/2, the field between the adjacent corners can be coupled to each other across the air gap for the filling factor larger than 0.5 and produce a similar resonance as in an air rod. Further increase of the grating depth can cause the groove of the grating forming metal–insulator–metal(MIM) structures and induce surface plasmon standing wave modes. Our investigations will not only be helpful for manipulating thermal emission properties according to applications, but also help us understand the coupling mechanism between the incident electromagnetism waves and gratings with different parameters in various research fields.展开更多
The spin fluctuation in rubidium atom gas is studied via all-optical spin noise spectroscopy(SNS).Experimental results show that the integrated SNS signal and its full width at half maximum(FWHM) strongly depend o...The spin fluctuation in rubidium atom gas is studied via all-optical spin noise spectroscopy(SNS).Experimental results show that the integrated SNS signal and its full width at half maximum(FWHM) strongly depend on the frequency detuning of the probe light under resonant and non-resonant conditions.The total integrated SNS signal can be well fitted with a single squared Faraday rotation spectrum and the FWHM dependence may be related to the absorption profile of the sample.展开更多
Multiphoton resonant excitation and frustrated tunneling ionization,manifesting the photonic and optical nature of the driving light via direct excitation and electron recapture,respectively,are complementary mechanis...Multiphoton resonant excitation and frustrated tunneling ionization,manifesting the photonic and optical nature of the driving light via direct excitation and electron recapture,respectively,are complementary mechanisms to access Rydberg state excitation(RSE)of atoms and molecules in an intense laser field.However,clear identification and manipulation of their individual contributions in the light-induced RSE process remain experimentally challenging.Here,we bridge this gap by exploring the dissociative and nondissociative RSE of H2 molecules using bicircular two-color laser pulses.Depending on the relative field strength and polarization helicity of the two colors,the RSE probability can be boosted by more than one order of magnitude by exploiting the laser waveform-dependent field effect.The role of the photon effect is readily strengthened with increasing relative strength of the second-harmonic field of the two colors regardless of the polarization helicity.As compared to the nondissociative RSE forming H2,the field effect in producing the dissociative RSE channel of eHt;HT is moderately suppressed,which is primarily accessed via a three-step sequential process separated by molecular bond stretching.Our work paves the way toward a comprehensive understanding of the interplay of the underlying field and photon effects in the strong-field RSE process,as well as facilitating the generation of Rydberg states optimized with tailored characteristics.展开更多
The relativistic configuration interaction method is employed to calculate the dielectronic recombination(DR) cross sections of helium-like krypton via the 1s2lnl ’(n = 2,3,...,15) resonances.Then,the resonant transf...The relativistic configuration interaction method is employed to calculate the dielectronic recombination(DR) cross sections of helium-like krypton via the 1s2lnl ’(n = 2,3,...,15) resonances.Then,the resonant transfer excitation(RTE) processes of Kr 34+ colliding with H,He,H 2,and CH x(x = 0-4) targets are investigated under the impulse approximation.The needed Compton profiles of targets are obtained from the Hartree-Fock wave functions.The RTE cross sections are strongly dependent on DR resonant energies and strengths,and the electron momentum distributions of the target.For H 2 and H targets,the ratio of their RTE cross sections changes from 1.85 for the 1s2l2l ’ to 1.88 for other resonances,which demonstrates the weak molecular effects on the Compton profiles of H 2.For CH x(x = 0-4) targets,the main contribution to the RTE cross section comes from the carbon atom since carbon carries 6 electrons;as the number of hydrogen increases in CH x,the RTE cross section almost increases by the same value,displaying the strong separate atom character for the hydrogen.However,further comparison of the individual orbital contributions of C(2p,2s,1s) and CH 4(1t 2,2a 1,1a 1) to the RTE cross sections shows that the molecular effects induce differences of about 25.1%,19.9%,and 0.2% between 2p-1t 2,2s-2a 1,and 1s-1a 1 orbitals,respectively.展开更多
High-order nonlinear multiphoton absorption is usually inefficient,but can be enhanced by designing resonant excitations between occupied and unoccupied energy levels.We conducted angle-resolved multi-photon photoemis...High-order nonlinear multiphoton absorption is usually inefficient,but can be enhanced by designing resonant excitations between occupied and unoccupied energy levels.We conducted angle-resolved multi-photon photoemission(mPPE)studies on the SnSe_(2)(001)surfaces excited by ultrashort laser pulses.By tuning photon energy and light polarization,we demonstrate the presence of a resonant four-photon photoemission(4PPE)process involving the occupied valence band(VB),the unoccupied second conduction band(CB2)and the unoccupied image-potential state(IPs)of SnSe_(2).In this 4PPE process,VB electrons of SnSe_(2) are resonantly excited into CB2 by adsorbing two photons,followed by the adsorption of another photon to populate the n=1 IPs before being emitted out to the vacuum by adsorbing one more photon.This results in a double-resonant 4PPE process,which exhibits approximately a 40 times enhancement in photoemission yields compared to cases where one of the resonant pathways,CB2→IPs,is inhibited by involving a virtual state instead of the IPs in the 4PPE.The double-resonant 4PPE process efficiently excite the bulk VB electrons outside the vacuum,like taking advantage of resonant“ladders”through two real empty electronic states of SnSe_(2).Our results highlight the important applications of mPPE in probing the band-structure,particularly the unoccupied states,of recently emerging main group dichalcogenide semiconductors.Furthermore,the discovered resonant mPPE process contributes to the exploration of their promising optoelectronic applications.展开更多
Multiple resonant excitations of surface plasmons in a graphene stratified slab are realized by Otto configuration at terahertz frequencies. The proposed graphene stratified slab consists of alternating dielectric lay...Multiple resonant excitations of surface plasmons in a graphene stratified slab are realized by Otto configuration at terahertz frequencies. The proposed graphene stratified slab consists of alternating dielectric layers and graphene sheets, and is sandwiched between a prism and another semi-infinite medium. Optical response and field distribution are determined by the transfer matrix method with the surface current density boundary condition.Multiple resonant excitations appear on the angular reflection spectrum, and are analyzed theoretically via the phase-matching condition. Furthermore, the effects of the system parameters are investigated. Among them, the Fermi levels can tune the corresponding resonances independently. The proposed concept can be engineered for promising applications, including angular selective or multiplex filters, multiple channel sensors, and directional delivery of energy.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.11076009 and 11374062)the Chinese Association of Atomic and Molecular Data,the Chinese National Fusion Project for ITER(Grant No.2015GB117000)the Leading Academic Discipline Project of Shanghai,China(Grant No.B107)
文摘Employing both the Dirac R-matrix and the relativistic distorted wave with independent process and isolated reso- nance approaches, we report resonance enhanced electron impact excitation data (specifically, effective collision strengths) among the lowest 41 levels from the n = 3 configurations of Cu XV. The results show that the latter approach can obtain resonance contributions reasonably well for most excitations of Cu XV, though a comparison between the two approaches shows that the close-coupling effects are truly significant for rather weak excitations, especially for two-electron excitations from the 3s3p4 to 3s23p23d configuration. Resonance contributions are significant (more than two orders of magnitude) for many excitations and dramatically influence the line intensity ratios associated with density diagnostics.
基金supported by the Taiwan Ministry of Science and Technology via grant#104-2116-M-001-006
文摘Earth's Coriolis force profoundly alters the eigen frequencies, eigen functions, and excitation of rotational normal modes. Some rotational modes of the solid mantle-fluid outer core-solid inner core Earth system are confirmed observationally and some remain elusive. Here we bring together from literature assertions about an excited resonance system in terms of the Green's function and temporal convolution. We raise caveats against taking the face values of the oscillational motion which have been "masqueraded" by the convolution, necessitating deconvolution for retrieving the excitation function which reflects the true variability. Lastly we exemplify successful applications of the deconvolution in estimating resonance complex frequencies.
基金Supported by the JSPS-NRF-NSFC A3 Foresight Program in the Field of Plasma Physics under Grant Nos 11261140328 and 2012K2A2A6000443the ’Thirteenth Five-Year’ Strategic Planning of Chinathe Funds of the Chinese Academy of Sciences and ASIPP
文摘We apply the reductive perturbation method to the simple electrostatic ion-temperature-gradient mode in an advanced fluid description. The fluid resonance turns out to play a major role for the excitation of zonal flows. This is the mechanism recently found to lead to the low-to-high (L-H) mode transition and to the nonlinear Dimits upshift in transport code simulations. It is important that we have taken the nonlinear temperature dynamics from the Reynolds stress as the convected diamagnetic flow. This has turned out to be the most relevant effect as found in transport simulations of the L-H transition, internal transport barriers and Dimits shift. This is the first time that an analytical method is applied to a system which numerically has been found to give the right experimental dynamics.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.12074430 and 11974423)。
文摘The creation and relaxation of double K-hole states 1s^(0)2s^(2)2p^(6)np(n≥3)of Ne^(1+)in the interaction with ultraintense ultrafast x-ray pulses are theoretically investigated.The x-ray photon energies are selected so that x-rays first photoionize1s^(22)s^(22)p^(6) of a neon atom to create a single K-hole state of 1s2s^(22)p^(6) of Ne^(1+),which is further excited resonantly to double K-hole states of ls^(0)2s^(2)2p^(6)np(n≥3).A time-dependent rate equation is used to investigate the creation and relaxation processes of 1s^(0)2s^(2)2p^(6)np,where the primary microscopic atomic processes including photoexcitation,spontaneous radiation,photoionization and Auger decay are considered.The calculated Auger electron energy spectra are compared with recent experimental results,which shows good agreement.The relative intensity of Auger electrons is very sensitive to the photon energy and bandwidth of x-ray pulses,which could be used as a diagnostic tool for x-ray free electron laser and atom experiments.
基金supported by the State Key Program of National Natural Science of China(Grant No.11232009)Shanghai Leading Academic Discipline Project(Grant No.S30106)
文摘A vibration-based energy harvester is essentially a resonator working in a limited frequency range.To increase the working frequency range is a challenging problem.This paper reveals a novel possibility for enhancing energy harvesting via internal resonance.An internal resonance energy harvester is proposed.The excitation is successively assumed as the Gaussian white noise,the colored noise defined by a second-order filter,the narrow-band noise,and exponentially correlated noise.The corresponding averaged root-meansquare output voltages are computed.Numerical results demonstrate that the internal resonance increases the operating bandwidth and the output voltage.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 1179041,11025417,and 10979007) the NSAF (Grant No. 10876043)
文摘The relativistic configuration interaction method is employed to calculate the dielectronic recombination(DR) cross sections of helium-like krypton via the 1s2lnl '(n = 2,3,...,15) resonances.Then,the resonant transfer excitation(RTE) processes of Kr 34+ colliding with H,He,H 2,and CH x(x = 0-4) targets are investigated under the impulse approximation.The needed Compton profiles of targets are obtained from the Hartree-Fock wave functions.The RTE cross sections are strongly dependent on DR resonant energies and strengths,and the electron momentum distributions of the target.For H 2 and H targets,the ratio of their RTE cross sections changes from 1.85 for the 1s2l2l ' to 1.88 for other resonances,which demonstrates the weak molecular effects on the Compton profiles of H 2.For CH x(x = 0-4) targets,the main contribution to the RTE cross section comes from the carbon atom since carbon carries 6 electrons;as the number of hydrogen increases in CH x,the RTE cross section almost increases by the same value,displaying the strong separate atom character for the hydrogen.However,further comparison of the individual orbital contributions of C(2p,2s,1s) and CH 4(1t 2,2a 1,1a 1) to the RTE cross sections shows that the molecular effects induce differences of about 25.1%,19.9%,and 0.2% between 2p-1t 2,2s-2a 1,and 1s-1a 1 orbitals,respectively.
基金Project supported by the National Natural Science Foundation of China (Grant Nos 10674036 and 10774033)Program for New Century Excellent Talents in UniversityProgram of Excellent Team in Harbin Institute of Technology
文摘This paper proposes a novel one-colour Xe-Kr laser induced collisional ionization system. Considering the level scheme of the system, it finds that the initial state of the reaction--the four 4f levels with even J of Xe-can be prepared through method of four-photon resonant excitation by dye laser with wavelength of -440 nm. Absorption of an additional photon (the transfer laser) of the same wavelength will complete the laser induced collisional ionization process. The resonance enhanced ionization spectrum of Xe by four laser photons at -440nm is measured through time-of-flight mass spectrometry, this aims at the preparation of the initial state of the system proposed. The Stark broadening of the measured spectrum is observed and consistent with the previous study. Analysis of the measured resonance ionization spectrum implies the feasibility of -440 nm four-photon resonant excitation of the initial 4f state of the Xe Kr system proposed in this paper, which prepares for a further experiment of laser induced collisional ionization.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.12074146 and 12074142)。
文摘Coherent electronic dynamics are of great significance in photo-induced processes and molecular magnetism.We theoretically investigate electronic dynamics of triatomic molecule H_(3)^(2+) by circularly polarized pulses,including electron density distributions,induced electronic currents,and ultrafast magnetic field generation.By comparing the results of the coherent resonant excitation and direct ionization,we found that for the coherent resonant excitation,the electron is localized and the coherent electron wave packet moves periodically between three protons,which can be attributed to the coherent superposition of the ground A′state and excited E+state.Whereas,for the direct single-photon ionization,the induced electronic currents mainly come from the free electron in the continuum state.It is found that there are differences in the intensity,phase,and frequency of the induced current and the generated magnetic field.The scheme allows one to control the induced electronic current and the ultrafast magnetic field generation.
基金Project supported by the National Natural Science Foundation of China(Grant No.11574020)the Project of Thousand Youth Talents in Chinathe Starting Grant of ShanghaiTech University。
文摘We investigate the dissociation dynamics of core-excited O_(2)molecules using a high-resolution energy-resolved electron-ion coincidence experimental setup.The excited cationic states with two valence holes and one Rydberg electron are created after spectator Auger decay induced by O 1s→(^(4)Σ_(u)^(-))3sσcore excitation in O_(2).From the energy correlation between the kinetic energy of the Auger electron and the ion kinetic energy release,we distinguish several dissociation channels.Rather complex dissociation channels of the spectator Auger final states are disclosed,which can be explained by the increased number of the crossing point due to the existence of Rydberg electron.The quantum system will evolve into different dissociation limits at each crossing point between the potential energy curves.
基金supported by the National Program on Key Basic Research Project of China under Grant No.2014CB339806Basic Research Key Project under Grant No.12JC1407100+1 种基金Major National Development Project of Scientific Instrument and Equipment under Grant No.2011YQ150021 and No.2012YQ14000504the National Natural Science Foundation of China under Grant No.11174207,No.61138001,No.61205094,and No.61307126
文摘The influence of air gaps on the response of transmission for a transverse-electric mode parallel-plate waveguide(TE-PPWG) with a single cavity and double cavities has been studied experimentally. As the air gap is larger than the resonant wavelength of high order cavity mode in the single deep grooved waveguide, only the fundamental cavity mode can be excited and single resonance can be observed in the transmission spectrum. Based on above observations, a tunable multiband terahertz(THz)notch filter has been proposed and the variation of air gap has turned out to be an effective method to select the band number. Experimental data and simulated results verify this band number tunability. This mechanical control mechanism for electromagnetic induced transparency(EIT) will open a door to design the tunable THz devices.
基金Project supported by the National Natural Science Foundation of China(Grant No.11174233)
文摘The phonon-assisted process of energy transfer aiming at exploring the newly emerging frontier between biology and physics is an issue of central interest.This article shows the important role of the intramolecular vibrational modes for excitation energy transfer in the photosynthetic systems.Based on a dimer system consisting of a donor and an acceptor modeled by two two-level systems,in which one of them is coupled to a high-energy vibrational mode,we derive an effective Hamiltonian describing the vibration-assisted coherent energy transfer process in the polaron frame.The effective Hamiltonian reveals in the case that the vibrational mode dynamically matches the energy detuning between the donor and the acceptor,the original detuned energy transfer becomes resonant energy transfer.In addition,the population dynamics and coherence dynamics of the dimer system with and without vibration-assistance are investigated numerically.It is found that,the energy transfer efficiency and the transfer time depend heavily on the interaction strength of the donor and the high-energy vibrational mode,as well as the vibrational frequency.The numerical results also indicate that the initial state and dissipation rate of the vibrational mode have little influence on the dynamics of the dimer system.Results obtained in this article are not only helpful to understand the natural photosynthesis,but also offer an optimal design principle for artificial photosynthesis.
文摘Based on excitation-resonance mass testing principle, a proper experiment testing system is designed for annular parts. The dynamics characters of the axis sleeve, which is made of a new Mn-Cu alloy and used as a vibration reductor in high acceleration rotary testing machine for fusee, is investigated. The relationship between stiffness coefficient and utilizing frequency is obtained, and the simplified dynamics model of crystal is established From the viewpoint of crystal microstructure of the Mn-Cu alloy, the experiment result is analyzed by the viscoelastic theory, and the characters of stress and strain in the condition of high frequency are discussed. The results indicate that the Mn-Cu alloy annular parts are fit to be used on the high accleration rotary testing machine for fusee.
基金supported by the National Natural Science Foundation of China(11372146)Research Fund for the Doctoral Program of Higher Education of China(20123305120007)+2 种基金Impact and Safety of Coastal Engineering Initiative,a COE Program of Zhejiang Provincial Government at Ningbo University(zj1110,zj1201,zj1229,and zj1203)Research Project Foundation of Zhejiang Educational Department(201327293)Young Doctoral Innovation Fund by Ningbo Polythchnic
文摘In this paper, the coupled extension and thickness- twist vibrations are studied for AT-cut quartz plates under Lateral Field Excitation (LFE) with variations along the x1- direction. Mindlin's two-dimensional equations are used for anisotropic crystal plates. Both free and electrically forced vibrations are considered. Important vibration characteristics are obtained, including dispersion relations, frequency spectra, and motional capacitances. It is shown that, to avoid the effects of the couplings between extension and thickness-twist vibrations, a series of discrete values of the length/thickness ratio of the crystal plate need to be excluded. The results are of fundamental significance for the design of LFE resonators and sensors.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 11174218 and 10674102)the Natural Science Foundation of Tianjin,China (Grant No. 05YFJMJC05200)
文摘Spectra of autoionizing states of the Sm atom in an energy region between 45948.9 cm^-1 and 46943.6 cm^-1 are systematically investigated by a three-color multi-step resonant excitation scheme with three different excitation paths.The three intermediate states,4f 66s7s 7F3,4f 66s7s 7F4,and 4f 66s7s 9F5 are employed for the three paths,respectively.Based on precise calibration of wavelength,the level energies of 112 autoionizing states are determined with the line widths and the relative line intensities of the related transitions.The possible influence of configuration interaction on the line shape of autoionizing state is also discussed.In addition,a unique value of J,the total angular momentum,is assigned to all detected states by comparing the three spectra obtained with the different excitation paths.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61378082 and 61675070)the Project of High-level Professionals in the Universities of Guangdong Province,China
文摘Thermal emission is often presented as a typical incoherent process. Incorporating periodic structures on the tungsten surface offers the possibility to obtain coherent thermal emission sources. Here we illustrate grating as an example to examine the influence of the geometric parameters on the thermal emission properties. It is found that for very shallow gratings, only surface plasmon polariton(SPP) modes can be excited and the emission efficiency is closely related with the filling factor. When the ratio of the depth to period of the grating is in the range from 1/20 to 1/2, the field between the adjacent corners can be coupled to each other across the air gap for the filling factor larger than 0.5 and produce a similar resonance as in an air rod. Further increase of the grating depth can cause the groove of the grating forming metal–insulator–metal(MIM) structures and induce surface plasmon standing wave modes. Our investigations will not only be helpful for manipulating thermal emission properties according to applications, but also help us understand the coupling mechanism between the incident electromagnetism waves and gratings with different parameters in various research fields.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.91321310 and 11404325)the National Basic Research Program of China(Grant No.2013CB922304)
文摘The spin fluctuation in rubidium atom gas is studied via all-optical spin noise spectroscopy(SNS).Experimental results show that the integrated SNS signal and its full width at half maximum(FWHM) strongly depend on the frequency detuning of the probe light under resonant and non-resonant conditions.The total integrated SNS signal can be well fitted with a single squared Faraday rotation spectrum and the FWHM dependence may be related to the absorption profile of the sample.
基金the National Key R&D Program of China(Grant No.2018YFA0306303)the National Natural Science Foundation of China(Grant Nos.11834004,61690224,92150105,11904103,12241407,and 12227807)the Science and Technology Commission of Shanghai Municipality(Grant No.21ZR1420100).
文摘Multiphoton resonant excitation and frustrated tunneling ionization,manifesting the photonic and optical nature of the driving light via direct excitation and electron recapture,respectively,are complementary mechanisms to access Rydberg state excitation(RSE)of atoms and molecules in an intense laser field.However,clear identification and manipulation of their individual contributions in the light-induced RSE process remain experimentally challenging.Here,we bridge this gap by exploring the dissociative and nondissociative RSE of H2 molecules using bicircular two-color laser pulses.Depending on the relative field strength and polarization helicity of the two colors,the RSE probability can be boosted by more than one order of magnitude by exploiting the laser waveform-dependent field effect.The role of the photon effect is readily strengthened with increasing relative strength of the second-harmonic field of the two colors regardless of the polarization helicity.As compared to the nondissociative RSE forming H2,the field effect in producing the dissociative RSE channel of eHt;HT is moderately suppressed,which is primarily accessed via a three-step sequential process separated by molecular bond stretching.Our work paves the way toward a comprehensive understanding of the interplay of the underlying field and photon effects in the strong-field RSE process,as well as facilitating the generation of Rydberg states optimized with tailored characteristics.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 1179041,11025417,and 10979007)the NSAF (Grant No. 10876043)
文摘The relativistic configuration interaction method is employed to calculate the dielectronic recombination(DR) cross sections of helium-like krypton via the 1s2lnl ’(n = 2,3,...,15) resonances.Then,the resonant transfer excitation(RTE) processes of Kr 34+ colliding with H,He,H 2,and CH x(x = 0-4) targets are investigated under the impulse approximation.The needed Compton profiles of targets are obtained from the Hartree-Fock wave functions.The RTE cross sections are strongly dependent on DR resonant energies and strengths,and the electron momentum distributions of the target.For H 2 and H targets,the ratio of their RTE cross sections changes from 1.85 for the 1s2l2l ’ to 1.88 for other resonances,which demonstrates the weak molecular effects on the Compton profiles of H 2.For CH x(x = 0-4) targets,the main contribution to the RTE cross section comes from the carbon atom since carbon carries 6 electrons;as the number of hydrogen increases in CH x,the RTE cross section almost increases by the same value,displaying the strong separate atom character for the hydrogen.However,further comparison of the individual orbital contributions of C(2p,2s,1s) and CH 4(1t 2,2a 1,1a 1) to the RTE cross sections shows that the molecular effects induce differences of about 25.1%,19.9%,and 0.2% between 2p-1t 2,2s-2a 1,and 1s-1a 1 orbitals,respectively.
基金the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XD30000000)the National Key R&D Program of China(Grant Nos.2018YFA0305802 and 2017YFA0303500)the National Natural Science Foundation of China(Grant No.11774267).Calculations were performed at the supercomputing center of WHU of China.
文摘High-order nonlinear multiphoton absorption is usually inefficient,but can be enhanced by designing resonant excitations between occupied and unoccupied energy levels.We conducted angle-resolved multi-photon photoemission(mPPE)studies on the SnSe_(2)(001)surfaces excited by ultrashort laser pulses.By tuning photon energy and light polarization,we demonstrate the presence of a resonant four-photon photoemission(4PPE)process involving the occupied valence band(VB),the unoccupied second conduction band(CB2)and the unoccupied image-potential state(IPs)of SnSe_(2).In this 4PPE process,VB electrons of SnSe_(2) are resonantly excited into CB2 by adsorbing two photons,followed by the adsorption of another photon to populate the n=1 IPs before being emitted out to the vacuum by adsorbing one more photon.This results in a double-resonant 4PPE process,which exhibits approximately a 40 times enhancement in photoemission yields compared to cases where one of the resonant pathways,CB2→IPs,is inhibited by involving a virtual state instead of the IPs in the 4PPE.The double-resonant 4PPE process efficiently excite the bulk VB electrons outside the vacuum,like taking advantage of resonant“ladders”through two real empty electronic states of SnSe_(2).Our results highlight the important applications of mPPE in probing the band-structure,particularly the unoccupied states,of recently emerging main group dichalcogenide semiconductors.Furthermore,the discovered resonant mPPE process contributes to the exploration of their promising optoelectronic applications.
基金National Natural Science Foundation of China(NSFC)(11604276,61601393,11501481)Key Scientific Project of Fujian Province in China(2015H0039)
文摘Multiple resonant excitations of surface plasmons in a graphene stratified slab are realized by Otto configuration at terahertz frequencies. The proposed graphene stratified slab consists of alternating dielectric layers and graphene sheets, and is sandwiched between a prism and another semi-infinite medium. Optical response and field distribution are determined by the transfer matrix method with the surface current density boundary condition.Multiple resonant excitations appear on the angular reflection spectrum, and are analyzed theoretically via the phase-matching condition. Furthermore, the effects of the system parameters are investigated. Among them, the Fermi levels can tune the corresponding resonances independently. The proposed concept can be engineered for promising applications, including angular selective or multiplex filters, multiple channel sensors, and directional delivery of energy.