This review provides a comprehensive overview of the progress in light-material interactions(LMIs),focusing on lasers and flash lights for energy conversion and storage applications.We discuss intricate LMI parameters...This review provides a comprehensive overview of the progress in light-material interactions(LMIs),focusing on lasers and flash lights for energy conversion and storage applications.We discuss intricate LMI parameters such as light sources,interaction time,and fluence to elucidate their importance in material processing.In addition,this study covers various light-induced photothermal and photochemical processes ranging from melting,crystallization,and ablation to doping and synthesis,which are essential for developing energy materials and devices.Finally,we present extensive energy conversion and storage applications demonstrated by LMI technologies,including energy harvesters,sensors,capacitors,and batteries.Despite the several challenges associated with LMIs,such as complex mechanisms,and high-degrees of freedom,we believe that substantial contributions and potential for the commercialization of future energy systems can be achieved by advancing optical technologies through comprehensive academic research and multidisciplinary collaborations.展开更多
Improving the capacitance and energy density is a significant challenge while developing practical and flexible energy storage system(ESS).Redox mediators(RMs),as redox-active electrolyte additives,can provide additio...Improving the capacitance and energy density is a significant challenge while developing practical and flexible energy storage system(ESS).Redox mediators(RMs),as redox-active electrolyte additives,can provide additional energy storing capability via electrochemical faradaic contribution on electrodes for high-performance flexible ESSs.Particularly,determining effective material combinations between electrodes and RMs is essential for maximizing surface faradaic redox reactions for energy-storage performance.In this study,an electrode-RM system comprising heterostructured hybrid(carbon fiber(CF)/MnO_(2)) faradaic electrodes and iodine RMs(I-RMs) in a redox-active electrolyte is investigated.The CF/MnO_(2)with the 1-RMs(CF/MnO_(2)-I) induces dominant catalytic faradaic interaction with the I-RMs,significantly enhancing the surface faradaic kinetics and increasing the overall energy-storage performance.The CF/MnO_(2)-I ESSs show a 12.6-fold(or higher) increased volumetric energy density of 793.81 mWh L^(-1)at a current of 10 μA relative to ESSs using CF/MnO_(2)without I-RMs(CF/MnO_(2)).Moreover,the CF/MnO_(2)-I retains 93.1% of its initial capacitance after 10,000 cycles,validating the excellent cyclability.Finally,the flexibility of the ESSs is tested at different bending angles(180° to 0°),demonstrating its feasibility for flexible and high-wear environments.Therefore,CF/MnO_(2)electrodes present a practical material combination for high-performance flexible energy-storage devices owing to the catalytic faradaic interaction with I-RMs.展开更多
We investigated the properties of polarons in a wurtzite ZnO/MgxZn1-xO quantum well by adopting a modified Lee–Low–Pines variational method, giving the ground state energy, transition energy, and phonon contribution...We investigated the properties of polarons in a wurtzite ZnO/MgxZn1-xO quantum well by adopting a modified Lee–Low–Pines variational method, giving the ground state energy, transition energy, and phonon contributions from various optical-phonon modes to the ground state energy as functions of the well width and Mg composition. In our calculations, we considered the effects of confined optical phonon modes, interface-optical phonon modes, and half-space phonon modes, as well as the anisotropy of the electron effective band mass, phonon frequency, and dielectric constant. Our numerical results indicate that the electron–optical phonon interactions importantly affect the polaronic energies in the ZnO/MgxZn1-xO quantum well. The electron–optical phonon interactions decrease the polaron energies. For quantum wells with narrower wells, the interface optical phonon and half-space phonon modes contribute more to the polaronic energies than the confined phonon modes. However, for wider quantum wells, the total contribution to the polaronic energy mainly comes from the confined modes. The contributions of the various phonon modes to the transition energy change differently with increasing well width. The contribution of the half-space phonons decreases slowly as the QW width increases, whereas the contributions of the confined and interface phonons reach a maximum at d ≈ 5.0 nm and then decrease slowly. However,the total contribution of phonon modes to the transition energy is negative and increases gradually with the QW width of d.As the composition x increases, the total contribution of phonons to the ground state energies increases slowly, but the total contributions of phonons to the transition energies decrease gradually. We analyze the physical reasons for these behaviors in detail.展开更多
This paper investigates the collective excitation and stability of low-dimensional Bose-Einstein condensates with two- and three-body interactions by the variational analysis of the time-dependent Gross-Pitaevskii-Gin...This paper investigates the collective excitation and stability of low-dimensional Bose-Einstein condensates with two- and three-body interactions by the variational analysis of the time-dependent Gross-Pitaevskii-Ginsburg equation. The spectrum of the low-energy excitation and the effective potential for the width of the condensate axe obtained. The results show that: (i) the repulsive two-body interaction among atoms makes the frequency red-shifted for the internal excitation and the repulsive or attractive three-body interaction always makes it blue-shifted; (ii) the region for the existence of the stable bound states is obtained by identifying the critical value of the two- and three-body interactions.展开更多
An offshore wind-wave hybrid platform could consistently and cost-effectively supply renewable power.A multi-objective optimization process is proposed for a hybrid platform with hydrodynamic coupling interaction.The ...An offshore wind-wave hybrid platform could consistently and cost-effectively supply renewable power.A multi-objective optimization process is proposed for a hybrid platform with hydrodynamic coupling interaction.The effects of various critical structural parameters,spacing values,and wave directions are studied for higher energy capture and offshore platform stability.Approximation models of various key parameters are established to optimize the hybrid system,with the objects of the power capture width ratio and the stability index of the platform.The optimization results are affected by the hydrodynamic coupling interaction,with a tendency to affect the higher frequency of hydrodynamic performance in the hybrid system.After the optimization,an appropriate spacing value effectively improves energy capture performance.The optimal array distance D_(Ff),D_(Fp),the optimal structural parameters R_(p),r_(p),d_(f),r_(f),and B_(PTO)are 11.57,12.75,5.1,3.3,1.5,6.5 m,and 80436 Nm s^(-1),respectively.The peak value of the wave energy converter capture width ratio in the hybrid system increases by almost 50%,with a 54%decrease in the stability index.展开更多
Using 19-year satellite altimetric data, variations in the eddy kinetic energy, energy exchanges and interaction between the eddy fi eld and mean fl ow are discussed for the Kuroshio south of Japan. In the seasonal cy...Using 19-year satellite altimetric data, variations in the eddy kinetic energy, energy exchanges and interaction between the eddy fi eld and mean fl ow are discussed for the Kuroshio south of Japan. In the seasonal cycle, the eddy kinetic energy level is a minimum in December/January and a maximum in April/May. In addition to seasonal variations, the eddy kinetic energy undergoes interannual changes. The energy transfers mainly from the mean fl ow to the eddy fi eld in the Kuroshio south of Japan, and dominant energy exchanges mainly occur along the Kuroshio path south of Japan in each year from 1993 to 2011. In addition, there is often barotropic instability south of Honshu. Regarding interactions between the eddy fi eld and mean fl ow, cyclonic and anticyclonic accelerations are also found along the Kuroshio path and they fl ank each other. There is cyclonic acceleration always imposed on southeast of Kyushu, and anticyclonic acceleration dominates south of Honshu from 2001 to mid-2005. Reynolds stress is used to explain the dynamic process of energy exchange. Furthermore, lag-correlation and linear regression analysis show that variability of the energy conversion rate and Reynolds stress involve responses to eddy acceleration at two time scales. The enhanced eddy acceleration induces large Reynolds stress, and enhanced Reynolds stress or barotropic instability further enforces energy transfer from the mean fl ow to the eddy fi eld.展开更多
We theoretically and numerically investigate the coherence of disordered bosonic gas with effective two- and three-body interactions within a two-site Bose-Hubbard model. By properly adjusting the two- and three-body ...We theoretically and numerically investigate the coherence of disordered bosonic gas with effective two- and three-body interactions within a two-site Bose-Hubbard model. By properly adjusting the two- and three-body interactions and the disorder, the coherence of the system exhibits new and interesting phenomena, including the resonance character of coherence against the disorder in the purely two- or three-body interactions system. More interestingly, the disorder and three-body interactions together can suppress the coherence of the purely three-body interactions system, which is different from the case in which the disorder and two-body interactions together can enhance the coherence in certain values of two.body interaction. Furthermore, when two- or three- body interactions are attractive or repulsive, the phase coherence exhibits completely different phenomena. In particular, if two- or three-body interactions are attractive, the coherence of the system can be significantly enhanced in certain regions. Correspondingly, the phase coherence of the system is strongly related to the effective interaction energy. The results provide a possible way for studying the coherence of bosonic gas with multi-atoms' interactions in the presence of the disorder.展开更多
In addition to the hexagonal crystals of class 6 mm, many piezoelectric materials (e.g., BaTiO3), piezomagnetic materials (e.g., CoFe2O4), and multiferroic com-posite materials (e.g., BaTiO3-CoFe2O4 composites)...In addition to the hexagonal crystals of class 6 mm, many piezoelectric materials (e.g., BaTiO3), piezomagnetic materials (e.g., CoFe2O4), and multiferroic com-posite materials (e.g., BaTiO3-CoFe2O4 composites) also exhibit symmetry of transverse isotropy after poling, with the isotropic plane perpendicular to the poling direction. In this paper, simple and elegant line-integral expressions are derived for extended displace-ments, extended stresses, self-energy, and interaction energy of arbitrarily shaped, three-dimensional (3D) dislocation loops with a constant extended Burgers vector in trans-versely isotropic magneto-electro-elastic (MEE) bimaterials (i.e., joined half-spaces). The derived solutions can also be simply reduced to those expressions for piezoelectric, piezo-magnetic, or purely elastic materials. Several numerical examples are given to show both the multi-field coupling effect and the interface/surface effect in transversely isotropic MEE materials.展开更多
The potential energy curves (PECs) of the ground state (^3∏) and three low-lying excited states (^1∑, ^3∑,^1∏) of CdSe dimer have been studied by employing quasirelativistic effective core potentials on the ...The potential energy curves (PECs) of the ground state (^3∏) and three low-lying excited states (^1∑, ^3∑,^1∏) of CdSe dimer have been studied by employing quasirelativistic effective core potentials on the basis of the complete active space self-consistent field method followed by multireference configuration interaction calculation. The four PECs are fitted to analytical potential energy functions using the Murrel-Sorbie potential function. Based on the PECs, the vibrational levels of the four states are determined by solving the Schrodinger equation of nuclear motion, and corresponding spectroscopic constants are accurately calculated. The equilibrium positions as well as the spectroscopic constants and the vibrational levels are reported. By our analysis, the ^3∏ state, of which the dissociation asymptote is Cd(^1S) + Se(^3p), is identified as a ground state of CdSe dimer, and the corresponding dissociation energy is estimated to be 0.39eV. However, the first excited state is only 1132.49cm^-1 above the ground state and the ^3∑ state is the highest in the four calculated states.展开更多
Based on the Burgers equation and Manley-Rowe equation, the derivation about nonlinear interaction of the acoustic waves has been done in this paper. After nonlinear interaction among the low-frequency weak waves and ...Based on the Burgers equation and Manley-Rowe equation, the derivation about nonlinear interaction of the acoustic waves has been done in this paper. After nonlinear interaction among the low-frequency weak waves and the pump wave, the analytical solutions of acoustic waves' amplitude in the field are deduced. The relationship between normalized energy of high-frequency and the change of acoustic energy before and after the nonlinear interaction of the acoustic waves is analyzed. The experimental results about the changes of the acoustic energy are presented. The study shows that new frequencies are generated and the energies of the low-frequency are modulated in a long term by the pump waves, which leads the energies of the low-frequency acoustic waves to change in the pulse trend in the process of the nonlinear interaction of the acoustic waves. The increase and decrease of the energies of the low-frequency are observed under certain typical conditions, which lays a foundation for practical engineering applications.展开更多
Copper-zinc alloy element for boiler energy saving was put in the intake of simulated boiler system to investigate the interaction and transfer of ions in water system both theoretically and experimentally.The fouling...Copper-zinc alloy element for boiler energy saving was put in the intake of simulated boiler system to investigate the interaction and transfer of ions in water system both theoretically and experimentally.The fouling was analyzed by scanning electron microscopy(SEM)and energy dispersive X-ray detector(EDX).The results show that the transfer of calcium and magnesium ions in heat-transfer-surface-water system is affected by zinc ions dissolved from the alloy because of primary battery reaction.Some calcium ions of calcium carbonate crystal are replaced by zinc ions,the growth of aragonite crystal nucleus is retarded,and the transition of calcium carbonate from aragonite to calcite is hampered.展开更多
Low energy ions exist widely in natural world, but people pay a little attention on. the interaction between low energy ions and matter, it is even more out of the question of studying on the relation of low energy io...Low energy ions exist widely in natural world, but people pay a little attention on. the interaction between low energy ions and matter, it is even more out of the question of studying on the relation of low energy ions and the complicated organism. The discovery of bioeffect induced by ion implantation has, however, opened a new branch in the field of ion beam application in life sciences. This paper reports recent advances in research on the role of low energy ions in Chemical synthesis of the biomolecules and application in genetic modification.展开更多
Jarzynski' identity (JI) method was suggested a promising tool for reconstructing free energy landscape of biomolecular interactions in numerical simulations and ex- periments. However, JI method has not yet been w...Jarzynski' identity (JI) method was suggested a promising tool for reconstructing free energy landscape of biomolecular interactions in numerical simulations and ex- periments. However, JI method has not yet been well tested in complex systems such as ligand-receptor molecular pairs. In this paper, we applied a huge number of steered molec- ular dynamics (SMD) simulations to dissociate the protease of human immunodeficiency type I virus (HIV-1 protease) and its inhibitors. We showed that because of intrinsic com- plexity of the ligand-receptor system, the energy barrier pre- dicted by JI method at high pulling rates is much higher than experimental results. However, with a slower pulling rate and fewer switch times of simulations, the predictions of JI method can approach to the experiments. These results sug- gested that the JI method is more appropriate for reconstruct- ing free energy landscape using the data taken from experi- ments, since the pulling rates used in experiments are often much slower than those in SMD simulations. Furthermore, we showed that a higher loading stiffness can produce higher precision of calculation of energy landscape because it yields a lower mean value and narrower bandwidth of work distri- bution in SMD simulations.展开更多
With the increasing demand for petroleum resources and environmental issues,new energy electric vehicles are increasingly being used.However,the large number of electric vehicles connected to the grid has brought new ...With the increasing demand for petroleum resources and environmental issues,new energy electric vehicles are increasingly being used.However,the large number of electric vehicles connected to the grid has brought new challenges to the operation of the grid.Firstly,A novel bidirectional interaction model is established based on modulation theory with nonlinear loads.Then,the electric energy measuring scheme of EVs for V2G is derived under the conditions of distorted power loads.The scheme is composed of fundamental electric energy,fundamental-distorted electric energy,distorted-fundamental electric energy and distorted electric energy.And the characteristics of each electric energy are analyzed.Finally,the correctness of the model and energy measurement method is verified by three simulation cases:the impact signals,the fluctuating signals,and the harmonic signals.展开更多
The author of this paper once attempted to propose a unified framework for gauge fields based on the mathematical and physical picture of the principal fiber bundle: that is, to believe that our universe may have more...The author of this paper once attempted to propose a unified framework for gauge fields based on the mathematical and physical picture of the principal fiber bundle: that is, to believe that our universe may have more fundamental interactions than the four, and these fundamental gauge fields are only components on the bottom manifold (i.e. our universe) projected by a unified gauge potential of the principal fiber bundle manifold;these components can satisfy the transformation of gauge potential, or even be transformed from one basic interaction gauge potential to another basic interaction gauge potential, and can be summarized into a unified equation, namely the generalized gauge equation expression, corresponding to gauge transformation invariance;so the invariance of gauge transformation is a necessary condition for unified field theory, and the four (or more) fundamental interaction fields of the universe are unified in a unified gauge field defined by the connection on the principal fiber bundle. In this paper, the author continues to propose a model of large-scale (gravitational) fundamental interactions in the universe based on the mathematical and physical picture of the principal fiber bundle, attempting to explain that dark matter and dark energy are merely reflections of these gravitational fundamental interactions that deviate in intensity from the gravitational fundamental interactions of the solar system at galaxy scales or some cosmic scales which are much larger than the solar system. All these “gravitational” fundamental interactions originate from the unified gauge field of the universe, namely the connection or curvature on the principal fiber bundle. These interactions are their projected representations on the bottom manifold (i.e. our universe) by different cross-sections (gauge transformations). These projection representations of the universe certainly are described by the generalized gauge equation or curvature similarity equation, and under the guidance of curvature gauge transformation factors, oscillate and evolve between the curvatures 1→0→-1→0→1 of the universe.展开更多
Allowing for all combinations of internal single-bond rotamers, 1,296 unique trial structures of γ-Aminobutyric acid (GABA) are obtained. All of these structures are optimized at the M06-2X level of theory and a to...Allowing for all combinations of internal single-bond rotamers, 1,296 unique trial structures of γ-Aminobutyric acid (GABA) are obtained. All of these structures are optimized at the M06-2X level of theory and a total of 68 local minimal conformers are found. The nine low-lying conformers are used for further studies. According to the calculated relative Gibbs free energies at M06-2X level of theory, we find that the dispersion is important for the relative energy of GABA. The intramolecular hydrogen bonds and byperconjugative interaction and their effects on the conformational stability are studied. The results show that both of them have great influence on the conformers. The vertical ionization energies (VIE) are calculated and match the experimental data well. The results show that the neutral GABA in the gas phase is a multi-conformer system and at least four conformations exist.展开更多
The stability and collective excitation of Bose-Einstein condensates with both two- and three-body interactions in a two-dimensional anhaxmonic trap (i.e., harmonic plus quartic trap) are investigated. By using the ...The stability and collective excitation of Bose-Einstein condensates with both two- and three-body interactions in a two-dimensional anhaxmonic trap (i.e., harmonic plus quartic trap) are investigated. By using the variational method, the influence of the three-body interaction and the anharmonicity on the stability axe discussed in detail. It is found that the anhaxmonicity of the trap and the three-body interaction have significant effect on the stability and collective excitations of the system.展开更多
Based on a single ion model, Hamiltonian of the simplest form about magnetocrystalline anisotropy for Tb3+ ion was solved by using the numerical method. The relation between the stabilization energy, crystal field coe...Based on a single ion model, Hamiltonian of the simplest form about magnetocrystalline anisotropy for Tb3+ ion was solved by using the numerical method. The relation between the stabilization energy, crystal field coefficient B20 and the magnetic exchange interaction was studied as temperature approaches to 0 K. The results show that the stabilization energy contributed by Tb3+ is linear with crystal field coefficient B20 approximately, but it is insensitive to the change of magnetic exchange interaction for the strong magnetic substances such as TbCo5, Tb2Co17 and Tb2Fe14B compounds.展开更多
The shape transition between the vibrational U(5)and deformed c-unstable O(6)dynamical symmetries of sd interacting boson model has been investigated by considering a modified O(6)Hamiltonian,providing that the coeffi...The shape transition between the vibrational U(5)and deformed c-unstable O(6)dynamical symmetries of sd interacting boson model has been investigated by considering a modified O(6)Hamiltonian,providing that the coefficients of the Casimir operator of O(5)are N-dependent,where N is the total number of bosons.The modified O(6)Hamiltonian does not contain the number operator of the d boson,which is responsible for the vibrational motions.In addition,the deformation features can be achieved without using the SU(3)limit by adding to the O(6)dynamical symmetry the three-body interaction[QQQ]^(0),where Q is the O(6)symmetric quadrupole operator.Moreover,triaxiality can be generated through the inclusion of the cubic d-boson interaction[d+d+d+]^(3)·∣ddd∣^(3).The classical limit of the potential energy surface(PES),which represents the expected value of the total Hamiltonian in a coherent state,is studied and examined.The modified O(6)model is applied to the even–even^124-132 Xe isotopes.The parameters for the Hamiltonian and the PESs are calculated using a simulated search program to obtain the minimum root mean square deviation between the calculated and experimental excitation energies and B(E2)values for a number of low-lying levels.A good agreement between the calculations and experiment results is found.展开更多
A three-body model composed of two geological bodies and a structural body was developed to explore how ground-support systems respond to axial loads in underground spaces. A detailed method was designed to fabricate ...A three-body model composed of two geological bodies and a structural body was developed to explore how ground-support systems respond to axial loads in underground spaces. A detailed method was designed to fabricate physical scale-model specimens for testing. Three types of specimens were constructed to investigate how three different materials reacted to each other under load. The three types of specimens were called the weak-rock model, hard-rock model and mixed model. The results of uniaxial compression tests show that the mechanical behaviour of a three-body structural support is closely related to the interaction between the three bodies, but owing to different mechanisms, the three types of material behave very differently. To explain the test results, numerical simulations were conducted to explore fully the load responses of the three-body model specimens. The numerical simulations verify the hypotheses proposed for how the three types of material interact.展开更多
基金supported by the National Research Foundation of Korea(Grant number:NRF-2023R1A2C2005864)supported by the National Research Foundation of Korea(NRF)grant funded by the Korea government(MSIT)(RS-2024-00406240)+3 种基金supported by a National Research Foundation of Korea(NRF)Grant funded by the Korean Government(MSIT)(No.2022R1A2C1003853)supported by a National Research Foundation of Korea(NRF)Grant funded by the Korean Government(MSIT)(No.RS-2023-00217661)Technology Innovation Program(RS-2022-00155961,Development of a high-efficiency drying system for carbon reduction and high-loading electrodes by a flash light source)funded by the Ministry of Trade&,Energy(MOTIE,Korea)supported by a National Research Foundation of Korea(NRF)Grant funded by the Korean Government(MSIT)(No.2022R1A2C4001497).
文摘This review provides a comprehensive overview of the progress in light-material interactions(LMIs),focusing on lasers and flash lights for energy conversion and storage applications.We discuss intricate LMI parameters such as light sources,interaction time,and fluence to elucidate their importance in material processing.In addition,this study covers various light-induced photothermal and photochemical processes ranging from melting,crystallization,and ablation to doping and synthesis,which are essential for developing energy materials and devices.Finally,we present extensive energy conversion and storage applications demonstrated by LMI technologies,including energy harvesters,sensors,capacitors,and batteries.Despite the several challenges associated with LMIs,such as complex mechanisms,and high-degrees of freedom,we believe that substantial contributions and potential for the commercialization of future energy systems can be achieved by advancing optical technologies through comprehensive academic research and multidisciplinary collaborations.
基金supported by the National Research Foundation of Korea grant funded by the Korean government (MSIT)(2020R1A2C1101039)the Commercializations Promotion Agency for R&D Outcomes (COMPA) grant funded by the Korea government(MSIT)(2021E200)+1 种基金supported by“Regional Innovation Strategy (RIS)” through the National Research Foundation of Korea (NRF) funded by the Ministry of Education(MOE)(2021RIS-004)supported by the Soonchunhyang University Research Fund。
文摘Improving the capacitance and energy density is a significant challenge while developing practical and flexible energy storage system(ESS).Redox mediators(RMs),as redox-active electrolyte additives,can provide additional energy storing capability via electrochemical faradaic contribution on electrodes for high-performance flexible ESSs.Particularly,determining effective material combinations between electrodes and RMs is essential for maximizing surface faradaic redox reactions for energy-storage performance.In this study,an electrode-RM system comprising heterostructured hybrid(carbon fiber(CF)/MnO_(2)) faradaic electrodes and iodine RMs(I-RMs) in a redox-active electrolyte is investigated.The CF/MnO_(2)with the 1-RMs(CF/MnO_(2)-I) induces dominant catalytic faradaic interaction with the I-RMs,significantly enhancing the surface faradaic kinetics and increasing the overall energy-storage performance.The CF/MnO_(2)-I ESSs show a 12.6-fold(or higher) increased volumetric energy density of 793.81 mWh L^(-1)at a current of 10 μA relative to ESSs using CF/MnO_(2)without I-RMs(CF/MnO_(2)).Moreover,the CF/MnO_(2)-I retains 93.1% of its initial capacitance after 10,000 cycles,validating the excellent cyclability.Finally,the flexibility of the ESSs is tested at different bending angles(180° to 0°),demonstrating its feasibility for flexible and high-wear environments.Therefore,CF/MnO_(2)electrodes present a practical material combination for high-performance flexible energy-storage devices owing to the catalytic faradaic interaction with I-RMs.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11264027 and 11364030)the Project of Prairie Excellent Specialist of Inner Mongolia,Chinathe "Thousand,Hundred and Ten" Talent Training Project Foundation of Inner Mongolia Normal University,China(Grant No.RCPY-2-2012-K-039)
文摘We investigated the properties of polarons in a wurtzite ZnO/MgxZn1-xO quantum well by adopting a modified Lee–Low–Pines variational method, giving the ground state energy, transition energy, and phonon contributions from various optical-phonon modes to the ground state energy as functions of the well width and Mg composition. In our calculations, we considered the effects of confined optical phonon modes, interface-optical phonon modes, and half-space phonon modes, as well as the anisotropy of the electron effective band mass, phonon frequency, and dielectric constant. Our numerical results indicate that the electron–optical phonon interactions importantly affect the polaronic energies in the ZnO/MgxZn1-xO quantum well. The electron–optical phonon interactions decrease the polaron energies. For quantum wells with narrower wells, the interface optical phonon and half-space phonon modes contribute more to the polaronic energies than the confined phonon modes. However, for wider quantum wells, the total contribution to the polaronic energy mainly comes from the confined modes. The contributions of the various phonon modes to the transition energy change differently with increasing well width. The contribution of the half-space phonons decreases slowly as the QW width increases, whereas the contributions of the confined and interface phonons reach a maximum at d ≈ 5.0 nm and then decrease slowly. However,the total contribution of phonon modes to the transition energy is negative and increases gradually with the QW width of d.As the composition x increases, the total contribution of phonons to the ground state energies increases slowly, but the total contributions of phonons to the transition energies decrease gradually. We analyze the physical reasons for these behaviors in detail.
基金supported by the Natural Science Foundation of Shaanxi University of Science and Technology,China (Grant Nos SUST-ZX08-27 and SUST-ZX07-32)
文摘This paper investigates the collective excitation and stability of low-dimensional Bose-Einstein condensates with two- and three-body interactions by the variational analysis of the time-dependent Gross-Pitaevskii-Ginsburg equation. The spectrum of the low-energy excitation and the effective potential for the width of the condensate axe obtained. The results show that: (i) the repulsive two-body interaction among atoms makes the frequency red-shifted for the internal excitation and the repulsive or attractive three-body interaction always makes it blue-shifted; (ii) the region for the existence of the stable bound states is obtained by identifying the critical value of the two- and three-body interactions.
基金the National Natural Science Foundation of China(No.U2006229)the Research on the Qingdao Science and Technology Development Projects(No.18-1-2-20-zhc)supported by the Innovation Program approved by the Ministry of Industry and Information Technology of PR China([2016]24)。
文摘An offshore wind-wave hybrid platform could consistently and cost-effectively supply renewable power.A multi-objective optimization process is proposed for a hybrid platform with hydrodynamic coupling interaction.The effects of various critical structural parameters,spacing values,and wave directions are studied for higher energy capture and offshore platform stability.Approximation models of various key parameters are established to optimize the hybrid system,with the objects of the power capture width ratio and the stability index of the platform.The optimization results are affected by the hydrodynamic coupling interaction,with a tendency to affect the higher frequency of hydrodynamic performance in the hybrid system.After the optimization,an appropriate spacing value effectively improves energy capture performance.The optimal array distance D_(Ff),D_(Fp),the optimal structural parameters R_(p),r_(p),d_(f),r_(f),and B_(PTO)are 11.57,12.75,5.1,3.3,1.5,6.5 m,and 80436 Nm s^(-1),respectively.The peak value of the wave energy converter capture width ratio in the hybrid system increases by almost 50%,with a 54%decrease in the stability index.
基金Supported by the Knowledge Innovation Program of Chinese Academy of Sciences(No.KZCX2-EW-201)the Basic Research Program of Science and Technology Projects of Qingdao(No.11-1-4-95-jch)
文摘Using 19-year satellite altimetric data, variations in the eddy kinetic energy, energy exchanges and interaction between the eddy fi eld and mean fl ow are discussed for the Kuroshio south of Japan. In the seasonal cycle, the eddy kinetic energy level is a minimum in December/January and a maximum in April/May. In addition to seasonal variations, the eddy kinetic energy undergoes interannual changes. The energy transfers mainly from the mean fl ow to the eddy fi eld in the Kuroshio south of Japan, and dominant energy exchanges mainly occur along the Kuroshio path south of Japan in each year from 1993 to 2011. In addition, there is often barotropic instability south of Honshu. Regarding interactions between the eddy fi eld and mean fl ow, cyclonic and anticyclonic accelerations are also found along the Kuroshio path and they fl ank each other. There is cyclonic acceleration always imposed on southeast of Kyushu, and anticyclonic acceleration dominates south of Honshu from 2001 to mid-2005. Reynolds stress is used to explain the dynamic process of energy exchange. Furthermore, lag-correlation and linear regression analysis show that variability of the energy conversion rate and Reynolds stress involve responses to eddy acceleration at two time scales. The enhanced eddy acceleration induces large Reynolds stress, and enhanced Reynolds stress or barotropic instability further enforces energy transfer from the mean fl ow to the eddy fi eld.
基金Supported by the National Natural Science Foundation of China under Grant Nos 11475027,11274255 and 11305132the Specialized Research Fund for the Doctoral Program of Higher Education of China under Grand No 20136203110001+1 种基金the Natural Science Foundation of Gansu Province under Grant No 1506RJYA131the Creation of Science and Technology of Northwest Normal University under Grant Nos NWNU-KJCXGC-03-48 and NWNU-LKQN-12-12
文摘We theoretically and numerically investigate the coherence of disordered bosonic gas with effective two- and three-body interactions within a two-site Bose-Hubbard model. By properly adjusting the two- and three-body interactions and the disorder, the coherence of the system exhibits new and interesting phenomena, including the resonance character of coherence against the disorder in the purely two- or three-body interactions system. More interestingly, the disorder and three-body interactions together can suppress the coherence of the purely three-body interactions system, which is different from the case in which the disorder and two-body interactions together can enhance the coherence in certain values of two.body interaction. Furthermore, when two- or three- body interactions are attractive or repulsive, the phase coherence exhibits completely different phenomena. In particular, if two- or three-body interactions are attractive, the coherence of the system can be significantly enhanced in certain regions. Correspondingly, the phase coherence of the system is strongly related to the effective interaction energy. The results provide a possible way for studying the coherence of bosonic gas with multi-atoms' interactions in the presence of the disorder.
基金Project supported by the National Project of Scientific and Technical Supporting Programs Funded by Ministry of Science&Technology of China(No.2009BAG12A01-A03-2)the National Natural Science Foundation of China(Nos.10972196,11090333,11172273,and 11321202)
文摘In addition to the hexagonal crystals of class 6 mm, many piezoelectric materials (e.g., BaTiO3), piezomagnetic materials (e.g., CoFe2O4), and multiferroic com-posite materials (e.g., BaTiO3-CoFe2O4 composites) also exhibit symmetry of transverse isotropy after poling, with the isotropic plane perpendicular to the poling direction. In this paper, simple and elegant line-integral expressions are derived for extended displace-ments, extended stresses, self-energy, and interaction energy of arbitrarily shaped, three-dimensional (3D) dislocation loops with a constant extended Burgers vector in trans-versely isotropic magneto-electro-elastic (MEE) bimaterials (i.e., joined half-spaces). The derived solutions can also be simply reduced to those expressions for piezoelectric, piezo-magnetic, or purely elastic materials. Several numerical examples are given to show both the multi-field coupling effect and the interface/surface effect in transversely isotropic MEE materials.
基金Project supported by the national Natural Science Foundation of China (Grant No 10674114).
文摘The potential energy curves (PECs) of the ground state (^3∏) and three low-lying excited states (^1∑, ^3∑,^1∏) of CdSe dimer have been studied by employing quasirelativistic effective core potentials on the basis of the complete active space self-consistent field method followed by multireference configuration interaction calculation. The four PECs are fitted to analytical potential energy functions using the Murrel-Sorbie potential function. Based on the PECs, the vibrational levels of the four states are determined by solving the Schrodinger equation of nuclear motion, and corresponding spectroscopic constants are accurately calculated. The equilibrium positions as well as the spectroscopic constants and the vibrational levels are reported. By our analysis, the ^3∏ state, of which the dissociation asymptote is Cd(^1S) + Se(^3p), is identified as a ground state of CdSe dimer, and the corresponding dissociation energy is estimated to be 0.39eV. However, the first excited state is only 1132.49cm^-1 above the ground state and the ^3∑ state is the highest in the four calculated states.
基金financially supported by the Scientific Research Fund of Heilongjiang Provincial Education Department(Grant No.12541132)the Natural Science Youth Foundation of Heilongjiang Province of China(Grant No.QC2015082)
文摘Based on the Burgers equation and Manley-Rowe equation, the derivation about nonlinear interaction of the acoustic waves has been done in this paper. After nonlinear interaction among the low-frequency weak waves and the pump wave, the analytical solutions of acoustic waves' amplitude in the field are deduced. The relationship between normalized energy of high-frequency and the change of acoustic energy before and after the nonlinear interaction of the acoustic waves is analyzed. The experimental results about the changes of the acoustic energy are presented. The study shows that new frequencies are generated and the energies of the low-frequency are modulated in a long term by the pump waves, which leads the energies of the low-frequency acoustic waves to change in the pulse trend in the process of the nonlinear interaction of the acoustic waves. The increase and decrease of the energies of the low-frequency are observed under certain typical conditions, which lays a foundation for practical engineering applications.
基金This work was financially supported by the Key Technologies R&D Program of Tianjin(No.06YFGZGX02400).
文摘Copper-zinc alloy element for boiler energy saving was put in the intake of simulated boiler system to investigate the interaction and transfer of ions in water system both theoretically and experimentally.The fouling was analyzed by scanning electron microscopy(SEM)and energy dispersive X-ray detector(EDX).The results show that the transfer of calcium and magnesium ions in heat-transfer-surface-water system is affected by zinc ions dissolved from the alloy because of primary battery reaction.Some calcium ions of calcium carbonate crystal are replaced by zinc ions,the growth of aragonite crystal nucleus is retarded,and the transition of calcium carbonate from aragonite to calcite is hampered.
基金National Science & Technology Key ProgramNational Nature Science FOundation+1 种基金Chinese Academy of Sciences FoundationAnh
文摘Low energy ions exist widely in natural world, but people pay a little attention on. the interaction between low energy ions and matter, it is even more out of the question of studying on the relation of low energy ions and the complicated organism. The discovery of bioeffect induced by ion implantation has, however, opened a new branch in the field of ion beam application in life sciences. This paper reports recent advances in research on the role of low energy ions in Chemical synthesis of the biomolecules and application in genetic modification.
基金supported by the National Science Foundation of China (10732050,10872115 and 11025208)Excellent Young Scholars Research Fund of Beijing Institute of Technology
文摘Jarzynski' identity (JI) method was suggested a promising tool for reconstructing free energy landscape of biomolecular interactions in numerical simulations and ex- periments. However, JI method has not yet been well tested in complex systems such as ligand-receptor molecular pairs. In this paper, we applied a huge number of steered molec- ular dynamics (SMD) simulations to dissociate the protease of human immunodeficiency type I virus (HIV-1 protease) and its inhibitors. We showed that because of intrinsic com- plexity of the ligand-receptor system, the energy barrier pre- dicted by JI method at high pulling rates is much higher than experimental results. However, with a slower pulling rate and fewer switch times of simulations, the predictions of JI method can approach to the experiments. These results sug- gested that the JI method is more appropriate for reconstruct- ing free energy landscape using the data taken from experi- ments, since the pulling rates used in experiments are often much slower than those in SMD simulations. Furthermore, we showed that a higher loading stiffness can produce higher precision of calculation of energy landscape because it yields a lower mean value and narrower bandwidth of work distri- bution in SMD simulations.
基金This work is supported by China Postdoctoral Science Foundation(2021M690798)Guizhou Province Science and Technology Plan Project(No.[2021]General 085)+1 种基金National Natural Science Foundation of China(No.61603034)the Fundamental Research Funds for the Central Universities(Nos.FRF-BD-19-002A,FRF-DF-20-14).
文摘With the increasing demand for petroleum resources and environmental issues,new energy electric vehicles are increasingly being used.However,the large number of electric vehicles connected to the grid has brought new challenges to the operation of the grid.Firstly,A novel bidirectional interaction model is established based on modulation theory with nonlinear loads.Then,the electric energy measuring scheme of EVs for V2G is derived under the conditions of distorted power loads.The scheme is composed of fundamental electric energy,fundamental-distorted electric energy,distorted-fundamental electric energy and distorted electric energy.And the characteristics of each electric energy are analyzed.Finally,the correctness of the model and energy measurement method is verified by three simulation cases:the impact signals,the fluctuating signals,and the harmonic signals.
文摘The author of this paper once attempted to propose a unified framework for gauge fields based on the mathematical and physical picture of the principal fiber bundle: that is, to believe that our universe may have more fundamental interactions than the four, and these fundamental gauge fields are only components on the bottom manifold (i.e. our universe) projected by a unified gauge potential of the principal fiber bundle manifold;these components can satisfy the transformation of gauge potential, or even be transformed from one basic interaction gauge potential to another basic interaction gauge potential, and can be summarized into a unified equation, namely the generalized gauge equation expression, corresponding to gauge transformation invariance;so the invariance of gauge transformation is a necessary condition for unified field theory, and the four (or more) fundamental interaction fields of the universe are unified in a unified gauge field defined by the connection on the principal fiber bundle. In this paper, the author continues to propose a model of large-scale (gravitational) fundamental interactions in the universe based on the mathematical and physical picture of the principal fiber bundle, attempting to explain that dark matter and dark energy are merely reflections of these gravitational fundamental interactions that deviate in intensity from the gravitational fundamental interactions of the solar system at galaxy scales or some cosmic scales which are much larger than the solar system. All these “gravitational” fundamental interactions originate from the unified gauge field of the universe, namely the connection or curvature on the principal fiber bundle. These interactions are their projected representations on the bottom manifold (i.e. our universe) by different cross-sections (gauge transformations). These projection representations of the universe certainly are described by the generalized gauge equation or curvature similarity equation, and under the guidance of curvature gauge transformation factors, oscillate and evolve between the curvatures 1→0→-1→0→1 of the universe.
基金Project supported by the Science Foundation of Henan Provincial Educational Committee,China(Grant Nos.2011A140015 and 12A140006)the Doctoral Research Fund of Henan Normal University,China(Grant No.525449)
文摘Allowing for all combinations of internal single-bond rotamers, 1,296 unique trial structures of γ-Aminobutyric acid (GABA) are obtained. All of these structures are optimized at the M06-2X level of theory and a total of 68 local minimal conformers are found. The nine low-lying conformers are used for further studies. According to the calculated relative Gibbs free energies at M06-2X level of theory, we find that the dispersion is important for the relative energy of GABA. The intramolecular hydrogen bonds and byperconjugative interaction and their effects on the conformational stability are studied. The results show that both of them have great influence on the conformers. The vertical ionization energies (VIE) are calculated and match the experimental data well. The results show that the neutral GABA in the gas phase is a multi-conformer system and at least four conformations exist.
基金The project by the National Natural Science Foundation of China under Grant No.10774120by the Natural Science Foundation of Gansu Province,China under Grant No.3ZS051-A25-013by Creation of Science and Technology of Northwest Normal University,China under Grant No.NWNU-KJCXGC-03-17
文摘The stability and collective excitation of Bose-Einstein condensates with both two- and three-body interactions in a two-dimensional anhaxmonic trap (i.e., harmonic plus quartic trap) are investigated. By using the variational method, the influence of the three-body interaction and the anharmonicity on the stability axe discussed in detail. It is found that the anhaxmonicity of the trap and the three-body interaction have significant effect on the stability and collective excitations of the system.
文摘Based on a single ion model, Hamiltonian of the simplest form about magnetocrystalline anisotropy for Tb3+ ion was solved by using the numerical method. The relation between the stabilization energy, crystal field coefficient B20 and the magnetic exchange interaction was studied as temperature approaches to 0 K. The results show that the stabilization energy contributed by Tb3+ is linear with crystal field coefficient B20 approximately, but it is insensitive to the change of magnetic exchange interaction for the strong magnetic substances such as TbCo5, Tb2Co17 and Tb2Fe14B compounds.
文摘The shape transition between the vibrational U(5)and deformed c-unstable O(6)dynamical symmetries of sd interacting boson model has been investigated by considering a modified O(6)Hamiltonian,providing that the coefficients of the Casimir operator of O(5)are N-dependent,where N is the total number of bosons.The modified O(6)Hamiltonian does not contain the number operator of the d boson,which is responsible for the vibrational motions.In addition,the deformation features can be achieved without using the SU(3)limit by adding to the O(6)dynamical symmetry the three-body interaction[QQQ]^(0),where Q is the O(6)symmetric quadrupole operator.Moreover,triaxiality can be generated through the inclusion of the cubic d-boson interaction[d+d+d+]^(3)·∣ddd∣^(3).The classical limit of the potential energy surface(PES),which represents the expected value of the total Hamiltonian in a coherent state,is studied and examined.The modified O(6)model is applied to the even–even^124-132 Xe isotopes.The parameters for the Hamiltonian and the PESs are calculated using a simulated search program to obtain the minimum root mean square deviation between the calculated and experimental excitation energies and B(E2)values for a number of low-lying levels.A good agreement between the calculations and experiment results is found.
基金Project(51674244)supported by the National Natural Science Foundation of ChinaProject(2014QNA47)supported by the Fundamental Research Funds for the Central Universities,ChinaProject(BK20151145)supported by the Natural Science Foundation of Jiangsu Province,China
文摘A three-body model composed of two geological bodies and a structural body was developed to explore how ground-support systems respond to axial loads in underground spaces. A detailed method was designed to fabricate physical scale-model specimens for testing. Three types of specimens were constructed to investigate how three different materials reacted to each other under load. The three types of specimens were called the weak-rock model, hard-rock model and mixed model. The results of uniaxial compression tests show that the mechanical behaviour of a three-body structural support is closely related to the interaction between the three bodies, but owing to different mechanisms, the three types of material behave very differently. To explain the test results, numerical simulations were conducted to explore fully the load responses of the three-body model specimens. The numerical simulations verify the hypotheses proposed for how the three types of material interact.