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Hybrid pedestrian positioning system using wearable inertial sensors and ultrasonic ranging
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作者 Lin Qi Yu Liu +2 位作者 Chuanshun Gao Tao Feng Yue Yu 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2024年第3期327-338,共12页
Pedestrian positioning system(PPS)using wearable inertial sensors has wide applications towards various emerging fields such as smart healthcare,emergency rescue,soldier positioning,etc.The performance of traditional ... Pedestrian positioning system(PPS)using wearable inertial sensors has wide applications towards various emerging fields such as smart healthcare,emergency rescue,soldier positioning,etc.The performance of traditional PPS is limited by the cumulative error of inertial sensors,complex motion modes of pedestrians,and the low robustness of the multi-sensor collaboration structure.This paper presents a hybrid pedestrian positioning system using the combination of wearable inertial sensors and ultrasonic ranging(H-PPS).A robust two nodes integration structure is developed to adaptively combine the motion data acquired from the single waist-mounted and foot-mounted node,and enhanced by a novel ellipsoid constraint model.In addition,a deep-learning-based walking speed estimator is proposed by considering all the motion features provided by different nodes,which effectively reduces the cumulative error originating from inertial sensors.Finally,a comprehensive data and model dual-driven model is presented to effectively combine the motion data provided by different sensor nodes and walking speed estimator,and multi-level constraints are extracted to further improve the performance of the overall system.Experimental results indicate that the proposed H-PPS significantly improves the performance of the single PPS and outperforms existing algorithms in accuracy index under complex indoor scenarios. 展开更多
关键词 Pedestrian positioning system Wearable inertial sensors Ultrasonic ranging Deep-learning Data and model dual-driven
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Design and Implementation of Batch Calibration System for Platinum Resistance Temperature Sensors
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作者 Hui LIANG Tianwen SONG Yun XIAN 《Meteorological and Environmental Research》 CAS 2023年第5期19-23,共5页
Developing a calibration and collection system of platinum resistance temperature sensor using Python language environment can read the information returned by the serial port and automatically generate an"Temper... Developing a calibration and collection system of platinum resistance temperature sensor using Python language environment can read the information returned by the serial port and automatically generate an"Temperature Sensor Calibration Record Table"excel table with the current date as the file name.It can collect data from 10 platinum resistance temperature sensors at once,achieving automation and improving work efficiency. 展开更多
关键词 PYTHON Air temperature sensor COLLECTION
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An Activity Recognition System at Home Based on CO2 Sensors
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作者 Hiroyuki Matsubara 《Journal of Computer and Communications》 2023年第11期64-77,共14页
Activity recognition of indoor occupants using indirect sensing with less privacy violation is one of the hot research topics. This paper proposes a CO<sub>2</sub> sensor-based indoor occupant activity mon... Activity recognition of indoor occupants using indirect sensing with less privacy violation is one of the hot research topics. This paper proposes a CO<sub>2</sub> sensor-based indoor occupant activity monitoring system. Using the IoT sensor node that contains CO<sub>2</sub> sensors, the measured CO<sub>2</sub> concentrations in three locations (laboratory, office, and bedroom) were stored in a cloud server for up to 35 days starting July 1, 2023. The CO<sub>2</sub> measurements stored at 30-second intervals were statistically processed to produce a heat-mapped display of the hourly average or maximum CO<sub>2</sub> concentration. From the heatmap visualizations of CO<sub>2</sub> concentration, the proposed system estimated meeting, heating water using a portable stove, and sleep for the occupants’ activity recognition. 展开更多
关键词 Activity Recognition CO2 Sensor Internet of Things (IoT) Low Privacy-Intrusion Heat Map
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Collaborative positioning for swarms:A brief survey of vision,LiDAR and wireless sensors based methods
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作者 Zeyu Li Changhui Jiang +3 位作者 Xiaobo Gu Ying Xu Feng zhou Jianhui Cui 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2024年第3期475-493,共19页
As positioning sensors,edge computation power,and communication technologies continue to develop,a moving agent can now sense its surroundings and communicate with other agents.By receiving spatial information from bo... As positioning sensors,edge computation power,and communication technologies continue to develop,a moving agent can now sense its surroundings and communicate with other agents.By receiving spatial information from both its environment and other agents,an agent can use various methods and sensor types to localize itself.With its high flexibility and robustness,collaborative positioning has become a widely used method in both military and civilian applications.This paper introduces the basic fundamental concepts and applications of collaborative positioning,and reviews recent progress in the field based on camera,LiDAR(Light Detection and Ranging),wireless sensor,and their integration.The paper compares the current methods with respect to their sensor type,summarizes their main paradigms,and analyzes their evaluation experiments.Finally,the paper discusses the main challenges and open issues that require further research. 展开更多
关键词 Collaborative positioning VISION LIDAR Wireless sensors Sensor fusion
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Progress of Proximity Sensors for Potential Applications in Electronic Skins
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作者 Runnan Zou Yanhong Tong +3 位作者 Jiayi Liu Jing Sun Da Xian Qingxin Tang 《Transactions of Tianjin University》 EI CAS 2024年第1期40-62,共23页
Recently,electronic skins and fl exible wearable devices have been developed for widespread applications in medical monitoring,artifi cial intelligence,human–machine interaction,and artifi cial prosthetics.Flexible p... Recently,electronic skins and fl exible wearable devices have been developed for widespread applications in medical monitoring,artifi cial intelligence,human–machine interaction,and artifi cial prosthetics.Flexible proximity sensors can accurately perceive external objects without contact,introducing a new way to achieve an ultrasensitive perception of objects.This article reviews the progress of fl exible capacitive proximity sensors,fl exible triboelectric proximity sensors,and fl exible gate-enhanced proximity sensors,focusing on their applications in the electronic skin fi eld.Herein,their working mechanism,materials,preparation methods,and research progress are discussed in detail.Finally,we summarize the future challenges in developing fl exible proximity sensors. 展开更多
关键词 Capacitive proximity sensors Triboelectric proximity sensors Gate-enhanced proximity sensors Flexible wearable devices Electronic skins
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Advances of Electrochemical and Electrochemiluminescent Sensors Based on Covalent Organic Frameworks
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作者 Yue Cao Ru Wu +2 位作者 Yan‑Yan Gao Yang Zhou Jun‑Jie Zhu 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第2期395-422,共28页
Covalent organic frameworks(COFs),a rapidly developing category of crystalline conjugated organic polymers,possess highly ordered structures,large specific surface areas,stable chemical properties,and tunable pore mic... Covalent organic frameworks(COFs),a rapidly developing category of crystalline conjugated organic polymers,possess highly ordered structures,large specific surface areas,stable chemical properties,and tunable pore microenvironments.Since the first report of boroxine/boronate ester-linked COFs in 2005,COFs have rapidly gained popularity,showing important application prospects in various fields,such as sensing,catalysis,separation,and energy storage.Among them,COFs-based electrochemical(EC)sensors with upgraded analytical performance are arousing extensive interest.In this review,therefore,we summarize the basic properties and the general synthesis methods of COFs used in the field of electroanalytical chemistry,with special emphasis on their usages in the fabrication of chemical sensors,ions sensors,immunosensors,and aptasensors.Notably,the emerged COFs in the electrochemiluminescence(ECL)realm are thoroughly covered along with their preliminary applications.Additionally,final conclusions on state-of-the-art COFs are provided in terms of EC and ECL sensors,as well as challenges and prospects for extending and improving the research and applications of COFs in electroanalytical chemistry. 展开更多
关键词 Covalent organic frameworks ELECTROCHEMISTRY ELECTROCHEMILUMINESCENCE sensors
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Combined CNN-LSTM Deep Learning Algorithms for Recognizing Human Physical Activities in Large and Distributed Manners:A Recommendation System
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作者 Ameni Ellouze Nesrine Kadri +1 位作者 Alaa Alaerjan Mohamed Ksantini 《Computers, Materials & Continua》 SCIE EI 2024年第4期351-372,共22页
Recognizing human activity(HAR)from data in a smartphone sensor plays an important role in the field of health to prevent chronic diseases.Daily and weekly physical activities are recorded on the smartphone and tell t... Recognizing human activity(HAR)from data in a smartphone sensor plays an important role in the field of health to prevent chronic diseases.Daily and weekly physical activities are recorded on the smartphone and tell the user whether he is moving well or not.Typically,smartphones and their associated sensing devices operate in distributed and unstable environments.Therefore,collecting their data and extracting useful information is a significant challenge.In this context,the aimof this paper is twofold:The first is to analyze human behavior based on the recognition of physical activities.Using the results of physical activity detection and classification,the second part aims to develop a health recommendation system to notify smartphone users about their healthy physical behavior related to their physical activities.This system is based on the calculation of calories burned by each user during physical activities.In this way,conclusions can be drawn about a person’s physical behavior by estimating the number of calories burned after evaluating data collected daily or even weekly following a series of physical workouts.To identify and classify human behavior our methodology is based on artificial intelligence models specifically deep learning techniques like Long Short-Term Memory(LSTM),stacked LSTM,and bidirectional LSTM.Since human activity data contains both spatial and temporal information,we proposed,in this paper,to use of an architecture allowing the extraction of the two types of information simultaneously.While Convolutional Neural Networks(CNN)has an architecture designed for spatial information,our idea is to combine CNN with LSTM to increase classification accuracy by taking into consideration the extraction of both spatial and temporal data.The results obtained achieved an accuracy of 96%.On the other side,the data learned by these algorithms is prone to error and uncertainty.To overcome this constraint and improve performance(96%),we proposed to use the fusion mechanisms.The last combines deep learning classifiers tomodel non-accurate and ambiguous data to obtain synthetic information to aid in decision-making.The Voting and Dempster-Shafer(DS)approaches are employed.The results showed that fused classifiers based on DS theory outperformed individual classifiers(96%)with the highest accuracy level of 98%.Also,the findings disclosed that participants engaging in physical activities are healthy,showcasing a disparity in the distribution of physical activities between men and women. 展开更多
关键词 Human physical activities smartphone sensors deep learning distributed monitoring recommendation system uncertainty HEALTHY CALORIES
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Observer-based dynamic event-triggered control for distributed parameter systems over mobile sensor-plus-actuator networks
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作者 穆文英 庄波 邱芳 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第4期237-243,共7页
We develop a policy of observer-based dynamic event-triggered state feedback control for distributed parameter systems over a mobile sensor-plus-actuator network.It is assumed that the mobile sensing devices that prov... We develop a policy of observer-based dynamic event-triggered state feedback control for distributed parameter systems over a mobile sensor-plus-actuator network.It is assumed that the mobile sensing devices that provide spatially averaged state measurements can be used to improve state estimation in the network.For the purpose of decreasing the update frequency of controller and unnecessary sampled data transmission, an efficient dynamic event-triggered control policy is constructed.In an event-triggered system, when an error signal exceeds a specified time-varying threshold, it indicates the occurrence of a typical event.The global asymptotic stability of the event-triggered closed-loop system and the boundedness of the minimum inter-event time can be guaranteed.Based on the linear quadratic optimal regulator, the actuator selects the optimal displacement only when an event occurs.A simulation example is finally used to verify that the effectiveness of such a control strategy can enhance the system performance. 展开更多
关键词 distributed parameter systems event-triggered control mobile sensors mobile actuators
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Implantable Electrochemical Microsensors for In Vivo Monitoring of Animal Physiological Information
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作者 Jin Zhou Shenghan Zhou +4 位作者 Peidi Fan Xunjia Li Yibin Ying Jianfeng Ping Yuxiang Pan 《Nano-Micro Letters》 SCIE EI CSCD 2024年第3期183-211,共29页
In vivo monitoring of animal physiological information plays a crucial role in promptly alerting humans to potential diseases in animals and aiding in the exploration of mechanisms underlying human diseases.Currently,... In vivo monitoring of animal physiological information plays a crucial role in promptly alerting humans to potential diseases in animals and aiding in the exploration of mechanisms underlying human diseases.Currently,implantable electrochemical microsensors have emerged as a prominent area of research.These microsensors not only fulfill the technical requirements for monitoring animal physiological information but also offer an ideal platform for integration.They have been extensively studied for their ability to monitor animal physiological information in a minimally invasive manner,characterized by their bloodless,painless features,and exceptional performance.The development of implantable electrochemical microsensors for in vivo monitoring of animal physiological information has witnessed significant scientific and technological advancements through dedicated efforts.This review commenced with a comprehensive discussion of the construction of microsensors,including the materials utilized and the methods employed for fabrication.Following this,we proceeded to explore the various implantation technologies employed for electrochemical microsensors.In addition,a comprehensive overview was provided of the various applications of implantable electrochemical microsensors,specifically in the monitoring of diseases and the investigation of disease mechanisms.Lastly,a concise conclusion was conducted on the recent advancements and significant obstacles pertaining to the practical implementation of implantable electrochemical microsensors. 展开更多
关键词 Electrochemical microsensors Implantable sensors In vivo monitoring Animal physiological information
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An Ingenious IoT Based Crop Prediction System Using ML and EL
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作者 Shabana Ramzan Yazeed Yasin Ghadi +2 位作者 Hanan Aljuaid Aqsa Mahmood Basharat Ali 《Computers, Materials & Continua》 SCIE EI 2024年第4期183-199,共17页
Traditional farming procedures are time-consuming and expensive as based on manual labor. Farmers haveno proper knowledge to select which crop is suitable to grow according to the environmental factors and soilcharact... Traditional farming procedures are time-consuming and expensive as based on manual labor. Farmers haveno proper knowledge to select which crop is suitable to grow according to the environmental factors and soilcharacteristics. This is the main reason for the low yield of crops and the economic crisis in the agricultural sectorof the different countries. The use of modern technologies such as the Internet of Things (IoT), machine learning,and ensemble learning can facilitate farmers to observe different factors such as soil electrical conductivity (EC),and environmental factors like temperature to improve crop yield. These parameters play a vital role in suggestinga suitable crop to cope the food scarcity. This paper proposes a systemcomprised of twomodules, first module usesstatic data and the second module takes hybrid data collection (IoT-based real-time data and manual data) withmachine learning and ensemble learning algorithms to suggest the suitable crop in the farm to maximize the yield.Python is used to train the model that predicts the crop. This system proposed an intelligent and low-cost solutionfor the farmers to process the data and predict the suitable crop.We implemented the proposed system in the field.The efficiency and accuracy of the proposed system are confirmed by the generated results to predict the crop. 展开更多
关键词 Machine learning Internet of Things sensors ensemble learning
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Recent progress on nanomaterial-based electrochemical dissolved oxygen sensors
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作者 Shaoqi Zhang Tao Liu +1 位作者 Zhenyu Chu Wanqin Jin 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2024年第4期103-119,共17页
Dissolved oxygen(DO)usually refers to the amount of oxygen dissolved in water.In the environment,medicine,and fermentation industries,the DO level needs to be accurate and capable of online monitoring to guide the pre... Dissolved oxygen(DO)usually refers to the amount of oxygen dissolved in water.In the environment,medicine,and fermentation industries,the DO level needs to be accurate and capable of online monitoring to guide the precise control of water quality,clinical treatment,and microbial metabolism.Compared with other analytical methods,the electrochemical strategy is superior in its fast response,low cost,high sensitivity,and portable device.However,an electrochemical DO sensor faces a trade-off between sensitivity and long-term stability,which strongly limits its practical applications.To solve this problem,various advanced nanomaterials have been proposed to promote detection performance owing to their excellent electrocatalysis,conductivity,and chemical stability.Therefore,in this review,we focus on the recent progress of advanced nanomaterial-based electrochemical DO sensors.Through the comparison of the working principles on the main analysis techniques toward DO,the advantages of the electrochemical method are discussed.Emphasis is placed on recently developed nanomaterials that exhibit special characteristics,including nanostructures and preparation routes,to benefit DO determination.Specifically,we also introduce some interesting research on the configuration design of the electrode and device,which is rarely introduced.Then,the different requirements of the electrochemical DO sensors in different application fields are included to provide brief guidance on the selection of appropriate nanomaterials.Finally,the main challenges are evaluated to propose future development prospects and detection strategies for nanomaterial-based electrochemical sensors. 展开更多
关键词 NANOMATERIAL Dissolved oxygen Electrochemical sensor NANOSTRUCTURES Detection principles
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Security Analysis in Smart Agriculture: Insights from a Cyber-Physical System Application
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作者 Ahmed Redha Mahlous 《Computers, Materials & Continua》 SCIE EI 2024年第6期4781-4803,共23页
Smart agriculture modifies traditional farming practices,and offers innovative approaches to boost production and sustainability by leveraging contemporary technologies.In today’s world where technology is everything... Smart agriculture modifies traditional farming practices,and offers innovative approaches to boost production and sustainability by leveraging contemporary technologies.In today’s world where technology is everything,these technologies are utilized to streamline regular tasks and procedures in agriculture,one of the largest and most significant industries in every nation.This research paper stands out from existing literature on smart agriculture security by providing a comprehensive analysis and examination of security issues within smart agriculture systems.Divided into three main sections-security analysis,system architecture and design and risk assessment of Cyber-Physical Systems(CPS)applications-the study delves into various elements crucial for smart farming,such as data sources,infrastructure components,communication protocols,and the roles of different stakeholders such as farmers,agricultural scientists and researchers,technology providers,government agencies,consumers and many others.In contrast to earlier research,this work analyzes the resilience of smart agriculture systems using approaches such as threat modeling,penetration testing,and vulnerability assessments.Important discoveries highlight the concerns connected to unsecured communication protocols,possible threats from malevolent actors,and vulnerabilities in IoT devices.Furthermore,the study suggests enhancements for CPS applications,such as strong access controls,intrusion detection systems,and encryption protocols.In addition,risk assessment techniques are applied to prioritize mitigation tactics and detect potential hazards,addressing issues like data breaches,system outages,and automated farming process sabotage.The research sets itself apart even more by presenting a prototype CPS application that makes use of a digital temperature sensor.This application was first created using a Tinkercad simulator and then using actual hardware with Arduino boards.The CPS application’s defenses against potential threats and vulnerabilities are strengthened by this integrated approach,which distinguishes this research for its depth and usefulness in the field of smart agriculture security. 展开更多
关键词 Smart agriculture cyber-physical system IOT security temperature sensor threats VULNERABILITIES
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Nanomaterial-assisted wearable glucose biosensors for noninvasive real-time monitoring:Pioneering point-of-care and beyond
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作者 Moein Safarkhani Abdullah Aldhaher +5 位作者 Golnaz Heidari Ehsan Nazarzadeh Zare Majid Ebrahimi Warkiani Omid Akhavan YunSuk Huh Navid Rabiee 《Nano Materials Science》 EI CAS CSCD 2024年第3期263-283,共21页
This review explores glucose monitoring and management strategies,emphasizing the need for reliable and userfriendly wearable sensors that are the next generation of sensors for continuous glucose detection.In additio... This review explores glucose monitoring and management strategies,emphasizing the need for reliable and userfriendly wearable sensors that are the next generation of sensors for continuous glucose detection.In addition,examines key strategies for designing glucose sensors that are multi-functional,reliable,and cost-effective in a variety of contexts.The unique features of effective diabetes management technology are highlighted,with a focus on using nano/biosensor devices that can quickly and accurately detect glucose levels in the blood,improving patient treatment and control of potential diabetes-related infections.The potential of next-generation wearable and touch-sensitive nano biomedical sensor engineering designs for providing full control in assessing implantable,continuous glucose monitoring is also explored.The challenges of standardizing drug or insulin delivery doses,low-cost,real-time detection of increased blood sugar levels in diabetics,and early digital health awareness controls for the adverse effects of injectable medication are identified as unmet needs.Also,the market for biosensors is expected to expand significantly due to the rising need for portable diagnostic equipment and an ever-increasing diabetic population.The paper concludes by emphasizing the need for further research and development of glucose biosensors to meet the stringent requirements for sensitivity and specificity imposed by clinical diagnostics while being cost-effective,stable,and durable. 展开更多
关键词 Glucose sensor BIOSENSOR Wearable devices NONINVASIVE Real-time monitoring
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MXene-Based Elastomer Mimetic StretchableSensors: Design, Properties, and Applications
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作者 Poushali Das Parham Khoshbakht Marvi +5 位作者 Sayan Ganguly Xiaowu(Shirley)Tang Bo Wang Seshasai Srinivasan Amin Reza Rajabzadeh Andreas Rosenkranz 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第7期295-342,共48页
Flexible sensors based on MXene-polymer composites are highly prospective for next-generation wearable electronics used in human-machine interfaces.One of the motivating factors behind the progress of flexible sensors... Flexible sensors based on MXene-polymer composites are highly prospective for next-generation wearable electronics used in human-machine interfaces.One of the motivating factors behind the progress of flexible sensors is the steady arrival of new conductive materials.MXenes,a new family of 2D nanomaterials,have been draw-ing attention since the last decade due to their high electronic conduc-tivity,processability,mechanical robustness and chemical tunability.In this review,we encompass the fabrication of MXene-based polymeric nanocomposites,their structure-property relationship,and applications in the flexible sensor domain.Moreover,our discussion is not only lim-ited to sensor design,their mechanism,and various modes of sensing platform,but also their future perspective and market throughout the world.With our article,we intend to fortify the bond between flexible matrices and MXenes thus promoting the swift advancement of flexible MXene-sensors for wearable technologies. 展开更多
关键词 Flexible sensor 2D nanomaterials MXene Wearable and conductive Applications
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Electrochemical biosensors for point-of-care testing
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作者 Jinsol Kim Juho Jeong Seung Hwan Ko 《Bio-Design and Manufacturing》 SCIE EI CAS CSCD 2024年第4期548-565,共18页
Point-of-care testing(POCT)is the practice of diagnosing and monitoring diseases where the patient is located,as opposed to traditional treatment conducted solely in a medical laboratory or other clinical setting.POCT... Point-of-care testing(POCT)is the practice of diagnosing and monitoring diseases where the patient is located,as opposed to traditional treatment conducted solely in a medical laboratory or other clinical setting.POCT has been less common in the recent past due to a lack of portable medical devices capable of facilitating effective medical testing.However,recent growth has occurred in this field due to advances in diagnostic technologies,device miniaturization,and progress in wearable electronics.Among these developments,electrochemical sensors have attracted interest in the POCT field due to their high sensitivity,compact size,and affordability.They are used in various applications,from disease diagnosis to health status monitoring.In this paper we explore recent advancements in electrochemical sensors,the methods of fabricating them,and the various types of sensing mechanisms that can be used.Furthermore,we delve into methods for immobilizing specific biorecognition elements,including enzymes,antibodies,and aptamers,onto electrode surfaces and how these sensors are used in real-world POCT settings. 展开更多
关键词 Point-of-care testing(POCT) Electrochemical sensor ENZYME ANTIBODY Health care
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MXene Key Composites:A New Arena for Gas Sensors
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作者 Yitong Wang Yuhua Wang +2 位作者 Min Jian Qinting Jiang Xifei Li 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第10期350-391,共42页
With the development of science and technology,the scale of industrial production continues to grow,and the types and quantities of gas raw materials used in industrial production and produced during the production pr... With the development of science and technology,the scale of industrial production continues to grow,and the types and quantities of gas raw materials used in industrial production and produced during the production process are also constantly increasing.These gases include flammable and explosive gases,and even contain toxic gases.Therefore,it is very important and necessary for gas sensors to detect and monitor these gases quickly and accurately.In recent years,a new two-dimensional material called MXene has attracted widespread attention in various applications.Their abundant surface functional groups and sites,excellent current conductivity,tunable surface chemistry,and outstanding stability make them promising for gas sensor applications.Since the birth of MXene materials,researchers have utilized the efficient and convenient solution etching preparation,high flexibility,and easily functionalize MXene with other materials to pre-pare composites for gas sensing.This has opened a new chapter in high-performance gas sensing materials and provided a new approach for advanced sensor research.However,previous reviews on MXene-based composite materials in gas sensing only focused on the performance of gas sensing,without systematically explaining the gas sensing mechanisms generated by different gases,as well as summarizing and predicting the advantages and disadvantages of MXene-based composite materials.This article reviews the latest progress in the application of MXene-based composite materials in gas sensing.Firstly,a brief summary was given of the commonly used methods for preparing gas sens-ing device structures,followed by an introduction to the key attributes of MXene related to gas sensing performance.This article focuses on the performance of MXene-based composite materials used for gas sensing,such as MXene/graphene,MXene/Metal oxide,MXene/Transition metal sulfides(TMDs),MXene/Metal-organic framework(MOF),MXene/Polymer.It summarizes the advantages and disadvantages of MXene com-posite materials with different composites and discusses the possible gas sensing mechanisms of MXene-based composite materials for different gases.Finally,future directions and inroads of MXenes-based composites in gas sensing are presented and discussed. 展开更多
关键词 MXene Compound material Gas sensor Gas sensitive preparation Gas sensitivity performance
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Isomeric fluorescence sensors for wide range detection of ionizing radiations
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作者 Jimin Han Tianyu Yang +1 位作者 Li Yang Yuanjian Li 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2024年第4期247-257,共11页
In order to achieve a wider range of ionizing radiations detection,novel fluorescence sensing materials have been developed that utilize the fluorescence enhancement phenomenon caused by the intramolecular photoinduce... In order to achieve a wider range of ionizing radiations detection,novel fluorescence sensing materials have been developed that utilize the fluorescence enhancement phenomenon caused by the intramolecular photoinduced electron transfer(PET)effect.Two perylene diimide isomers PDI-P and PDI-B were designed and synthesized,and their molecular structures were characterized by high-resolution Fourier transform mass spectrometry(HRMS),nuclear magnetic resonance hydrogen and carbon spectroscopy(~1H and~(13)C NMR).The interaction between ionizing radiation and fluorescent molecules was simulated by HCl titration.The results show that combining PDIs and HCl can improve fluorescence through the retro-PET process.Despite the similarities in chemical structures,the fluorescent enhancement multiple of PDI-B with aromatic amine as electron donor is much higher than that of PDI-P with alkyl amine.In the direct irradiation experiments of ionizing radiation,the emission enhancement multiples of PDI-P and PDI-B are 2.01 and 45.4,respectively.Furthermore,density functional theory(DFT)and time-dependent density functional theory(TDDFT)calculations indicate that the HOMO and HOMO-1 energy ranges of PDI-P and PDI-B are 0.54 e V and 1.13 e V,respectively.A wider energy range has a stronger driving force on electrons,which is conducive to fluorescence quenching.Both femtosecond transient absorption spectroscopy(fs-TAS)and transient fluorescence spectroscopy(TFS)tests show that PDI-B has shorter charge separation lifetime and higher electron transfer rate constant.Although both isomers can significantly reduce LOD during PET process,PDI-B with aromatic amine has a wider detection range of 0.118—240 Gy due to its larger emission enhancement,which is a leap of three orders of magnitude.It breaks through the detection range of gamma radiation reported in existing studies,and provides theoretical support for the further study of sensitive and effective new materials for ionizing radiation detection. 展开更多
关键词 Perylene imide Intramolecular PET Ionizing radiation detection Fluorescence sensor ISOMERS
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A crosstalk-free dual-mode sweat sensing system for naked-eye sweat loss quantification via changes in structural reflectance
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作者 Bowen Zhong Hao Xu +3 位作者 Xiaokun Qin Lingchen Liu Hailong Wang Lili Wang 《Bio-Design and Manufacturing》 SCIE EI CAS CSCD 2024年第4期428-438,共11页
Sweat loss monitoring is important for understanding the body’s thermoregulation and hydration status,as well as for comprehensive sweat analysis.Despite recent advances,developing a low-cost,scalable,and universal m... Sweat loss monitoring is important for understanding the body’s thermoregulation and hydration status,as well as for comprehensive sweat analysis.Despite recent advances,developing a low-cost,scalable,and universal method for the fabrication of colorimetric microfluidics designed for sweat loss monitoring remains challenging.In this study,we propose a novel laserengraved surface roughening strategy for various flexible substrates.This process permits the construction of microchannels that show distinct structural reflectance changes before and after sweat filling.By leveraging these unique optical properties,we have developed a fully laser-engraved microfluidic device for the quantification of naked-eye sweat loss.This sweat loss sensor is capable of a volume resolution of 0.5µL and a total volume capacity of 11µL,and can be customized to meet different performance requirements.Moreover,we report the development of a crosstalk-free dual-mode sweat microfluidic system that integrates an Ag/AgCl chloride sensor and a matching wireless measurement flexible printed circuit board.This integrated system enables the real-time monitoring of colorimetric sweat loss signals and potential ion concentration signals without crosstalk.Finally,we demonstrate the potential practical use of this microfluidic sweat loss sensor and its integrated system for sports medicine via on-body studies. 展开更多
关键词 Sweat loss sensor Microfluidic design Structural reflectance Dual-mode integration Crosstalk-free
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The Fabrication and Detection Performance of High Sensitivity Au-Ag Alloy Nanostar/Paper Flexible Surface Enhanced Raman Spectroscopy Sensors
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作者 邓芷盈 WANG Tianyi +4 位作者 CAO Shiyi ZHAO Yuan HAN Xiaoyu 张继红 谢俊 《Journal of Wuhan University of Technology(Materials Science)》 SCIE EI CAS CSCD 2024年第2期436-443,共8页
Au-Ag alloy nanostars based flexible paper surface enhanced Raman spectroscopy sensors were fabricated through simple nanostar coating on regular office paper,and the surface enhanced Raman spectroscopy detection perf... Au-Ag alloy nanostars based flexible paper surface enhanced Raman spectroscopy sensors were fabricated through simple nanostar coating on regular office paper,and the surface enhanced Raman spectroscopy detection performances were investigated using crystal violet dye analyte.Au-Ag nanostars with sharp tips were synthesized via metal ions reduction method.Transmission electron microscope images,X-Ray diffraction pattern and energy dispersive spectroscopy elemental mapping confirmed the nanostar geometry and Au/Ag components of the nanostructure.UV-Vis-NIR absorption spectrum shows wide local surface plasmon resonance induced optical extinction.In addition,finite-difference time-domain simulation shows much stronger electromagnetic field from nanostars than from sphere nanoparticle.The effect of coating layer on Raman signal intensities was discussed,and optimized 5-layer coating with best Raman signal was obtained.The Au-Ag nanostatrs homogeneously distribute on paper fiber surface.The detection limit is 10-10 M,and the relationship between analyte concentrations and Raman signal intensities shows well linear,for potential quantitative analysis.The calculated enhancement factor is 4.795×10^(6).The flexible paper surface enhanced Raman spectroscopy sensors could be applied for trace chemical and biology molecule detection. 展开更多
关键词 surface-enhanced raman gold-silver alloy nanostars paper-based SERS sensor FLEXIBILITY
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Building Feedback-Regulation System Through Atomic Design for Highly Active SO_(2)Sensing
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作者 Xin Jia Panzhe Qiao +8 位作者 Xiaowu Wang Muyu Yan Yang Chen Bao-Li An Pengfei Hu Bo Lu Jing Xu Zhenggang Xue Jiaqiang Xu 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第7期343-357,共15页
Reasonably constructing an atomic interface is pronouncedly essential for surface-related gas-sensing reaction.Herein,we present an ingen-ious feedback-regulation system by changing the interactional mode between sing... Reasonably constructing an atomic interface is pronouncedly essential for surface-related gas-sensing reaction.Herein,we present an ingen-ious feedback-regulation system by changing the interactional mode between single Pt atoms and adjacent S species for high-efficiency SO_(2)sensing.We found that the single Pt sites on the MoS_(2)surface can induce easier volatiliza-tion of adjacent S species to activate the whole inert S plane.Reversely,the activated S species can provide a feedback role in tailoring the antibonding-orbital electronic occupancy state of Pt atoms,thus creating a combined system involving S vacancy-assisted single Pt sites(Pt-Vs)to synergistically improve the adsorption ability of SO_(2)gas molecules.Further-more,in situ Raman,ex situ X-ray photoelectron spectroscopy testing and density functional theory analysis demonstrate the intact feedback-regulation system can expand the electron transfer path from single Pt sites to whole Pt-MoS_(2)supports in SO_(2)gas atmosphere.Equipped with wireless-sensing modules,the final Pt1-MoS_(2)-def sensors array can further realize real-time monitoring of SO_(2)levels and cloud-data storage for plant growth.Such a fundamental understanding of the intrinsic link between atomic interface and sensing mechanism is thus expected to broaden the rational design of highly effective gas sensors. 展开更多
关键词 Feedback-regulation system Atomic interface SO_(2)sensor Single-atom sensing mechanism Intelligent-sensing array
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